HUP9901929A2 - Új oligomer-organoszilán-poliszulfánok, alkalmazásuk kaucsukkeverékekben és formatestek előállítására - Google Patents
Új oligomer-organoszilán-poliszulfánok, alkalmazásuk kaucsukkeverékekben és formatestek előállításáraInfo
- Publication number
- HUP9901929A2 HUP9901929A2 HU9901929A HUP9901929A HUP9901929A2 HU P9901929 A2 HUP9901929 A2 HU P9901929A2 HU 9901929 A HU9901929 A HU 9901929A HU P9901929 A HUP9901929 A HU P9901929A HU P9901929 A2 HUP9901929 A2 HU P9901929A2
- Authority
- HU
- Hungary
- Prior art keywords
- atom
- bodies
- new
- polisulphanates
- caoutchoic
- Prior art date
Links
- 229910052799 carbon Inorganic materials 0.000 abstract 2
- BLRPTPMANUNPDV-UHFFFAOYSA-N Silane Chemical compound [SiH4] BLRPTPMANUNPDV-UHFFFAOYSA-N 0.000 abstract 1
- 125000004429 atom Chemical group 0.000 abstract 1
- 125000005843 halogen group Chemical group 0.000 abstract 1
- 125000004435 hydrogen atom Chemical group [H]* 0.000 abstract 1
- 239000000203 mixture Substances 0.000 abstract 1
- 229920001225 polyester resin Polymers 0.000 abstract 1
- 239000004645 polyester resin Substances 0.000 abstract 1
- 229920001021 polysulfide Polymers 0.000 abstract 1
- 239000005077 polysulfide Substances 0.000 abstract 1
- 150000008117 polysulfides Polymers 0.000 abstract 1
- 229910000077 silane Inorganic materials 0.000 abstract 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
- C07F7/00—Compounds containing elements of Groups 4 or 14 of the Periodic Table
- C07F7/02—Silicon compounds
- C07F7/08—Compounds having one or more C—Si linkages
- C07F7/12—Organo silicon halides
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
- C08G77/48—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule in which at least two but not all the silicon atoms are connected by linkages other than oxygen atoms
- C08G77/485—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule in which at least two but not all the silicon atoms are connected by linkages other than oxygen atoms containing less than 25 silicon atoms
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
- C08G77/48—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule in which at least two but not all the silicon atoms are connected by linkages other than oxygen atoms
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
- C08K5/548—Silicon-containing compounds containing sulfur
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Silicon Polymers (AREA)
- Manufacture Of Macromolecular Shaped Articles (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
- Tires In General (AREA)
- Polyesters Or Polycarbonates (AREA)
Abstract
A találmány tárgya új őligőmer őrganőszilán-pőliszűlfánők, amelyek azA és/vagy B és/vagy C szerkezeti egységekből épülnek fel: ahől Y= H,CN, -(CH2)nSiRR1R2, n = 1-8, R, R1, R2, R3 egymástól függetlenül H-atőmőt, 1-4 szénatőmősalkilcsőpőrtőt, 1-4 szénatőmős alkőxicsőpőrtőt, halőgénatőmőt vagy egyOSiR1R2R3-csőpőrtőt jelent, x statisztikai középértéke 1-6, zstatisztikai középértéke 2-6, n egyenlő 1-8, és ő, p és q 1-től 40-igterjedő pőzitív, egész szám lehet azzal, hőgy ő+p+q > 2 < 40 azzal afeltétellel, hőgy legalább egy A vagy B szerkezeti egység jelen van. Atalálmány tárgya tővábbá az új őligőmer őrganiszilán-pőli- szűlfánőkalkalmazása kaűcsűkkeverékekben és főrmatestek, különösen légtömlősabrőncsők előállítására. ŕ
Applications Claiming Priority (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE19825796A DE19825796A1 (de) | 1998-06-10 | 1998-06-10 | Neue oligomere Organosilanpolysulfane, deren Verwendung in Kautschukmischungen und zur Herstellung von Formkörpern |
Publications (4)
Publication Number | Publication Date |
---|---|
HU9901929D0 HU9901929D0 (en) | 1999-08-30 |
HUP9901929A2 true HUP9901929A2 (hu) | 1999-12-28 |
HUP9901929A3 HUP9901929A3 (en) | 2000-10-30 |
HU221746B1 HU221746B1 (hu) | 2002-12-28 |
Family
ID=7870435
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
HU9901929A HU221746B1 (hu) | 1998-06-10 | 1999-06-09 | Új oligomer-organoszilán-poliszulfánok, alkalmazásuk kaucsukkeverékekben és formatestek előállítására |
Country Status (21)
Country | Link |
---|---|
US (1) | US6331605B1 (hu) |
EP (1) | EP0964021B1 (hu) |
JP (1) | JP4376999B2 (hu) |
KR (1) | KR100699183B1 (hu) |
CN (1) | CN1209365C (hu) |
AT (1) | ATE266694T1 (hu) |
BR (1) | BR9902232A (hu) |
CA (1) | CA2273873A1 (hu) |
DE (2) | DE19825796A1 (hu) |
ES (1) | ES2216376T3 (hu) |
HU (1) | HU221746B1 (hu) |
ID (1) | ID22866A (hu) |
IL (1) | IL130312A (hu) |
MY (1) | MY118650A (hu) |
PL (1) | PL333617A1 (hu) |
PT (1) | PT964021E (hu) |
RU (1) | RU2217446C2 (hu) |
TR (1) | TR199901295A2 (hu) |
TW (1) | TW546326B (hu) |
UA (1) | UA64732C2 (hu) |
ZA (1) | ZA993900B (hu) |
Families Citing this family (59)
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US6548573B1 (en) * | 1999-12-20 | 2003-04-15 | Caterpillar Inc | Composition and process for making a water and mud repellant rubber |
DE10044989A1 (de) | 2000-09-11 | 2002-03-21 | Bayer Ag | Flüssige schwefelhaltige Oligosiloxane und ihre Verwendung in Kautschukmischungen |
WO2002096914A2 (en) * | 2001-04-30 | 2002-12-05 | Crompton Corporation | Hybrid silicon-containing coupling agents for filled elastomer compositions |
DE10132941A1 (de) | 2001-07-06 | 2003-01-23 | Degussa | Oligomere Organosilane, Verfahren zu deren Herstellung und deren Verwendung |
DE10132942A1 (de) | 2001-07-06 | 2003-01-23 | Degussa | Siloxan-Oligomere, Verfahren zu deren Herstellung und deren Verwendung |
JP4450149B2 (ja) * | 2002-06-20 | 2010-04-14 | 信越化学工業株式会社 | 有機珪素化合物、その製造方法、及びゴム用配合剤 |
DE10354616A1 (de) * | 2003-11-21 | 2005-06-23 | Degussa Ag | Kautschukmischungen |
MY164448A (en) * | 2003-12-15 | 2017-12-15 | Ciba Holding Inc | Coupling agents between filler and elastomer |
DE102004030737A1 (de) * | 2004-06-25 | 2006-01-12 | Degussa Ag | Verfahren und Vorrichtung zur Extraktion von Stoffen aus silanmodifizierten Füllstoffen |
US7960576B2 (en) * | 2004-08-13 | 2011-06-14 | Momentive Performance Materials Inc. | Diol-derived organofunctional silane and compositions containing same |
US7928258B2 (en) | 2004-08-20 | 2011-04-19 | Momentive Performance Materials Inc. | Cyclic diol-derived blocked mercaptofunctional silane compositions |
DE102004061014A1 (de) * | 2004-12-18 | 2006-06-29 | Degussa Ag | Kautschukmischungen |
ES2626229T3 (es) | 2005-03-24 | 2017-07-24 | Bridgestone Corporation | Compuesto de caucho reforzado con sílice con baja emisión de compuestos orgánicos volátiles (COV) |
DE102005020535B3 (de) * | 2005-05-03 | 2006-06-08 | Degussa Ag | Verfahren zur Herstellung von Mercaptoorganyl(alkoxysilanen) |
JP4879521B2 (ja) * | 2005-06-14 | 2012-02-22 | 住友ゴム工業株式会社 | ゴム組成物 |
DE102005038791A1 (de) * | 2005-08-17 | 2007-02-22 | Degussa Ag | Organosiliciumverbindungen, ihre Herstellung und ihre Verwendung |
US7776967B2 (en) * | 2005-12-16 | 2010-08-17 | Continental Ag | Polyorganosiloxane composition for use in unsaturated elastomer, article made therefrom, and associated method |
US7652162B2 (en) * | 2005-12-16 | 2010-01-26 | Momentive Performance Materials Inc. | Polyorganosiloxane composition, and associated method |
US7560513B2 (en) * | 2005-12-16 | 2009-07-14 | Continental Ag | Polyorganosiloxane composition for use in unsaturated elastomer, article made therefrom, and associated method |
DE102005060122A1 (de) * | 2005-12-16 | 2007-06-21 | Degussa Gmbh | Verfahren zur Herstellung von (Mercaptoorganyl)alkylpolyethersilanen |
US7919650B2 (en) * | 2006-02-21 | 2011-04-05 | Momentive Performance Materials Inc. | Organofunctional silanes and their mixtures |
US7510670B2 (en) | 2006-02-21 | 2009-03-31 | Momentive Performance Materials Inc. | Free flowing filler composition based on organofunctional silane |
US7718819B2 (en) * | 2006-02-21 | 2010-05-18 | Momentive Performance Materials Inc. | Process for making organofunctional silanes and mixtures thereof |
US7504456B2 (en) * | 2006-02-21 | 2009-03-17 | Momentive Performance Materials Inc. | Rubber composition containing organofunctional silane |
DE102006027235A1 (de) * | 2006-06-09 | 2008-01-17 | Evonik Degussa Gmbh | Kautschukmischungen |
US7550540B2 (en) * | 2006-08-14 | 2009-06-23 | Momentive Performance Materials Inc. | Rubber composition and articles therefrom both comprising mercapto-functional silane |
US8008519B2 (en) * | 2006-08-14 | 2011-08-30 | Momentive Performance Materials Inc. | Process for making mercapto-functional silane |
US8097744B2 (en) * | 2006-08-14 | 2012-01-17 | Momentive Performance Materials Inc. | Free flowing filler composition comprising mercapto-functional silane |
US7915368B2 (en) | 2007-05-23 | 2011-03-29 | Bridgestone Corporation | Method for making alkoxy-modified silsesquioxanes |
US8501895B2 (en) | 2007-05-23 | 2013-08-06 | Bridgestone Corporation | Method for making alkoxy-modified silsesquioxanes and amino alkoxy-modified silsesquioxanes |
KR100894417B1 (ko) * | 2007-09-06 | 2009-04-24 | 제일모직주식회사 | 갭 필 능력이 개선된 반도체 미세 갭 필용 유기실란계중합체 및 이를 이용한 반도체 미세 갭 필용 조성물 |
US7816435B2 (en) * | 2007-10-31 | 2010-10-19 | Momentive Performance Materials Inc. | Halo-functional silane, process for its preparation, rubber composition containing same and articles manufactured therefrom |
US8962746B2 (en) | 2007-12-27 | 2015-02-24 | Bridgestone Corporation | Methods of making blocked-mercapto alkoxy-modified silsesquioxane compounds |
US8513371B2 (en) | 2007-12-31 | 2013-08-20 | Bridgestone Corporation | Amino alkoxy-modified silsesquioxanes and method of preparation |
US8794282B2 (en) | 2007-12-31 | 2014-08-05 | Bridgestone Corporation | Amino alkoxy-modified silsesquioxane adhesives for improved metal adhesion and metal adhesion retention to cured rubber |
CN101318971B (zh) * | 2008-03-17 | 2010-12-15 | 南京曙光硅烷化工有限公司 | 一种减少含硫硅烷中乙醇的方法 |
FR2947552B1 (fr) * | 2009-05-20 | 2011-08-26 | Michelin Soc Tech | Agent de couplage organosilane |
US8642691B2 (en) | 2009-12-28 | 2014-02-04 | Bridgestone Corporation | Amino alkoxy-modified silsesquioxane adhesives for improved metal adhesion and metal adhesion retention to cured rubber |
JP5420620B2 (ja) * | 2011-10-27 | 2014-02-19 | 住友ゴム工業株式会社 | ゴム組成物 |
DE112013001701B4 (de) * | 2012-03-23 | 2019-06-19 | The Yokohama Rubber Co., Ltd. | Luftreifen |
US9499009B2 (en) * | 2012-06-27 | 2016-11-22 | The Yokohama Rubber Co., Ltd. | Rubber composition for tire treads and pneumatic tire using same |
JP5929847B2 (ja) * | 2012-06-27 | 2016-06-08 | 信越化学工業株式会社 | オルガノポリシロキサン及びその製造方法 |
KR101625027B1 (ko) | 2013-02-25 | 2016-05-27 | 요코하마 고무 가부시키가이샤 | 타이어 트레드용 고무 조성물 및 이것을 이용하는 공기입 타이어 |
EP2960289B1 (en) | 2013-02-25 | 2020-12-02 | The Yokohama Rubber Co., Ltd. | Rubber composition for tires, and pneumatic tire using same |
EP2960288B1 (en) * | 2013-02-25 | 2019-10-30 | The Yokohama Rubber Co., Ltd. | Rubber composition for tire tread, and pneumatic tire |
JP5907309B2 (ja) * | 2013-02-25 | 2016-04-26 | 横浜ゴム株式会社 | 重荷重タイヤ用ゴム組成物および空気入りタイヤ |
JP6476554B2 (ja) * | 2013-02-25 | 2019-03-06 | 横浜ゴム株式会社 | タイヤサイドウォール用ゴム組成物およびそれを用いた空気入りタイヤ |
JP6287324B2 (ja) * | 2013-02-25 | 2018-03-07 | 横浜ゴム株式会社 | スタッドレスタイヤ用ゴム組成物およびスタッドレスタイヤ |
JP6476555B2 (ja) * | 2013-02-25 | 2019-03-06 | 横浜ゴム株式会社 | タイヤトレッド用ゴム組成物および空気入りタイヤ |
JP6481253B2 (ja) * | 2013-02-25 | 2019-03-13 | 横浜ゴム株式会社 | タイヤ用ゴム組成物及びこれを用いる空気入りタイヤ |
WO2014129661A1 (ja) * | 2013-02-25 | 2014-08-28 | 横浜ゴム株式会社 | タイヤトレッド用ゴム組成物及びこれを用いる空気入りタイヤ |
JP5910568B2 (ja) * | 2013-04-23 | 2016-04-27 | 信越化学工業株式会社 | 有機官能基含有オルガノポリシロキサンの製造方法 |
KR101572106B1 (ko) | 2013-08-20 | 2015-11-26 | 한국타이어 주식회사 | 타이어 트레드용 고무 조성물 및 이를 이용하여 제조한 타이어 |
CN104513982B (zh) * | 2013-09-27 | 2019-01-22 | 东友精细化工有限公司 | 用于液晶显示器的阵列基板的制造方法 |
DE102014200563A1 (de) * | 2014-01-15 | 2015-07-16 | Evonik Industries Ag | Oligomere Organosilane, deren Herstellung und Verwendung in Kautschukmischungen |
EP3241221A4 (en) | 2014-12-31 | 2018-08-08 | Bridgestone Corporation | Amino alkoxy-modified silsesquioxane adhesives for adhering steel alloy to rubber |
CN106800571B (zh) * | 2017-01-17 | 2019-03-08 | 荆州市江汉精细化工有限公司 | 一种环状含硫硅烷低聚物及制备方法 |
JP2021130730A (ja) * | 2020-02-18 | 2021-09-09 | 信越化学工業株式会社 | オルガノポリシロキサン、ゴム組成物およびタイヤ |
WO2024088789A1 (en) | 2022-10-24 | 2024-05-02 | Evonik Operations Gmbh | Oligomeric organosilanes, preparation thereof and use thereof in rubber mixtures |
Family Cites Families (14)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE1210192B (de) | 1961-04-10 | 1966-02-03 | Max Schmidt Dipl Chem Dr | Verfahren zur Herstellung von Disilathioaetherderivaten |
US3873489A (en) * | 1971-08-17 | 1975-03-25 | Degussa | Rubber compositions containing silica and an organosilane |
BE787691A (fr) * | 1971-08-17 | 1973-02-19 | Degussa | Composes organosiliciques contenant du soufre |
DE2141159C3 (de) * | 1971-08-17 | 1983-11-24 | Degussa Ag, 6000 Frankfurt | Schwefel enthaltende Organosiliciumverbindungen |
US4044037A (en) * | 1974-12-24 | 1977-08-23 | Union Carbide Corporation | Sulfur containing silane coupling agents |
DE3226091C2 (de) * | 1982-07-13 | 1986-11-20 | Degussa Ag, 6000 Frankfurt | Polymere Di-, Tri- oder Tetrasulfide, Verfahren zu ihrer Herstellung und Verwendung |
EP0191929B1 (de) * | 1985-02-08 | 1989-05-03 | Hüls Aktiengesellschaft | Haftvermittler zur Herstellung von Vulkanisaten mit gutem Füllstoff/Kautschuk-Verbund |
DD299187B5 (de) * | 1990-07-13 | 1996-05-15 | Huels Silicone Gmbh | Verfahren zur Herstellung von schwefelhaltigen Organosiliciumverbindungen |
DE4415658A1 (de) * | 1994-05-04 | 1995-11-09 | Bayer Ag | Schwefelhaltige Organosiliciumverbindungen enthaltende Kautschukmischungen |
US5580919A (en) | 1995-03-14 | 1996-12-03 | The Goodyear Tire & Rubber Company | Silica reinforced rubber composition and use in tires |
FR2743564A1 (fr) * | 1996-01-11 | 1997-07-18 | Michelin & Cie | Compositions de caoutchouc pour enveloppes de pneumatiques a base de silices contenant un additif de renforcement a base d'un polyorganosiloxane fonctionnalise et d'un compose organosilane . |
US5663358A (en) | 1996-01-22 | 1997-09-02 | The Goodyear Tire & Rubber Company | Process for the preparation of organosilicon disulfide compounds |
DE19702046A1 (de) * | 1996-07-18 | 1998-01-22 | Degussa | Gemische von Organosilanpolysulfanen und ein Verfahren zur Herstellung von diese Gemische enthaltenden Kautschukmischungen |
DE19651849A1 (de) * | 1996-12-13 | 1998-06-18 | Degussa | Verfahren zur Herstellung von Bis(silylorganyl)-polysulfanen |
-
1998
- 1998-06-10 DE DE19825796A patent/DE19825796A1/de not_active Ceased
-
1999
- 1999-06-02 AT AT99110615T patent/ATE266694T1/de not_active IP Right Cessation
- 1999-06-02 EP EP99110615A patent/EP0964021B1/de not_active Expired - Lifetime
- 1999-06-02 DE DE59909445T patent/DE59909445D1/de not_active Expired - Lifetime
- 1999-06-02 PT PT99110615T patent/PT964021E/pt unknown
- 1999-06-02 ES ES99110615T patent/ES2216376T3/es not_active Expired - Lifetime
- 1999-06-04 IL IL13031299A patent/IL130312A/xx not_active IP Right Cessation
- 1999-06-04 TW TW088109327A patent/TW546326B/zh not_active IP Right Cessation
- 1999-06-07 JP JP15986999A patent/JP4376999B2/ja not_active Expired - Lifetime
- 1999-06-09 CA CA002273873A patent/CA2273873A1/en not_active Abandoned
- 1999-06-09 PL PL99333617A patent/PL333617A1/xx not_active Application Discontinuation
- 1999-06-09 RU RU99113941/04A patent/RU2217446C2/ru not_active IP Right Cessation
- 1999-06-09 MY MYPI99002355A patent/MY118650A/en unknown
- 1999-06-09 TR TR1999/01295A patent/TR199901295A2/xx unknown
- 1999-06-09 HU HU9901929A patent/HU221746B1/hu not_active IP Right Cessation
- 1999-06-10 ZA ZA9903900A patent/ZA993900B/xx unknown
- 1999-06-10 ID IDP990559D patent/ID22866A/id unknown
- 1999-06-10 BR BR9902232-0A patent/BR9902232A/pt not_active Application Discontinuation
- 1999-06-10 US US09/329,370 patent/US6331605B1/en not_active Expired - Lifetime
- 1999-06-10 KR KR1019990021578A patent/KR100699183B1/ko not_active IP Right Cessation
- 1999-06-10 CN CNB991080319A patent/CN1209365C/zh not_active Expired - Lifetime
- 1999-06-10 UA UA99063220A patent/UA64732C2/uk unknown
Also Published As
Publication number | Publication date |
---|---|
ATE266694T1 (de) | 2004-05-15 |
KR20000006080A (ko) | 2000-01-25 |
EP0964021A3 (de) | 2001-09-26 |
UA64732C2 (uk) | 2004-03-15 |
JP2000038395A (ja) | 2000-02-08 |
HUP9901929A3 (en) | 2000-10-30 |
TR199901295A3 (tr) | 2000-01-21 |
CN1273975A (zh) | 2000-11-22 |
DE19825796A1 (de) | 1999-12-16 |
DE59909445D1 (de) | 2004-06-17 |
HU221746B1 (hu) | 2002-12-28 |
TW546326B (en) | 2003-08-11 |
US6331605B1 (en) | 2001-12-18 |
RU2217446C2 (ru) | 2003-11-27 |
TR199901295A2 (xx) | 2000-01-21 |
ZA993900B (en) | 1999-12-10 |
HU9901929D0 (en) | 1999-08-30 |
KR100699183B1 (ko) | 2007-03-27 |
CN1209365C (zh) | 2005-07-06 |
IL130312A (en) | 2005-06-19 |
MY118650A (en) | 2004-12-31 |
ES2216376T3 (es) | 2004-10-16 |
PL333617A1 (en) | 1999-12-20 |
ID22866A (id) | 1999-12-16 |
IL130312A0 (en) | 2000-06-01 |
EP0964021B1 (de) | 2004-05-12 |
CA2273873A1 (en) | 1999-12-10 |
PT964021E (pt) | 2004-09-30 |
BR9902232A (pt) | 2000-05-23 |
EP0964021A2 (de) | 1999-12-15 |
JP4376999B2 (ja) | 2009-12-02 |
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