CN101449338B - 用于后处理废核燃料及制备混合的铀-钚氧化物的方法 - Google Patents

用于后处理废核燃料及制备混合的铀-钚氧化物的方法 Download PDF

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CN101449338B
CN101449338B CN2007800188112A CN200780018811A CN101449338B CN 101449338 B CN101449338 B CN 101449338B CN 2007800188112 A CN2007800188112 A CN 2007800188112A CN 200780018811 A CN200780018811 A CN 200780018811A CN 101449338 B CN101449338 B CN 101449338B
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plutonium
uranium
neptunium
aqueous phase
solvent
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CN101449338A (zh
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P·巴龙
B·丹
M·马松
F·德兰
J-L·埃曼
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Ou Annuofenjie
Ou Annuoxunhuan
Ou Annuozaixunhuan
Commissariat a lEnergie Atomique et aux Energies Alternatives CEA
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Areva NC SA
Commissariat a lEnergie Atomique CEA
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    • G—PHYSICS
    • G21—NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21C—NUCLEAR REACTORS
    • G21C19/00—Arrangements for treating, for handling, or for facilitating the handling of, fuel or other materials which are used within the reactor, e.g. within its pressure vessel
    • G21C19/42—Reprocessing of irradiated fuel
    • G21C19/44—Reprocessing of irradiated fuel of irradiated solid fuel
    • G21C19/46—Aqueous processes, e.g. by using organic extraction means, including the regeneration of these means
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G43/00—Compounds of uranium
    • C01G43/003—Preparation involving a liquid-liquid extraction, an adsorption or an ion-exchange
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G43/00—Compounds of uranium
    • C01G43/01—Oxides; Hydroxides
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G56/00—Compounds of transuranic elements
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G56/00—Compounds of transuranic elements
    • C01G56/001—Preparation involving a liquid-liquid extraction, an adsorption or an ion-exchange
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E30/00—Energy generation of nuclear origin
    • Y02E30/30—Nuclear fission reactors
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02W—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00—Technologies for solid waste management
    • Y02W30/50—Reuse, recycling or recovery technologies

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Physics & Mathematics (AREA)
  • Engineering & Computer Science (AREA)
  • Geology (AREA)
  • General Life Sciences & Earth Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Plasma & Fusion (AREA)
  • General Engineering & Computer Science (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Inorganic Compounds Of Heavy Metals (AREA)
  • Extraction Or Liquid Replacement (AREA)
  • Oxygen, Ozone, And Oxides In General (AREA)
CN2007800188112A 2006-05-24 2007-05-23 用于后处理废核燃料及制备混合的铀-钚氧化物的方法 Active CN101449338B (zh)

Applications Claiming Priority (5)

Application Number Priority Date Filing Date Title
FR0604717A FR2901627B1 (fr) 2006-05-24 2006-05-24 Procede de retraitement d'un combustible nucleaire use et de preparation d'un oxyde mixte d'uranium et de plutonium
FR06/04717 2006-05-24
US85302406P 2006-10-20 2006-10-20
US60/853,024 2006-10-20
PCT/EP2007/055024 WO2007135178A1 (en) 2006-05-24 2007-05-23 Process for reprocessing a spent nuclear fuel and of preparing a mixed uranium-plutonium oxide

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CN101449338A CN101449338A (zh) 2009-06-03
CN101449338B true CN101449338B (zh) 2012-10-24

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US (2) US20090184298A1 (enExample)
EP (1) EP2022061B1 (enExample)
JP (1) JP5325098B2 (enExample)
KR (1) KR101386696B1 (enExample)
CN (1) CN101449338B (enExample)
AT (1) ATE447231T1 (enExample)
DE (1) DE602007003013D1 (enExample)
ES (1) ES2334852T3 (enExample)
FR (1) FR2901627B1 (enExample)
RU (1) RU2431896C2 (enExample)
WO (1) WO2007135178A1 (enExample)
ZA (1) ZA200809415B (enExample)

Families Citing this family (52)

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FR2901627B1 (fr) * 2006-05-24 2009-05-01 Commissariat Energie Atomique Procede de retraitement d'un combustible nucleaire use et de preparation d'un oxyde mixte d'uranium et de plutonium
JP5193687B2 (ja) * 2008-05-30 2013-05-08 株式会社東芝 使用済み燃料再処理方法
US20100158772A1 (en) * 2008-06-13 2010-06-24 Decode Biostructures, Inc. Nanovolume microcapillary crystallization system
JP5132476B2 (ja) * 2008-08-12 2013-01-30 株式会社東芝 使用済核燃料の再処理方法および遠心抽出装置
DE102008042518A1 (de) 2008-10-01 2010-04-08 Robert Bosch Gmbh Verfahren zur Auswahl von zu ergreifenden Sicherheitsmaßnahmen zur Erhöhung einer Sicherheit von Fahrzeuginsassen
US8571167B2 (en) * 2009-06-01 2013-10-29 Advanced Reactor Concepts LLC Particulate metal fuels used in power generation, recycling systems, and small modular reactors
FR2947663B1 (fr) 2009-07-02 2011-07-29 Areva Nc Procede ameliore de traitement de combustibles nucleaires uses
FR2948385B1 (fr) 2009-07-27 2011-09-23 Commissariat Energie Atomique Procede de recuperation selective de l'americium a partir d'une phase aqueuse nitrique
FR2948384B1 (fr) 2009-07-27 2011-09-23 Commissariat Energie Atomique Augmentation du facteur de separation entre l'americium et le curium et/ou entre des lanthanides dans une operation d'extraction liquide-liquide
FR2954354B1 (fr) * 2009-12-22 2012-01-13 Commissariat Energie Atomique Procede de purification de l'uranium d'un concentre d'uranium naturel
JP2013517479A (ja) 2010-01-13 2013-05-16 アドバンスト・リアクター・コンセプツ・エルエルシー シースで被覆された環状の金属核燃料
RU2713473C2 (ru) 2010-02-22 2020-02-05 Эдвансд Риэктор Консептс Ллк Система ядерного реактора и способ получения ядерной энергии
US8741237B1 (en) * 2010-04-12 2014-06-03 U.S. Department Of Energy Solvent extraction system for plutonium colloids and other oxide nano-particles
FR2960690B1 (fr) * 2010-05-27 2012-06-29 Commissariat Energie Atomique Procede de traitement de combustibles nucleaires uses ne necessitant pas d'operation de desextraction reductrice du plutonium
RU2456244C2 (ru) * 2010-08-30 2012-07-20 Федеральное государственное унитарное предприятие "Производственное объединение "Маяк" Способ переработки отработанных стекловолокнистых аэрозольных фильтров
FR2968014B1 (fr) 2010-11-25 2012-12-28 Commissariat Energie Atomique Procede de separation de l'americium des autres elements metalliques presents dans une phase aqueuse acide ou organique et ses applications
JP5737931B2 (ja) * 2010-12-24 2015-06-17 三菱重工業株式会社 抽出装置および使用済核燃料の再処理施設
JP5758209B2 (ja) * 2011-06-14 2015-08-05 株式会社東芝 使用済み燃料再処理方法
JP5784476B2 (ja) * 2011-12-09 2015-09-24 株式会社東芝 ウランの回収方法
RU2502142C1 (ru) * 2012-04-19 2013-12-20 Федеральное государственное унитарное предприятие "Научно-исследовательский институт Научно-производственное объединение "ЛУЧ" (ФГУП "НИИ НПО "ЛУЧ") Способ переработки уран-молибденовой композиции
RU2537013C2 (ru) * 2012-12-07 2014-12-27 Открытое акционерное общество "Радиевый институт имени В.Г. Хлопина" Топливная композиция для водоохлаждаемых реакторов аэс на тепловых нейтронах
CN103305702B (zh) * 2013-07-08 2014-12-24 中国原子能科学研究院 一种从Purex流程的2AW+2DW中放废液中回收和纯化镎的工艺
FR3015760B1 (fr) 2013-12-20 2016-01-29 Commissariat Energie Atomique Procede de traitement d'un combustible nucleaire use comprenant une etape de decontamination de l'uranium(vi) en au moins un actinide(iv) par complexation de cet actinide(iv)
GB2538687B (en) * 2014-04-14 2020-12-30 Advanced Reactor Concepts LLC Ceramic nuclear fuel dispersed in a metallic alloy matrix
RU2561508C1 (ru) * 2014-04-29 2015-08-27 Федеральное государственное унитарное предприятие "Научно-исследовательский технологический институт имени А.П. Александрова" Способ иммобилизации стронций-цезиевой фракции высокоактивных отходов включением в геокерамические матрицы
CN104407062A (zh) * 2014-09-11 2015-03-11 上海大学 一种快速分析磷酸三异戊酯的方法
JP6479398B2 (ja) * 2014-10-10 2019-03-06 三菱重工業株式会社 再処理施設
FR3039696B1 (fr) 2015-07-29 2017-07-28 Commissariat Energie Atomique Procede de traitement en un cycle, exempt d'operation de desextraction reductrice du plutonium, d'une solution aqueuse nitrique de dissolution d'un combustible nucleaire use
FR3039547B1 (fr) 2015-07-29 2017-08-25 Areva Nc Nouveaux n,n-dialkylamides dissymetriques, leur synthese et leurs utilisations
FR3042903B1 (fr) * 2015-10-21 2017-12-08 Commissariat Energie Atomique Utilisation d'acides hydroxyiminoalcanoiques comme agents anti-nitreux dans des operations de desextraction reductrice du plutonium
CN106119578B (zh) * 2016-06-27 2018-10-09 中国原子能科学研究院 一种草酸钚沉淀母液中硝酸-草酸浓缩与破坏的一体化方法
CN107845432B (zh) * 2016-09-20 2019-09-17 中核四〇四有限公司 一种mox球磨粉末混料方法
CN107845433B (zh) * 2016-09-20 2019-09-17 中核四〇四有限公司 一种mox粉末成形剂与润滑剂添加方法
JP6896561B2 (ja) * 2016-09-26 2021-06-30 株式会社東芝 軽水炉用燃料集合体、軽水炉炉心、軽水炉用燃料集合体製造方法およびｍｏｘ燃料集合体製造方法
CN107610796B (zh) * 2017-08-29 2019-08-13 中核四0四有限公司 Mox制备过程不合格粉末回收方法
WO2019115394A1 (en) 2017-12-11 2019-06-20 Orano Cycle Method for preparing a powder comprising particles of triuranium octoxide and particles of plutonium dioxide
FR3074794B1 (fr) 2017-12-11 2020-01-10 Areva Nc Procede de preparation d'une poudre comprenant des particules de sesquioxyde d'uranium et des particules de dioxyde de plutonium
CN108267347A (zh) * 2017-12-27 2018-07-10 中核四0四有限公司 一种采用tbp萃取剂测定mox芯块中银杂质含量的方法
CN108630332B (zh) * 2018-03-26 2021-06-18 中国核电工程有限公司 一种草酸盐沉淀过滤母液中草酸根的破坏装置及破坏方法
CN109234534B (zh) * 2018-08-08 2019-11-08 中国原子能科学研究院 一种从高放废液中共萃取三价锕系和三价镧系元素的工艺
CN109402413B (zh) * 2018-10-30 2020-11-03 中国工程物理研究院核物理与化学研究所 一种乏燃料元件裂变产物中钯的回收方法
CN109735859B (zh) * 2019-03-18 2020-10-09 中国原子能科学研究院 一种3-戊基肼及其盐的用途
CN112309601B (zh) * 2019-07-26 2023-04-11 中国科学院大连化学物理研究所 一种稀释剂及其制备和应用
KR102293451B1 (ko) * 2019-11-08 2021-08-25 한국원자력연구원 금속연료 폐기물을 이용한 금속연료심 제조방법 및 이 방법에 의해 제조된 금속연료심
CN112940781B (zh) * 2019-12-10 2022-10-25 中国科学院大连化学物理研究所 一种稀释剂和其制备与应用
CN112941346A (zh) * 2019-12-10 2021-06-11 中国科学院大连化学物理研究所 一种稀释剂及其制备和应用
RU2727140C1 (ru) * 2020-01-28 2020-07-21 Федеральное государственное унитарное предприятие "Горно-химический комбинат" (ФГУП "ГХК") Способ экстракционной переработки облученного ядерного топлива
CN111863303B (zh) * 2020-06-10 2022-08-05 中国原子能科学研究院 一种purex流程含钚团聚物的溶解与回收方法
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CN113241208B (zh) * 2021-06-22 2024-05-14 中国原子能科学研究院 用于钚尾端处理的容纳装置、蒸发煅烧系统及方法
FR3139408B1 (fr) 2022-09-02 2024-09-13 Commissariat Energie Atomique Procédé de désextraction d’uranium(vi) et d’un actinide(iv) d’une solution organique par précipitation oxalique
WO2024238826A1 (en) * 2023-05-16 2024-11-21 Shine Technologies, Llc Methods and systems of partitioning, transmuting, and recycling used nuclear fuel

Citations (7)

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Publication number Priority date Publication date Assignee Title
GB1206775A (en) * 1962-12-26 1970-09-30 Gen Electric Neptunium recovery process
GB2004407A (en) * 1977-09-16 1979-03-28 British Nuclear Fuels Ltd Purification of plutonium
US4278559A (en) * 1978-02-16 1981-07-14 Electric Power Research Institute Method for processing spent nuclear reactor fuel
CN1277725A (zh) * 1997-10-31 2000-12-20 英国核燃料公共有限公司 核燃料的后处理方法
CN1290397A (zh) * 1998-02-11 2001-04-04 不列颠核燃料有限公司 核燃料再加工
CN1448959A (zh) * 2003-04-04 2003-10-15 清华大学 一种乏燃料后端处理一体化的方法
FR2870841A1 (fr) * 2004-05-28 2005-12-02 Commissariat Energie Atomique Procede de coprecipitation d'actinides a des etats d'oxydation distincts et procede de preparation de composes mixtes d'actinides

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DE2838541A1 (de) * 1977-09-16 1979-04-05 British Nuclear Fuels Ltd Verfahren zur reinigung einer plutonium enthaltenden phase
FR2607823B1 (fr) * 1986-12-03 1989-02-17 Commissariat Energie Atomique Procede pour separer le technetium present dans un solvant organique avec du zirconium et au moins un autre metal tel que l'uranium ou le plutonium, utilisable notamment pour le retraitement des combustibles nucleaires irradies
RU2132578C1 (ru) * 1997-06-16 1999-06-27 Научно-производственное объединение "Радиевый институт им.В.Г.Хлопина" Способ переработки облученного ядерного топлива (оят) аэс
FR2815035B1 (fr) * 2000-10-05 2003-03-07 Commissariat Energie Atomique Procede de coprecipitation d'actinides et procede de preparation d'oxydes mixtes d'actinides
FR2862804B1 (fr) * 2003-11-20 2006-01-13 Commissariat Energie Atomique Procede de separation de l'uranium (vi) d'actinides (iv) et/ou (vi)et ses utilisations
FR2901627B1 (fr) * 2006-05-24 2009-05-01 Commissariat Energie Atomique Procede de retraitement d'un combustible nucleaire use et de preparation d'un oxyde mixte d'uranium et de plutonium

Patent Citations (7)

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Publication number Priority date Publication date Assignee Title
GB1206775A (en) * 1962-12-26 1970-09-30 Gen Electric Neptunium recovery process
GB2004407A (en) * 1977-09-16 1979-03-28 British Nuclear Fuels Ltd Purification of plutonium
US4278559A (en) * 1978-02-16 1981-07-14 Electric Power Research Institute Method for processing spent nuclear reactor fuel
CN1277725A (zh) * 1997-10-31 2000-12-20 英国核燃料公共有限公司 核燃料的后处理方法
CN1290397A (zh) * 1998-02-11 2001-04-04 不列颠核燃料有限公司 核燃料再加工
CN1448959A (zh) * 2003-04-04 2003-10-15 清华大学 一种乏燃料后端处理一体化的方法
FR2870841A1 (fr) * 2004-05-28 2005-12-02 Commissariat Energie Atomique Procede de coprecipitation d'actinides a des etats d'oxydation distincts et procede de preparation de composes mixtes d'actinides

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US7887767B2 (en) 2011-02-15
EP2022061B1 (en) 2009-10-28
US20070290178A1 (en) 2007-12-20
FR2901627B1 (fr) 2009-05-01
FR2901627A1 (fr) 2007-11-30
EP2022061A1 (en) 2009-02-11
DE602007003013D1 (de) 2009-12-10
JP2009537838A (ja) 2009-10-29
KR101386696B1 (ko) 2014-04-18
ES2334852T3 (es) 2010-03-16
KR20090010217A (ko) 2009-01-29
RU2431896C2 (ru) 2011-10-20
ZA200809415B (en) 2009-10-28
JP5325098B2 (ja) 2013-10-23
RU2008151145A (ru) 2010-06-27
US20090184298A1 (en) 2009-07-23
WO2007135178A1 (en) 2007-11-29
CN101449338A (zh) 2009-06-03
ATE447231T1 (de) 2009-11-15

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