JP3565425B2 - 窒化ケイ素質粉末の製造方法および窒化ケイ素質焼結体の製造方法 - Google Patents
窒化ケイ素質粉末の製造方法および窒化ケイ素質焼結体の製造方法 Download PDFInfo
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- JP3565425B2 JP3565425B2 JP2000284957A JP2000284957A JP3565425B2 JP 3565425 B2 JP3565425 B2 JP 3565425B2 JP 2000284957 A JP2000284957 A JP 2000284957A JP 2000284957 A JP2000284957 A JP 2000284957A JP 3565425 B2 JP3565425 B2 JP 3565425B2
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- silicon nitride
- powder
- sintered body
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- thermal conductivity
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- 229910052581 Si3N4 Inorganic materials 0.000 title claims description 138
- HQVNEWCFYHHQES-UHFFFAOYSA-N silicon nitride Chemical compound N12[Si]34N5[Si]62N3[Si]51N64 HQVNEWCFYHHQES-UHFFFAOYSA-N 0.000 title claims description 132
- 239000000843 powder Substances 0.000 title claims description 91
- 238000004519 manufacturing process Methods 0.000 title claims description 20
- 239000002245 particle Substances 0.000 claims description 48
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 claims description 36
- 239000001301 oxygen Substances 0.000 claims description 36
- 229910052760 oxygen Inorganic materials 0.000 claims description 36
- 238000000034 method Methods 0.000 claims description 26
- AXZKOIWUVFPNLO-UHFFFAOYSA-N magnesium;oxygen(2-) Chemical compound [O-2].[Mg+2] AXZKOIWUVFPNLO-UHFFFAOYSA-N 0.000 claims description 24
- 239000000395 magnesium oxide Substances 0.000 claims description 23
- CPLXHLVBOLITMK-UHFFFAOYSA-N magnesium oxide Inorganic materials [Mg]=O CPLXHLVBOLITMK-UHFFFAOYSA-N 0.000 claims description 23
- 229910052761 rare earth metal Inorganic materials 0.000 claims description 23
- 238000010438 heat treatment Methods 0.000 claims description 20
- 238000005245 sintering Methods 0.000 claims description 20
- IJGRMHOSHXDMSA-UHFFFAOYSA-N nitrogen Substances N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 claims description 16
- 229910052769 Ytterbium Inorganic materials 0.000 claims description 11
- 239000002994 raw material Substances 0.000 claims description 11
- 229910052727 yttrium Inorganic materials 0.000 claims description 11
- 239000012298 atmosphere Substances 0.000 claims description 10
- 238000006243 chemical reaction Methods 0.000 claims description 8
- 229910052757 nitrogen Inorganic materials 0.000 claims description 8
- 239000011230 binding agent Substances 0.000 claims description 4
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 claims description 3
- 229910004298 SiO 2 Inorganic materials 0.000 claims description 3
- 239000007789 gas Substances 0.000 claims description 3
- 238000000227 grinding Methods 0.000 claims description 3
- 239000001257 hydrogen Substances 0.000 claims description 3
- 229910052739 hydrogen Inorganic materials 0.000 claims description 3
- 230000001590 oxidative effect Effects 0.000 claims description 3
- 150000001875 compounds Chemical class 0.000 claims description 2
- 230000007704 transition Effects 0.000 claims description 2
- QJGQUHMNIGDVPM-UHFFFAOYSA-N nitrogen group Chemical group [N] QJGQUHMNIGDVPM-UHFFFAOYSA-N 0.000 claims 1
- 239000000758 substrate Substances 0.000 description 25
- 238000005452 bending Methods 0.000 description 11
- 229910052746 lanthanum Inorganic materials 0.000 description 10
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- VYPSYNLAJGMNEJ-UHFFFAOYSA-N silicon dioxide Inorganic materials O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 description 9
- 229910052782 aluminium Inorganic materials 0.000 description 8
- 239000000377 silicon dioxide Substances 0.000 description 8
- 229910052681 coesite Inorganic materials 0.000 description 7
- 229910052906 cristobalite Inorganic materials 0.000 description 7
- 238000010304 firing Methods 0.000 description 7
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- 229910052751 metal Inorganic materials 0.000 description 7
- 239000002184 metal Substances 0.000 description 7
- 229910052682 stishovite Inorganic materials 0.000 description 7
- 229910052905 tridymite Inorganic materials 0.000 description 7
- 229910052742 iron Inorganic materials 0.000 description 6
- 238000013001 point bending Methods 0.000 description 6
- RYGMFSIKBFXOCR-UHFFFAOYSA-N Copper Chemical compound [Cu] RYGMFSIKBFXOCR-UHFFFAOYSA-N 0.000 description 5
- 239000011248 coating agent Substances 0.000 description 5
- 238000000576 coating method Methods 0.000 description 5
- 229910052802 copper Inorganic materials 0.000 description 5
- 239000010949 copper Substances 0.000 description 5
- PMHQVHHXPFUNSP-UHFFFAOYSA-M copper(1+);methylsulfanylmethane;bromide Chemical compound Br[Cu].CSC PMHQVHHXPFUNSP-UHFFFAOYSA-M 0.000 description 5
- 230000007423 decrease Effects 0.000 description 5
- 239000000463 material Substances 0.000 description 5
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- 229910052684 Cerium Inorganic materials 0.000 description 4
- 229910052692 Dysprosium Inorganic materials 0.000 description 4
- 229910052688 Gadolinium Inorganic materials 0.000 description 4
- 238000000354 decomposition reaction Methods 0.000 description 4
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- 230000000694 effects Effects 0.000 description 4
- 229910052710 silicon Inorganic materials 0.000 description 4
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- 238000012360 testing method Methods 0.000 description 4
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 3
- XUIMIQQOPSSXEZ-UHFFFAOYSA-N Silicon Chemical compound [Si] XUIMIQQOPSSXEZ-UHFFFAOYSA-N 0.000 description 3
- YXFVVABEGXRONW-UHFFFAOYSA-N Toluene Chemical compound CC1=CC=CC=C1 YXFVVABEGXRONW-UHFFFAOYSA-N 0.000 description 3
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 description 3
- 229910052799 carbon Inorganic materials 0.000 description 3
- 239000000919 ceramic Substances 0.000 description 3
- 238000001816 cooling Methods 0.000 description 3
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- 229910052749 magnesium Inorganic materials 0.000 description 3
- 239000011812 mixed powder Substances 0.000 description 3
- 238000002156 mixing Methods 0.000 description 3
- 238000000465 moulding Methods 0.000 description 3
- 239000012299 nitrogen atmosphere Substances 0.000 description 3
- 238000012545 processing Methods 0.000 description 3
- NIQCNGHVCWTJSM-UHFFFAOYSA-N Dimethyl phthalate Chemical compound COC(=O)C1=CC=CC=C1C(=O)OC NIQCNGHVCWTJSM-UHFFFAOYSA-N 0.000 description 2
- 229910052691 Erbium Inorganic materials 0.000 description 2
- LFQSCWFLJHTTHZ-UHFFFAOYSA-N Ethanol Chemical compound CCO LFQSCWFLJHTTHZ-UHFFFAOYSA-N 0.000 description 2
- 229910052689 Holmium Inorganic materials 0.000 description 2
- LRHPLDYGYMQRHN-UHFFFAOYSA-N N-Butanol Chemical compound CCCCO LRHPLDYGYMQRHN-UHFFFAOYSA-N 0.000 description 2
- 229910052779 Neodymium Inorganic materials 0.000 description 2
- 229910052772 Samarium Inorganic materials 0.000 description 2
- HCHKCACWOHOZIP-UHFFFAOYSA-N Zinc Chemical compound [Zn] HCHKCACWOHOZIP-UHFFFAOYSA-N 0.000 description 2
- 230000002159 abnormal effect Effects 0.000 description 2
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- 229910052725 zinc Inorganic materials 0.000 description 2
- 239000011701 zinc Substances 0.000 description 2
- PZZOEXPDTYIBPI-UHFFFAOYSA-N 2-[[2-(4-hydroxyphenyl)ethylamino]methyl]-3,4-dihydro-2H-naphthalen-1-one Chemical compound C1=CC(O)=CC=C1CCNCC1C(=O)C2=CC=CC=C2CC1 PZZOEXPDTYIBPI-UHFFFAOYSA-N 0.000 description 1
- KXLUWEYBZBGJRZ-POEOZHCLSA-N Canin Chemical compound O([C@H]12)[C@]1([C@](CC[C@H]1C(=C)C(=O)O[C@@H]11)(C)O)[C@@H]1[C@@]1(C)[C@@H]2O1 KXLUWEYBZBGJRZ-POEOZHCLSA-N 0.000 description 1
- GPFVKTQSZOQXLY-UHFFFAOYSA-N Chrysartemin A Natural products CC1(O)C2OC2C34OC3(C)CC5C(CC14)OC(=O)C5=C GPFVKTQSZOQXLY-UHFFFAOYSA-N 0.000 description 1
- 229910052693 Europium Inorganic materials 0.000 description 1
- CWYNVVGOOAEACU-UHFFFAOYSA-N Fe2+ Chemical compound [Fe+2] CWYNVVGOOAEACU-UHFFFAOYSA-N 0.000 description 1
- 229910052765 Lutetium Inorganic materials 0.000 description 1
- 229910052777 Praseodymium Inorganic materials 0.000 description 1
- 229910000831 Steel Inorganic materials 0.000 description 1
- 229910052775 Thulium Inorganic materials 0.000 description 1
- 238000002441 X-ray diffraction Methods 0.000 description 1
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- 150000001412 amines Chemical class 0.000 description 1
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- 229910052788 barium Inorganic materials 0.000 description 1
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- FBSAITBEAPNWJG-UHFFFAOYSA-N dimethyl phthalate Natural products CC(=O)OC1=CC=CC=C1OC(C)=O FBSAITBEAPNWJG-UHFFFAOYSA-N 0.000 description 1
- 229960001826 dimethylphthalate Drugs 0.000 description 1
- 229910001873 dinitrogen Inorganic materials 0.000 description 1
- 238000010292 electrical insulation Methods 0.000 description 1
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- 239000010959 steel Substances 0.000 description 1
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Priority Applications (9)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
JP2000284957A JP3565425B2 (ja) | 2000-09-20 | 2000-09-20 | 窒化ケイ素質粉末の製造方法および窒化ケイ素質焼結体の製造方法 |
DE2001165080 DE10165080B4 (de) | 2000-09-20 | 2001-09-19 | Siliciumnitrid-Pulver und -Sinterkörper sowie Verfahren zu deren Herstellung und Leiterplatte damit |
DE10146227.1A DE10146227B4 (de) | 2000-09-20 | 2001-09-19 | Siliciumnitrid-Sinterkörper, Leiterplatte und thermoelektrisches Modul |
DE10165107.4A DE10165107B3 (de) | 2000-09-20 | 2001-09-19 | Substrat mit Siliciumnitrid-Sinterkörper und Leiterplatte |
KR1020010058380A KR100833962B1 (ko) | 2000-09-20 | 2001-09-20 | 질화규소 분말, 질화규소 소결체, 질화규소 소결체 기판,및 그 질화규소 소결체 기판을 포함한 회로기판 및열전소자 모듈 |
CNB011379634A CN1192989C (zh) | 2000-09-20 | 2001-09-20 | 氮化硅粉、其烧结体、基板、及由此的电路板和热电元件模块 |
US09/956,033 US6846765B2 (en) | 2000-09-20 | 2001-09-20 | Silicon nitride powder, silicon nitride sintered body, sintered silicon nitride substrate, and circuit board and thermoelectric module comprising such sintered silicon nitride substrate |
US10/998,657 US7031166B2 (en) | 2000-09-20 | 2004-11-30 | Silicon nitride powder, silicon nitride sintered body, sintered silicon nitride substrate, and circuit board and thermoelectric module comprising such sintered silicon nitride substrate |
KR1020070095109A KR100836150B1 (ko) | 2000-09-20 | 2007-09-19 | 질화규소 소결체, 질화규소 소결체의 제조 방법 및 질화규소 소결체 기판, 이러한 질화 규소 소결체 기판을 포함하는 회로 기판 |
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JP2000284957A JP3565425B2 (ja) | 2000-09-20 | 2000-09-20 | 窒化ケイ素質粉末の製造方法および窒化ケイ素質焼結体の製造方法 |
Related Child Applications (1)
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JP2004130790A Division JP4089974B2 (ja) | 2004-04-27 | 2004-04-27 | 窒化ケイ素質粉末、窒化ケイ素質焼結体及びこれを用いた電子部品用回路基板 |
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JP2002097005A JP2002097005A (ja) | 2002-04-02 |
JP2002097005A5 JP2002097005A5 (enrdf_load_stackoverflow) | 2004-08-05 |
JP3565425B2 true JP3565425B2 (ja) | 2004-09-15 |
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JP2000284957A Expired - Lifetime JP3565425B2 (ja) | 2000-09-20 | 2000-09-20 | 窒化ケイ素質粉末の製造方法および窒化ケイ素質焼結体の製造方法 |
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Families Citing this family (18)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP3797905B2 (ja) * | 2000-10-27 | 2006-07-19 | 株式会社東芝 | 窒化けい素セラミックス基板およびそれを用いた窒化けい素セラミックス回路基板並びにその製造方法 |
JP4518020B2 (ja) * | 2005-12-26 | 2010-08-04 | 日立金属株式会社 | 窒化ケイ素質焼結体およびそれを用いた回路基板。 |
JP5200741B2 (ja) * | 2007-08-01 | 2013-06-05 | 三菱化学株式会社 | 結晶性窒化珪素及びその製造方法、並びに、それを用いた蛍光体、該蛍光体含有組成物、発光装置、照明装置、画像表示装置、焼結体及び顔料 |
US9184595B2 (en) | 2008-09-27 | 2015-11-10 | Witricity Corporation | Wireless energy transfer in lossy environments |
US8324759B2 (en) | 2008-09-27 | 2012-12-04 | Witricity Corporation | Wireless energy transfer using magnetic materials to shape field and reduce loss |
US8304935B2 (en) | 2008-09-27 | 2012-11-06 | Witricity Corporation | Wireless energy transfer using field shaping to reduce loss |
EP2377839B1 (en) | 2009-01-13 | 2016-10-26 | Hitachi Metals, Ltd. | Silicon nitride substrate manufacturing method |
JP2010173877A (ja) * | 2009-01-28 | 2010-08-12 | Taiheiyo Cement Corp | 窒化珪素焼結体 |
JP5289090B2 (ja) * | 2009-02-16 | 2013-09-11 | 太平洋セメント株式会社 | セラミックス部材 |
JP5910498B2 (ja) * | 2010-08-04 | 2016-05-11 | 宇部興産株式会社 | 珪窒化物蛍光体用窒化珪素粉末並びにそれを用いたCaAlSiN3系蛍光体、Sr2Si5N8系蛍光体、(Sr,Ca)AlSiN3系蛍光体及びLa3Si6N11系蛍光体、及びその製造方法 |
KR101762473B1 (ko) | 2010-08-19 | 2017-07-27 | 우베 고산 가부시키가이샤 | 규질화물 형광체용 질화규소 분말 및 그것을 이용한 Sr3Al3Si13O2N21계 형광체, β-사이알론 형광체, 그리고 그들의 제조방법 |
WO2012090542A1 (ja) * | 2010-12-28 | 2012-07-05 | 宇部興産株式会社 | 多結晶シリコンインゴット鋳造用鋳型及びその製造方法並びに多結晶シリコンインゴット鋳造用鋳型の離型材用窒化珪素粉末及びそれを含有したスラリー |
CN103842473B (zh) * | 2011-10-12 | 2016-02-10 | 宇部兴产株式会社 | 氧氮化物荧光体粉末、氧氮化物荧光体粉末制造用氮化硅粉末及氧氮化物荧光体粉末的制造方法 |
KR101794410B1 (ko) * | 2015-08-17 | 2017-11-07 | 한국과학기술원 | 고 열전도도 질화규소 소결체 및 이의 제조 방법 |
JP6729224B2 (ja) * | 2015-11-26 | 2020-07-22 | 三菱マテリアル株式会社 | セラミックス/アルミニウム接合体、絶縁回路基板、パワーモジュール、ledモジュール、熱電モジュール |
KR102067144B1 (ko) * | 2017-06-26 | 2020-01-16 | 주식회사 엘지화학 | 질화규소 소결체의 제조 방법, 질화규소 소결체 및 이를 이용한 방열 기판 |
KR101901172B1 (ko) * | 2018-05-23 | 2018-09-27 | (주)존인피니티 | 전기절연성이 우수한 고열전도성 질화규소 세라믹스 기판 |
WO2023176500A1 (ja) * | 2022-03-16 | 2023-09-21 | 株式会社 東芝 | 窒化珪素焼結体およびそれを用いた耐摩耗性部材 |
Family Cites Families (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JPH0829923B2 (ja) * | 1989-12-07 | 1996-03-27 | 電気化学工業株式会社 | 窒化ケイ素粉末 |
JP3486642B2 (ja) * | 1992-11-27 | 2004-01-13 | 独立行政法人物質・材料研究機構 | 窒化ケイ素原料粉末の高純度化処理方法 |
JP3501317B2 (ja) * | 1995-07-21 | 2004-03-02 | 日産自動車株式会社 | 高熱伝導率窒化ケイ素質焼結体および窒化ケイ素質焼結体製絶縁基板 |
JPH11349381A (ja) * | 1998-06-08 | 1999-12-21 | Hitachi Metals Ltd | 窒化ケイ素焼結体およびそれからなるスパッタターゲット |
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- 2000-09-20 JP JP2000284957A patent/JP3565425B2/ja not_active Expired - Lifetime
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