CN1677728A - 高温燃料电池的阳极材料 - Google Patents
高温燃料电池的阳极材料 Download PDFInfo
- Publication number
- CN1677728A CN1677728A CNA2005100624612A CN200510062461A CN1677728A CN 1677728 A CN1677728 A CN 1677728A CN A2005100624612 A CNA2005100624612 A CN A2005100624612A CN 200510062461 A CN200510062461 A CN 200510062461A CN 1677728 A CN1677728 A CN 1677728A
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- China
- Prior art keywords
- anode
- netted
- fuel cell
- layer
- heterogeneous
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Pending
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- 239000010405 anode material Substances 0.000 title claims abstract description 33
- 239000000446 fuel Substances 0.000 title claims abstract description 33
- 239000002245 particle Substances 0.000 claims abstract description 35
- 239000000919 ceramic Substances 0.000 claims abstract description 27
- 238000000034 method Methods 0.000 claims abstract description 22
- 230000008859 change Effects 0.000 claims abstract description 13
- 238000005245 sintering Methods 0.000 claims abstract description 11
- 230000002427 irreversible effect Effects 0.000 claims abstract description 9
- 239000000463 material Substances 0.000 claims abstract description 8
- 239000011343 solid material Substances 0.000 claims abstract description 8
- 239000000203 mixture Substances 0.000 claims abstract description 7
- 229910010293 ceramic material Inorganic materials 0.000 claims abstract description 6
- 239000002131 composite material Substances 0.000 claims abstract description 4
- 238000005259 measurement Methods 0.000 claims abstract description 3
- 239000007769 metal material Substances 0.000 claims abstract description 3
- 239000000758 substrate Substances 0.000 claims description 29
- 238000007254 oxidation reaction Methods 0.000 claims description 23
- 230000003647 oxidation Effects 0.000 claims description 22
- 229910052751 metal Inorganic materials 0.000 claims description 15
- 239000002184 metal Substances 0.000 claims description 15
- 238000007689 inspection Methods 0.000 claims description 9
- 238000010008 shearing Methods 0.000 claims description 8
- 230000006641 stabilisation Effects 0.000 claims description 8
- 239000003792 electrolyte Substances 0.000 claims description 6
- 230000002829 reductive effect Effects 0.000 claims description 6
- 150000001875 compounds Chemical class 0.000 claims description 5
- 230000033116 oxidation-reduction process Effects 0.000 claims description 5
- MCMNRKCIXSYSNV-UHFFFAOYSA-N Zirconium dioxide Chemical compound O=[Zr]=O MCMNRKCIXSYSNV-UHFFFAOYSA-N 0.000 claims description 4
- 239000007784 solid electrolyte Substances 0.000 claims description 4
- 238000005516 engineering process Methods 0.000 claims description 3
- 238000004519 manufacturing process Methods 0.000 claims description 3
- 238000005096 rolling process Methods 0.000 claims description 2
- 238000007650 screen-printing Methods 0.000 claims description 2
- 238000011105 stabilization Methods 0.000 claims description 2
- 230000008569 process Effects 0.000 abstract description 6
- 238000010998 test method Methods 0.000 abstract 2
- 238000011156 evaluation Methods 0.000 abstract 1
- PXHVJJICTQNCMI-UHFFFAOYSA-N Nickel Chemical compound [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 description 6
- 238000006722 reduction reaction Methods 0.000 description 6
- 239000007772 electrode material Substances 0.000 description 5
- 239000007789 gas Substances 0.000 description 5
- 230000009467 reduction Effects 0.000 description 5
- 238000007906 compression Methods 0.000 description 4
- 230000002349 favourable effect Effects 0.000 description 4
- 239000011159 matrix material Substances 0.000 description 4
- -1 oxonium ion Chemical class 0.000 description 4
- 230000006835 compression Effects 0.000 description 3
- 230000008602 contraction Effects 0.000 description 3
- 229910052759 nickel Inorganic materials 0.000 description 3
- CURLTUGMZLYLDI-UHFFFAOYSA-N Carbon dioxide Chemical compound O=C=O CURLTUGMZLYLDI-UHFFFAOYSA-N 0.000 description 2
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 description 2
- 239000004020 conductor Substances 0.000 description 2
- 238000011026 diafiltration Methods 0.000 description 2
- 238000010586 diagram Methods 0.000 description 2
- 238000009826 distribution Methods 0.000 description 2
- 239000010408 film Substances 0.000 description 2
- 230000014509 gene expression Effects 0.000 description 2
- 239000001257 hydrogen Substances 0.000 description 2
- 229910052739 hydrogen Inorganic materials 0.000 description 2
- 229910052760 oxygen Inorganic materials 0.000 description 2
- 230000035699 permeability Effects 0.000 description 2
- 230000002441 reversible effect Effects 0.000 description 2
- 238000007569 slipcasting Methods 0.000 description 2
- 238000005507 spraying Methods 0.000 description 2
- 208000010392 Bone Fractures Diseases 0.000 description 1
- UGFAIRIUMAVXCW-UHFFFAOYSA-N Carbon monoxide Chemical compound [O+]#[C-] UGFAIRIUMAVXCW-UHFFFAOYSA-N 0.000 description 1
- MYMOFIZGZYHOMD-UHFFFAOYSA-N Dioxygen Chemical compound O=O MYMOFIZGZYHOMD-UHFFFAOYSA-N 0.000 description 1
- 206010017076 Fracture Diseases 0.000 description 1
- 230000009471 action Effects 0.000 description 1
- 239000000654 additive Substances 0.000 description 1
- 230000000996 additive effect Effects 0.000 description 1
- 230000008485 antagonism Effects 0.000 description 1
- 230000004888 barrier function Effects 0.000 description 1
- 239000011324 bead Substances 0.000 description 1
- 230000006399 behavior Effects 0.000 description 1
- 230000015572 biosynthetic process Effects 0.000 description 1
- 229910002092 carbon dioxide Inorganic materials 0.000 description 1
- 239000001569 carbon dioxide Substances 0.000 description 1
- 229910002091 carbon monoxide Inorganic materials 0.000 description 1
- 238000006243 chemical reaction Methods 0.000 description 1
- 238000002485 combustion reaction Methods 0.000 description 1
- 230000001010 compromised effect Effects 0.000 description 1
- 238000010276 construction Methods 0.000 description 1
- 230000001419 dependent effect Effects 0.000 description 1
- 238000001514 detection method Methods 0.000 description 1
- 229910001882 dioxygen Inorganic materials 0.000 description 1
- 208000002173 dizziness Diseases 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 230000005611 electricity Effects 0.000 description 1
- 238000003487 electrochemical reaction Methods 0.000 description 1
- 238000003411 electrode reaction Methods 0.000 description 1
- 239000010419 fine particle Substances 0.000 description 1
- 238000005755 formation reaction Methods 0.000 description 1
- 238000010438 heat treatment Methods 0.000 description 1
- 238000005184 irreversible process Methods 0.000 description 1
- 229910044991 metal oxide Inorganic materials 0.000 description 1
- 150000004706 metal oxides Chemical class 0.000 description 1
- 150000002739 metals Chemical class 0.000 description 1
- 239000012299 nitrogen atmosphere Substances 0.000 description 1
- 239000001301 oxygen Substances 0.000 description 1
- 238000007747 plating Methods 0.000 description 1
- 230000000717 retained effect Effects 0.000 description 1
- 239000000126 substance Substances 0.000 description 1
- 239000010409 thin film Substances 0.000 description 1
- 230000009466 transformation Effects 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 1
Images
Classifications
-
- H—ELECTRICITY
- H04—ELECTRIC COMMUNICATION TECHNIQUE
- H04L—TRANSMISSION OF DIGITAL INFORMATION, e.g. TELEGRAPHIC COMMUNICATION
- H04L1/00—Arrangements for detecting or preventing errors in the information received
- H04L1/22—Arrangements for detecting or preventing errors in the information received using redundant apparatus to increase reliability
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/88—Processes of manufacture
- H01M4/8878—Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
- H01M4/8882—Heat treatment, e.g. drying, baking
- H01M4/8885—Sintering or firing
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B22—CASTING; POWDER METALLURGY
- B22F—WORKING METALLIC POWDER; MANUFACTURE OF ARTICLES FROM METALLIC POWDER; MAKING METALLIC POWDER; APPARATUS OR DEVICES SPECIALLY ADAPTED FOR METALLIC POWDER
- B22F3/00—Manufacture of workpieces or articles from metallic powder characterised by the manner of compacting or sintering; Apparatus specially adapted therefor ; Presses and furnaces
- B22F3/10—Sintering only
- B22F3/11—Making porous workpieces or articles
- B22F3/1103—Making porous workpieces or articles with particular physical characteristics
- B22F3/1112—Making porous workpieces or articles with particular physical characteristics comprising hollow spheres or hollow fibres
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B22—CASTING; POWDER METALLURGY
- B22F—WORKING METALLIC POWDER; MANUFACTURE OF ARTICLES FROM METALLIC POWDER; MAKING METALLIC POWDER; APPARATUS OR DEVICES SPECIALLY ADAPTED FOR METALLIC POWDER
- B22F3/00—Manufacture of workpieces or articles from metallic powder characterised by the manner of compacting or sintering; Apparatus specially adapted therefor ; Presses and furnaces
- B22F3/10—Sintering only
- B22F3/11—Making porous workpieces or articles
- B22F3/1103—Making porous workpieces or articles with particular physical characteristics
- B22F3/1118—Making porous workpieces or articles with particular physical characteristics comprising internal reinforcements
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B22—CASTING; POWDER METALLURGY
- B22F—WORKING METALLIC POWDER; MANUFACTURE OF ARTICLES FROM METALLIC POWDER; MAKING METALLIC POWDER; APPARATUS OR DEVICES SPECIALLY ADAPTED FOR METALLIC POWDER
- B22F3/00—Manufacture of workpieces or articles from metallic powder characterised by the manner of compacting or sintering; Apparatus specially adapted therefor ; Presses and furnaces
- B22F3/10—Sintering only
- B22F3/11—Making porous workpieces or articles
- B22F3/1143—Making porous workpieces or articles involving an oxidation, reduction or reaction step
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/8605—Porous electrodes
- H01M4/8621—Porous electrodes containing only metallic or ceramic material, e.g. made by sintering or sputtering
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/8647—Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/90—Selection of catalytic material
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
- H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M2004/8678—Inert electrodes with catalytic activity, e.g. for fuel cells characterised by the polarity
- H01M2004/8684—Negative electrodes
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/10—Fuel cells with solid electrolytes
- H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
- H01M2008/1293—Fuel cells with solid oxide electrolytes
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M2300/00—Electrolytes
- H01M2300/0017—Non-aqueous electrolytes
- H01M2300/0065—Solid electrolytes
- H01M2300/0068—Solid electrolytes inorganic
- H01M2300/0071—Oxides
- H01M2300/0074—Ion conductive at high temperature
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Electrochemistry (AREA)
- Manufacturing & Machinery (AREA)
- General Chemical & Material Sciences (AREA)
- Mechanical Engineering (AREA)
- Thermal Sciences (AREA)
- Physics & Mathematics (AREA)
- Composite Materials (AREA)
- Materials Engineering (AREA)
- Ceramic Engineering (AREA)
- Life Sciences & Earth Sciences (AREA)
- Sustainable Development (AREA)
- Sustainable Energy (AREA)
- Computer Networks & Wireless Communication (AREA)
- Signal Processing (AREA)
- Inert Electrodes (AREA)
- Fuel Cell (AREA)
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
EP04405189 | 2004-03-29 | ||
EP04405189.4 | 2004-03-29 |
Publications (1)
Publication Number | Publication Date |
---|---|
CN1677728A true CN1677728A (zh) | 2005-10-05 |
Family
ID=34932048
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
CNA2005100624612A Pending CN1677728A (zh) | 2004-03-29 | 2005-03-28 | 高温燃料电池的阳极材料 |
Country Status (5)
Country | Link |
---|---|
US (1) | US7691524B2 (ja) |
JP (1) | JP5234698B2 (ja) |
KR (1) | KR20060044867A (ja) |
CN (1) | CN1677728A (ja) |
AU (1) | AU2005201308A1 (ja) |
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN105431375A (zh) * | 2013-11-01 | 2016-03-23 | Lg化学株式会社 | 燃料电池及其制备方法 |
Families Citing this family (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
KR101154217B1 (ko) * | 2006-01-09 | 2012-06-18 | 생-고뱅 세라믹스 앤드 플라스틱스, 인코포레이티드 | 다공성 전극들을 갖는 연료 전지 부품 |
Family Cites Families (20)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
JP2511121B2 (ja) * | 1988-09-08 | 1996-06-26 | 三菱重工業株式会社 | 燃料電池の電極の製造方法 |
JPH0498766A (ja) * | 1990-08-14 | 1992-03-31 | Mitsubishi Heavy Ind Ltd | 固体電解質型燃料電池の燃料電極の製造方法 |
JP3246678B2 (ja) * | 1992-07-31 | 2002-01-15 | 三井造船株式会社 | 固体電解質型燃料電池の電極体の製造方法 |
NL9202087A (nl) * | 1992-12-01 | 1994-07-01 | Stichting Energie | Werkwijze voor het aanbrengen van een cermet electrodelaag op een gesinterd elektroliet. |
JPH08287926A (ja) * | 1995-04-17 | 1996-11-01 | Nippon Telegr & Teleph Corp <Ntt> | 固体電解質型燃料電池の製造方法 |
JPH08306361A (ja) * | 1995-04-28 | 1996-11-22 | Central Res Inst Of Electric Power Ind | 固体電解質燃料電池用燃料極材料およびその製造方法 |
US5993986A (en) * | 1995-11-16 | 1999-11-30 | The Dow Chemical Company | Solide oxide fuel cell stack with composite electrodes and method for making |
US5670270A (en) * | 1995-11-16 | 1997-09-23 | The Dow Chemical Company | Electrode structure for solid state electrochemical devices |
JP3380681B2 (ja) * | 1996-06-27 | 2003-02-24 | 京セラ株式会社 | 固体電解質型燃料電池セルの製造方法 |
JPH1021929A (ja) * | 1996-06-28 | 1998-01-23 | Kyocera Corp | 固体電解質型燃料電池セル |
US6790474B1 (en) | 1996-12-20 | 2004-09-14 | Tokyo Gas Co., Ltd. | Fuel electrode of solid oxide fuel cell and process for the production of the same |
JPH10247501A (ja) * | 1997-02-28 | 1998-09-14 | Toto Ltd | 固体電解質型燃料電池の燃料極の形成方法 |
JPH10241702A (ja) * | 1997-02-28 | 1998-09-11 | Mitsubishi Heavy Ind Ltd | 固体電解質型電気化学セルの燃料極 |
US5908713A (en) * | 1997-09-22 | 1999-06-01 | Siemens Westinghouse Power Corporation | Sintered electrode for solid oxide fuel cells |
DE19819453A1 (de) | 1998-04-30 | 1999-11-11 | Forschungszentrum Juelich Gmbh | SOFC-Brennstoffzelle mit einer Anodenzwischenschicht |
DE10031102C2 (de) * | 2000-06-30 | 2003-03-06 | Forschungszentrum Juelich Gmbh | Verfahren zur Herstellung eines Verbundkörpers, insbesondere einer Elektrode mit temperaturbeständiger Leitfähigkeit |
NL1016458C2 (nl) * | 2000-10-23 | 2002-05-01 | Stichting En Onderzoek Ct Nede | Anodesamenstel. |
US8114551B2 (en) | 2002-03-04 | 2012-02-14 | Sulzer Hexis Ag | Porous structured body for a fuel cell anode |
JP3976181B2 (ja) * | 2002-07-19 | 2007-09-12 | 東邦瓦斯株式会社 | 固体酸化物燃料電池単セル及びこれを用いた固体酸化物燃料電池 |
JP4201247B2 (ja) * | 2002-08-06 | 2008-12-24 | 財団法人電力中央研究所 | 固体酸化物形燃料電池用燃料極材料 |
-
2005
- 2005-02-21 JP JP2005043402A patent/JP5234698B2/ja not_active Expired - Fee Related
- 2005-03-15 US US11/081,351 patent/US7691524B2/en not_active Expired - Fee Related
- 2005-03-24 AU AU2005201308A patent/AU2005201308A1/en not_active Abandoned
- 2005-03-28 CN CNA2005100624612A patent/CN1677728A/zh active Pending
- 2005-03-28 KR KR1020050025634A patent/KR20060044867A/ko not_active Application Discontinuation
Cited By (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN105431375A (zh) * | 2013-11-01 | 2016-03-23 | Lg化学株式会社 | 燃料电池及其制备方法 |
CN105431375B (zh) * | 2013-11-01 | 2018-01-23 | Lg化学株式会社 | 燃料电池及其制备方法 |
Also Published As
Publication number | Publication date |
---|---|
JP5234698B2 (ja) | 2013-07-10 |
JP2005285750A (ja) | 2005-10-13 |
AU2005201308A1 (en) | 2005-10-13 |
US7691524B2 (en) | 2010-04-06 |
US20060083979A1 (en) | 2006-04-20 |
KR20060044867A (ko) | 2006-05-16 |
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WD01 | Invention patent application deemed withdrawn after publication |