JP6727855B2 - 蓄電装置 - Google Patents
蓄電装置 Download PDFInfo
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- JP6727855B2 JP6727855B2 JP2016039614A JP2016039614A JP6727855B2 JP 6727855 B2 JP6727855 B2 JP 6727855B2 JP 2016039614 A JP2016039614 A JP 2016039614A JP 2016039614 A JP2016039614 A JP 2016039614A JP 6727855 B2 JP6727855 B2 JP 6727855B2
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- Prior art keywords
- positive electrode
- negative electrode
- sample
- active material
- power storage
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- 238000002076 thermal analysis method Methods 0.000 description 1
- QHGNHLZPVBIIPX-UHFFFAOYSA-N tin(II) oxide Inorganic materials [Sn]=O QHGNHLZPVBIIPX-UHFFFAOYSA-N 0.000 description 1
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- 229910000314 transition metal oxide Inorganic materials 0.000 description 1
- WFKWXMTUELFFGS-UHFFFAOYSA-N tungsten Chemical compound [W] WFKWXMTUELFFGS-UHFFFAOYSA-N 0.000 description 1
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Classifications
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- H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
- H01G11/54—Electrolytes
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- H01G11/62—Liquid electrolytes characterised by the solute, e.g. salts, anions or cations therein
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- H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
- H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
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- H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
- H01G11/04—Hybrid capacitors
- H01G11/06—Hybrid capacitors with one of the electrodes allowing ions to be reversibly doped thereinto, e.g. lithium ion capacitors [LIC]
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- H—ELECTRICITY
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- H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
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- H01M4/36—Selection of substances as active materials, active masses, active liquids
- H01M4/58—Selection of substances as active materials, active masses, active liquids of inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy; of polyanionic structures, e.g. phosphates, silicates or borates
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- H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
- H01G11/10—Multiple hybrid or EDL capacitors, e.g. arrays or modules
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- H—ELECTRICITY
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- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M2300/00—Electrolytes
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- H01M2300/0091—Composites in the form of mixtures
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- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/10—Energy storage using batteries
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/13—Energy storage using capacitors
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
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- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
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- Inorganic Chemistry (AREA)
- Materials Engineering (AREA)
- Physics & Mathematics (AREA)
- Condensed Matter Physics & Semiconductors (AREA)
- General Physics & Mathematics (AREA)
- Secondary Cells (AREA)
- Electric Double-Layer Capacitors Or The Like (AREA)
- Cell Separators (AREA)
- Battery Electrode And Active Subsutance (AREA)
- Primary Cells (AREA)
Description
本実施の形態では、本発明の一態様の蓄電装置について図1〜図7を用いて説明する。
セパレータは、単層構造であっても積層構造であってもよい。例えば、ポリフェニレンサルファイドを有するセパレータと、他のセパレータと、の積層構造であってもよい。
電解液は、イオン液体及びアルカリ金属塩を有する。電解液は他の材料を含んでいてもよい。また、複数種のイオン液体やアルカリ金属塩を含んでいてもよい。
集電体は、蓄電装置内で顕著な化学変化を引き起こさずに高い導電性を示す限り、特別な制限はない。正極集電体及び負極集電体には、例えば、ステンレス、金、白金、亜鉛、鉄、ニッケル、銅、アルミニウム、チタン、タンタル、マンガン等の金属、これらの合金、又は焼結した炭素などをそれぞれ用いることができる。または、銅もしくはステンレス鋼を炭素、ニッケルもしくはチタン等で被覆して用いてもよい。または、シリコン、チタン、ネオジム、スカンジウム、モリブデンなどの耐熱性を向上させる元素が添加されたアルミニウム合金を用いることができる。または、シリコンと反応してシリサイドを形成する金属元素で集電体を形成してもよい。シリコンと反応してシリサイドを形成する金属元素としては、ジルコニウム、チタン、ハフニウム、バナジウム、ニオブ、タンタル、クロム、モリブデン、タングステン、コバルト、ニッケル等がある。
活物質層は、活物質を含む。活物質とは、キャリアであるイオンの挿入・脱離に関わる物質のみを指すが、本明細書等では、本来「活物質」である材料に加えて、導電助剤や結着剤などを含めたものも、活物質層と呼ぶ。
外装体509は、電解液508と接する面、すなわち内側の面が電解液508と顕著な反応を生じないことが好ましい。また、電池セル500の外部から電池セル500内に水分が混入すると、電解液508の成分等と水との反応が生じる場合がある。よって外装体509は、水分の透過性が低いことが好ましい。
本実施の形態では、本発明の一態様の蓄電装置について図8〜図15を用いて説明する。
図8及び図9に、本発明の一態様の蓄電装置である、捲回体を用いた蓄電池の構成例を示す。
次に、捲回体を用いた蓄電池の一例として、円筒型の蓄電池を示す。
図12に、本発明の一態様の蓄電装置である、コイン型の蓄電池の一例を示す。図12(A)はコイン型(単層偏平型)の蓄電池の外観図であり、図12(B)、(C)は、その断面図の一例である。
次に、蓄電システムの構造例について、図13〜図15を用いて説明する。ここで蓄電システムとは、例えば、蓄電装置を搭載した機器を指す。本実施の形態で説明する蓄電システムは、本発明の一態様の蓄電装置を有する。
本実施の形態では、本発明の一態様である、可撓性を有する蓄電装置について、図16〜図23を用いて説明する。本発明の一態様の蓄電装置は、湾曲した形状であってもよい。また、本発明の一態様の蓄電装置は、可撓性を有し、湾曲した状態と湾曲していない状態の双方の状態において使用できてもよい。
図16(A)に二次電池200の斜視図を示し、図16(B)に二次電池200の上面図を示す。
図20(A)に二次電池250の斜視図を示し、図20(B)に二次電池250の上面図を示す。また、図20(C1)に第1の電極組立体230の断面図を示し、図20(C2)に第2の電極組立体231の断面図を示す。
本実施の形態では、本発明の一態様の蓄電装置の使用例について図24〜図27を用いて説明する。
負極の作製方法は、本実施例の試料全てにおいて共通である。
正極の作製方法は、試料1A、比較試料1C、及び比較試料1Dの3つにおいては共通である。なお、試料1Bのみ作製方法が異なるため、後述する。
正極活物質には比表面積15.6m2/gのLiFePO4を用い、結着剤としてPVdFを用い、導電助剤としてグラフェンを用いた。なお、グラフェンは、スラリーを作製する際には酸化グラフェンであり、電極塗布後に還元処理を施した。LiFePO4、PVdF、及びグラフェンの配合は、LiFePO4:酸化グラフェン:PVdF=94.2:0.8:5.0(wt%)とした。
負極活物質に比表面積6.3m2/g、平均粒径15μmの球状化天然黒鉛を用いた。また、結着剤としてCMC−Na及びSBRを用いた。用いたCMC−Naの重合度は600〜800、1%水溶液として用いた場合の水溶液粘度は300mPa・s〜500mPa・sの範囲の値であった。導電助剤として気相成長炭素繊維(VGCF(登録商標):Vapor−Grown Carbon Fiber)を用いた。黒鉛、VGCF(登録商標)、CMC−Na、及びSBRの配合は、黒鉛:VGCF(登録商標):CMC−Na:SBR=95:2:1.5:1.5(wt%)とした。
正極活物質には比表面積15.6m2/gのLiFePO4を用い、結着剤としてPVdFを用い、導電助剤としてグラフェンを用いた。なお、グラフェンは、スラリーを作製する際には酸化グラフェンであり、電極塗布後に還元処理を施した。LiFePO4、PVdF、及びグラフェンの配合は、LiFePO4:酸化グラフェン:PVdF=94.4:0.6:5.0(wt%)とした。
正極活物質には平均粒子径10μmのLiCoO2を用い、結着剤としてPVdFを用い、導電助剤としてアセチレンブラックを用いた。LiCoO2、PVdF、及びアセチレンブラックの配合は、LiCoO2:アセチレンブラック:PVdF=90:5:5(wt%)とした。
上記実施例で用いたHMI−FSAの合成例について説明する。
1H NMR(CDCl3,300MHz):δ=0.86−0.91(m、3H)、1.33−1.37(m、6H)、1.83−1.91(m、2H)、3.96(s、3H)、4.18(t、J=7.8Hz、2H)、7.27−7.30(m、2H)、8.66(s、1H)。
11 フィルム
12 正極集電体
13 セパレータ
14 負極集電体
18 正極活物質層
19 負極活物質層
102 活物質層
115 封止層
118 接合部
119 導入口
200 二次電池
203 セパレータ
203a 領域
203b 領域
207 外装体
211 正極
211a 正極
215 負極
215a 負極
220 封止層
221 正極リード
225 負極リード
230 電極組立体
231 電極組立体
250 二次電池
281 タブ領域
282 タブ領域
300 蓄電池
301 正極缶
302 負極缶
303 ガスケット
304 正極
305 正極集電体
306 正極活物質層
307 負極
308 負極集電体
309 負極活物質層
310 セパレータ
500 電池セル
501 正極集電体
502 正極活物質層
503 正極
504 負極集電体
505 負極活物質層
506 負極
507 セパレータ
508 電解液
509 外装体
510 正極リード
511 負極リード
512 接合部
513 湾曲部
514 接合部
600 蓄電池
601 正極キャップ
602 電池缶
603 正極端子
604 正極
605 セパレータ
606 負極
607 負極端子
608 絶縁板
609 絶縁板
611 PTC素子
612 安全弁機構
900 回路基板
910 ラベル
911 端子
912 回路
913 蓄電池
914 アンテナ
915 アンテナ
916 層
917 層
918 アンテナ
919 端子
920 表示装置
921 センサ
922 端子
951 端子
952 端子
980 蓄電池
981 フィルム
982 フィルム
990 蓄電池
991 外装体
992 外装体
993 捲回体
994 負極
995 正極
996 セパレータ
997 端子
998 端子
1200 蓄電装置
7100 携帯表示装置
7101 筐体
7102 表示部
7103 操作ボタン
7104 蓄電装置
7110 携帯情報端末
7111 筐体
7112 表示部
7113 操作ボタン
7114 蓄電装置
7200 携帯情報端末
7201 筐体
7202 表示部
7203 バンド
7204 バックル
7205 操作ボタン
7206 入出力端子
7207 アイコン
7300 表示装置
7304 表示部
7400 携帯電話機
7401 筐体
7402 表示部
7403 操作ボタン
7404 外部接続ポート
7405 スピーカ
7406 マイク
7407 蓄電装置
8000 表示装置
8001 筐体
8002 表示部
8003 スピーカ部
8004 蓄電装置
8021 充電装置
8022 ケーブル
8100 照明装置
8101 筐体
8102 光源
8103 蓄電装置
8104 天井
8105 側壁
8106 床
8107 窓
8200 室内機
8201 筐体
8202 送風口
8203 蓄電装置
8204 室外機
8300 電気冷凍冷蔵庫
8301 筐体
8302 冷蔵室用扉
8303 冷凍室用扉
8304 蓄電装置
8400 自動車
8401 ヘッドライト
8500 自動車
9600 タブレット型端末
9625 スイッチ
9626 スイッチ
9627 電源スイッチ
9628 操作スイッチ
9629 留め具
9630 筐体
9631 表示部
9631a 表示部
9631b 表示部
9632a 領域
9632b 領域
9633 太陽電池
9634 充放電制御回路
9635 蓄電体
9636 DCDCコンバータ
9637 コンバータ
9638 操作キー
9639 ボタン
9640 可動部
Claims (7)
- 正極、負極、セパレータ、及び電解液を有し、
前記セパレータは、前記正極と前記負極の間に位置し、
前記セパレータは、ポリフェニレンサルファイドを有し、
前記正極は、グラフェンを有し、
前記電解液は、イオン液体及びアルカリ金属塩を有する、蓄電装置。 - 請求項1において、
前記アルカリ金属塩は、リチウムビス(フルオロスルホニル)アミドである、蓄電装置。 - 請求項1又は2において、
前記イオン液体は、カチオン及びアニオンを有し、
前記カチオンは、1以上の置換基を有する5員環のヘテロ芳香環を有し、
前記1以上の置換基が有する炭素数の合計が2以上10以下である、蓄電装置。 - 請求項3において、
前記カチオンは、1−ブチル−3−メチルイミダゾリウムカチオンである、蓄電装置。 - 請求項1乃至4のいずれか一項において、
前記負極は、黒鉛を有する、蓄電装置。 - 請求項1乃至5のいずれか一項に記載の蓄電装置であり、
可撓性を有する、蓄電装置。 - 請求項1乃至6のいずれか一項に記載の蓄電装置であり、
0℃における放電容量が、25℃における放電容量の80%以上であり、
100℃における放電容量が、25℃における放電容量の80%以上である、蓄電装置。
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-
2016
- 2016-02-29 US US15/056,353 patent/US20160268064A1/en not_active Abandoned
- 2016-03-02 JP JP2016039614A patent/JP6727855B2/ja active Active
- 2016-03-04 KR KR1020160026098A patent/KR102530983B1/ko active IP Right Grant
- 2016-03-08 CN CN202210549336.8A patent/CN114824652A/zh active Pending
- 2016-03-08 CN CN201610131079.0A patent/CN105958002A/zh active Pending
- 2016-10-04 JP JP2016196361A patent/JP6096364B2/ja active Active
-
2020
- 2020-07-01 JP JP2020113891A patent/JP2020170715A/ja not_active Withdrawn
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2022
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JP6096364B2 (ja) | 2017-03-15 |
US20160268064A1 (en) | 2016-09-15 |
CN105958002A (zh) | 2016-09-21 |
JP2016207641A (ja) | 2016-12-08 |
JP2022119877A (ja) | 2022-08-17 |
KR20160110131A (ko) | 2016-09-21 |
JP7365454B2 (ja) | 2023-10-19 |
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