DE102015215309A1 - Präparationstechnik von kohlenwasserstoffselektiven Gasdiffusionselektroden basierend auf Cu-haltigen-Katalysatoren - Google Patents
Präparationstechnik von kohlenwasserstoffselektiven Gasdiffusionselektroden basierend auf Cu-haltigen-Katalysatoren Download PDFInfo
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- DE102015215309A1 DE102015215309A1 DE102015215309.6A DE102015215309A DE102015215309A1 DE 102015215309 A1 DE102015215309 A1 DE 102015215309A1 DE 102015215309 A DE102015215309 A DE 102015215309A DE 102015215309 A1 DE102015215309 A1 DE 102015215309A1
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- 239000000758 substrate Substances 0.000 description 1
- 239000011593 sulfur Substances 0.000 description 1
- 229910052717 sulfur Inorganic materials 0.000 description 1
- 230000009897 systematic effect Effects 0.000 description 1
- 238000010345 tape casting Methods 0.000 description 1
- 230000002123 temporal effect Effects 0.000 description 1
- BFKJFAAPBSQJPD-UHFFFAOYSA-N tetrafluoroethene Chemical group FC(F)=C(F)F BFKJFAAPBSQJPD-UHFFFAOYSA-N 0.000 description 1
- 238000007669 thermal treatment Methods 0.000 description 1
- 239000010409 thin film Substances 0.000 description 1
- XOLBLPGZBRYERU-UHFFFAOYSA-N tin dioxide Chemical compound O=[Sn]=O XOLBLPGZBRYERU-UHFFFAOYSA-N 0.000 description 1
- 229910001887 tin oxide Inorganic materials 0.000 description 1
- GWBUNZLLLLDXMD-UHFFFAOYSA-H tricopper;dicarbonate;dihydroxide Chemical compound [OH-].[OH-].[Cu+2].[Cu+2].[Cu+2].[O-]C([O-])=O.[O-]C([O-])=O GWBUNZLLLLDXMD-UHFFFAOYSA-H 0.000 description 1
- 238000007704 wet chemistry method Methods 0.000 description 1
- 229910001928 zirconium oxide Inorganic materials 0.000 description 1
Images
Classifications
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- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
- C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
- C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
- C25B11/073—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material
- C25B11/091—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of at least one catalytic element and at least one catalytic compound; consisting of two or more catalytic elements or catalytic compounds
- C25B11/095—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of at least one catalytic element and at least one catalytic compound; consisting of two or more catalytic elements or catalytic compounds at least one of the compounds being organic
-
- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B3/00—Electrolytic production of organic compounds
- C25B3/20—Processes
- C25B3/25—Reduction
-
- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
- C25B11/02—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form
- C25B11/03—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form perforated or foraminous
- C25B11/031—Porous electrodes
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- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
- C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
- C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
-
- C—CHEMISTRY; METALLURGY
- C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
- C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
- C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
- C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
- C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
- C25B11/055—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the substrate or carrier material
- C25B11/057—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the substrate or carrier material consisting of a single element or compound
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- Materials Engineering (AREA)
- Metallurgy (AREA)
- Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)
- Electrodes For Compound Or Non-Metal Manufacture (AREA)
- Catalysts (AREA)
Priority Applications (10)
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| DE102015215309.6A DE102015215309A1 (de) | 2015-08-11 | 2015-08-11 | Präparationstechnik von kohlenwasserstoffselektiven Gasdiffusionselektroden basierend auf Cu-haltigen-Katalysatoren |
| DK16741915.9T DK3307924T3 (da) | 2015-08-11 | 2016-07-19 | Teknik til fremstilling af carbonhydrid-selektive gasdiffusionselektroder på basis af Cu-holdige katalysatorer |
| PCT/EP2016/067165 WO2017025285A1 (de) | 2015-08-11 | 2016-07-19 | Präparationstechnik von kohlenwasserstoffselektiven gasdiffusionselektroden basierend auf cu-haltigen-katalysatoren |
| EP16741915.9A EP3307924B1 (de) | 2015-08-11 | 2016-07-19 | Präparationstechnik von kohlenwasserstoffselektiven gasdiffusionselektroden basierend auf cu-haltigen-katalysatoren |
| US15/751,216 US20180230612A1 (en) | 2015-08-11 | 2016-07-19 | Method For Monitoring A Process For Powder-Bed Based Additive Manufacturing Of A Component And Such A System |
| PL16741915T PL3307924T3 (pl) | 2015-08-11 | 2016-07-19 | Sposób wytwarzania dyfuzyjnych elektrod gazowych selektywnych wobec węglowodorów bazujących na zawierających Cu katalizatorach |
| CN201680046786.8A CN107923052B (zh) | 2015-08-11 | 2016-07-19 | 基于含铜的催化剂的烃选择性气体扩散电极的制备技术 |
| ES16741915T ES2746118T3 (es) | 2015-08-11 | 2016-07-19 | Técnica de preparación de electrodos de difusión de gas selectivos a los hidrocarburos, a base de catalizadores que contienen Cu |
| AU2016305184A AU2016305184B2 (en) | 2015-08-11 | 2016-07-19 | Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts |
| SA518390888A SA518390888B1 (ar) | 2015-08-11 | 2018-02-06 | طريقة تحضير أقطاب توزيع الغاز انتقائية -الهيدروكربون اعتمادا على المحفزات المحتوية على النحاس |
Applications Claiming Priority (1)
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| DE102015215309.6A DE102015215309A1 (de) | 2015-08-11 | 2015-08-11 | Präparationstechnik von kohlenwasserstoffselektiven Gasdiffusionselektroden basierend auf Cu-haltigen-Katalysatoren |
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| DE102015215309A1 true DE102015215309A1 (de) | 2017-02-16 |
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| US (1) | US20180230612A1 (ko) |
| EP (1) | EP3307924B1 (ko) |
| CN (1) | CN107923052B (ko) |
| AU (1) | AU2016305184B2 (ko) |
| DE (1) | DE102015215309A1 (ko) |
| DK (1) | DK3307924T3 (ko) |
| ES (1) | ES2746118T3 (ko) |
| PL (1) | PL3307924T3 (ko) |
| SA (1) | SA518390888B1 (ko) |
| WO (1) | WO2017025285A1 (ko) |
Cited By (16)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| DE102017203903A1 (de) * | 2017-03-09 | 2018-09-13 | Siemens Aktiengesellschaft | Schwerlösliche Salze als Zuschlag zu Gasdiffusionselektroden zur Erhöhung der CO2-Selektivität bei hohen Stromdichten |
| DE102017204096A1 (de) | 2017-03-13 | 2018-09-13 | Siemens Aktiengesellschaft | Herstellung von Gasdiffusionselektroden mit Ionentransport-Harzen zur elektrochemischen Reduktion von CO2 zu chemischen Wertstoffen |
| DE102017203900A1 (de) | 2017-03-09 | 2018-09-13 | Siemens Aktiengesellschaft | Elektroden umfassend in Festkörperelektrolyten eingebrachtes Metall |
| DE102017208518A1 (de) | 2017-05-19 | 2018-11-22 | Siemens Aktiengesellschaft | Herstellung von dendritischen Elektrokatalysatoren zur Reduktion von CO2 und/oder CO |
| DE102017208610A1 (de) * | 2017-05-22 | 2018-11-22 | Siemens Aktiengesellschaft | Zwei-Membran-Aufbau zur elektrochemischen Reduktion von CO2 |
| WO2019015919A1 (de) * | 2017-07-18 | 2019-01-24 | Siemens Aktiengesellschaft | Co2-elektrolyseur |
| DE102017118118A1 (de) * | 2017-08-09 | 2019-02-14 | Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. | Elektrode für eine insbesondere bioelektrochemische Zelle |
| DE102017219766A1 (de) * | 2017-11-07 | 2019-05-09 | Siemens Aktiengesellschaft | Anordnung für die Kohlendioxid-Elektrolyse |
| DE102018212409A1 (de) | 2017-11-16 | 2019-05-16 | Siemens Aktiengesellschaft | Kohlenwasserstoff-selektive Elektrode |
| DE102018202184A1 (de) * | 2018-02-13 | 2019-08-14 | Siemens Aktiengesellschaft | Separatorlose Doppel-GDE-Zelle zur elektrochemischen Umsetzung |
| DE102018105115A1 (de) * | 2018-03-06 | 2019-09-12 | Deutsches Zentrum für Luft- und Raumfahrt e.V. | Elektrode, Zelleneinheit und Elektrolyseur |
| DE102018205571A1 (de) * | 2018-03-29 | 2019-10-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode, eine Elektrolyseanordnung sowie ein Verfahren zum Betreiben einer Elektrolyseanlage |
| WO2020001850A1 (de) | 2018-06-27 | 2020-01-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode zur kohlendioxid-verwertung, verfahren zu deren herstellung sowie elektrolysezelle mit gasdiffusionselektrode |
| DE102020205393A1 (de) | 2020-04-29 | 2021-11-04 | Siemens Aktiengesellschaft | Bimetallische und multimetallische Katalysatoren zur selektiven Elektroreduzierung von CO2 und/oder CO zu Kohlenwasserstoffen und Oxygenaten |
| DE102020206449A1 (de) | 2020-05-25 | 2021-11-25 | Siemens Aktiengesellschaft | Verfahren zum Befestigen einer Elektrode |
| DE102020206448A1 (de) | 2020-05-25 | 2021-11-25 | Siemens Aktiengesellschaft | Vorrichtung zum Befestigen einer Elektrode |
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| JP6622237B2 (ja) | 2017-03-14 | 2019-12-18 | 株式会社東芝 | 二酸化炭素電解装置 |
| JP6672211B2 (ja) * | 2017-03-21 | 2020-03-25 | 株式会社東芝 | 二酸化炭素電解装置および二酸化炭素電解方法 |
| US11299811B2 (en) * | 2018-01-29 | 2022-04-12 | Board Of Regents, The University Of Texas System | Continuous flow reactor and hybrid electro-catalyst for high selectivity production of C2H4 from CO2 and water via electrolysis |
| DE102018210457A1 (de) * | 2018-06-27 | 2020-01-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode zur Kohlendioxid-Verwertung, Verfahren zu deren Herstellung sowie Elektrolysezelle mit Gasdiffusionselektrode |
| DK3827114T3 (da) | 2018-07-23 | 2023-07-24 | Governing Council Univ Toronto | Katalysatorer til elektrokemisk co2 -reduktion og tilknyttede fremgangsmåder |
| CN109695048B (zh) * | 2019-02-28 | 2020-08-07 | 武汉大学 | 自支撑碳基体表面原位电化学生长纳米碳化物基电催化膜层的方法及应用 |
| CN111074294B (zh) * | 2019-12-12 | 2021-12-14 | 中国科学技术大学 | 一种铜合金材料电催化二氧化碳制备含碳化合物的方法 |
| CN115084540B (zh) * | 2021-03-10 | 2025-03-21 | 上海大学 | 一种具有亲水微孔层的气体扩散电极及其制备方法和应用 |
| CN114574889B (zh) * | 2021-12-13 | 2024-10-15 | 中国科学技术大学 | 一种气体扩散电极及其制备方法和应用 |
| CN114481184A (zh) * | 2021-12-21 | 2022-05-13 | 上海交通大学 | 一种用于二氧化碳电化学还原的气体扩散层及其制备方法 |
| CN114908375B (zh) * | 2022-05-25 | 2024-08-13 | 中国科学技术大学 | 电催化co2还原中具有稳定活性位点的铜催化剂及其制备方法与应用 |
| WO2024155694A2 (en) * | 2023-01-17 | 2024-07-25 | Texas Tech University System | Sonochemical synthesis methods and related applications |
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| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| DE102017203903A1 (de) * | 2017-03-09 | 2018-09-13 | Siemens Aktiengesellschaft | Schwerlösliche Salze als Zuschlag zu Gasdiffusionselektroden zur Erhöhung der CO2-Selektivität bei hohen Stromdichten |
| WO2018162202A1 (de) | 2017-03-09 | 2018-09-13 | Siemens Aktiengesellschaft | Schwerlösliche salze als zuschlag zu gasdiffusionselektroden zur erhöhung der co2-selektivität bei hohen stromdichten |
| DE102017203900A1 (de) | 2017-03-09 | 2018-09-13 | Siemens Aktiengesellschaft | Elektroden umfassend in Festkörperelektrolyten eingebrachtes Metall |
| CN110382741A (zh) * | 2017-03-09 | 2019-10-25 | 西门子股份公司 | 难溶性盐作为气体扩散电极中的添加剂用于提高在高电流密度下的co２选择性 |
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| WO2018166739A1 (de) | 2017-03-13 | 2018-09-20 | Siemens Aktiengesellschaft | Herstellung von gasdiffusionselektroden mit ionentransport-harzen zur elektrochemischen reduktion von co2 zu chemischen wertstoffen |
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| DE102017208610A1 (de) * | 2017-05-22 | 2018-11-22 | Siemens Aktiengesellschaft | Zwei-Membran-Aufbau zur elektrochemischen Reduktion von CO2 |
| US11932954B2 (en) | 2017-05-22 | 2024-03-19 | Siemens Energy Global GmbH & Co. KG | Two-membrane construction for electrochemically reducing CO2 |
| WO2019015919A1 (de) * | 2017-07-18 | 2019-01-24 | Siemens Aktiengesellschaft | Co2-elektrolyseur |
| DE102017118118A1 (de) * | 2017-08-09 | 2019-02-14 | Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. | Elektrode für eine insbesondere bioelektrochemische Zelle |
| DE102017219766A1 (de) * | 2017-11-07 | 2019-05-09 | Siemens Aktiengesellschaft | Anordnung für die Kohlendioxid-Elektrolyse |
| DE102018212409A1 (de) | 2017-11-16 | 2019-05-16 | Siemens Aktiengesellschaft | Kohlenwasserstoff-selektive Elektrode |
| WO2019096540A1 (de) | 2017-11-16 | 2019-05-23 | Siemens Aktiengesellschaft | Ethylenselektive elektrode mit gemischt-valentem cu4o3-katalysator |
| WO2019096985A1 (de) | 2017-11-16 | 2019-05-23 | Siemens Aktiengesellschaft | Kohlenwasserstoff-selektive elektrode |
| US11846031B2 (en) | 2017-11-16 | 2023-12-19 | Siemens Energy Global GmbH & Co. KG | Hydrocarbon-selective electrode |
| DE102018202184A1 (de) * | 2018-02-13 | 2019-08-14 | Siemens Aktiengesellschaft | Separatorlose Doppel-GDE-Zelle zur elektrochemischen Umsetzung |
| US12018393B2 (en) | 2018-02-13 | 2024-06-25 | Siemens Energy Global GmbH & Co. KG | Separatorless dual GDE cell for electrochemical reactions |
| DE102018105115A1 (de) * | 2018-03-06 | 2019-09-12 | Deutsches Zentrum für Luft- und Raumfahrt e.V. | Elektrode, Zelleneinheit und Elektrolyseur |
| DE102018205571A1 (de) * | 2018-03-29 | 2019-10-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode, eine Elektrolyseanordnung sowie ein Verfahren zum Betreiben einer Elektrolyseanlage |
| WO2020001850A1 (de) | 2018-06-27 | 2020-01-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode zur kohlendioxid-verwertung, verfahren zu deren herstellung sowie elektrolysezelle mit gasdiffusionselektrode |
| DE102018210458A1 (de) | 2018-06-27 | 2020-01-02 | Siemens Aktiengesellschaft | Gasdiffusionselektrode zur Kohlendioxid-Verwertung, Verfahren zu deren Herstellung sowie Elektrolysezelle mit Gasdiffusionselektrode |
| DE102020205393A1 (de) | 2020-04-29 | 2021-11-04 | Siemens Aktiengesellschaft | Bimetallische und multimetallische Katalysatoren zur selektiven Elektroreduzierung von CO2 und/oder CO zu Kohlenwasserstoffen und Oxygenaten |
| DE102020206449A1 (de) | 2020-05-25 | 2021-11-25 | Siemens Aktiengesellschaft | Verfahren zum Befestigen einer Elektrode |
| DE102020206448A1 (de) | 2020-05-25 | 2021-11-25 | Siemens Aktiengesellschaft | Vorrichtung zum Befestigen einer Elektrode |
| WO2021239338A1 (de) | 2020-05-25 | 2021-12-02 | Siemens Aktiengesellschaft | Verfahren zum befestigen einer elektrode |
| WO2021239340A1 (de) | 2020-05-25 | 2021-12-02 | Siemens Aktiengesellschaft | Vorrichtung zur platzierung eines elektrochemisch aktiven elements in einer elektrochemischen zelle, ihre herstellung und verwendung |
Also Published As
| Publication number | Publication date |
|---|---|
| ES2746118T3 (es) | 2020-03-04 |
| US20180230612A1 (en) | 2018-08-16 |
| WO2017025285A1 (de) | 2017-02-16 |
| SA518390888B1 (ar) | 2021-10-10 |
| EP3307924B1 (de) | 2019-06-19 |
| DK3307924T3 (da) | 2019-09-02 |
| AU2016305184B2 (en) | 2019-02-28 |
| EP3307924A1 (de) | 2018-04-18 |
| CN107923052B (zh) | 2020-06-19 |
| CN107923052A (zh) | 2018-04-17 |
| PL3307924T3 (pl) | 2020-01-31 |
| AU2016305184A1 (en) | 2018-02-01 |
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