YU49164B - Fungicidni derivati 2-imidazolin-5-ona i 2-imidazolin-5-tiona - Google Patents

Fungicidni derivati 2-imidazolin-5-ona i 2-imidazolin-5-tiona

Info

Publication number
YU49164B
YU49164B YU109092A YU109092A YU49164B YU 49164 B YU49164 B YU 49164B YU 109092 A YU109092 A YU 109092A YU 109092 A YU109092 A YU 109092A YU 49164 B YU49164 B YU 49164B
Authority
YU
Yugoslavia
Prior art keywords
carbon atoms
group
radical
alkyl
optionally substituted
Prior art date
Application number
YU109092A
Other languages
English (en)
Other versions
YU109092A (sh
Inventor
Guy Lacroix
Raymond Peignier
Regis Pepin
Original Assignee
Bayer Cropscience Sa.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Bayer Cropscience Sa. filed Critical Bayer Cropscience Sa.
Publication of YU109092A publication Critical patent/YU109092A/sh
Publication of YU49164B publication Critical patent/YU49164B/sh

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Classifications

    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D401/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
    • C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
    • C07D401/04—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings directly linked by a ring-member-to-ring-member bond
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
    • A01N43/48—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with two nitrogen atoms as the only ring hetero atoms
    • A01N43/50—1,3-Diazoles; Hydrogenated 1,3-diazoles
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C331/00—Derivatives of thiocyanic acid or of isothiocyanic acid
    • C07C331/16—Isothiocyanates
    • C07C331/18—Isothiocyanates having isothiocyanate groups bound to acyclic carbon atoms
    • C07C331/20—Isothiocyanates having isothiocyanate groups bound to acyclic carbon atoms of a saturated carbon skeleton
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C333/00—Derivatives of thiocarbamic acids, i.e. compounds containing any of the groups, the nitrogen atom not being part of nitro or nitroso groups
    • C07C333/14—Dithiocarbamic acids; Derivatives thereof
    • C07C333/18—Esters of dithiocarbamic acids
    • C07C333/20—Esters of dithiocarbamic acids having nitrogen atoms of dithiocarbamate groups bound to hydrogen atoms or to acyclic carbon atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D233/00—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings
    • C07D233/54—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having two double bonds between ring members or between ring members and non-ring members
    • C07D233/66—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having two double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • C07D233/84—Sulfur atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D233/00—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings
    • C07D233/54—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having two double bonds between ring members or between ring members and non-ring members
    • C07D233/66—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, not condensed with other rings having two double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • C07D233/86—Oxygen and sulfur atoms, e.g. thiohydantoin
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D401/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
    • C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
    • C07D401/06—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D401/00—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
    • C07D401/02—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
    • C07D401/12—Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings linked by a chain containing hetero atoms as chain links
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D405/00—Heterocyclic compounds containing both one or more hetero rings having oxygen atoms as the only ring hetero atoms, and one or more rings having nitrogen as the only ring hetero atom
    • C07D405/02—Heterocyclic compounds containing both one or more hetero rings having oxygen atoms as the only ring hetero atoms, and one or more rings having nitrogen as the only ring hetero atom containing two hetero rings
    • C07D405/06—Heterocyclic compounds containing both one or more hetero rings having oxygen atoms as the only ring hetero atoms, and one or more rings having nitrogen as the only ring hetero atom containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D409/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having sulfur atoms as the only ring hetero atoms
    • C07D409/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having sulfur atoms as the only ring hetero atoms containing two hetero rings
    • C07D409/06—Heterocyclic compounds containing two or more hetero rings, at least one ring having sulfur atoms as the only ring hetero atoms containing two hetero rings linked by a carbon chain containing only aliphatic carbon atoms
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D417/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00
    • C07D417/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings
    • C07D417/12—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings linked by a chain containing hetero atoms as chain links

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Agronomy & Crop Science (AREA)
  • Pest Control & Pesticides (AREA)
  • Plant Pathology (AREA)
  • Health & Medical Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Dentistry (AREA)
  • General Health & Medical Sciences (AREA)
  • Wood Science & Technology (AREA)
  • Zoology (AREA)
  • Environmental Sciences (AREA)
  • Plural Heterocyclic Compounds (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)
  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)
  • Nitrogen Condensed Heterocyclic Rings (AREA)

Abstract

Jedinjenja iz grupe imidazolimoma ili imidazolintiona, naznacena time, sto odgovaraju opstoj formuli I: u kojoj -W je atom sumpora ili kiseonika ili S=O grupa, -A predstavlja O ili S, -n je 0 ili 1, -B predstavlja N(R5) ili O ili S ili C(R5) (R6) ili SO2 ili C=O, -R1 i R2, koji su identicni ili razliciti, predstavljaju: -H, pod uslovom da jedna od dve grupe je razlicita od H, ili -aliki ili haloalkil radikal sa 1 do 6 ugljenikovih atoma, ili -alkoksialkil, alkiltioalkil, alkilsulfonil-alkil, monoalkilaminoalkil, alkenil ili alkinil radikal sa 2 do 6 ugljenikovih atoma, ili -dialkilaminoalkil ili cikloalkil radikal sa 3 do 7 ugljenikovih atoma, ili -aril radikal, koji obuhvata fenil, naftil, tienil, furil, piridil, benzotienil, benzofuril, hinolinil, izohinolinil ili metilendioksifenil, opciono supstituisan sa 1 do 3 grupe izabrane od R7 ili -arilalkil, ariloksialkil, ariltioalkil ili arilsulfonilalkil radikal, izrazi aril i alkil imaju gore navedena znacenja, ili -R1 i R2 mogu obrazovati, sa ugljenikom za koji su vezani na prstenu, jedan karbociklicni ili heterociklicni prsten koji ima od 5 do 7 atoma, koji se mogu spojiti sa fenilom, opciono supstituisanim sa 1 do 3 grupe izabrane od R7; -R3 predstavlja: -alkil grupu sa 1 do 6 ugljenikovih atoma, ili -alkoksialkil, alkiltioalkil, alkilsulfonil-alkil, haloalkil, cijanoalkil, tiocijanato-alkil, oksoalkil, alkenil ili alkinil grupu od 2 do 6 ugljenikovih atoma, ili -dialkilaminalkil, alkoksikarbonilalkil ili N-alkilkarbamoilalkil grupu od 3 do 6 ugljenikovih atoma, ili -N,N-dialkilkarbamoilalkil grupu od 4 do 8 ugljenikovih atoma, ili -arilalkil grupu, alkil deo je radikal od 1 do 6 ugljenikovih atoma i aril deo je fenil, naftil, tienil, furil ili piridil, opciono supstituisan sa 1 do 3 grupe izabrane od R7; -R4 predstavlja: -atom vodonika kada n je 1, ili -alkil grupu od 1 do 6 ugljenikovih atoma, ili -alkoksialkil, alkiltioalkil, haloalkil, cijanoalkil, tiocijanatoalkil, alkenil ili alkinil grupu od 2 do 6 ugljenikovih atoma, ili -dialkilaminoalkil, alkoksikarbonilalkil ili N-alkilkarbamoilalkil grupu od 3 do 6 ugljenikovih atoma, ili -N,N-dialkilkarbamoilalkil grupu od 4 do 8 ugljenikovih atoma ili - aril radikal koji ukljucuje fenil, naftil, tienil, furil, piridil, pirimidil, piridazinil, pirazinil, benzotienil, benzofuril, hinolinil, izohinolinil ili metilendioksifenil, opciono supstituisan sa 1 do 3 grupe izabrane od R7 ili - arilalkil, ariloksialkil, ariltioalkil ili arilsulfonialkil radikal, izrazi aril i aikil imaju gore data znacenja, ili - amino grupa disupstiuisana sa 2 identicne ili razlicite grupe izabrne od: - alkil radikal od 1 do 6 ugljenikovih atoma, - alkoksialkil, alkenil ili alkinil radikal od 3 do 6 atoma ugljenika, - cikloalkil radikal od 3 do 7 atoma ugljenika, - arilalkil, kao sto je gore definisan, fenil ili naftil radikal, opciono supftuisan sa 1 do 3 grupe izabrane od R7, ili - tienilmetil ili furfuril radikal, -pirolidino, piperidino, morfolino ili piperazino grupa opci
YU109092A 1991-12-20 1992-12-18 Fungicidni derivati 2-imidazolin-5-ona i 2-imidazolin-5-tiona YU49164B (sh)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
FR9116200A FR2685328B1 (fr) 1991-12-20 1991-12-20 Derives de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.

Publications (2)

Publication Number Publication Date
YU109092A YU109092A (sh) 1995-10-03
YU49164B true YU49164B (sh) 2004-05-12

Family

ID=9420553

Family Applications (1)

Application Number Title Priority Date Filing Date
YU109092A YU49164B (sh) 1991-12-20 1992-12-18 Fungicidni derivati 2-imidazolin-5-ona i 2-imidazolin-5-tiona

Country Status (32)

Country Link
EP (1) EP0551048B1 (sh)
JP (1) JP3462516B2 (sh)
KR (1) KR100263576B1 (sh)
CN (1) CN1035594C (sh)
AP (1) AP405A (sh)
AT (1) ATE221878T1 (sh)
AU (2) AU651021B2 (sh)
BR (1) BR9204699A (sh)
CA (1) CA2085192C (sh)
CZ (1) CZ287207B6 (sh)
DE (1) DE69232719T2 (sh)
DK (1) DK0551048T3 (sh)
EC (1) ECSP920893A (sh)
EG (1) EG19910A (sh)
ES (1) ES2176186T3 (sh)
FI (1) FI119732B (sh)
FR (1) FR2685328B1 (sh)
HR (1) HRP921456B1 (sh)
HU (1) HU215384B (sh)
IL (2) IL104091A (sh)
MA (1) MA22747A1 (sh)
MX (1) MX9207383A (sh)
MY (1) MY110823A (sh)
NZ (1) NZ245489A (sh)
PL (1) PL170819B1 (sh)
PT (1) PT551048E (sh)
RU (1) RU2111207C1 (sh)
SI (1) SI9200391B (sh)
SK (1) SK283470B6 (sh)
TW (1) TW267928B (sh)
YU (1) YU49164B (sh)
ZA (1) ZA929772B (sh)

Families Citing this family (23)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3931907A1 (de) * 1989-09-25 1991-04-04 Henkel Kgaa Waessriges lackoverspray-schutzcoating fuer spritzkabinen sowie verfahren zu dessen herstellung
FR2685328B1 (fr) * 1991-12-20 1995-12-01 Rhone Poulenc Agrochimie Derives de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.
FR2706455B1 (fr) * 1993-06-18 1995-08-04 Rhone Poulenc Agrochimie Dérivés optiquement actifs de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.
US6002016A (en) * 1991-12-20 1999-12-14 Rhone-Poulenc Agrochimie Fungicidal 2-imidazolin-5-ones and 2-imidazoline-5-thiones
FR2706456B1 (fr) * 1993-06-18 1996-06-28 Rhone Poulenc Agrochimie Dérivés optiquement actifs de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.
FR2698359B1 (fr) * 1992-11-25 1995-10-27 Rhone Poulenc Agrochimie Derives de 2-alkoxy 2-imidazoline-5-ones fongicides.
EP1008589A1 (en) * 1992-05-22 2000-06-14 E.I. Du Pont De Nemours & Company Incorporated Fungicidal imidazolinones
US6008370A (en) * 1992-11-25 1999-12-28 Rhone-Poulenc Agrochimie Fungicidal-2-alkoxy/haloalkoxy-1-(mono- or disubstituted)amino-4,4-disubstituted-2-imidazolin-5-ones
FR2716192B1 (fr) * 1994-02-17 1996-04-12 Rhone Poulenc Agrochimie Dérivés de 2-imidazoline-5-ones fongicides.
AU1892495A (en) * 1994-03-09 1995-09-25 Rhone-Poulenc Agrochimie Pesticide substituted 2-imidazolinones
FR2721022B1 (fr) * 1994-06-10 1996-07-19 Rhone Poulenc Agrochimie Dérivés de 5-imino 2-imidazolines fongicides.
FR2722499B1 (fr) * 1994-07-13 1996-08-23 Rhone Poulenc Agrochimie Nouveaux derives de 2-imidazoline-5-ones fongicides
FR2722652B1 (fr) 1994-07-22 1997-12-19 Rhone Poulenc Agrochimie Composition fongicide comprenant une 2-imidazoline-5-one
JPH09183725A (ja) * 1995-09-01 1997-07-15 Pfizer Inc ガン治療用治療剤
FR2751327A1 (fr) 1996-07-22 1998-01-23 Rhone Poulenc Agrochimie Intermediaires pour la preparation de 2-imidazoline-5-ones
UA61064C2 (uk) * 1997-12-02 2003-11-17 Рон-Пуленк Агро Синергічна фунгіцидна композиція, що містить 2-інідазолін-5-он та спосіб боротьби з фітопатогенними грибками культур
UA70327C2 (uk) 1998-06-08 2004-10-15 Баєр Акціенгезельшафт Спосіб боротьби з фітопатогенними хворобами сільськогосподарських рослин та фунгіцидна композиція
FR2783401B1 (fr) * 1998-09-21 2000-10-20 Rhone Poulenc Agrochimie Nouvelles compositions fongicides
EP1092712A1 (en) * 1999-10-13 2001-04-18 E.I. Du Pont De Nemours And Company Process for preparing fungicidal oxazolidinones and imidazolinones
NZ536029A (en) 2002-04-24 2006-09-29 Basf Ag Alcohol alkoxylates as adjuvants for agrotechnical applications
CN101863835B (zh) * 2010-06-29 2012-10-10 渤海大学 S-取代-5,5-二苯基-2-硫代海因衍生物的合成方法
CN103081915A (zh) * 2011-11-07 2013-05-08 深圳诺普信农化股份有限公司 一种杀菌组合物
EP2622961A1 (en) 2012-02-02 2013-08-07 Bayer CropScience AG Acive compound combinations

Family Cites Families (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2329276A1 (fr) * 1975-10-29 1977-05-27 Roussel Uclaf Nouvelles imidazolidines substituees, procede de preparation, application comme medicament et compositions les renfermant
DE3305203A1 (de) * 1983-02-16 1984-08-16 Bayer Ag, 5090 Leverkusen N-sulfenylierte hydantoine, ein verfahren zu ihrer herstellung und ihre verwendung als mikrobizide
DE3340595A1 (de) * 1983-11-10 1985-05-23 Hoechst Ag, 6230 Frankfurt Imidazolinone, verfahren zu ihrer herstellung und ihre verwendung im pflanzenschutz
WO1988007040A1 (en) * 1987-03-20 1988-09-22 E.I. Du Pont De Nemours And Company Fungicidal aminotriazoles and aminoimidazoles
EP0469061A1 (en) * 1989-04-21 1992-02-05 E.I. Du Pont De Nemours And Company Fungicidal oxazolidinones
PT97078B (pt) * 1990-03-20 1997-07-31 Sanofi Sa Processo para a preparacao de derivados heterociclicos n-substituidos e de composicoes farmaceuticas que os contem
FR2671348B1 (fr) * 1991-01-09 1993-03-26 Roussel Uclaf Nouvelles phenylimidazolidines, leur procede de preparation, leur application comme medicaments et les compositions pharmaceutiques les renfermant.
FR2706456B1 (fr) * 1993-06-18 1996-06-28 Rhone Poulenc Agrochimie Dérivés optiquement actifs de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.
FR2685328B1 (fr) * 1991-12-20 1995-12-01 Rhone Poulenc Agrochimie Derives de 2-imidazoline-5-ones et 2-imidazoline-5-thiones fongicides.
EP1008589A1 (en) * 1992-05-22 2000-06-14 E.I. Du Pont De Nemours & Company Incorporated Fungicidal imidazolinones

Also Published As

Publication number Publication date
SK375392A3 (en) 1995-02-08
MY110823A (en) 1999-05-31
JP3462516B2 (ja) 2003-11-05
EP0551048B1 (fr) 2002-08-07
CN1074215A (zh) 1993-07-14
JPH05271198A (ja) 1993-10-19
PL170819B1 (pl) 1997-01-31
AU671389B2 (en) 1996-08-22
AP9200466A0 (en) 1993-01-31
HU9204030D0 (en) 1993-04-28
KR100263576B1 (ko) 2000-08-01
AU651021B2 (en) 1994-07-07
HUT69748A (en) 1995-09-28
NZ245489A (en) 1996-03-26
SK283470B6 (sk) 2003-08-05
CN1035594C (zh) 1997-08-13
EP0551048A1 (fr) 1993-07-14
HRP921456B1 (en) 2007-04-30
FI119732B (fi) 2009-02-27
IL121465A0 (en) 1998-02-08
AP405A (en) 1995-09-03
HRP921456A2 (en) 1995-08-31
MA22747A1 (fr) 1993-07-01
BR9204699A (pt) 1993-06-22
TW267928B (sh) 1996-01-11
CA2085192C (fr) 2007-02-20
PL297064A1 (en) 1993-12-13
IL104091A (en) 1998-06-15
YU109092A (sh) 1995-10-03
ZA929772B (en) 1993-06-14
AU7449994A (en) 1995-01-05
MX9207383A (es) 1993-06-01
SI9200391A (en) 1993-06-30
HU215384B (hu) 1999-04-28
FI925763A0 (fi) 1992-12-18
CZ375392A3 (en) 1993-09-15
DE69232719T2 (de) 2003-04-03
PT551048E (pt) 2002-12-31
ECSP920893A (es) 1994-02-02
ATE221878T1 (de) 2002-08-15
EG19910A (en) 1996-05-31
DK0551048T3 (da) 2002-12-02
DE69232719D1 (de) 2002-09-12
RU2111207C1 (ru) 1998-05-20
CZ287207B6 (cs) 2000-10-11
FR2685328B1 (fr) 1995-12-01
SI9200391B (sl) 2002-02-28
AU3031092A (en) 1993-07-01
ES2176186T3 (es) 2002-12-01
CA2085192A1 (fr) 1993-06-21
FI925763A (fi) 1993-06-21
FR2685328A1 (fr) 1993-06-25
IL104091A0 (en) 1993-05-13

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