JP2015516499A - 導電性ダイ取付けフィルムの接着を改善するための鎖延長されたエポキシ - Google Patents
導電性ダイ取付けフィルムの接着を改善するための鎖延長されたエポキシ Download PDFInfo
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- JP2015516499A JP2015516499A JP2015512653A JP2015512653A JP2015516499A JP 2015516499 A JP2015516499 A JP 2015516499A JP 2015512653 A JP2015512653 A JP 2015512653A JP 2015512653 A JP2015512653 A JP 2015512653A JP 2015516499 A JP2015516499 A JP 2015516499A
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- IISBACLAFKSPIT-UHFFFAOYSA-N CC(C)(c(cc1)ccc1O)c(cc1)ccc1O Chemical compound CC(C)(c(cc1)ccc1O)c(cc1)ccc1O IISBACLAFKSPIT-UHFFFAOYSA-N 0.000 description 1
- RXNYJUSEXLAVNQ-UHFFFAOYSA-N Oc(cc1)ccc1C(c(cc1)ccc1O)=O Chemical compound Oc(cc1)ccc1C(c(cc1)ccc1O)=O RXNYJUSEXLAVNQ-UHFFFAOYSA-N 0.000 description 1
- QIGBRXMKCJKVMJ-UHFFFAOYSA-N Oc(cc1)ccc1O Chemical compound Oc(cc1)ccc1O QIGBRXMKCJKVMJ-UHFFFAOYSA-N 0.000 description 1
- VPWNQTHUCYMVMZ-UHFFFAOYSA-N Oc(cc1)ccc1S(c(cc1)ccc1O)(=O)=O Chemical compound Oc(cc1)ccc1S(c(cc1)ccc1O)(=O)=O VPWNQTHUCYMVMZ-UHFFFAOYSA-N 0.000 description 1
- VWGKEVWFBOUAND-UHFFFAOYSA-N Oc(cc1)ccc1Sc(cc1)ccc1O Chemical compound Oc(cc1)ccc1Sc(cc1)ccc1O VWGKEVWFBOUAND-UHFFFAOYSA-N 0.000 description 1
- PXKLMJQFEQBVLD-UHFFFAOYSA-N Oc1ccc(Cc(cc2)ccc2O)cc1 Chemical compound Oc1ccc(Cc(cc2)ccc2O)cc1 PXKLMJQFEQBVLD-UHFFFAOYSA-N 0.000 description 1
- GHMLBKRAJCXXBS-UHFFFAOYSA-N Oc1cccc(O)c1 Chemical compound Oc1cccc(O)c1 GHMLBKRAJCXXBS-UHFFFAOYSA-N 0.000 description 1
Classifications
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- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J9/00—Adhesives characterised by their physical nature or the effects produced, e.g. glue sticks
- C09J9/02—Electrically-conducting adhesives
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G59/00—Polycondensates containing more than one epoxy group per molecule; Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups
- C08G59/18—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing
- C08G59/182—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing using pre-adducts of epoxy compounds with curing agents
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
- C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
- C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
- C08G73/12—Unsaturated polyimide precursors
- C08G73/124—Unsaturated polyimide precursors the unsaturated precursors containing oxygen in the form of ether bonds in the main chain
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
- C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
- C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
- C08G73/12—Unsaturated polyimide precursors
- C08G73/125—Unsaturated polyimide precursors the unsaturated precursors containing atoms other than carbon, hydrogen, oxygen or nitrogen in the main chain
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
- C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
- C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
- C08G73/12—Unsaturated polyimide precursors
- C08G73/126—Unsaturated polyimide precursors the unsaturated precursors being wholly aromatic
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G73/00—Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
- C08G73/06—Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
- C08G73/10—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
- C08G73/12—Unsaturated polyimide precursors
- C08G73/126—Unsaturated polyimide precursors the unsaturated precursors being wholly aromatic
- C08G73/127—Unsaturated polyimide precursors the unsaturated precursors being wholly aromatic containing oxygen in the form of ether bonds in the main chain
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/10—Metal compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L63/00—Compositions of epoxy resins; Compositions of derivatives of epoxy resins
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J163/00—Adhesives based on epoxy resins; Adhesives based on derivatives of epoxy resins
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J179/00—Adhesives based on macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing nitrogen, with or without oxygen, or carbon only, not provided for in groups C09J161/00 - C09J177/00
- C09J179/04—Polycondensates having nitrogen-containing heterocyclic rings in the main chain; Polyhydrazides; Polyamide acids or similar polyimide precursors
- C09J179/08—Polyimides; Polyester-imides; Polyamide-imides; Polyamide acids or similar polyimide precursors
- C09J179/085—Unsaturated polyimide precursors
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- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Health & Medical Sciences (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Adhesives Or Adhesive Processes (AREA)
- Conductive Materials (AREA)
Abstract
Description
A.芳香族エポキシ(式中、nは、0〜25の範囲の値を有する。)(58wt%)
得られた鎖延長されたエポキシでは、総エポキシ官能基(芳香族エポキシおよび脂肪族エポキシの両方に由来)のフェノール官能基に対するモル比は1.4であり、芳香族エポキシの脂肪族エポキシに対するモル比は0.5である。
Claims (14)
- (i)熱硬化性樹脂と、
(ii)任意に、フィルム形成性樹脂と、
(iii)導電性充填剤と、
(iv)多官能性フェノールと多官能性芳香族エポキシおよび多官能性脂肪族エポキシの混合物との反応から調製される鎖延長されたエポキシと、
を含む導電性接着剤組成物。 - 前記鎖延長されたエポキシが、総組成物の1〜20wt%の量で、前記組成物中に存在する、請求項1に記載の導電性接着剤組成物。
- 前記鎖延長されたエポキシ中の、総エポキシ官能基の前記フェノール官能基に対する化学量論比が、0.05〜30の範囲である、請求項1に記載の導電性接着剤組成物。
- 前記熱硬化性樹脂が、4,4’−ジフェニルメタンビスマレイミド、4,4’−ジフェニルエーテルビスマレイミド、4,4’−ジフェニルスルホンビスマレイミド、フェニルメタンマレイミド、m−フェニレンビスマレイミド、2,2’−ビス[4−(4−マレイミドフェノキシ)フェニル]プロパン、3,3’−ジメチル−5,5’−ジエチル−4,4’−ジフェニルメタンビスマレイミド、4−メチル−1,3−フェニレンビスマレイミド、1,6’−ビスマレイミド−(2,2,4−トリメチル)ヘキサン、1,3−ビス(3−マレイミドフェノキシ)ベンゼンおよび1,3−ビス(4−マレイミドフェノキシ)ベンゼンからなる群より選択されるビスマレイミドである、請求項1に記載の導電性接着剤組成物。
- 前記熱硬化性樹脂が、総組成物の約0.5wt%〜約40wt%の量で存在する、請求項1に記載の導電性接着剤組成物。
- 前記フィルム形成性樹脂が存在し、カルボキシ末端ブタジエンアクリロニトリルおよび液体または粘性エポキシ樹脂の付加体、ポリ[メタクリル酸メチル]−b−ポリ(アクリル酸ブチル)−b−ポリ[メタクリル酸メチル]、ポリ[スチレン−b−ポリブタジエン−b−ポリ[メタクリル酸メチル]、ブタジエンゴムおよびスチレンゴムからなる群より選択される、請求項1に記載の導電性接着剤組成物。
- 前記フィルム形成性樹脂が、総組成物の最大約30wt%の量で、前記導電性組成物中に存在する、請求項11に記載の導電性接着剤組成物。
- 前記導電性充填剤が、カーボンブラック、グラファイト、金、銀、銅、白金、パラジウム、ニッケル、アルミニウム、銀めっき銅、銀めっきアルミニウム、ビスマス、スズ、ビスマス−スズ合金、銀めっきファイバー、炭化ケイ素、窒化ホウ素、ダイヤモンド、アルミナおよび合金42からなる群より選択される、請求項1に記載の導電性接着剤組成物。
- 前記導電性充填剤が、総組成物の80wt%以上の量で、前記導電性組成物中に存在する、請求項1に記載の導電性接着剤組成物。
Applications Claiming Priority (5)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US201261648284P | 2012-05-17 | 2012-05-17 | |
US61/648,284 | 2012-05-17 | ||
US13/833,322 US9200184B2 (en) | 2012-05-17 | 2013-03-15 | Chain extended epoxy to improve adhesion of conductive die attach film |
US13/833,322 | 2013-03-15 | ||
PCT/US2013/035405 WO2013172993A1 (en) | 2012-05-17 | 2013-04-05 | Chain extended epoxy to improve adhesion of conductive die attach film |
Publications (3)
Publication Number | Publication Date |
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JP2015516499A true JP2015516499A (ja) | 2015-06-11 |
JP2015516499A5 JP2015516499A5 (ja) | 2016-01-21 |
JP5956068B2 JP5956068B2 (ja) | 2016-07-20 |
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Application Number | Title | Priority Date | Filing Date |
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JP2015512653A Active JP5956068B2 (ja) | 2012-05-17 | 2013-04-05 | 導電性ダイ取付けフィルムの接着を改善するための鎖延長されたエポキシ |
Country Status (7)
Country | Link |
---|---|
US (1) | US9200184B2 (ja) |
EP (1) | EP2850146B1 (ja) |
JP (1) | JP5956068B2 (ja) |
KR (1) | KR101617988B1 (ja) |
CN (1) | CN104302724B (ja) |
TW (1) | TWI530548B (ja) |
WO (1) | WO2013172993A1 (ja) |
Cited By (6)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP5972489B1 (ja) * | 2016-02-10 | 2016-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP5972490B1 (ja) * | 2016-02-10 | 2016-08-17 | 古河電気工業株式会社 | 導電性接着剤組成物ならびにこれを用いた導電性接着フィルムおよびダイシング・ダイボンディングフィルム |
JP5989928B1 (ja) * | 2016-02-10 | 2016-09-07 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP6005312B1 (ja) * | 2016-02-10 | 2016-10-12 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP6005313B1 (ja) * | 2016-02-10 | 2016-10-12 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
KR20180070595A (ko) * | 2015-10-15 | 2018-06-26 | 헨켈 아이피 앤드 홀딩 게엠베하 | 접착제 제제에서 전도성 충전제로서 니켈 및 니켈 함유 합금의 용도 |
Families Citing this family (5)
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CN104371623A (zh) * | 2014-11-13 | 2015-02-25 | 无锡中洁能源技术有限公司 | 一种导热导电胶剂及其制备方法 |
EP3294799A4 (en) * | 2015-05-08 | 2018-11-21 | Henkel IP & Holding GmbH | Sinterable films and pastes and methods for the use thereof |
JP6563700B2 (ja) * | 2015-06-10 | 2019-08-21 | 京セラ株式会社 | 半導体接着用樹脂組成物、半導体接着用シート及びそれを用いた半導体装置 |
EP3540025B1 (en) | 2016-11-10 | 2023-09-13 | Kyocera Corporation | Semiconductor-bonding resin composition, semiconductor-bonding sheet, and semiconductor device using semiconductor-bonding sheet |
JP2019173023A (ja) * | 2019-06-03 | 2019-10-10 | 京セラ株式会社 | 半導体接着用シート及びそれを用いた半導体装置 |
Citations (2)
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JPH04339883A (ja) * | 1991-05-16 | 1992-11-26 | Hitachi Chem Co Ltd | 導電性エポキシ接着フィルム |
KR20090055394A (ko) * | 2007-11-28 | 2009-06-02 | (주)에버텍엔터프라이즈 | 저습성 및 고신뢰성을 갖는 다이 접착용 전기 전도성 접착조성물 |
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-
2013
- 2013-03-15 US US13/833,322 patent/US9200184B2/en active Active
- 2013-04-05 EP EP13790039.5A patent/EP2850146B1/en active Active
- 2013-04-05 KR KR1020147031763A patent/KR101617988B1/ko active IP Right Grant
- 2013-04-05 JP JP2015512653A patent/JP5956068B2/ja active Active
- 2013-04-05 WO PCT/US2013/035405 patent/WO2013172993A1/en active Application Filing
- 2013-04-05 CN CN201380025636.5A patent/CN104302724B/zh active Active
- 2013-04-29 TW TW102115306A patent/TWI530548B/zh active
Patent Citations (2)
Publication number | Priority date | Publication date | Assignee | Title |
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JPH04339883A (ja) * | 1991-05-16 | 1992-11-26 | Hitachi Chem Co Ltd | 導電性エポキシ接着フィルム |
KR20090055394A (ko) * | 2007-11-28 | 2009-06-02 | (주)에버텍엔터프라이즈 | 저습성 및 고신뢰성을 갖는 다이 접착용 전기 전도성 접착조성물 |
Cited By (19)
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KR20180070595A (ko) * | 2015-10-15 | 2018-06-26 | 헨켈 아이피 앤드 홀딩 게엠베하 | 접착제 제제에서 전도성 충전제로서 니켈 및 니켈 함유 합금의 용도 |
KR102645616B1 (ko) * | 2015-10-15 | 2024-03-11 | 헨켈 아게 운트 코. 카게아아 | 접착제 제제에서 전도성 충전제로서 니켈 및 니켈 함유 합금의 용도 |
JP2018538381A (ja) * | 2015-10-15 | 2018-12-27 | ヘンケル アイピー アンド ホールディング ゲゼルシャフト ミット ベシュレンクテル ハフツング | 接着剤配合物中の伝導性充填材としてのニッケル及びニッケル含有合金の使用 |
WO2017138255A1 (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP2017141364A (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP2017141365A (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
WO2017138256A1 (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着剤組成物ならびにこれを用いた導電性接着フィルムおよびダイシング・ダイボンディングフィルム |
JP2017141367A (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着剤組成物ならびにこれを用いた導電性接着フィルムおよびダイシング・ダイボンディングフィルム |
JP5972489B1 (ja) * | 2016-02-10 | 2016-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
WO2017138254A1 (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP6005313B1 (ja) * | 2016-02-10 | 2016-10-12 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP2017141366A (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP2017141363A (ja) * | 2016-02-10 | 2017-08-17 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP6005312B1 (ja) * | 2016-02-10 | 2016-10-12 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
JP5989928B1 (ja) * | 2016-02-10 | 2016-09-07 | 古河電気工業株式会社 | 導電性接着フィルムおよびこれを用いたダイシング・ダイボンディングフィルム |
US11136479B2 (en) | 2016-02-10 | 2021-10-05 | Furukawa Electric Co., Ltd. | Electrically conductive adhesive film and dicing-die bonding film using the same |
US11230649B2 (en) | 2016-02-10 | 2022-01-25 | Furukawa Electric Co., Ltd. | Electrically conductive adhesive film and dicing-die bonding film using the same |
US11306225B2 (en) | 2016-02-10 | 2022-04-19 | Furukawa Electric Co., Ltd. | Electrically conductive adhesive agent composition, and electrically conductive adhesive film and dicing-die-bonding film using the same |
JP5972490B1 (ja) * | 2016-02-10 | 2016-08-17 | 古河電気工業株式会社 | 導電性接着剤組成物ならびにこれを用いた導電性接着フィルムおよびダイシング・ダイボンディングフィルム |
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Publication number | Publication date |
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TWI530548B (zh) | 2016-04-21 |
KR101617988B1 (ko) | 2016-05-03 |
JP5956068B2 (ja) | 2016-07-20 |
CN104302724A (zh) | 2015-01-21 |
EP2850146A1 (en) | 2015-03-25 |
WO2013172993A1 (en) | 2013-11-21 |
CN104302724B (zh) | 2017-06-16 |
EP2850146B1 (en) | 2019-02-13 |
US20130306916A1 (en) | 2013-11-21 |
EP2850146A4 (en) | 2015-12-16 |
KR20150018786A (ko) | 2015-02-24 |
US9200184B2 (en) | 2015-12-01 |
TW201402771A (zh) | 2014-01-16 |
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