WO2006120804A1 - Membre protecteur adhesif - Google Patents

Membre protecteur adhesif Download PDF

Info

Publication number
WO2006120804A1
WO2006120804A1 PCT/JP2006/305774 JP2006305774W WO2006120804A1 WO 2006120804 A1 WO2006120804 A1 WO 2006120804A1 JP 2006305774 W JP2006305774 W JP 2006305774W WO 2006120804 A1 WO2006120804 A1 WO 2006120804A1
Authority
WO
WIPO (PCT)
Prior art keywords
pressure
adhesive
sensitive adhesive
protective member
base material
Prior art date
Application number
PCT/JP2006/305774
Other languages
English (en)
Japanese (ja)
Inventor
Keiji Oka
Original Assignee
Piac Co., Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Piac Co., Ltd. filed Critical Piac Co., Ltd.
Priority to JP2007526828A priority Critical patent/JP4510084B2/ja
Publication of WO2006120804A1 publication Critical patent/WO2006120804A1/fr

Links

Classifications

    • A—HUMAN NECESSITIES
    • A61—MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61F—FILTERS IMPLANTABLE INTO BLOOD VESSELS; PROSTHESES; DEVICES PROVIDING PATENCY TO, OR PREVENTING COLLAPSING OF, TUBULAR STRUCTURES OF THE BODY, e.g. STENTS; ORTHOPAEDIC, NURSING OR CONTRACEPTIVE DEVICES; FOMENTATION; TREATMENT OR PROTECTION OF EYES OR EARS; BANDAGES, DRESSINGS OR ABSORBENT PADS; FIRST-AID KITS
    • A61F13/00—Bandages or dressings; Absorbent pads
    • A61F13/10—Bandages or dressings; Absorbent pads specially adapted for fingers, hands, or arms; Finger-stalls; Nail-protectors
    • A61F13/104—Bandages or dressings; Absorbent pads specially adapted for fingers, hands, or arms; Finger-stalls; Nail-protectors for the hands or fingers
    • A61F13/105—Bandages or dressings; Absorbent pads specially adapted for fingers, hands, or arms; Finger-stalls; Nail-protectors for the hands or fingers for the fingers; Finger-stalls; Nail-protectors
    • A—HUMAN NECESSITIES
    • A61—MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61P—SPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
    • A61P17/00—Drugs for dermatological disorders

Definitions

  • the present invention relates to an adhesive protective member, and more particularly, to an adhesive protective member having excellent usability because it can be applied with the back side of a finger exposed.
  • liquid bandages mainly composed of a hydrophilic colloidal water-soluble high molecule, a liquid hydrocarbon compound, and a drug have been proposed as salve prevention ointments and cut ointments (for example, Patent Document 1).
  • a film 104 provided with air holes 103 is coated with an adhesive, and the overall shape thereof is a circular part that is attached to each of the belly side and the back side of the finger.
  • the shape of the part with the constricted part 101 between 102 and the length of the part to be affixed to the abdomen and back of the finger is about the length from the fingertip to the front of the first joint.
  • a fingernail covering tape 100 is proposed in which the minimum width of the part 101 is approximately the same as or slightly narrower than the width of the fingernail, and is provided with a non-adhesive knot part 106 corresponding to the position of the constricted part 101. (For example, see Patent Document 2).
  • Patent Document 1 JP 2001-97848 (Claims)
  • Patent Document 2 JP-A-11-19118 (Claims)
  • Patent Document 1 the liquid adhesive bandage disclosed in Patent Document 1 has poor adhesion to the skin and tends to be insufficiently protected against biting spots and cuts, while being difficult to apply uniformly, When using computers, mobile phones, etc., or when hairdressers wash their hair, they tend to feel uncomfortable with their fingers! With nephew! A problem was seen.
  • the fingernail coating tape disclosed in Patent Document 2 has the advantage that it is difficult to peel off because it covers the fingernail, but when using a personal computer or a mobile phone, the finger feels uncomfortable. There was a big problem.
  • the present inventor can apply the planar shape with the back side of the finger exposed, while selectively covering the portion where the bite or cut occurs.
  • the present invention has been completed by finding that an excellent usability can be obtained even when a personal computer, a mobile phone, or the like is used.
  • an object of the present invention is to provide a pressure-sensitive adhesive protective member that can selectively coat a portion where biting or cutting has occurred, has excellent protection, and provides an excellent feeling of use.
  • At least the pressure-sensitive adhesive layer and the base material, and the surface side of the finger along the longitudinal direction of the finger or the force of applying so as to cover the periphery of the fingernail surface A pressure-sensitive adhesive protection member is provided so that the planar shape of the pressure-sensitive adhesive protection member is approximately crescent, oval, circular, square, or polygonal. The problem can be solved.
  • the planar shape of the adhesive protection member by setting the planar shape of the adhesive protection member to a predetermined shape, it can be applied with the back side of the finger exposed, while it may be bitten or cut around the fingernail or along the longitudinal direction of the finger. Only the resulting part can be coated. Therefore, it is necessary to protect the biting points and cuts effectively without causing a sense of incongruity to the finger. Can do.
  • the planar shape of the adhesive protective member is a substantially crescent shape, and that the scabs generated around the fingernail are protected.
  • the scabs generated around the fingernails can be effectively protected.
  • JIS-L-1096 compliant is 400% or more, and it is preferable to laminate a reinforcing peeling member on the surface of the substrate.
  • the side surface of the adhesive protection member and the side surface of another adhesion protection member include an engagement member for engagement.
  • the moisture permeability of the substrate measured in accordance with JIS Z-0208 should be a value within the range of 100 to 900 g / m 2 '24Hrs. Is preferred.
  • the pressure-sensitive adhesive layer contains an inorganic filler in the range of 0.1 to LO weight% with respect to the total amount. It is preferable that it is composed of an adhesive.
  • the first embodiment includes at least a pressure-sensitive adhesive layer and a base material, and covers the surface side of the finger along the longitudinal direction of the finger or the force applied to cover the periphery of the fingernail.
  • the adhesive protection member is a sticking protection member in which the planar shape of the adhesion protection member is approximately crescent, oval, circular, square, or polygonal.
  • it includes at least an adhesive layer 14 and a base material 12, and is used for adhesion protection so as to cover the periphery of the fingernail so as to cover the surface.
  • the adhesive protection member 10 of the first embodiment is suitable for scab protection, and the finger is removed with the peeling member 16 removed. It is intended to be used by sticking so that the area around the nail 30 is covered. That is, it is used in a state where it covers a part of the side surface of the finger 31 but does not cover the back side of the finger 31 so that the finger does not feel strange.
  • an embodiment of the adhesive protection member 10 of the first embodiment will be described mainly as an adhesion protection member for scabs.
  • Examples of the base material that constitutes a part of the adhesive protective member include, but are not limited to, polyurethane film, polyester film, chlorinated film, olefin film, polycarbonate film, polysulfone film, polyphenylene sulfide film, A polyimide film, paper, a film containing a fiber, etc. are mentioned.
  • the form of the substrate is not particularly limited.
  • it may be a mesh-like material, or a woven or non-woven fabric.
  • a mesh-like material is used as a non-woven fabric, it can be used as an adhesive protective member for scabs that is extremely excellent in cushioning and air permeability.
  • a woven fabric made of polyester fiber or the like the moisture permeability can be kept low, and the adhesive protection member for peas can be made excellent in followability to finger movement.
  • the elongation rate of the base material is 400% or more because excellent usability is easily obtained. A value within the range is more preferable.
  • a reinforcing release member 16 ′ should be laminated on the surface of the base material 12, as shown in FIG. 1 (c). Is preferred. By laminating the reinforcing release member in this way, it can be easily applied to a predetermined location, can selectively cover the portion where the bite or cut has occurred, and can also be used as a process paper at the time of manufacture. It is also possible to demonstrate the function.
  • the reinforcing peeling member exhibits a function as a reinforcing member in addition to the function as a peeling member. Therefore, the reinforcing peeling member includes a reinforcing material such as a fiber or an inorganic filler, or is thicker than a normal peeling member. It is preferable to increase the mechanical strength.
  • the thickness of the base material to be applied is a value within the range of 5 to 2,000 m. The reason for this is that if the thickness of the base material to be applied is less than 5 m, the mechanical strength is lowered and may not be suitable for use as an adhesive protective member for scab.
  • the thickness of the strong base material exceeds 2,000 m, it will become excessively thick and difficult to handle. This is because they may be peeled off. Therefore, it is more preferable to set the thickness of the base material to a value in the range of 10 to: L, OOO / zm, and it is more preferable to set a value in the range of 20-500 ⁇ m.
  • the elongation percentage of the base material (based on JIS-L-1096) is 400% or more and the thickness of the base material is 10 to 30 / ⁇ ⁇ , excellent usability is obtained. It can be said that it is easy to obtain.
  • the planar shape of the adhesive protection member is approximately three. It is characterized by being a moon, ellipse, circle, square, or polygon. Then, in order to apply the cover around the fingernail so as to cover the surface of the fingernail, as shown in FIG. 1 (a), the planar shape of the base material 12 can be covered around the fingernail. In addition, it is more preferable to have a substantially crescent shape. That is, a force that is an example of a substantially crescent shape, as shown in FIG.
  • the distance (tl) between the inner side surface 10a and the outer side surface 10b arranged approximately square is a value of about 2 to 30 mm.
  • the distance (t2) between the inner side surface 10a and the outer side surface 10b on the right side surface 10c and the left side surface 10d is a value smaller than tl and a value of about 0.5 to 20 mm.
  • the distance (t3) between the tip of the right side surface 10c and the tip of the left side surface 10d is a value of about 5 to 25 mm.
  • planar shape makes it easier to follow the movement of the finger, reduces the load on the adhesive layer, and does not easily peel off.
  • an inner side surface 10a of a substantially crescent-shaped adhesive protection member 10 and an outer side surface 10b of another substantially crescent-shaped adhesive protection member 10 It is preferable to provide an engaging member 11 for engaging with each other. That is, even if the inner side surface 10a of the substantially crescent-shaped adhesive protection member 10 and the outer side surface 10b of another adjacent substantially crescent-shaped adhesive protection member 10 are partial, they are engaged and contacted as sides. It is preferable to have In the case of the adhesive protecting member 10 shown in FIG. 3, the flat portion located at the center of the inner side surface 10a and the outer side surface 10b is the engaging member 11 in this case.
  • this configuration allows a plurality of adhesive protection members to be arranged without gaps, which is extremely advantageous in terms of space saving. Further, if a plurality of adhesive protection members can be arranged without gaps, the plurality of adhesive protection members can be formed by continuous cutting, which is advantageous in terms of the manufacturing process.
  • the distance (t ′ 1) between the inner side surface 10a and the square-arranged outer side surface 10b is the inner side surface 10a of the right side surface 10c and the left side surface 10d, and The distance between the outer side surface 10b and the distance (2) is substantially equal to about 2 to 30 mm. Further, the distance (3) between the tip of the right side surface 10c and the tip of the left side surface 10d is a value of about 5 to 25 mm.
  • the substantially crescent-shaped planar shape basically consists of straight portions, and the right side surface 10c and the left side surface More preferably, both 10d and the linear partial force are configured.
  • flap portions 10e and 10f are provided on the side surface of the substantially crescent-shaped adhesive protection member 10.
  • the shape of the flap portion is not particularly limited, but various shapes such as a semicircular shape, an oval shape, a rectangular shape, a square shape, a triangular shape, and a corrugated shape can be employed.
  • a water repellent treatment layer including a sizing layer 11 on the surface of the substrate 12.
  • such a water repellent layer also constitutes, for example, fluorine resin or silicone resin.
  • the moisture permeability of the substrate measured in accordance with JIS Z-0208 is preferably set to a value in the range of 100 to 900 gZm 2 '24Hrs.
  • the reason for this is that by controlling the moisture permeability of the base material in this way, it is easy to prevent the entry of liquid substances from the outside even in the water work, the outside work, or the medical field, etc. This is not only preferable, but also because it can effectively prevent the adhesive protective member from peeling off.
  • the moisture permeability of the substrate to a value within the range of 150 ⁇ 800gZm 2 '24Hrs More preferably, the value is more preferably in the range of 200 to 700 gZm 2 ′ 24 Hrs.
  • the water vapor permeability of the measured substrate is 1000 g / m 2 ⁇ 24Hrs or more! /.
  • an identification mark corresponding to the type of the fingernail or a decorative layer 13 is provided on the surface of the base material 12.
  • the adhesive protection member 10 of the optimum size can be clearly identified. This is because the ease of use when using the adhesive protective member 10 can be remarkably improved.
  • the type of the pressure-sensitive adhesive constituting the pressure-sensitive adhesive layer is not particularly limited.
  • an organopolysiloxane pressure sensitive adhesive as a main component in the adhesive layer.
  • organopolysiloxane pressure-sensitive adhesive can provide appropriate adhesion to the skin, while improving creep resistance, water resistance, and chemical resistance. It is because it can do.
  • organopolysiloxane pressure-sensitive adhesive for example, a silicone resin having a structure represented by the general formula (1) or the general formula (2) is blended and dehydrated and condensed. Organopolysiloxane obtained by this is preferable.
  • R and R are each a methyl group or a phenyl group, and n is 10 to L000.
  • m represents an integer of 10 to 10,000.
  • R 1 and R 2 are each a methyl group or a phenyl group.
  • the mole ratio of the phenyl group is preferably set to a value in the range of 25Z75 to 98Z2, more preferably in the range of 85/15 to 95/5. preferable.
  • n and m are usually in the range of 2000 to 200,000 cP of pressure-sensitive adhesive, considering the workability of forming an adhesive layer on the nonwoven fabric. It is preferable to adjust the value to be (25 ° C).
  • an inorganic filler in the range of 0.1 to 10% by weight based on the total amount in the organopolysiloxane pressure-sensitive adhesive.
  • the amount of the inorganic filler added is set to a value in the range of 1 to LO weight%, preferably in the range of 3 to 7 weight% with respect to the total amount.
  • the organopolysiloxane pressure-sensitive adhesive may remain on the skin as an adherend, and the added amount is less than 10% by weight. In such a case, the cohesive strength of the pressure-sensitive adhesive is excessively improved, and the pressure-sensitive adhesive strength may be significantly reduced.
  • the inorganic filler in the range of 0.5 to 8% by weight, more preferably 1 to 5% by weight, based on the total amount.
  • the average particle diameter of the inorganic filler contained in the organopolysiloxane-based pressure-sensitive adhesive is preferably 1 to 20 ⁇ m, preferably 4 to 12 ⁇ m.
  • the inorganic filler tends to aggregate and it is difficult to uniformly disperse it in the organopolysiloxane pressure sensitive adhesive. This is because there may be cases.
  • the average particle diameter of the inorganic filler exceeds 10 m, the thickness of the formed adhesive layer is usually 25 to 30 / ⁇ ⁇ , so that the inorganic filler protrudes on the surface and becomes rough. This is because a feeling may be given.
  • the sedimentation rate of the inorganic filler in the organopolysiloxane pressure-sensitive adhesive increases in the manufacturing process, making it difficult to achieve a uniform dispersion state. This is because there are cases.
  • the inorganic filler include, for example, one kind of calcium carbonate, bentonite, titanium oxide, zinc oxide, carion, silica, or a combination of two or more kinds.
  • organopolysiloxane pressure sensitive adhesive 10-30% by weight of the total amount
  • organopolysiloxane pressure sensitive adhesive 100% by weight of the total amount
  • a typical example of such an acrylic pressure-sensitive adhesive is, for example, an acrylic copolymer mainly composed of 2-ethylhexyl acrylate and butyl acrylate.
  • the blending ratio of 2-ethylhexyl acrylate and butyl acrylate is adjusted to be 20:80 to 80:20, preferably 20:80 to 40:60 by weight. .
  • the proportion of 2-ethylhexyl acrylate is excessively large, the cohesive force of the pressure-sensitive adhesive tends to be too low and the pressure-sensitive adhesive force tends to decrease.
  • acrylamide or vinyl carboxylic acid may be blended within a range not exceeding 5% by weight with respect to the total amount.
  • the viscosity of the acrylic pressure-sensitive adhesive is preferably set to a value within the range of 500 to 20000 cP (25 ° C.).
  • organic peroxides such as peroxybenzoyl and peroxyditamyl and platinum catalysts are used. It is preferable to add in the range of 1.5 to 3% by weight based on the solid content of the organopolysiloxane adhesive.
  • a preparation can be added to the pressure-sensitive adhesive composition as a kind of additive so as to exhibit a predetermined medicinal effect.
  • the type of such a preparation is not particularly limited.
  • anti-inflammatory drugs for example, anti-inflammatory drugs, anti-inflammatory analgesics, coronary vasodilators, asthma drugs, antihypertensive drugs, antihistamines, tranquilizers, antibiotics, anesthetics
  • one kind of vitamin preparation or a combination of two or more kinds can be mentioned.
  • the amount of the preparation added varies depending on the type of preparation and the application of the pressure-sensitive adhesive composition.
  • the value is within a range of 0.1 to 30% by mass with respect to the total amount of the pressure-sensitive adhesive composition. Can preferable.
  • additives it is preferable to add various additives to the pressure-sensitive adhesive composition.
  • the peel adhesive strength (mode: T-mode peel, adherend: stainless steel plate, peel speed: 300 mmZmin) of the adhesive protective member compliant with JIS Z0237 it is preferable to set the peel adhesive strength (mode: T-mode peel, adherend: stainless steel plate, peel speed: 300 mmZmin) of the adhesive protective member compliant with JIS Z0237 to a value within the range of 300 to 2000 gZ25 mm.
  • the strong peel adhesion is less than 300 gZ25 mmmm, it peels easily from the skin and the like, and may have a poor function as an adhesive protective member.
  • the strong peel adhesion exceeds 2000 g / 25 mm, it may be difficult to remove the adhesive from the skin, or the skin irritation may be excessively high, resulting in discomfort during use. Because there is.
  • the peel adhesive strength of the strong adhesive protection member it is more preferable to set the peel adhesive strength of the strong adhesive protection member to a value in the range of 500 to 1500 g / 25 mm, and it is more preferable to set the value in the range of 900 to 1200 g / 25 mm.
  • the second embodiment includes at least a pressure-sensitive adhesive layer and a base material, and covers the surface side of the finger along the longitudinal direction of the finger or the force of applying so as to cover the periphery of the fingernail.
  • a method for producing an adhesive protection member wherein the planar shape of the adhesion protection member is approximately crescent, oval, circular, quadrangular, or polygonal. It is a manufacturing method of the adhesion protection member containing these process (a)-(b).
  • the pressure-sensitive adhesive layer 14 is formed on the peeling member 16.
  • the method for forming the pressure-sensitive adhesive layer 14 is not particularly limited, but the pressure-sensitive adhesive composition is uniformly applied onto the substrate using, for example, a roll coater, comma coater, knife coater, or the like. Thus, it can be easily manufactured.
  • the type of the pressure-sensitive adhesive composition it is also preferable to heat-treat under certain conditions in order to scatter the solvent or to perform a crosslinking treatment.
  • a reinforcing release member 16 composed of a silicone release paper, a silicone release film, or the like is laminated on the surface in advance.
  • the substrate 12 is further laminated on the pressure-sensitive adhesive layer 14 on the peeling member 16.
  • the method of laminating the base material 12 is not particularly limited, but for example, a laminate, a press roll, or the like can be used.
  • the laminate with the substrate 12 laminated using the cutting jig 20 is cut into a predetermined shape as shown in Fig.
  • This is a process for forming the protective member 10.
  • a cutter, knife, laser, cutting frame, etc. can be used as the cutting jig 20.
  • FIG. L (a) to (b) are a plan view and a cross-sectional view of an adhesive protective member (adhesive protective member for scabs) according to the present invention, and (c) includes a reinforcing peeling member.
  • FIG. 3 is a cross-sectional view of an adhesive protection member (adhesive protection member for scabs).
  • FIG. 2 (a) and (b) are diagrams for explaining the usage state of the adhesive protective member (sticky adhesive protective member) of the present invention.
  • FIG. 3 is a diagram for explaining a state in which a plurality of adhesive protection members are arranged side by side.
  • ⁇ 4 It is a plan view of an adhesive protective member provided with a flap.
  • FIG. 5 (a) to (c) are diagrams used to explain a water-repellent treatment layer of an adhesive protective member, a base material as a nonwoven fabric, and a decoration layer.
  • FIG. 6 (a) to (d) are views for explaining a method for producing an adhesive protective member.
  • FIG. 7 is a schematic view showing a conventional fingernail covering tape.
  • Adhesive protective member (adhesive protective member for sharks)

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  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Dermatology (AREA)
  • Engineering & Computer Science (AREA)
  • Veterinary Medicine (AREA)
  • Public Health (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Animal Behavior & Ethology (AREA)
  • Vascular Medicine (AREA)
  • Heart & Thoracic Surgery (AREA)
  • Biomedical Technology (AREA)
  • Bioinformatics & Cheminformatics (AREA)
  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Nuclear Medicine, Radiotherapy & Molecular Imaging (AREA)
  • Organic Chemistry (AREA)
  • Pharmacology & Pharmacy (AREA)
  • Adhesive Tapes (AREA)
  • Medicinal Preparation (AREA)

Abstract

Membre protecteur adhésif permettant des sensations d'utilisation excellentes sans provoquer d'inconfort même lors de l'utilisation d'un ordinateur personnel ou d'un téléphone mobile. Le membre protecteur adhésif selon l'invention comprend au moins une couche d'agent adhésif et un matériau de base et doit être collé sur un ongle de façon à en recouvrir la surface périphérique ou sur un doigt de façon à en recouvrir la surface dans le sens de la longueur. Le membre protecteur adhésif présente une forme sensiblement en chevron, elliptique, circulaire, carrée ou polygonale dans une vue en plan.
PCT/JP2006/305774 2005-05-10 2006-03-23 Membre protecteur adhesif WO2006120804A1 (fr)

Priority Applications (1)

Application Number Priority Date Filing Date Title
JP2007526828A JP4510084B2 (ja) 2005-05-10 2006-03-23 さかむけ用粘着保護部材およびその製造方法

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2005-136945 2005-05-10
JP2005136945 2005-05-10

Publications (1)

Publication Number Publication Date
WO2006120804A1 true WO2006120804A1 (fr) 2006-11-16

Family

ID=37396322

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/JP2006/305774 WO2006120804A1 (fr) 2005-05-10 2006-03-23 Membre protecteur adhesif

Country Status (2)

Country Link
JP (2) JP4510084B2 (fr)
WO (1) WO2006120804A1 (fr)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2017130838A1 (fr) * 2016-01-29 2017-08-03 王子ホールディングス株式会社 Bandage adhésif
EP3211687A1 (fr) * 2016-02-24 2017-08-30 Nitto Denko Corporation Bande isolante

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JP2004222749A (ja) * 2003-01-17 2004-08-12 Daisuke Irie 指先用絆創膏

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JPH0666651U (ja) * 1993-03-02 1994-09-20 泰男 佐藤 指先用ガーゼ付ばんそうこう
JP2004222749A (ja) * 2003-01-17 2004-08-12 Daisuke Irie 指先用絆創膏

Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2017130838A1 (fr) * 2016-01-29 2017-08-03 王子ホールディングス株式会社 Bandage adhésif
CN108601678A (zh) * 2016-01-29 2018-09-28 王子控股株式会社 创可贴
US11266539B2 (en) 2016-01-29 2022-03-08 Oji Holdings Corporation Adhesive tape
EP3211687A1 (fr) * 2016-02-24 2017-08-30 Nitto Denko Corporation Bande isolante
CN107118704A (zh) * 2016-02-24 2017-09-01 日东电工株式会社 绝缘带

Also Published As

Publication number Publication date
JP4927967B2 (ja) 2012-05-09
JP4510084B2 (ja) 2010-07-21
JPWO2006120804A1 (ja) 2008-12-18
JP2010148932A (ja) 2010-07-08

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