HUP0002178A2 - Herbicid hatású 4-(3-heterociklil-benzoil)-pirazolok, előállításuk és alkalmazásuk - Google Patents
Herbicid hatású 4-(3-heterociklil-benzoil)-pirazolok, előállításuk és alkalmazásukInfo
- Publication number
- HUP0002178A2 HUP0002178A2 HU0002178A HUP0002178A HUP0002178A2 HU P0002178 A2 HUP0002178 A2 HU P0002178A2 HU 0002178 A HU0002178 A HU 0002178A HU P0002178 A HUP0002178 A HU P0002178A HU P0002178 A2 HUP0002178 A2 HU P0002178A2
- Authority
- HU
- Hungary
- Prior art keywords
- alkyl
- alkoxy
- halo
- optionally substituted
- alkoxycarbonyl
- Prior art date
Links
- 230000002363 herbicidal effect Effects 0.000 title 1
- 150000003217 pyrazoles Chemical class 0.000 title 1
- 125000000217 alkyl group Chemical group 0.000 abstract 24
- 125000003545 alkoxy group Chemical group 0.000 abstract 7
- 125000005843 halogen group Chemical group 0.000 abstract 6
- 125000004453 alkoxycarbonyl group Chemical group 0.000 abstract 4
- 125000003342 alkenyl group Chemical group 0.000 abstract 3
- 125000000304 alkynyl group Chemical group 0.000 abstract 3
- 125000000753 cycloalkyl group Chemical group 0.000 abstract 3
- 125000005090 alkenylcarbonyl group Chemical group 0.000 abstract 2
- 125000003282 alkyl amino group Chemical group 0.000 abstract 2
- 125000004448 alkyl carbonyl group Chemical group 0.000 abstract 2
- 125000004414 alkyl thio group Chemical group 0.000 abstract 2
- 125000001188 haloalkyl group Chemical group 0.000 abstract 2
- 125000000623 heterocyclic group Chemical group 0.000 abstract 2
- 125000005092 alkenyloxycarbonyl group Chemical group 0.000 abstract 1
- 125000005196 alkyl carbonyloxy group Chemical group 0.000 abstract 1
- 125000004644 alkyl sulfinyl group Chemical group 0.000 abstract 1
- 125000004390 alkyl sulfonyl group Chemical group 0.000 abstract 1
- 125000005087 alkynylcarbonyl group Chemical group 0.000 abstract 1
- 125000005225 alkynyloxycarbonyl group Chemical group 0.000 abstract 1
- 125000003917 carbamoyl group Chemical group [H]N([H])C(*)=O 0.000 abstract 1
- 125000003178 carboxy group Chemical group [H]OC(*)=O 0.000 abstract 1
- 125000006254 cycloalkyl carbonyl group Chemical group 0.000 abstract 1
- 125000004433 nitrogen atom Chemical group N* 0.000 abstract 1
- 125000001997 phenyl group Chemical group [H]C1=C([H])C([H])=C(*)C([H])=C1[H] 0.000 abstract 1
- 125000002924 primary amino group Chemical group [H]N([H])* 0.000 abstract 1
- 150000003839 salts Chemical class 0.000 abstract 1
- 125000004434 sulfur atom Chemical group 0.000 abstract 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D419/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen, oxygen, and sulfur atoms as the only ring hetero atoms
- C07D419/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen, oxygen, and sulfur atoms as the only ring hetero atoms containing two hetero rings
- C07D419/10—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen, oxygen, and sulfur atoms as the only ring hetero atoms containing two hetero rings linked by a carbon chain containing aromatic rings
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D231/00—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings
- C07D231/02—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings
- C07D231/10—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings having two or three double bonds between ring members or between ring members and non-ring members
- C07D231/14—Heterocyclic compounds containing 1,2-diazole or hydrogenated 1,2-diazole rings not condensed with other rings having two or three double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
- C07D231/18—One oxygen or sulfur atom
- C07D231/20—One oxygen atom attached in position 3 or 5
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D261/00—Heterocyclic compounds containing 1,2-oxazole or hydrogenated 1,2-oxazole rings
- C07D261/02—Heterocyclic compounds containing 1,2-oxazole or hydrogenated 1,2-oxazole rings not condensed with other rings
- C07D261/04—Heterocyclic compounds containing 1,2-oxazole or hydrogenated 1,2-oxazole rings not condensed with other rings having one double bond between ring members or between a ring member and a non-ring member
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D261/00—Heterocyclic compounds containing 1,2-oxazole or hydrogenated 1,2-oxazole rings
- C07D261/20—Heterocyclic compounds containing 1,2-oxazole or hydrogenated 1,2-oxazole rings condensed with carbocyclic rings or ring systems
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D413/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and oxygen atoms as the only ring hetero atoms
- C07D413/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and oxygen atoms as the only ring hetero atoms containing two hetero rings
- C07D413/10—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and oxygen atoms as the only ring hetero atoms containing two hetero rings linked by a carbon chain containing aromatic rings
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07D—HETEROCYCLIC COMPOUNDS
- C07D417/00—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00
- C07D417/02—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings
- C07D417/10—Heterocyclic compounds containing two or more hetero rings, at least one ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for by group C07D415/00 containing two hetero rings linked by a carbon chain containing aromatic rings
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Agricultural Chemicals And Associated Chemicals (AREA)
- Plural Heterocyclic Compounds (AREA)
Abstract
A találmány szerinti 4-(3-heterőciklil-benzőil)-pirazőlők (I)általánős képletében R1, R1 hidrőgén-, halőgénatőm, nitrő-, cianő-,alkil-, halőgén-alkil-, alkőxi-, halőgén-alkőxi-, alkil-tiő-, halőgén-alkil-tiő-, alkil-szűlfinil-, halőgén-alkil-szűlfinil-, alkil-szűlfőnil-, halőgén-alkil-szűlfőnil-, szűlfamőil-, N-alkil-szűlfamőil-, N,N-dialkil-szűlfamőil-, N-(alkil-szűlfőnil)-aminő-, N-(halőgén-alkil-szűlfőnil)-aminő-, N-alkil-N-(alkil-szűlfőnil)-aminő-vagy N-alkil-N-(halőgén-alkil-szűlfőnil)-aminő-csőpőrt, R2 adőttesetben szűbsztitűált őlyan 5- vagy 6-tagú heterőciklűsős csőpőrt,amely az őxigén-, kén- és nitrőgénatőmők közül heterőatőmként egy-négyegymással azőnős vagy egymástól eltérő atőmőt tartalmaz; R4 hidrőgén-,halőgénatőm vagy alkilcsőpőrt; R5 a 4-es helyzetű szénatőmján átkapcsőlódó (II) általánős képletű pirazőlszármazék, amelyben R6alkilcsőpőrt, R7 halőgén-alkenil-, halőgén-alkinil-, ciklőalkil-,fenil-, heterőciklil-, dialkil-tiőkarbamőil-csőpőrt, -C(O)-R, -C(O)-OR' vagy -C(O)NRR' általánős képletű csőpőrt, amelyekben R alkil-,fenil-, alkenil-, fenil-alkenil-, alkinil- vagy heterőciklilcsőpőrt.R', R' alkil-, alkenil-, alkinil-, fenil- vagy heterőciklilcsőpőrt, Rhidrőgénatőm, alkil- vagy alkőxicsőpőrt, és R7, R, R', R és R'csőpőrtőkban az alkil-, ciklőalkil-, fenil-, heterőciklil- ésalkőxicsőpőrtők adőtt esetben szűbsztitűálva vannak, R8 hidrőgénatőm,alkil- vagy halőgén-alkil-csőpőrt.. A találmány tárgyát képezik avegyületek mezőgazdaságilag alkalmazható sói is, tővábbá eljáráselőállításűkra, hatóanyagként ezeket tartalmazó győmirtó készítmények,eljárás a készítmények előállítására és a győmők irtására, valamint ahatóanyagők és az ezeket tartalmazó készítmények alkalmazása képezi. ŕ
Applications Claiming Priority (3)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| DE19701446 | 1997-01-17 | ||
| DE19740494 | 1997-09-15 | ||
| PCT/EP1998/000070 WO1998031682A1 (de) | 1997-01-17 | 1998-01-08 | 4-(3-heterocyclyl-1-benzoyl)pyrazole und ihre verwendung als herbizide |
Publications (3)
| Publication Number | Publication Date |
|---|---|
| HUP0002178A2 true HUP0002178A2 (hu) | 2000-09-28 |
| HUP0002178A3 HUP0002178A3 (en) | 2002-01-28 |
| HU226012B1 HU226012B1 (en) | 2008-02-28 |
Family
ID=26033168
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| HU0002178A HU226012B1 (en) | 1997-01-17 | 1998-01-08 | Herbicidal 4-(3-heterocyclyl-1-benzoyl)pyrazoles, preparation and use thereof |
Country Status (31)
| Country | Link |
|---|---|
| US (1) | US6165944A (hu) |
| EP (1) | EP0958292B1 (hu) |
| JP (1) | JP4259620B2 (hu) |
| KR (2) | KR20060025610A (hu) |
| CN (1) | CN1104429C (hu) |
| AR (1) | AR012836A1 (hu) |
| AT (1) | ATE350380T1 (hu) |
| AU (1) | AU742514B2 (hu) |
| BG (1) | BG64389B1 (hu) |
| BR (1) | BR9806917B1 (hu) |
| CA (1) | CA2277893C (hu) |
| CZ (1) | CZ298050B6 (hu) |
| DE (1) | DE59813869D1 (hu) |
| DK (1) | DK0958292T3 (hu) |
| EA (1) | EA009338B1 (hu) |
| EE (1) | EE05291B1 (hu) |
| ES (1) | ES2279569T3 (hu) |
| GE (1) | GEP20022765B (hu) |
| HU (1) | HU226012B1 (hu) |
| IL (1) | IL130778A0 (hu) |
| MX (1) | MX209959B (hu) |
| NO (1) | NO314728B1 (hu) |
| NZ (1) | NZ336640A (hu) |
| PL (1) | PL195943B1 (hu) |
| PT (1) | PT958292E (hu) |
| SI (1) | SI0958292T1 (hu) |
| SK (1) | SK286364B6 (hu) |
| TR (1) | TR199901665T2 (hu) |
| TW (1) | TW513414B (hu) |
| UA (1) | UA60325C2 (hu) |
| WO (1) | WO1998031682A1 (hu) |
Families Citing this family (39)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| AU1670897A (en) * | 1996-03-26 | 1997-10-17 | Nippon Soda Co., Ltd. | 3-(isoxazol-5-yl)-substituted benzoic acid derivatives and process for producing the same |
| HU228459B1 (en) * | 1997-01-17 | 2013-03-28 | Basf Ag | (3-heterocyclyl-substituted benzoyl)-pyrazole derivatives, preparation and intermediates thereof, and their use as herbicide |
| WO1999021852A1 (fr) * | 1997-10-27 | 1999-05-06 | Nippon Soda Co., Ltd. | Nouveaux derives de benzoylpyrazole et herbicides |
| BR9814832A (pt) * | 1997-10-30 | 2000-10-03 | Nippon Soda Co | Composto, e, herbicida |
| CZ299064B6 (cs) * | 1998-05-11 | 2008-04-16 | Basf Aktiengesellschaft | Zpusob výroby isoxazolu |
| DE19846792A1 (de) * | 1998-10-10 | 2000-04-13 | Hoechst Schering Agrevo Gmbh | Benzoylcyclohexandione, Verfahren zur ihrer Herstellung und ihre Verwendung als Herbizide und Pflanzenwachstumsregulatoren |
| EP1135388B1 (de) * | 1998-12-04 | 2003-09-10 | Basf Aktiengesellschaft | 3-(heterocyclyl)-substituierte benzoylpyrazole |
| CZ20011961A3 (cs) * | 1998-12-04 | 2002-02-13 | Basf Aktiengesellschaft | 3-(Heterocyclyl)+benzoylpyrazolové deriváty |
| DE19914140A1 (de) | 1999-03-27 | 2000-09-28 | Bayer Ag | Substituierte Benzoylpyrazole |
| US6541642B1 (en) | 1999-03-29 | 2003-04-01 | Nippon Soda Co., Ltd. | Process for the preparation of (e)-3-(1-propenyl)isoxazoline |
| CA2372500A1 (en) | 1999-04-27 | 2000-11-02 | Basf Aktiengesellschaft | Phosphoric benzoyl derivatives and their use as herbicides |
| AR024845A1 (es) | 1999-08-06 | 2002-10-30 | Basf Ag | Derivados de 1-cicloalquilpirazolil-benzoilo y sus sales, procedimiento para obtener dichos derivados, las composiciones herbicidas que los contienen y supreparacion, el procedimiento para controlar el crecimiento de plantas indeseadas con dichos derivados y el uso de dichos derivados como herbicida |
| DE19946853A1 (de) | 1999-09-30 | 2001-04-05 | Bayer Ag | Substituierte Arylketone |
| WO2001040221A2 (de) * | 1999-12-02 | 2001-06-07 | Basf Aktiengesellschaft | Cyclopropyl-anellierte 3-(4,5-dihydroisoxazol-3-yl)-substituierte benzoylpyrazole als herbizide |
| CN1402723A (zh) * | 1999-12-02 | 2003-03-12 | 巴斯福股份公司 | 作为除草剂的3－(4,5－二氢异噁唑－3－基)－取代的苯甲酰基吡唑 |
| CZ20022195A3 (cs) * | 1999-12-22 | 2003-03-12 | Basf Aktiengesellschaft | 3-(4,5-dihydroisoxazol-5-yl)benzoylpyrazoly |
| WO2001053275A2 (de) * | 2000-01-17 | 2001-07-26 | Bayer Aktiengesellschaft | Substituierte arylketone |
| AR032779A1 (es) * | 2000-12-11 | 2003-11-26 | Basf Ag | Derivados de ciclohexenona de benzazolonas, acidos benzazolonacarboxilicos, agentes que contienen por lo menos un derivado de ciclohexenona, procedimiento para combatir el crecimiento indeseado de plantas y uso de dichos derivados como herbicidas |
| BR0209099B1 (pt) | 2001-04-27 | 2013-04-24 | composiÇço seletivamente herbicida e mÉtodo para controlar o desenvolvimento de plantas indesejadas em colheitas de plantas éteis. | |
| WO2002090336A1 (de) * | 2001-05-09 | 2002-11-14 | Bayer Cropscience Ag | Substituierte arylketone |
| DE10136449A1 (de) * | 2001-05-09 | 2002-11-14 | Bayer Ag | Substituierte Arylketone |
| DE10138577A1 (de) * | 2001-05-21 | 2002-11-28 | Bayer Ag | Substituierte Benzoylpyrazole |
| DE10142336A1 (de) * | 2001-08-30 | 2003-03-20 | Bayer Cropscience Ag | Selektive Herbizide enthaltend ein Tetrazolinon-Derivat |
| DE10142333A1 (de) * | 2001-08-30 | 2003-03-20 | Bayer Cropscience Ag | Herbizide Mischungen auf Basis von substituierten Arylketonen |
| JP2005502701A (ja) * | 2001-09-11 | 2005-01-27 | バイエル クロップサイエンス ゲーエムベーハー | ３−ブロモメチル安息香酸の製造方法 |
| DE10159659A1 (de) * | 2001-12-05 | 2003-06-26 | Bayer Cropscience Ag | Herbizide auf Basis von substituierten Carbonsäureaniliden |
| DE10209645A1 (de) * | 2002-03-05 | 2003-09-18 | Bayer Cropscience Ag | Substituierte Arylketone |
| US20050239654A1 (en) * | 2002-07-23 | 2005-10-27 | Elmar Kibler | Synergistically acting herbicidal mixtures |
| WO2004010779A2 (en) * | 2002-07-24 | 2004-02-05 | Basf Aktiengesellschaft | Synergistically acting herbicidal mixtures |
| UA94003C2 (uk) * | 2006-11-28 | 2011-03-25 | Ишихара Санджай Кайша, Лтд. | Сполуки бензоїлпіразолу, гербіцид на їх основі та спосіб боротьби з небажаними рослинами |
| MX2010005231A (es) * | 2007-11-12 | 2010-05-27 | Du Pont | Mezcla herbicida. |
| WO2011067184A1 (de) | 2009-12-01 | 2011-06-09 | Basf Se | 3- (4, 5 -dihydroisoxazol- 5 -yl) benzoylpyrazolverbindungen und ihre mischungen mit safenern |
| DK2921492T3 (en) * | 2011-12-27 | 2017-12-11 | Bayer Ip Gmbh | HETEROARYLPIPERIDINE AND ¿PIPERAZINE DERIVATIVES |
| CN105399674B (zh) | 2015-12-31 | 2017-02-15 | 青岛清原化合物有限公司 | 吡唑类化合物或其盐、制备方法、除草剂组合物及用途 |
| CN105503728B (zh) | 2015-12-31 | 2017-03-22 | 青岛清原化合物有限公司 | 吡唑类化合物或其盐、制备方法、除草剂组合物及用途 |
| CN107629046B (zh) * | 2017-10-24 | 2021-07-06 | 青岛清原化合物有限公司 | 吡唑酮类化合物或其盐、除草剂组合物及用途 |
| WO2020114212A1 (zh) * | 2018-12-07 | 2020-06-11 | 青岛清原化合物有限公司 | 4-(3-杂环基-1-苯甲酰基)吡唑类化合物或其盐、制备方法、除草剂组合物及用途 |
| CN114787134B (zh) * | 2019-10-08 | 2023-12-19 | 沈阳中化农药化工研发有限公司 | 一种含烯的羧酸酯类化合物及其应用 |
| CN112624974B (zh) * | 2019-10-08 | 2024-01-30 | 沈阳中化农药化工研发有限公司 | 一种肉桂羧酸酯类化合物及其应用 |
Family Cites Families (7)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JPS58185568A (ja) * | 1982-04-24 | 1983-10-29 | Nissan Chem Ind Ltd | ピラゾ−ル誘導体，その製造方法および該誘導体を含有する選択性除草剤 |
| JPS58206568A (ja) * | 1982-05-25 | 1983-12-01 | Sankyo Co Ltd | ピラゾ−ル誘導体及び除草剤 |
| US4744815A (en) * | 1985-05-11 | 1988-05-17 | Nissan Chemical Industries, Ltd. | 4-benzoyl-1-alkyl (alkenyl) - pyrazoles, composition containing them, herbicidal method of using them, and intermediate in their preparation |
| IL85659A (en) * | 1987-03-17 | 1992-03-29 | Nissan Chemical Ind Ltd | 4-benzoylpyrazole derivatives,method for their preparation and herbicidal compositions containing them |
| KR19980702466A (ko) * | 1995-02-24 | 1998-07-15 | 페라 스타르크, 요헨 카르크 | 피라졸-4-일-벤조일 유도체 및 제초제로서의 그의 용도 |
| WO1997041105A1 (fr) * | 1996-04-26 | 1997-11-06 | Nippon Soda Co., Ltd. | Nouveaux derives de benzene a substitution heterocycle et herbicides |
| AU3297397A (en) * | 1996-06-06 | 1998-01-05 | E.I. Du Pont De Nemours And Company | Herbicidal pyridinyl and pyrazolylphenyl ketones |
-
1997
- 1997-01-08 US US09/091,292 patent/US6165944A/en not_active Expired - Fee Related
-
1998
- 1998-01-08 WO PCT/EP1998/000070 patent/WO1998031682A1/de active IP Right Grant
- 1998-01-08 EP EP98907930A patent/EP0958292B1/de not_active Expired - Lifetime
- 1998-01-08 DE DE59813869T patent/DE59813869D1/de not_active Expired - Lifetime
- 1998-01-08 MX MX9906600A patent/MX209959B/es not_active IP Right Cessation
- 1998-01-08 CN CN98802992A patent/CN1104429C/zh not_active Expired - Fee Related
- 1998-01-08 EE EEP199900292A patent/EE05291B1/xx not_active IP Right Cessation
- 1998-01-08 JP JP53362198A patent/JP4259620B2/ja not_active Expired - Fee Related
- 1998-01-08 BR BRPI9806917-9A patent/BR9806917B1/pt not_active IP Right Cessation
- 1998-01-08 CA CA002277893A patent/CA2277893C/en not_active Expired - Fee Related
- 1998-01-08 IL IL13077898A patent/IL130778A0/xx unknown
- 1998-01-08 SI SI9830875T patent/SI0958292T1/sl unknown
- 1998-01-08 KR KR1020067003690A patent/KR20060025610A/ko not_active Application Discontinuation
- 1998-01-08 KR KR19997006464A patent/KR100571463B1/ko not_active IP Right Cessation
- 1998-01-08 SK SK919-99A patent/SK286364B6/sk not_active IP Right Cessation
- 1998-01-08 NZ NZ336640A patent/NZ336640A/xx unknown
- 1998-01-08 TR TR1999/01665T patent/TR199901665T2/xx unknown
- 1998-01-08 HU HU0002178A patent/HU226012B1/hu not_active IP Right Cessation
- 1998-01-08 EA EA199900619A patent/EA009338B1/ru not_active IP Right Cessation
- 1998-01-08 PT PT98907930T patent/PT958292E/pt unknown
- 1998-01-08 PL PL98334849A patent/PL195943B1/pl not_active IP Right Cessation
- 1998-01-08 ES ES98907930T patent/ES2279569T3/es not_active Expired - Lifetime
- 1998-01-08 CZ CZ0252299A patent/CZ298050B6/cs not_active IP Right Cessation
- 1998-01-08 DK DK98907930T patent/DK0958292T3/da active
- 1998-01-08 AT AT98907930T patent/ATE350380T1/de not_active IP Right Cessation
- 1998-01-08 GE GEAP19984962A patent/GEP20022765B/en unknown
- 1998-01-08 AU AU66133/98A patent/AU742514B2/en not_active Ceased
- 1998-01-15 TW TW087100464A patent/TW513414B/zh not_active IP Right Cessation
- 1998-01-16 AR ARP980100214A patent/AR012836A1/es active IP Right Grant
- 1998-08-01 UA UA99084709A patent/UA60325C2/uk unknown
-
1999
- 1999-07-16 NO NO19993522A patent/NO314728B1/no not_active IP Right Cessation
- 1999-08-13 BG BG103663A patent/BG64389B1/bg unknown
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