BG61038B1 - Катализирани катионактивни лакови свързващи вещества, техно- логии за производството им и тяхното приложение - Google Patents
Катализирани катионактивни лакови свързващи вещества, техно- логии за производството им и тяхното приложение Download PDFInfo
- Publication number
- BG61038B1 BG61038B1 BG99193A BG9919394A BG61038B1 BG 61038 B1 BG61038 B1 BG 61038B1 BG 99193 A BG99193 A BG 99193A BG 9919394 A BG9919394 A BG 9919394A BG 61038 B1 BG61038 B1 BG 61038B1
- Authority
- BG
- Bulgaria
- Prior art keywords
- bismuth
- lacquer
- parts
- lacquer binders
- acid
- Prior art date
Links
Classifications
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
- C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
- C09D5/44—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes for electrophoretic applications
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
- C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
- C09D5/44—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes for electrophoretic applications
- C09D5/4488—Cathodic paints
- C09D5/4492—Cathodic paints containing special additives, e.g. grinding agents
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G59/00—Polycondensates containing more than one epoxy group per molecule; Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups
- C08G59/18—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing
- C08G59/68—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing characterised by the catalysts used
- C08G59/681—Metal alcoholates, phenolates or carboxylates
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/04—Oxygen-containing compounds
- C08K5/09—Carboxylic acids; Metal salts thereof; Anhydrides thereof
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/04—Oxygen-containing compounds
- C08K5/09—Carboxylic acids; Metal salts thereof; Anhydrides thereof
- C08K5/098—Metal salts of carboxylic acids
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
- C09D133/00—Coating compositions based on homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Coating compositions based on derivatives of such polymers
- C09D133/04—Homopolymers or copolymers of esters
- C09D133/06—Homopolymers or copolymers of esters of esters containing only carbon, hydrogen and oxygen, the oxygen atom being present only as part of the carboxyl radical
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
- C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
- C09D5/02—Emulsion paints including aerosols
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Life Sciences & Earth Sciences (AREA)
- Health & Medical Sciences (AREA)
- Wood Science & Technology (AREA)
- Materials Engineering (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Molecular Biology (AREA)
- Dispersion Chemistry (AREA)
- Paints Or Removers (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
AT0112292A AT397820B (de) | 1992-05-29 | 1992-05-29 | Katalysatorhältige kationische lackbindemittel, verfahren zu ihrer herstellung und ihre verwendung |
AT0257192A AT399889B (de) | 1992-12-24 | 1992-12-24 | Verfahren zur herstellung von katalysatorhältigen lackbindemitteln und deren verwendung |
PCT/AT1993/000091 WO1993024578A2 (de) | 1992-05-29 | 1993-05-27 | Katalysierte kationische lackbindemittel, verfahren zu ihrer herstellung und ihre verwendung |
Publications (2)
Publication Number | Publication Date |
---|---|
BG99193A BG99193A (bg) | 1995-09-29 |
BG61038B1 true BG61038B1 (bg) | 1996-09-30 |
Family
ID=25594960
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
BG99193A BG61038B1 (bg) | 1992-05-29 | 1994-11-18 | Катализирани катионактивни лакови свързващи вещества, техно- логии за производството им и тяхното приложение |
Country Status (22)
Country | Link |
---|---|
US (1) | US5554700A (zh) |
EP (1) | EP0642558B2 (zh) |
JP (1) | JP2951406B2 (zh) |
KR (1) | KR0157077B1 (zh) |
CN (1) | CN1034281C (zh) |
AU (1) | AU666385B2 (zh) |
BG (1) | BG61038B1 (zh) |
BR (1) | BR9306440A (zh) |
CA (1) | CA2118124C (zh) |
CZ (1) | CZ282509B6 (zh) |
DE (1) | DE59303987D1 (zh) |
ES (1) | ES2092824T5 (zh) |
GR (1) | GR3021166T3 (zh) |
HU (1) | HU216086B (zh) |
MX (1) | MX9303117A (zh) |
PL (1) | PL171420B1 (zh) |
RO (1) | RO115061B1 (zh) |
RU (1) | RU2109783C1 (zh) |
SI (1) | SI9300285B (zh) |
SK (1) | SK279801B6 (zh) |
UA (1) | UA42691C2 (zh) |
WO (1) | WO1993024578A2 (zh) |
Families Citing this family (51)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE4330002C1 (de) * | 1993-09-04 | 1995-03-23 | Herberts Gmbh | Verfahren zur Lackierung von metallischen Substraten und Anwendung des Verfahrens |
AT398987B (de) * | 1993-09-07 | 1995-02-27 | Vianova Kunstharz Ag | Verfahren zur herstellung von wismutsalze enthaltenden zubereitungen und deren verwendung als katalysatorkomponente in kathodisch abscheidbaren elektrotauchlacken |
TW368523B (en) * | 1994-03-17 | 1999-09-01 | Fry Metals Inc | Bismuth coating protection for copper |
NL9400513A (nl) * | 1994-03-31 | 1995-11-01 | Bichemie Coatings Bv | Toepassing van lactaten bij de bereiding van reversibele bekledingssamenstellingen, de aldus verkregen lactaten bevattende bekledingssamenstellingen, de toepassing van deze bekledingssamenstellingen bij het bekleden van substraten en voortbrengselen, alsmede substraten en voortbrengselen, die met deze bekledingssamenstellingen zijn bekleed. |
DE4423139A1 (de) * | 1994-07-01 | 1996-01-04 | Hoechst Ag | Härtung von kataphoretischen Tauchlacken mit Wismutkatalysatoren |
DE4434593A1 (de) * | 1994-09-28 | 1996-04-04 | Herberts Gmbh | Verfahren zur Herstellung einer korrosionsschützenden, gut haftenden Lackierung und die dabei erhaltenen Werkstücke |
DE19613685C1 (de) * | 1996-04-05 | 1997-09-11 | Herberts Gmbh | Säurefreie Katalysatorpaste, deren Herstellung und Verwendung bei der kathodischen Elektrotauchlackierung |
US5908912A (en) * | 1996-09-06 | 1999-06-01 | Ppg Industries Ohio, Inc. | Electrodepositable coating composition containing bismuth and amino acid materials and electrodeposition method |
WO1998049367A1 (en) | 1997-04-28 | 1998-11-05 | Fry's Metals, Inc. | Bismuth coating protection for copper |
DE69837091D1 (de) * | 1997-07-29 | 2007-03-29 | Kansai Paint Co Ltd | Kationische elektrotauchlackierung-zusammensetzung |
DE69837014T3 (de) | 1997-12-12 | 2012-10-25 | Kansai Paint Co., Ltd. | Cationische elektrotauchlackzusammensetzung |
JPH11279461A (ja) * | 1998-01-29 | 1999-10-12 | Kansai Paint Co Ltd | カチオン電着塗料 |
US5972189A (en) * | 1998-05-29 | 1999-10-26 | Ppg Industries Ohio, Inc. | Electrodepositable coating composition containing bismuth diorganodithiocarbamates and method of electrodeposition |
US6156823A (en) * | 1998-12-04 | 2000-12-05 | E. I. Du Pont De Nemours And Company | Bismuth oxide catalyst for cathodic electrocoating compositions |
DE19908144C1 (de) * | 1999-02-25 | 2000-03-16 | Herberts Gmbh & Co Kg | Kathodisch abscheidbare Tauchlacke, deren Herstellung und Verwendung |
US6190524B1 (en) | 1999-03-26 | 2001-02-20 | Ppg Industries Ohio, Inc. | Organosulfur bismuth compounds and their use in electrodepositable coating compositions |
DE10001222A1 (de) | 2000-01-14 | 2001-08-09 | Basf Coatings Ag | Beschichtung, enthaltend kolloidal verteiltes metallisches Bismut |
AT410442B (de) * | 2001-06-15 | 2003-04-25 | Solutia Austria Gmbh | Wässrige bindemittel |
GB0120598D0 (en) * | 2001-08-24 | 2001-10-17 | Rice Michael J P | A handlebar assembly |
KR20030033680A (ko) * | 2001-10-24 | 2003-05-01 | 허회욱 | 양돈용 무쇠 급이통 |
US6811667B2 (en) * | 2002-03-04 | 2004-11-02 | E. I. Du Pont De Nemours And Company | Cathodic electrodeposition coating agents containing bismuth complexes, preparation and use thereof |
DE10236347A1 (de) * | 2002-08-08 | 2004-02-19 | Basf Coatings Ag | Wäßrige Elektrotauchlacke, ihre Verwendung in Verfahren zur Beschichtung elektrisch leitfähiger Substrate sowie die Verwendung von Bismutverbindungen in diesen wäßrigen Elektrotauchlacken |
DE10236350A1 (de) * | 2002-08-08 | 2004-02-19 | Basf Coatings Ag | Bismutverbindungen enthaltende Elektrotauchlacke (ETL) |
US7374650B2 (en) * | 2002-08-22 | 2008-05-20 | E.I. Du Pont De Nemours & Company | Cathodic electrodeposition coating agents containing bismuth salts together with yttrium and/or neodymium compounds, production and use thereof |
US7351319B2 (en) * | 2003-01-24 | 2008-04-01 | E. I. Du Pont De Nemours & Co. | Cathodic electrodeposition coating compositions containing bismuth compounds and dicarboxylic acids, production and use thereof |
US7632386B2 (en) * | 2003-08-28 | 2009-12-15 | E.I. Du Pont De Nemours And Company | Process for producing coatings on electrically conductive substrates by cathodic electrodeposition coating |
US7211182B2 (en) * | 2003-09-23 | 2007-05-01 | E. I. Du Pont De Nemours And Company | Process for producing coatings on electrically conductive substrates by cathodic electrodeposition coating |
US8389653B2 (en) * | 2006-03-30 | 2013-03-05 | Basf Corporation | Method of catalyzing a reaction to form a urethane coating and a complex for use in the method |
US7867570B2 (en) * | 2006-10-26 | 2011-01-11 | Basf Coatings Gmbh | Method of producing a coating having metal coordinating and film-forming materials |
US7759436B2 (en) * | 2006-10-26 | 2010-07-20 | Basf Coatings Gmbh | Film-former of resin with nonionic metal coordinating structure and crosslinker-reactive group |
US7772334B2 (en) * | 2006-10-26 | 2010-08-10 | Basf Coatings Gmbh | Crosslinker of reactive functional groups and nonionic metal coordinating structure-containing alkyl or aromatic compound |
DE102007038824A1 (de) | 2007-08-16 | 2009-02-19 | Basf Coatings Ag | Einsatz von Bismutsubnitrat in Elektrotauchlacken |
DE102008016220A1 (de) | 2008-03-27 | 2009-10-01 | Basf Coatings Ag | Elektrotauchlacke enthaltend Polymethylenharnstoff |
US9382638B2 (en) | 2008-12-29 | 2016-07-05 | Basf Corporation | Electrocoat composition and process replacing phosphate pretreatment |
US8815066B2 (en) | 2008-12-29 | 2014-08-26 | Basf Coatings Gmbh | Coating composition with phosphorous-containing resins and organometallic compounds |
US8192603B2 (en) * | 2008-12-29 | 2012-06-05 | Basf Coatings Gmbh | Electrocoat composition and process replacing phosphate pretreatment |
US8702943B2 (en) * | 2008-12-29 | 2014-04-22 | Basf Coatings Gmbh | Electrocoat composition and process replacing phosphate pretreatment |
US8961768B2 (en) | 2008-12-29 | 2015-02-24 | Basf Corporation | Metal containing integrated electrocoat for better corrosion resistance |
US20100167071A1 (en) * | 2008-12-29 | 2010-07-01 | Basf Corporation | Pyridine group-containing electrocoat composition with metal oxide |
CN103183608B (zh) * | 2011-12-30 | 2015-02-04 | 广东先导稀材股份有限公司 | 次水杨酸铋的制备方法 |
EP2862905A1 (en) | 2013-10-17 | 2015-04-22 | ALLNEX AUSTRIA GmbH | Cationic water-dilutable binders |
WO2015070931A1 (de) | 2013-11-18 | 2015-05-21 | Basf Coatings Gmbh | Wässrige beschichtungszusammensetzung zur tauchlack-beschichtung elektrisch leitfähiger substrate enthaltend bismut in gelöst vorliegender form |
JP6375385B2 (ja) | 2013-11-18 | 2018-08-15 | ビーエーエスエフ コーティングス ゲゼルシャフト ミット ベシュレンクテル ハフツングBASF Coatings GmbH | 溶解と非溶解両方のビスマスを含む導電性基材のための水性ディップコーティング組成物 |
JP6374016B2 (ja) | 2013-11-18 | 2018-08-15 | ビーエーエスエフ コーティングス ゲゼルシャフト ミット ベシュレンクテル ハフツングBASF Coatings GmbH | Bi(III)含有組成物を使用して導電性基材をディップコーティングするための2段階法 |
ES2662416T3 (es) * | 2013-11-19 | 2018-04-06 | Henkel Ag & Co. Kgaa | Composición acuosa de recubrimiento para el recubrimiento con pintura de inmersión de sustratos eléctricamente conductores que contienen óxido de aluminio |
US9982147B2 (en) | 2013-12-10 | 2018-05-29 | Basf Coatings Gmbh | Aqueous dip-coating composition for electroconductive substrates, comprising bismuth and a phosphorus-containing, amine-blocked compound |
MX2017009782A (es) | 2015-02-10 | 2017-10-27 | Valspar Sourcing Inc | Sistema de electrodeposicion novedoso. |
CN106349451B (zh) * | 2015-07-14 | 2020-11-13 | 罗门哈斯公司 | 用于制备疏水改性环氧烷氨基甲酸酯聚合物的方法 |
JP2018184489A (ja) | 2015-09-25 | 2018-11-22 | 日本ペイント・オートモーティブコーティングス株式会社 | カチオン電着塗料組成物の調製方法 |
MX2021012611A (es) | 2019-04-15 | 2021-11-12 | Basf Coatings Gmbh | Composicion acuosa de recubrimiento por inmersion para sustratos electricamente conductores, que comprende bismuto mas litio. |
US20230193056A1 (en) | 2020-05-25 | 2023-06-22 | Basf Coatings Gmbh | Bismuth Containing Electrocoating Material with Improved Catalytic Activity |
Family Cites Families (18)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JPS538568B2 (zh) † | 1974-09-20 | 1978-03-30 | ||
CA1097449A (en) * | 1975-08-01 | 1981-03-10 | Karl F. Schimmel | Pigment grinding vehicle |
US4009133A (en) * | 1975-08-01 | 1977-02-22 | Ppg Industries, Inc. | Electrodepositable epoxy resins having quaternary groups carrying blocked NCO, and aqueous dispersions |
JPS5218746A (en) * | 1975-08-01 | 1977-02-12 | Ppg Industries Inc | Resin vehicle for cathode electrodeposition |
US4040924A (en) * | 1975-08-01 | 1977-08-09 | Ppg Industries, Inc. | Aqueous cationic electrodeposition of epoxy resins having quaternary groups carrying blocked NCO |
US4007154A (en) * | 1975-08-01 | 1977-02-08 | Ppg Industries, Inc. | Novel pigment paste for cationic electrodeposition |
US4362847A (en) * | 1980-05-22 | 1982-12-07 | Shell Oil Company | Heat-curable thermosetting resin binder compositions comprising a non-acidic resinous compound, a non-acidic polyester cross-linking agent, and a transesterification catalyst |
EP0107089B1 (en) * | 1982-09-30 | 1987-05-06 | Ppg Industries, Inc. | Novel pigment grinding vehicle |
US4485259A (en) * | 1982-09-30 | 1984-11-27 | Ppg Industries, Inc. | Pigment grinding vehicle |
AU547702B2 (en) * | 1982-09-30 | 1985-10-31 | Ppg Industries, Inc. | Amine modified epoxy |
CA1254328A (en) * | 1983-10-17 | 1989-05-16 | William G. Boberski | Water-dispersible polymers containing metal chelating groups |
AT380264B (de) * | 1984-10-22 | 1986-05-12 | Vianova Kunstharz Ag | Verfahren zur herstellung von bindemitteln fuer pigmentpasten fuer wasserverduennbare lacke |
JPH0676567B2 (ja) * | 1986-06-16 | 1994-09-28 | 関西ペイント株式会社 | カチオン電着塗料用樹脂組成物 |
US4715898A (en) * | 1986-06-30 | 1987-12-29 | Ppg Industries, Inc. | Sulfonium resins useful as pigment grinding vehicles in cationic electrodeposition |
AU595938B2 (en) * | 1986-10-16 | 1990-04-12 | Nippon Paint Co., Ltd. | Electrodeposition coating composition |
ZA891937B (en) * | 1988-04-04 | 1990-11-28 | Ppg Industries Inc | Pigment grinding vehicles containing quaternary ammonium and ternary sulfonium groups |
DE3812251A1 (de) † | 1988-04-13 | 1989-10-26 | Herberts Gmbh | Wasserverduennbare bindemittel und deren verwendung fuer ueberzugsmittel insbesondere im kraftfahrzeugbau |
JP2983370B2 (ja) † | 1991-04-16 | 1999-11-29 | 関西ペイント株式会社 | 電着塗料組成物 |
-
1993
- 1993-05-27 JP JP6500009A patent/JP2951406B2/ja not_active Expired - Lifetime
- 1993-05-27 MX MX9303117A patent/MX9303117A/es not_active IP Right Cessation
- 1993-05-27 SK SK1415-94A patent/SK279801B6/sk not_active IP Right Cessation
- 1993-05-27 WO PCT/AT1993/000091 patent/WO1993024578A2/de active IP Right Grant
- 1993-05-27 AU AU42936/93A patent/AU666385B2/en not_active Ceased
- 1993-05-27 BR BR9306440A patent/BR9306440A/pt not_active IP Right Cessation
- 1993-05-27 PL PL93306423A patent/PL171420B1/pl unknown
- 1993-05-27 UA UA94119090A patent/UA42691C2/uk unknown
- 1993-05-27 ES ES93912386T patent/ES2092824T5/es not_active Expired - Lifetime
- 1993-05-27 DE DE59303987T patent/DE59303987D1/de not_active Expired - Lifetime
- 1993-05-27 CZ CZ942796A patent/CZ282509B6/cs not_active IP Right Cessation
- 1993-05-27 US US08/343,448 patent/US5554700A/en not_active Expired - Lifetime
- 1993-05-27 HU HUP9403403A patent/HU216086B/hu not_active IP Right Cessation
- 1993-05-27 EP EP93912386A patent/EP0642558B2/de not_active Expired - Lifetime
- 1993-05-27 KR KR1019940704283A patent/KR0157077B1/ko not_active IP Right Cessation
- 1993-05-27 RO RO94-01897A patent/RO115061B1/ro unknown
- 1993-05-27 CA CA002118124A patent/CA2118124C/en not_active Expired - Lifetime
- 1993-05-27 RU RU94046121A patent/RU2109783C1/ru active
- 1993-05-28 SI SI9300285A patent/SI9300285B/sl not_active IP Right Cessation
- 1993-05-28 CN CN93106492A patent/CN1034281C/zh not_active Expired - Lifetime
-
1994
- 1994-11-18 BG BG99193A patent/BG61038B1/bg unknown
-
1996
- 1996-09-26 GR GR960402411T patent/GR3021166T3/el unknown
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