WO2009020045A1 - 芳香族炭化水素の製造方法 - Google Patents

芳香族炭化水素の製造方法 Download PDF

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Publication number
WO2009020045A1
WO2009020045A1 PCT/JP2008/063773 JP2008063773W WO2009020045A1 WO 2009020045 A1 WO2009020045 A1 WO 2009020045A1 JP 2008063773 W JP2008063773 W JP 2008063773W WO 2009020045 A1 WO2009020045 A1 WO 2009020045A1
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WO
WIPO (PCT)
Prior art keywords
aromatic hydrocarbons
production
contact
molybdenum
solid catalyst
Prior art date
Application number
PCT/JP2008/063773
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English (en)
French (fr)
Inventor
Toru Nishimura
Shinobu Aoki
Yan Liu
Original Assignee
Mitsui Chemicals, Inc.
Agency For Science, Technology And Research
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Publication date
Application filed by Mitsui Chemicals, Inc., Agency For Science, Technology And Research filed Critical Mitsui Chemicals, Inc.
Priority to JP2009526417A priority Critical patent/JP5266225B2/ja
Priority to EP08791988.2A priority patent/EP2184269B1/en
Priority to CN200880101268A priority patent/CN101765575A/zh
Priority to US12/452,990 priority patent/US20100185034A1/en
Publication of WO2009020045A1 publication Critical patent/WO2009020045A1/ja

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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J29/00—Catalysts comprising molecular sieves
    • B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
    • B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • B01J29/70—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups B01J29/08 - B01J29/65
    • B01J29/78—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups B01J29/08 - B01J29/65 containing arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B01J29/7876—MWW-type, e.g. MCM-22, ERB-1, ITQ-1, PSH-3 or SSZ-25
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J29/00—Catalysts comprising molecular sieves
    • B01J29/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites
    • B01J29/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • B01J29/40—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the pentasil type, e.g. types ZSM-5, ZSM-8 or ZSM-11, as exemplified by patent documents US3702886, GB1334243 and US3709979, respectively
    • B01J29/48—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of the pentasil type, e.g. types ZSM-5, ZSM-8 or ZSM-11, as exemplified by patent documents US3702886, GB1334243 and US3709979, respectively containing arsenic, antimony, bismuth, vanadium, niobium tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0201—Impregnation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/08—Heat treatment
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/16—Reducing
    • B01J37/18—Reducing with gases containing free hydrogen
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
    • C07C2/76—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by condensation of hydrocarbons with partial elimination of hydrogen
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2529/00—Catalysts comprising molecular sieves
    • C07C2529/04—Catalysts comprising molecular sieves having base-exchange properties, e.g. crystalline zeolites, pillared clays
    • C07C2529/06—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof
    • C07C2529/70—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups C07C2529/08 - C07C2529/65
    • C07C2529/78—Crystalline aluminosilicate zeolites; Isomorphous compounds thereof of types characterised by their specific structure not provided for in groups C07C2529/08 - C07C2529/65 containing arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2400/00—Products obtained by processes covered by groups C10G9/00 - C10G69/14
    • C10G2400/30—Aromatics

Abstract

　本発明は、モリブデン含有固体触媒を用いて芳香族炭化水素を製造する方法であって、モリブデン含有固体触媒を活性化させ、高い収率を長時間維持し、メタンを主成分とする低級炭化水素ガスから効率的に芳香族炭化水素を製造する方法を提供することを課題としている。 　本発明の芳香族炭化水素の製造方法は、モリブデン含有固体触媒と、低級炭化水素および水素ガスから選ばれる１種以上の予備接触ガスとを予備接触させる工程と、予備接触させた触媒とメタンを主成分とする原料ガスとを接触させて反応させ、芳香族炭化水素を生成させる反応工程とを有し、予備接触の開始温度が反応温度よりも低温であり、予備接触の開始から終了までの温度が反応温度を超えないことを特徴としている。
PCT/JP2008/063773 2007-08-03 2008-07-31 芳香族炭化水素の製造方法 WO2009020045A1 (ja)

Priority Applications (4)

Application Number Priority Date Filing Date Title
JP2009526417A JP5266225B2 (ja) 2007-08-03 2008-07-31 芳香族炭化水素の製造方法
EP08791988.2A EP2184269B1 (en) 2007-08-03 2008-07-31 Process for production of aromatic hydrocarbons
CN200880101268A CN101765575A (zh) 2007-08-03 2008-07-31 芳香族烃的制造方法
US12/452,990 US20100185034A1 (en) 2007-08-03 2008-07-31 Process for producing aromatic hydrocarbon

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007-203221 2007-08-03
JP2007203221 2007-08-03

Publications (1)

Publication Number Publication Date
WO2009020045A1 true WO2009020045A1 (ja) 2009-02-12

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Country Status (5)

Country Link
US (1) US20100185034A1 (ja)
EP (1) EP2184269B1 (ja)
JP (1) JP5266225B2 (ja)
CN (1) CN101765575A (ja)
WO (1) WO2009020045A1 (ja)

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JP2012522899A (ja) * 2009-04-06 2012-09-27 ビーエーエスエフ ソシエタス・ヨーロピア 電気化学的に水素を除去することによって、天然ガスを芳香族化合物に変換する方法
WO2014027670A1 (ja) * 2012-08-16 2014-02-20 三井化学株式会社 触媒組成物、および該触媒組成物を用いた芳香族炭化水素の製造方法
US9079169B2 (en) 2010-05-12 2015-07-14 Shell Oil Company Methane aromatization catalyst, method of making and method of using the catalyst
CN111203259A (zh) * 2020-02-24 2020-05-29 湘潭大学 核壳型微波催化剂的制备方法及其在硫化氢分解中的应用

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