JP5904371B2 - リチウム二次電池用活物質、リチウム二次電池用電極及びリチウム二次電池 - Google Patents

リチウム二次電池用活物質、リチウム二次電池用電極及びリチウム二次電池 Download PDF

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JP5904371B2
JP5904371B2 JP2012535047A JP2012535047A JP5904371B2 JP 5904371 B2 JP5904371 B2 JP 5904371B2 JP 2012535047 A JP2012535047 A JP 2012535047A JP 2012535047 A JP2012535047 A JP 2012535047A JP 5904371 B2 JP5904371 B2 JP 5904371B2
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active material
lithium
lithium secondary
secondary battery
plane
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JPWO2012039413A1 (ja
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遠藤　大輔
大輔 遠藤
禎弘 片山
禎弘 片山
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GS Yuasa International Ltd
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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/131—Electrodes based on mixed oxides or hydroxides, or on mixtures of oxides or hydroxides, e.g. LiCoOx
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G45/00—Compounds of manganese
    • C01G45/12—Manganates manganites or permanganates
    • C01G45/1221—Manganates or manganites with a manganese oxidation state of Mn(III), Mn(IV) or mixtures thereof
    • C01G45/1228—Manganates or manganites with a manganese oxidation state of Mn(III), Mn(IV) or mixtures thereof of the type [MnO2]n-, e.g. LiMnO2, Li[MxMn1-x]O2
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G51/00—Compounds of cobalt
    • C01G51/40—Cobaltates
    • C01G51/42—Cobaltates containing alkali metals, e.g. LiCoO2
    • C01G51/44—Cobaltates containing alkali metals, e.g. LiCoO2 containing manganese
    • C01G51/50—Cobaltates containing alkali metals, e.g. LiCoO2 containing manganese of the type [MnO2]n-, e.g. Li(CoxMn1-x)O2, Li(MyCoxMn1-x-y)O2
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G53/00—Compounds of nickel
    • C01G53/40—Nickelates
    • C01G53/42—Nickelates containing alkali metals, e.g. LiNiO2
    • C01G53/44—Nickelates containing alkali metals, e.g. LiNiO2 containing manganese
    • C01G53/50—Nickelates containing alkali metals, e.g. LiNiO2 containing manganese of the type [MnO2]n-, e.g. Li(NixMn1-x)O2, Li(MyNixMn1-x-y)O2
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H01M10/0525—Rocking-chair batteries, i.e. batteries with lithium insertion or intercalation in both electrodes; Lithium-ion batteries
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/139—Processes of manufacture
    • H01M4/1391—Processes of manufacture of electrodes based on mixed oxides or hydroxides, or on mixtures of oxides or hydroxides, e.g. LiCoOx
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/362—Composites
    • H01M4/364—Composites as mixtures
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/38—Selection of substances as active materials, active masses, active liquids of elements or alloys
    • H01M4/381—Alkaline or alkaline earth metals elements
    • H01M4/382—Lithium
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/50—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese
    • H01M4/505—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese of mixed oxides or hydroxides containing manganese for inserting or intercalating light metals, e.g. LiMn2O4 or LiMn2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/52—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron
    • H01M4/525—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron of mixed oxides or hydroxides containing iron, cobalt or nickel for inserting or intercalating light metals, e.g. LiNiO2, LiCoO2 or LiCoOxFy
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00—Crystal-structural characteristics
    • C01P2002/50—Solid solutions
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00—Crystal-structural characteristics
    • C01P2002/50—Solid solutions
    • C01P2002/52—Solid solutions containing elements as dopants
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00—Crystal-structural characteristics
    • C01P2002/70—Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data
    • C01P2002/76—Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data by a space-group or by other symmetry indications
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00—Crystal-structural characteristics
    • C01P2002/70—Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data
    • C01P2002/77—Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data by unit-cell parameters, atom positions or structure diagrams
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00—Crystal-structural characteristics
    • C01P2002/80—Crystal-structural characteristics defined by measured data other than those specified in group C01P2002/70
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2004/00—Particle morphology
    • C01P2004/60—Particles characterised by their size
    • C01P2004/64—Nanometer sized, i.e. from 1-100 nanometer
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2006/00—Physical properties of inorganic compounds
    • C01P2006/12—Surface area
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2006/00—Physical properties of inorganic compounds
    • C01P2006/40—Electric properties
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
    • Y02T10/00—Road transport of goods or passengers
    • Y02T10/60—Other road transportation technologies with climate change mitigation effect
    • Y02T10/70—Energy storage systems for electromobility, e.g. batteries

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  • Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Composite Materials (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Inorganic Compounds Of Heavy Metals (AREA)
  • Secondary Cells (AREA)
JP2012535047A 2010-09-22 2011-09-21 リチウム二次電池用活物質、リチウム二次電池用電極及びリチウム二次電池 Active JP5904371B2 (ja)

Applications Claiming Priority (5)

Application Number Priority Date Filing Date Title
JP2010212383 2010-09-22
JP2010212383 2010-09-22
JP2010217905 2010-09-28
JP2010217905 2010-09-28
PCT/JP2011/071440 WO2012039413A1 (ja) 2010-09-22 2011-09-21 リチウム二次電池用活物質、リチウム二次電池用電極及びリチウム二次電池

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JPWO2012039413A1 JPWO2012039413A1 (ja) 2014-02-03
JP5904371B2 true JP5904371B2 (ja) 2016-04-13

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US (1) US9219273B2 (ko)
EP (1) EP2621002B1 (ko)
JP (1) JP5904371B2 (ko)
KR (1) KR101820814B1 (ko)
CN (1) CN103119761B (ko)
WO (1) WO2012039413A1 (ko)

Families Citing this family (51)

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JP6011838B2 (ja) * 2011-08-31 2016-10-19 トヨタ自動車株式会社 リチウム二次電池
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JP6090662B2 (ja) 2012-06-29 2017-03-08 株式会社Ｇｓユアサ リチウム二次電池用正極活物質、その製造方法、リチウム二次電池用電極、リチウム二次電池
JP6066306B2 (ja) 2012-07-04 2017-01-25 株式会社Ｇｓユアサ 非水電解質二次電池及び非水電解質二次電池の製造方法
JP6094797B2 (ja) * 2012-08-03 2017-03-15 株式会社Ｇｓユアサ リチウム二次電池用正極活物質、その製造方法、リチウム二次電池用電極、リチウム二次電池
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JP6175763B2 (ja) * 2012-08-28 2017-08-09 株式会社Ｇｓユアサ リチウム二次電池用正極活物質、その正極活物質の製造方法、リチウム二次電池用電極、及びリチウム二次電池
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JP6209435B2 (ja) * 2013-12-17 2017-10-04 住友化学株式会社 正極活物質、リチウムイオン二次電池用正極およびリチウムイオン二次電池
JP6486653B2 (ja) 2014-01-31 2019-03-20 パナソニック株式会社 非水電解質二次電池用正極活物質及び非水電解質二次電池
FR3023070A1 (fr) * 2014-06-27 2016-01-01 Renault Sas Procede de cyclage de batterie lithium-ion comprenant un materiau pour cathode a base d'oxyde lamellaire surlithie
US9660263B2 (en) 2014-12-23 2017-05-23 Sharp Kabushiki Kaisha Layered oxide materials for batteries
US9653731B2 (en) * 2014-12-23 2017-05-16 Sharp Kabushiki Kaisha Layered oxide materials for batteries
JP6474033B2 (ja) * 2015-01-29 2019-02-27 株式会社Ｇｓユアサ リチウム二次電池用正極活物質、リチウム二次電池用電極、及びリチウム二次電池
CN104684119B (zh) * 2015-02-12 2017-01-11 蒋军闽 一种远红外电热线的生产工艺
JP6624885B2 (ja) 2015-02-19 2019-12-25 パナソニック株式会社 非水電解質二次電池用正極活物質及び非水電解質二次電池
JP6164332B2 (ja) 2015-04-28 2017-07-19 日亜化学工業株式会社 ニッケルコバルト複合水酸化物粒子とその製造方法、非水系電解質二次電池用正極活物質とその製造方法、ならびに、非水系電解質二次電池
KR102447364B1 (ko) 2015-04-28 2022-09-26 니치아 카가쿠 고교 가부시키가이샤 니켈 코발트 복합 수산화물 입자 및 그 제조 방법, 비수용성 전해질 이차 전지용 양 전극 활물질 및 그 제조 방법, 및 비수용성 전해질 이차 전지
JP6583662B2 (ja) * 2015-05-21 2019-10-02 株式会社Ｇｓユアサ 非水電解質二次電池用正極活物質及び非水電解質二次電池
JP6825559B2 (ja) 2015-05-28 2021-02-03 株式会社Ｇｓユアサ 非水電解質二次電池用正極活物質、その製造方法、非水電解質二次電池用電極及び非水電解質二次電池
DE102015210895A1 (de) * 2015-06-15 2016-12-15 Robert Bosch Gmbh Na-dotiertes und Nb-, W- und/oder Mo-dotiertes HE-NCM
US10109854B2 (en) 2015-09-30 2018-10-23 Panasonic Corporation Positive electrode active material for nonaqueous electrolyte secondary batteries and nonaqueous electrolyte secondary battery
CN108432001B (zh) * 2015-11-11 2021-08-17 住友化学株式会社 正极活性物质的制造方法、正极活性物质、正极和锂离子二次电池
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JP7004959B2 (ja) * 2016-07-14 2022-01-21 株式会社Ｇｓユアサ リチウム遷移金属複合酸化物、遷移金属水酸化物前駆体、遷移金属水酸化物前駆体の製造方法、リチウム遷移金属複合酸化物の製造方法、非水電解質二次電池用正極活物質、非水電解質二次電池用電極、非水電解質二次電池及び蓄電装置
CN106207157A (zh) * 2016-07-20 2016-12-07 北京新能源汽车股份有限公司 掺杂层状锰酸锂及其制备方法和应用
WO2018025795A1 (ja) * 2016-08-04 2018-02-08 株式会社三徳 非水電解質二次電池用正極活物質、並びに該正極活物質を使用した正極及び二次電池
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FR3061903B1 (fr) * 2017-01-19 2019-05-31 Commissariat A L'energie Atomique Et Aux Energies Alternatives Procede de preparation de nanoparticules non agglomerees d'un oxyde lamellaire lithie
JP7191489B2 (ja) * 2017-07-14 2022-12-19 ビーエーエスエフ ソシエタス・ヨーロピア 電極活物質の製造方法
EP3660972B1 (en) * 2017-08-10 2024-06-05 GS Yuasa International Ltd. Non-aqueous electrolyte and non-aqueous electrolyte electricity storage element
DE102017217250A1 (de) * 2017-09-27 2019-03-28 Volkswagen Aktiengesellschaft Stabilisierte Ni-reiche Schichtoxide als Aktivmaterial für positive Elektroden von Lithium-Ionen-Batterien
CN107994221B (zh) * 2017-12-04 2020-03-20 中南大学 一种复相结构层状钠离子电池正极材料及制备方法
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CN112599765A (zh) * 2020-12-18 2021-04-02 西北工业大学 一种钠/钾掺杂的高性能富锂锰镍基正极材料及其制备方法
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