KR100522216B1 - 인산기함유 고체 고분자 전해질 (복합)막 및 그 제조방법 - Google Patents

인산기함유 고체 고분자 전해질 (복합)막 및 그 제조방법 Download PDF

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Publication number
KR100522216B1
KR100522216B1 KR10-2003-7005370A KR20037005370A KR100522216B1 KR 100522216 B1 KR100522216 B1 KR 100522216B1 KR 20037005370 A KR20037005370 A KR 20037005370A KR 100522216 B1 KR100522216 B1 KR 100522216B1
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South Korea
Prior art keywords
unsaturated monomer
group
acid group
polymer electrolyte
fuel cell
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Expired - Fee Related
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KR10-2003-7005370A
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English (en)
Korean (ko)
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KR20030078860A (ko
Inventor
이토이코
리쿠카와마사히로
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캐논 가부시끼가이샤
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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F30/00—Homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and containing phosphorus, selenium, tellurium or a metal
    • C08F30/02—Homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and containing phosphorus, selenium, tellurium or a metal containing phosphorus
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F230/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and containing phosphorus, selenium, tellurium or a metal
    • C08F230/02—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and containing phosphorus, selenium, tellurium or a metal containing phosphorus
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
    • H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
    • H01B1/06—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances
    • H01B1/12—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances organic substances
    • H01B1/122—Ionic conductors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1027—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having carbon, oxygen and other atoms, e.g. sulfonated polyethersulfones [S-PES]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1034—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having phosphorus, e.g. sulfonated polyphosphazenes [S-PPh]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1039—Polymeric electrolyte materials halogenated, e.g. sulfonated polyvinylidene fluorides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1058—Polymeric electrolyte materials characterised by a porous support having no ion-conducting properties
    • H01M8/106—Polymeric electrolyte materials characterised by a porous support having no ion-conducting properties characterised by the chemical composition of the porous support
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. in situ polymerisation or in situ crosslinking
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0082—Organic polymers
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0088—Composites
    • H01M2300/0094—Composites in the form of layered products, e.g. coatings
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T428/00—Stock material or miscellaneous articles
    • Y10T428/249921—Web or sheet containing structurally defined element or component
    • Y10T428/249953—Composite having voids in a component [e.g., porous, cellular, etc.]
    • Y10T428/249962—Void-containing component has a continuous matrix of fibers only [e.g., porous paper, etc.]
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T442/00—Fabric [woven, knitted, or nonwoven textile or cloth, etc.]
    • Y10T442/20—Coated or impregnated woven, knit, or nonwoven fabric which is not [a] associated with another preformed layer or fiber layer or, [b] with respect to woven and knit, characterized, respectively, by a particular or differential weave or knit, wherein the coating or impregnation is neither a foamed material nor a free metal or alloy layer
    • Y10T442/2418—Coating or impregnation increases electrical conductivity or anti-static quality

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  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Electrochemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Health & Medical Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Physics & Mathematics (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Laminated Bodies (AREA)
  • Secondary Cells (AREA)
  • Coating Of Shaped Articles Made Of Macromolecular Substances (AREA)
  • Primary Cells (AREA)
  • Macromonomer-Based Addition Polymer (AREA)
  • Polymerisation Methods In General (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
KR10-2003-7005370A 2000-10-19 2001-10-19 인산기함유 고체 고분자 전해질 (복합)막 및 그 제조방법 Expired - Fee Related KR100522216B1 (ko)

Applications Claiming Priority (5)

Application Number Priority Date Filing Date Title
JPJP-P-2000-00319390 2000-10-19
JP2000319390 2000-10-19
JPJP-P-2001-00204097 2001-07-04
JP2001204097 2001-07-04
PCT/JP2001/009209 WO2002033709A1 (fr) 2000-10-19 2001-10-19 (membranes) composites de polyelectrolytes solides portant des groupes d'acide phosphorique et leurs procedes de production

Publications (2)

Publication Number Publication Date
KR20030078860A KR20030078860A (ko) 2003-10-08
KR100522216B1 true KR100522216B1 (ko) 2005-10-14

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Family Applications (1)

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KR10-2003-7005370A Expired - Fee Related KR100522216B1 (ko) 2000-10-19 2001-10-19 인산기함유 고체 고분자 전해질 (복합)막 및 그 제조방법

Country Status (9)

Country Link
US (2) US7160968B2 (https=)
EP (1) EP1339072B1 (https=)
JP (2) JP4150180B2 (https=)
KR (1) KR100522216B1 (https=)
CN (2) CN101127401A (https=)
AU (3) AU2001295984B2 (https=)
DE (1) DE60137532D1 (https=)
NZ (1) NZ525916A (https=)
WO (1) WO2002033709A1 (https=)

Cited By (2)

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Publication number Priority date Publication date Assignee Title
KR100813515B1 (ko) 2006-09-11 2008-03-17 삼성에스디아이 주식회사 연료전지용 프로톤 전도체 및 이를 채용한 연료전지
KR101284176B1 (ko) * 2011-05-06 2013-07-09 한국과학기술연구원 블록 공중합체 전해질 복합막 및 이의 제조방법

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EP1487041B1 (en) 2002-03-07 2007-04-25 Nitto Denko Corporation Electrolyte film and solid polymer fuel cell using the same
JP3891484B2 (ja) * 2002-09-05 2007-03-14 株式会社ノリタケカンパニーリミテド 電解質膜およびその膜を備えた燃料電池
DE10242106A1 (de) * 2002-09-11 2004-04-15 Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. Phosphorgruppenhaltige Carbonsäurederivate mit organisch polymerisierbaren Gruppen
JP2005005046A (ja) * 2003-06-10 2005-01-06 Canon Inc シロキサン高分子電解質膜及びそれを用いた固体高分子型燃料電池
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KR101065374B1 (ko) * 2004-06-30 2011-09-16 삼성에스디아이 주식회사 연료전지용 고분자 막 및 그 제조방법
JP4573023B2 (ja) * 2004-07-23 2010-11-04 信越化学工業株式会社 燃料電池電解質膜用硬化性樹脂組成物並びに電解質膜、その製造方法及び電解質膜・電極接合体、その製造方法
JP5049459B2 (ja) * 2004-08-02 2012-10-17 ユニケミカル株式会社 ポリアクリロニトリル多孔質膜にリン酸基含有不飽和単量体（組成物）を含浸させ、（共）重合してなる固体高分子電解質複合膜及びその用途
KR100684730B1 (ko) * 2004-10-14 2007-02-20 삼성에스디아이 주식회사 직접 산화형 연료 전지용 고분자 전해질 막, 이의 제조 방법 및 이를 포함하는 직접 산화형 연료 전지 장치
JP5010823B2 (ja) * 2004-10-14 2012-08-29 三星エスディアイ株式会社 直接酸化型燃料電池用高分子電解質膜、その製造方法及びこれを含む直接酸化型燃料電池システム
JP4530847B2 (ja) * 2004-12-28 2010-08-25 ユニケミカル株式会社 リン酸基含有不飽和単量体及びビニル芳香族−共役ジエン系液状オリゴマーを共重合してなる固体高分子電解質膜並びにその用途
KR100712933B1 (ko) 2005-02-18 2007-05-02 대주전자재료 주식회사 고체 고분자 전해질막 및 이를 이용한 연료 전지
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US7517604B2 (en) * 2005-09-19 2009-04-14 3M Innovative Properties Company Fuel cell electrolyte membrane with acidic polymer
KR100693801B1 (ko) * 2005-10-17 2007-03-12 최영수 탱크로리용 밸브개폐장치
GB0615139D0 (en) * 2006-07-29 2006-09-06 Itm Fuel Cells Ltd Alternative membrane production method
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JP5110184B2 (ja) * 2010-10-19 2012-12-26 トヨタ自動車株式会社 ホスホン酸ポリマー、その製造方法及び燃料電池用電解質膜
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JP4491103B2 (ja) * 1999-12-27 2010-06-30 株式会社Kri 多分岐高分子、その製造方法、固体電解質及び電気化学素子
JP4082891B2 (ja) * 2001-11-07 2008-04-30 ユニケミカル株式会社 リン酸基含有重合体を含有する固体高分子電解質複合膜及びコーティング剤

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
KR100813515B1 (ko) 2006-09-11 2008-03-17 삼성에스디아이 주식회사 연료전지용 프로톤 전도체 및 이를 채용한 연료전지
KR101284176B1 (ko) * 2011-05-06 2013-07-09 한국과학기술연구원 블록 공중합체 전해질 복합막 및 이의 제조방법
US8802319B2 (en) 2011-05-06 2014-08-12 Korea Institute Of Science And Technology Block copolymer electrolyte composite membranes and methods of producing the same

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AU2001295984B2 (en) 2007-09-20
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JP2003086021A (ja) 2003-03-20
US20040044160A1 (en) 2004-03-04
CN101127401A (zh) 2008-02-20
WO2002033709A1 (fr) 2002-04-25
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AU2007205760B2 (en) 2009-10-01
US20060293475A1 (en) 2006-12-28
JP4685886B2 (ja) 2011-05-18
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AU2007205760A1 (en) 2007-08-30
EP1339072B1 (en) 2009-01-21
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AU9598401A (en) 2002-04-29
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NZ525916A (en) 2006-03-31

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