WO2008143027A1 - リチウムイオン二次電池、及び、その製造方法 - Google Patents

リチウムイオン二次電池、及び、その製造方法 Download PDF

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Publication number
WO2008143027A1
WO2008143027A1 PCT/JP2008/058616 JP2008058616W WO2008143027A1 WO 2008143027 A1 WO2008143027 A1 WO 2008143027A1 JP 2008058616 W JP2008058616 W JP 2008058616W WO 2008143027 A1 WO2008143027 A1 WO 2008143027A1
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WIPO (PCT)
Prior art keywords
electrode layer
layer
lithium ion
rechargeable battery
ion rechargeable
Prior art date
Application number
PCT/JP2008/058616
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English (en)
French (fr)
Inventor
Mamoru Baba
Shoichi Iwaya
Hitoshi Masumura
Noriyuki Sakai
Takayuki Fujita
Hiroshi Sasagawa
Hiroshi Sato
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Namics Corporation
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Publication date
Application filed by Namics Corporation filed Critical Namics Corporation
Priority to US12/599,941 priority Critical patent/US20100216032A1/en
Priority to CN2008800141411A priority patent/CN101675553B/zh
Priority to KR1020097020089A priority patent/KR101506045B1/ko
Priority to JP2009515152A priority patent/JP4797105B2/ja
Publication of WO2008143027A1 publication Critical patent/WO2008143027A1/ja
Priority to US13/932,375 priority patent/US9457512B2/en

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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B29—WORKING OF PLASTICS; WORKING OF SUBSTANCES IN A PLASTIC STATE IN GENERAL
    • B29C—SHAPING OR JOINING OF PLASTICS; SHAPING OF MATERIAL IN A PLASTIC STATE, NOT OTHERWISE PROVIDED FOR; AFTER-TREATMENT OF THE SHAPED PRODUCTS, e.g. REPAIRING
    • B29C65/00—Joining or sealing of preformed parts, e.g. welding of plastics materials; Apparatus therefor
    • B29C65/02—Joining or sealing of preformed parts, e.g. welding of plastics materials; Apparatus therefor by heating, with or without pressure
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/362—Composites
    • H01M4/366—Composites as layered products
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H01M10/0525—Rocking-chair batteries, i.e. batteries with lithium insertion or intercalation in both electrodes; Lithium-ion batteries
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
    • H01M10/0561—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of inorganic materials only
    • H01M10/0562—Solid materials
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/485—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of mixed oxides or hydroxides for inserting or intercalating light metals, e.g. LiTi2O4 or LiTi2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/50—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese
    • H01M4/505—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese of mixed oxides or hydroxides containing manganese for inserting or intercalating light metals, e.g. LiMn2O4 or LiMn2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/624—Electric conductive fillers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T29/00—Metal working
    • Y10T29/49—Method of mechanical manufacture
    • Y10T29/49002—Electrical device making
    • Y10T29/49108—Electric battery cell making
    • Y10T29/49112—Electric battery cell making including laminating of indefinite length material

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Inorganic Chemistry (AREA)
  • Composite Materials (AREA)
  • Materials Engineering (AREA)
  • Physics & Mathematics (AREA)
  • Condensed Matter Physics & Semiconductors (AREA)
  • General Physics & Mathematics (AREA)
  • Mechanical Engineering (AREA)
  • Secondary Cells (AREA)
  • Battery Electrode And Active Subsutance (AREA)

Abstract

電極層と電解質層を積層した多層全固体型のリチウムイオン二次電池では、電極層と電解質層の界面に充放電反応に寄与しない不純物層ができ、電池特性を劣化させるという問題があった。この対策として、界面に反応生成物を形成しない従来技術による電池では、界面の接合が十分強固なものとならないという問題があった。 電極層と電解質層を積層した後、焼成を行う工程で、電極層と電解質層の界面に充放電反応に寄与する反応生成物からなる中間層が形成されるように、電極層及び電解質層の材料を選択した。また、所定の混合比で活物質と導電性物質を混合したペーストを用い正極層、負極層を形成した。電極抵抗、界面抵抗の低減、充放電サイクル特性の改善が可能になった。  
PCT/JP2008/058616 2007-05-11 2008-05-09 リチウムイオン二次電池、及び、その製造方法 WO2008143027A1 (ja)

Priority Applications (5)

Application Number Priority Date Filing Date Title
US12/599,941 US20100216032A1 (en) 2007-05-11 2008-05-09 Lithium ion rechargeable battery and process for producing the lithium ion rechargeable battery
CN2008800141411A CN101675553B (zh) 2007-05-11 2008-05-09 锂离子二次电池及其制造方法
KR1020097020089A KR101506045B1 (ko) 2007-05-11 2008-05-09 리튬이온 2 차 전지 및 그 제조 방법
JP2009515152A JP4797105B2 (ja) 2007-05-11 2008-05-09 リチウムイオン二次電池、及び、その製造方法
US13/932,375 US9457512B2 (en) 2007-05-11 2013-07-01 Lithium ion rechargeable battery and process for producing the lithium ion rechargeable battery

Applications Claiming Priority (4)

Application Number Priority Date Filing Date Title
JP2007-127443 2007-05-11
JP2007127444 2007-05-11
JP2007127443 2007-05-11
JP2007-127444 2007-05-11

Related Child Applications (2)

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US12/599,941 A-371-Of-International US20100216032A1 (en) 2007-05-11 2008-05-09 Lithium ion rechargeable battery and process for producing the lithium ion rechargeable battery
US13/932,375 Division US9457512B2 (en) 2007-05-11 2013-07-01 Lithium ion rechargeable battery and process for producing the lithium ion rechargeable battery

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US (2) US20100216032A1 (ja)
JP (1) JP4797105B2 (ja)
KR (1) KR101506045B1 (ja)
CN (1) CN101675553B (ja)
TW (1) TWI527289B (ja)
WO (1) WO2008143027A1 (ja)

Cited By (29)

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JP2009181876A (ja) * 2008-01-31 2009-08-13 Ohara Inc リチウムイオン二次電池用積層体の製造方法
WO2010067818A1 (ja) * 2008-12-10 2010-06-17 ナミックス株式会社 リチウムイオン二次電池、及び、その製造方法
JP2010245024A (ja) * 2009-03-16 2010-10-28 Toyota Motor Corp 全固体二次電池
JP2011150817A (ja) * 2010-01-19 2011-08-04 Ohara Inc 全固体電池
JP2011198692A (ja) * 2010-03-23 2011-10-06 Namics Corp リチウムイオン二次電池及びその製造方法
US20120276439A1 (en) * 2009-12-21 2012-11-01 Namics Corporation Lithium ion secondary battery
WO2013133394A1 (ja) * 2012-03-07 2013-09-12 株式会社村田製作所 全固体電池
JP2014110149A (ja) * 2012-11-30 2014-06-12 Murata Mfg Co Ltd 全固体型電池用積層体
JP2014534591A (ja) * 2011-11-02 2014-12-18 アイ テン 薄膜リチウムイオンマイクロ電池の製造方法及びその方法により得られたマイクロ電池
JP2014534592A (ja) * 2011-11-02 2014-12-18 アイ テン 全固体薄膜電池の製造方法
JP2014535141A (ja) * 2011-11-02 2014-12-25 アイ テン リチウムイオン電池用の固体電解質薄膜の製造方法
JP2015191722A (ja) * 2014-03-27 2015-11-02 株式会社村田製作所 固体電解質及び全固体電池
JP2016507865A (ja) * 2012-12-31 2016-03-10 アイ テン 積層構造の全固体電池の製造方法
JP2016072077A (ja) * 2014-09-30 2016-05-09 セイコーエプソン株式会社 電極複合体、電極複合体の製造方法およびリチウム電池
JP2017107826A (ja) * 2015-12-11 2017-06-15 国立大学法人豊橋技術科学大学 電極及びその製造方法並びに全固体型リチウムイオン電池
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