WO2009069797A1 - ポリアミック酸溶液の製造方法およびポリアミック酸溶液 - Google Patents

ポリアミック酸溶液の製造方法およびポリアミック酸溶液 Download PDF

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Publication number
WO2009069797A1
WO2009069797A1 PCT/JP2008/071778 JP2008071778W WO2009069797A1 WO 2009069797 A1 WO2009069797 A1 WO 2009069797A1 JP 2008071778 W JP2008071778 W JP 2008071778W WO 2009069797 A1 WO2009069797 A1 WO 2009069797A1
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WIPO (PCT)
Prior art keywords
acid solution
polyamic acid
component
tetracarboxylic acid
diamine component
Prior art date
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PCT/JP2008/071778
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English (en)
French (fr)
Inventor
Takeshige Nakayama
Seiichirou Takabayashi
Tooru Murakami
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Ube Industries, Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Publication date
Application filed by Ube Industries, Ltd. filed Critical Ube Industries, Ltd.
Priority to CN200880125661XA priority Critical patent/CN101925633B/zh
Priority to JP2009543893A priority patent/JP5445136B2/ja
Priority to EP08855223A priority patent/EP2223954A4/en
Priority to US12/745,217 priority patent/US8816017B2/en
Publication of WO2009069797A1 publication Critical patent/WO2009069797A1/ja

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1003—Preparatory processes
    • C08G73/1007—Preparatory processes from tetracarboxylic acids or derivatives and diamines
    • C08G73/1028—Preparatory processes from tetracarboxylic acids or derivatives and diamines characterised by the process itself, e.g. steps, continuous
    • C08G73/1032—Preparatory processes from tetracarboxylic acids or derivatives and diamines characterised by the process itself, e.g. steps, continuous characterised by the solvent(s) used
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1003—Preparatory processes
    • C08G73/1007—Preparatory processes from tetracarboxylic acids or derivatives and diamines
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1003—Preparatory processes
    • C08G73/1007—Preparatory processes from tetracarboxylic acids or derivatives and diamines
    • C08G73/1028—Preparatory processes from tetracarboxylic acids or derivatives and diamines characterised by the process itself, e.g. steps, continuous
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1042—Copolyimides derived from at least two different tetracarboxylic compounds or two different diamino compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1046—Polyimides containing oxygen in the form of ether bonds in the main chain
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1046—Polyimides containing oxygen in the form of ether bonds in the main chain
    • C08G73/105—Polyimides containing oxygen in the form of ether bonds in the main chain with oxygen only in the diamino moiety
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1067—Wholly aromatic polyimides, i.e. having both tetracarboxylic and diamino moieties aromatically bound
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
    • C08G73/1067—Wholly aromatic polyimides, i.e. having both tetracarboxylic and diamino moieties aromatically bound
    • C08G73/1071—Wholly aromatic polyimides containing oxygen in the form of ether bonds in the main chain

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Macromolecular Compounds Obtained By Forming Nitrogen-Containing Linkages In General (AREA)

Abstract

　２０～８０モル％のパラフェニレンジアミンと８０～２０モル％のジアミノジフェニルエーテルとからなるジアミン成分と、１０～６０モル％の２，３，３’，４’－ビフェニルテトラカルボン酸二無水物と９０～４０モル％の３，３’，４，４’－ビフェニルテトラカルボン酸二無水物とからなるテトラカルボン酸成分とを溶媒中で反応させてポリアミック酸溶液を製造する方法であって、 　ジアミン成分と前記ジアミン成分に対して過剰モル量のテトラカルボン酸成分とを、前記テトラカルボン酸成分に対して１／３モル倍を越える量の水を含有する溶媒中で反応してポリアミック酸溶液を調製する前工程と、次いで、前記ポリアミック酸溶液へジアミン成分とテトラカルボン酸成分とが実質的に等モル量になるようにジアミン成分、又はジアミン成分及びテトラカルボン酸成分を加えて更に反応する後工程とを含むことを特徴とするポリアミック酸溶液を製造する方法に関する。
PCT/JP2008/071778 2007-11-29 2008-12-01 ポリアミック酸溶液の製造方法およびポリアミック酸溶液 WO2009069797A1 (ja)

Priority Applications (4)

Application Number Priority Date Filing Date Title
CN200880125661XA CN101925633B (zh) 2007-11-29 2008-12-01 用于制备聚酰胺酸溶液的方法和聚酰胺酸溶液
JP2009543893A JP5445136B2 (ja) 2007-11-29 2008-12-01 ポリアミック酸溶液の製造方法およびポリアミック酸溶液
EP08855223A EP2223954A4 (en) 2007-11-29 2008-12-01 PROCESS FOR PREPARING POLYAMIDE ACID SOLUTION AND POLYAMIDE ACID SOLUTION
US12/745,217 US8816017B2 (en) 2007-11-29 2008-12-01 Process for producing polyamic acid solution and polyamic acid solution

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007-308640 2007-11-29
JP2007308640 2007-11-29

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WO2009069797A1 true WO2009069797A1 (ja) 2009-06-04

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Country Status (6)

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US (1) US8816017B2 (ja)
EP (1) EP2223954A4 (ja)
JP (1) JP5445136B2 (ja)
KR (1) KR101540827B1 (ja)
CN (1) CN101925633B (ja)
WO (1) WO2009069797A1 (ja)

Cited By (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2009221398A (ja) * 2008-03-18 2009-10-01 Ube Ind Ltd ポリアミック酸溶液組成物、及びポリイミド膜
WO2012133594A1 (ja) * 2011-03-30 2012-10-04 宇部興産株式会社 ポリイミドフィルムおよびそれを用いた金属積層板
JP5409385B2 (ja) * 2007-12-06 2014-02-05 グンゼ株式会社 カーボンブラック分散ポリアミド酸溶液組成物、それを用いた半導電性ポリイミド樹脂ベルトの製造方法及び半導電性ポリイミド樹脂ベルト
WO2016056595A1 (ja) * 2014-10-08 2016-04-14 宇部興産株式会社 ポリイミド前駆体組成物、およびそれを用いた絶縁被覆層の製造方法
JP2017155168A (ja) * 2016-03-03 2017-09-07 日立化成デュポンマイクロシステムズ株式会社 樹脂組成物及びポリイミド樹脂膜
WO2022031303A1 (en) * 2020-08-07 2022-02-10 Zymergen Inc. Process for polyimide synthesis and polyimides made therefrom
JP7104162B2 (ja) 2017-11-10 2022-07-20 ピーアイ・アドバンスド・マテリアルズ・カンパニー・リミテッド 導体被覆用ポリアミック酸組成物

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WO2010150513A1 (ja) * 2009-06-23 2010-12-29 キヤノン株式会社 電極構造体及び蓄電デバイス
TWI569970B (zh) * 2011-06-14 2017-02-11 宇部興產股份有限公司 聚醯亞胺疊層體之製造方法及聚醯亞胺疊層體
KR102276288B1 (ko) * 2013-11-25 2021-07-12 삼성전자주식회사 폴리이미드 제조용 조성물, 폴리이미드, 상기 폴리이미드를 포함하는 성형품, 및 상기 성형품을 포함하는 디스플레이 장치
KR101847140B1 (ko) 2017-06-27 2018-04-10 한국화학연구원 고분자형 아민계 에폭시 수지 경화제와 이의 제조방법 및 이를 포함하는 에폭시 수지 조성물
CN113088076B (zh) * 2019-12-23 2022-09-06 中国科学院宁波材料技术与工程研究所 一种高性能聚酰亚胺模塑粉、其制备方法与应用
CN116145428A (zh) * 2022-12-05 2023-05-23 东华大学 一种水溶性聚酰胺酸盐上浆剂的制备方法和应用

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JPS5638324A (en) * 1979-09-06 1981-04-13 Ube Ind Ltd Preparation of polyimide solution
JPS57131248A (en) 1981-02-05 1982-08-14 Ube Ind Ltd Polyamic acid solution composition and preparation thereof
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JPS59204619A (ja) 1983-05-09 1984-11-20 Ube Ind Ltd 芳香族ポリアミツク酸溶液組成物
JPS61258836A (ja) * 1985-05-10 1986-11-17 Hitachi Chem Co Ltd ポリアミド酸溶液の製造方法
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JPS5638324A (en) * 1979-09-06 1981-04-13 Ube Ind Ltd Preparation of polyimide solution
JPS57131248A (en) 1981-02-05 1982-08-14 Ube Ind Ltd Polyamic acid solution composition and preparation thereof
JPS59164328A (ja) 1983-03-08 1984-09-17 Ube Ind Ltd 芳香族ポリアミツク酸溶液組成物
JPS59204619A (ja) 1983-05-09 1984-11-20 Ube Ind Ltd 芳香族ポリアミツク酸溶液組成物
JPS61258836A (ja) * 1985-05-10 1986-11-17 Hitachi Chem Co Ltd ポリアミド酸溶液の製造方法
JPS62115887A (ja) * 1985-11-15 1987-05-27 日東電工株式会社 フレキシブル印刷回路基板
JPH1180352A (ja) * 1997-09-12 1999-03-26 Ube Ind Ltd 貯蔵安定性の改良された耐熱性コ−ティング組成物およびポリイミド膜
WO2008059801A1 (fr) * 2006-11-13 2008-05-22 Ube Industries, Ltd. Procédé de fabrication d'une solution d'acide polyamide et solution d'acide polyamique

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Title
See also references of EP2223954A4 *

Cited By (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP5409385B2 (ja) * 2007-12-06 2014-02-05 グンゼ株式会社 カーボンブラック分散ポリアミド酸溶液組成物、それを用いた半導電性ポリイミド樹脂ベルトの製造方法及び半導電性ポリイミド樹脂ベルト
JP2009221398A (ja) * 2008-03-18 2009-10-01 Ube Ind Ltd ポリアミック酸溶液組成物、及びポリイミド膜
WO2012133594A1 (ja) * 2011-03-30 2012-10-04 宇部興産株式会社 ポリイミドフィルムおよびそれを用いた金属積層板
JPWO2012133594A1 (ja) * 2011-03-30 2014-07-28 宇部興産株式会社 ポリイミドフィルムおよびそれを用いた金属積層板
JP5904202B2 (ja) * 2011-03-30 2016-04-13 宇部興産株式会社 ポリイミドフィルムおよびそれを用いた金属積層板
WO2016056595A1 (ja) * 2014-10-08 2016-04-14 宇部興産株式会社 ポリイミド前駆体組成物、およびそれを用いた絶縁被覆層の製造方法
JP2017155168A (ja) * 2016-03-03 2017-09-07 日立化成デュポンマイクロシステムズ株式会社 樹脂組成物及びポリイミド樹脂膜
JP7104162B2 (ja) 2017-11-10 2022-07-20 ピーアイ・アドバンスド・マテリアルズ・カンパニー・リミテッド 導体被覆用ポリアミック酸組成物
WO2022031303A1 (en) * 2020-08-07 2022-02-10 Zymergen Inc. Process for polyimide synthesis and polyimides made therefrom

Also Published As

Publication number Publication date
CN101925633A (zh) 2010-12-22
JP5445136B2 (ja) 2014-03-19
US20100305295A1 (en) 2010-12-02
EP2223954A4 (en) 2012-10-31
KR101540827B1 (ko) 2015-07-30
CN101925633B (zh) 2013-10-30
KR20100098659A (ko) 2010-09-08
JPWO2009069797A1 (ja) 2011-04-21
EP2223954A1 (en) 2010-09-01
US8816017B2 (en) 2014-08-26

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