JPWO2019031080A1 - 排ガス浄化用のメタル基材及びそれを用いた排ガス浄化装置 - Google Patents
排ガス浄化用のメタル基材及びそれを用いた排ガス浄化装置 Download PDFInfo
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- 229910052751 metal Inorganic materials 0.000 title claims abstract description 73
- 239000002184 metal Substances 0.000 title claims abstract description 73
- 238000000746 purification Methods 0.000 title claims abstract description 46
- 239000000758 substrate Substances 0.000 title claims abstract description 32
- 239000011888 foil Substances 0.000 claims abstract description 148
- 239000000463 material Substances 0.000 claims abstract description 33
- 239000003054 catalyst Substances 0.000 claims description 13
- 239000011148 porous material Substances 0.000 abstract description 5
- 229910044991 metal oxide Inorganic materials 0.000 description 10
- 150000004706 metal oxides Chemical class 0.000 description 10
- 230000000052 comparative effect Effects 0.000 description 7
- 229910000510 noble metal Inorganic materials 0.000 description 6
- 238000002485 combustion reaction Methods 0.000 description 4
- 238000004080 punching Methods 0.000 description 4
- 238000004519 manufacturing process Methods 0.000 description 3
- 239000002243 precursor Substances 0.000 description 3
- 239000002002 slurry Substances 0.000 description 3
- KDLHZDBZIXYQEI-UHFFFAOYSA-N Palladium Chemical compound [Pd] KDLHZDBZIXYQEI-UHFFFAOYSA-N 0.000 description 2
- MCMNRKCIXSYSNV-UHFFFAOYSA-N Zirconium dioxide Chemical compound O=[Zr]=O MCMNRKCIXSYSNV-UHFFFAOYSA-N 0.000 description 2
- 239000011248 coating agent Substances 0.000 description 2
- 238000000576 coating method Methods 0.000 description 2
- 230000000694 effects Effects 0.000 description 2
- 238000010304 firing Methods 0.000 description 2
- 238000000034 method Methods 0.000 description 2
- 239000002245 particle Substances 0.000 description 2
- 230000002093 peripheral effect Effects 0.000 description 2
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical compound [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 description 2
- PNEYBMLMFCGWSK-UHFFFAOYSA-N aluminium oxide Inorganic materials [O-2].[O-2].[O-2].[Al+3].[Al+3] PNEYBMLMFCGWSK-UHFFFAOYSA-N 0.000 description 1
- 238000005219 brazing Methods 0.000 description 1
- CETPSERCERDGAM-UHFFFAOYSA-N ceric oxide Chemical compound O=[Ce]=O CETPSERCERDGAM-UHFFFAOYSA-N 0.000 description 1
- 229910000422 cerium(IV) oxide Inorganic materials 0.000 description 1
- 239000002131 composite material Substances 0.000 description 1
- 230000003247 decreasing effect Effects 0.000 description 1
- 230000006866 deterioration Effects 0.000 description 1
- 238000009792 diffusion process Methods 0.000 description 1
- 238000009826 distribution Methods 0.000 description 1
- 239000000446 fuel Substances 0.000 description 1
- 238000010030 laminating Methods 0.000 description 1
- 229910052763 palladium Inorganic materials 0.000 description 1
- 229910052697 platinum Inorganic materials 0.000 description 1
- 239000010970 precious metal Substances 0.000 description 1
- 229910001404 rare earth metal oxide Inorganic materials 0.000 description 1
- 229910052703 rhodium Inorganic materials 0.000 description 1
- 239000010948 rhodium Substances 0.000 description 1
- MHOVAHRLVXNVSD-UHFFFAOYSA-N rhodium atom Chemical compound [Rh] MHOVAHRLVXNVSD-UHFFFAOYSA-N 0.000 description 1
- 238000005096 rolling process Methods 0.000 description 1
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J35/00—Catalysts, in general, characterised by their form or physical properties
- B01J35/40—Catalysts, in general, characterised by their form or physical properties characterised by dimensions, e.g. grain size
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/92—Chemical or biological purification of waste gases of engine exhaust gases
- B01D53/94—Chemical or biological purification of waste gases of engine exhaust gases by catalytic processes
- B01D53/9404—Removing only nitrogen compounds
- B01D53/9409—Nitrogen oxides
- B01D53/9431—Processes characterised by a specific device
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J35/00—Catalysts, in general, characterised by their form or physical properties
- B01J35/50—Catalysts, in general, characterised by their form or physical properties characterised by their shape or configuration
- B01J35/56—Foraminous structures having flow-through passages or channels, e.g. grids or three-dimensional monoliths
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- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
- F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
- F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
- F01N3/24—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by constructional aspects of converting apparatus
- F01N3/28—Construction of catalytic reactors
- F01N3/2803—Construction of catalytic reactors characterised by structure, by material or by manufacturing of catalyst support
- F01N3/2807—Metal other than sintered metal
- F01N3/281—Metallic honeycomb monoliths made of stacked or rolled sheets, foils or plates
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
- F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
- F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
- F01N3/24—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by constructional aspects of converting apparatus
- F01N3/28—Construction of catalytic reactors
- F01N3/2803—Construction of catalytic reactors characterised by structure, by material or by manufacturing of catalyst support
- F01N3/2807—Metal other than sintered metal
- F01N3/281—Metallic honeycomb monoliths made of stacked or rolled sheets, foils or plates
- F01N3/2821—Metallic honeycomb monoliths made of stacked or rolled sheets, foils or plates the support being provided with means to enhance the mixing process inside the converter, e.g. sheets, plates or foils with protrusions or projections to create turbulence
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/10—Noble metals or compounds thereof
- B01D2255/102—Platinum group metals
- B01D2255/1021—Platinum
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2255/00—Catalysts
- B01D2255/10—Noble metals or compounds thereof
- B01D2255/102—Platinum group metals
- B01D2255/1025—Rhodium
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/92—Chemical or biological purification of waste gases of engine exhaust gases
- B01D53/94—Chemical or biological purification of waste gases of engine exhaust gases by catalytic processes
- B01D53/9445—Simultaneously removing carbon monoxide, hydrocarbons or nitrogen oxides making use of three-way catalysts [TWC] or four-way-catalysts [FWC]
- B01D53/945—Simultaneously removing carbon monoxide, hydrocarbons or nitrogen oxides making use of three-way catalysts [TWC] or four-way-catalysts [FWC] characterised by a specific catalyst
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
- B01J23/54—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
- B01J23/56—Platinum group metals
- B01J23/63—Platinum group metals with rare earths or actinides
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N2330/00—Structure of catalyst support or particle filter
- F01N2330/02—Metallic plates or honeycombs, e.g. superposed or rolled-up corrugated or otherwise deformed sheet metal
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N2330/00—Structure of catalyst support or particle filter
- F01N2330/02—Metallic plates or honeycombs, e.g. superposed or rolled-up corrugated or otherwise deformed sheet metal
- F01N2330/04—Methods of manufacturing
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N2330/00—Structure of catalyst support or particle filter
- F01N2330/30—Honeycomb supports characterised by their structural details
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N2330/00—Structure of catalyst support or particle filter
- F01N2330/30—Honeycomb supports characterised by their structural details
- F01N2330/38—Honeycomb supports characterised by their structural details flow channels with means to enhance flow mixing,(e.g. protrusions or projections)
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
- F01N3/02—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust
- F01N3/021—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust by means of filters
- F01N3/022—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust by means of filters characterised by specially adapted filtering structure, e.g. honeycomb, mesh or fibrous
- F01N3/0222—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust by means of filters characterised by specially adapted filtering structure, e.g. honeycomb, mesh or fibrous the structure being monolithic, e.g. honeycombs
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- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Materials Engineering (AREA)
- Organic Chemistry (AREA)
- Combustion & Propulsion (AREA)
- Health & Medical Sciences (AREA)
- Toxicology (AREA)
- Mechanical Engineering (AREA)
- General Engineering & Computer Science (AREA)
- Environmental & Geological Engineering (AREA)
- Analytical Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Biomedical Technology (AREA)
- Catalysts (AREA)
- Exhaust Gas Treatment By Means Of Catalyst (AREA)
- Exhaust Gas After Treatment (AREA)
- Vaporization, Distillation, Condensation, Sublimation, And Cold Traps (AREA)
Abstract
Description
《態様1》
波箔と平箔とが積層されて筒状になっている排ガス浄化用の孔あきメタル基材であって、
50個/平方インチ〜800個/平方インチのセルを有し、
前記波箔が、前記セルの平均開孔面積の2.0倍以上50倍以下の面積を有する複数の第1の孔を有し、
前記平箔が、前記セルの平均開孔面積の3.0倍以上100倍以下の面積を有する複数の第2の孔を有し、かつ
前記波箔の前記第1の孔の面積の平均値が、前記平箔の前記第2の孔の面積の平均値よりも小さい、
孔あきメタル基材。
《態様2》
前記波箔の前記第1の孔の合計面積が、前記波箔の全ての孔の合計面積の60%以上であり、かつ/又は前記平箔の前記第2の孔の合計面積が、前記平箔の全ての孔の合計面積の60%以上である、態様1に記載の孔あきメタル基材。
《態様3》
前記波箔の前記第1の孔が、3.0mm2〜100mm2の面積を有し、かつ前記平箔の前記第2の孔が、5.0mm2〜200mm2の面積を有する、態様1又は2に記載の孔あきメタル基材。
《態様4》
前記波箔の前記第1の孔の面積の平均値に対する、前記平箔の前記第2の孔の面積の平均値の比が、1.5〜10.0の範囲である、態様1〜3のいずれか一項に記載の孔あきメタル基材。
《態様5》
平箔及び波箔の開孔率が、それぞれ10%〜90%の範囲である、態様1〜4のいずれか一項に記載の孔あきメタル基材。
《態様6》
前記セルの平均開孔面積が、0.50mm2〜7.0mm2である、態様1〜5のいずれか一項に記載の孔あきメタル基材。
《態様7》
前記波箔及び前記平箔の厚みが、それぞれ20μm〜500μmの範囲である、態様1〜6のいずれか一項に記載の孔あきメタル基材。
《態様8》
態様1〜7のいずれか一項に記載の孔あきメタル基材、及び前記孔あきメタル基材上に形成された触媒層を有する、排ガス浄化装置。
1 波箔
1a 第1の孔
2 平箔
2a 第2の孔
3 セル
4 外筒
Claims (8)
- 波箔と平箔とが積層されて筒状になっている排ガス浄化用の孔あきメタル基材であって、
50個/平方インチ〜800個/平方インチのセルを有し、
前記波箔が、前記セルの平均開孔面積の2.0倍以上50倍以下の面積を有する複数の第1の孔を有し、
前記平箔が、前記セルの平均開孔面積の3.0倍以上100倍以下の面積を有する複数の第2の孔を有し、かつ
前記波箔の前記第1の孔の面積の平均値が、前記平箔の前記第2の孔の面積の平均値よりも小さい、
孔あきメタル基材。 - 前記波箔の前記第1の孔の合計面積が、前記波箔の全ての孔の合計面積の60%以上であり、かつ/又は前記平箔の前記第2の孔の合計面積が、前記平箔の全ての孔の合計面積の60%以上である、請求項1に記載の孔あきメタル基材。
- 前記波箔の前記第1の孔が、3.0mm2〜100mm2の面積を有し、かつ前記平箔の前記第2の孔が、5.0mm2〜200mm2の面積を有する、請求項1又は2に記載の孔あきメタル基材。
- 前記波箔の前記第1の孔の面積の平均値に対する、前記平箔の前記第2の孔の面積の平均値の比が、1.5〜10.0の範囲である、請求項1〜3のいずれか一項に記載の孔あきメタル基材。
- 平箔及び波箔の開孔率が、それぞれ10%〜90%の範囲である、請求項1〜4のいずれか一項に記載の孔あきメタル基材。
- 前記セルの平均開孔面積が、0.50mm2〜7.0mm2である、請求項1〜5のいずれか一項に記載の孔あきメタル基材。
- 前記波箔及び前記平箔の厚みが、それぞれ20μm〜500μmの範囲である、請求項1〜6のいずれか一項に記載の孔あきメタル基材。
- 請求項1〜7のいずれか一項に記載の孔あきメタル基材、及び前記孔あきメタル基材上に形成された触媒層を有する、排ガス浄化装置。
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JP2017153273 | 2017-08-08 | ||
JP2017153273 | 2017-08-08 | ||
PCT/JP2018/023890 WO2019031080A1 (ja) | 2017-08-08 | 2018-06-22 | 排ガス浄化用のメタル基材及びそれを用いた排ガス浄化装置 |
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JP6505336B1 JP6505336B1 (ja) | 2019-04-24 |
JPWO2019031080A1 true JPWO2019031080A1 (ja) | 2019-11-07 |
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US (1) | US11135577B2 (ja) |
EP (1) | EP3666377B1 (ja) |
JP (1) | JP6505336B1 (ja) |
CN (1) | CN110997142B (ja) |
TW (1) | TWI769281B (ja) |
WO (1) | WO2019031080A1 (ja) |
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JP7106565B2 (ja) | 2017-10-27 | 2022-07-26 | 株式会社キャタラー | メタル基材を用いた排ガス浄化装置及びその製造方法 |
JP6742457B1 (ja) * | 2019-02-05 | 2020-08-19 | 株式会社キャタラー | 排ガス浄化用のメタル基材及びそれを用いた排ガス浄化装置 |
CN113874111A (zh) * | 2019-05-24 | 2021-12-31 | 本田技研工业株式会社 | 废气净化催化剂结构体及其制造方法 |
JP2023123886A (ja) * | 2020-07-22 | 2023-09-06 | ヤマハ発動機株式会社 | 排ガス浄化装置、鞍乗型車両および排ガス浄化装置の製造方法 |
JP6975359B1 (ja) | 2021-07-30 | 2021-12-01 | 日鉄ケミカル&マテリアル株式会社 | 触媒担持用基材及び触媒担体 |
US20230080614A1 (en) * | 2021-09-15 | 2023-03-16 | Sentec E&E Co., Ltd. | Metal honeycomb substrate |
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CA1102706A (en) * | 1977-05-06 | 1981-06-09 | Rainer Scholz | Monolithic metal catalyst for the detoxication of the exhaust gases of internal combustion engines |
US4382323A (en) * | 1980-07-10 | 1983-05-10 | General Motors Corporation | Method for manufacturing a wound foil structure comprising distinct catalysts |
US4318888A (en) * | 1980-07-10 | 1982-03-09 | General Motors Corporation | Wound foil structure comprising distinct catalysts |
US4829655A (en) * | 1987-03-24 | 1989-05-16 | W. R. Grace & Co.-Conn. | Catalyst support and method for making same |
US4931421A (en) * | 1988-06-27 | 1990-06-05 | Motonobu Shibata | Catalyst carriers and a method for producing the same |
JPH02171232A (ja) * | 1988-12-23 | 1990-07-02 | Showa Aircraft Ind Co Ltd | ハニカム構造体 |
DE69420342T2 (de) * | 1993-02-12 | 2000-02-24 | Nippon Steel Corp., Tokio/Tokyo | Metallische wabenstruktur zur verwendung als katalysator und verfahren zu deren herstellung |
JPH06320014A (ja) * | 1993-03-17 | 1994-11-22 | Nippondenso Co Ltd | メタル担体 |
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2018
- 2018-06-22 CN CN201880051673.6A patent/CN110997142B/zh active Active
- 2018-06-22 US US16/633,522 patent/US11135577B2/en active Active
- 2018-06-22 WO PCT/JP2018/023890 patent/WO2019031080A1/ja unknown
- 2018-06-22 JP JP2018553174A patent/JP6505336B1/ja active Active
- 2018-06-22 EP EP18843816.2A patent/EP3666377B1/en active Active
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CN110997142A (zh) | 2020-04-10 |
CN110997142B (zh) | 2022-10-11 |
TW201909993A (zh) | 2019-03-16 |
TWI769281B (zh) | 2022-07-01 |
EP3666377A1 (en) | 2020-06-17 |
US20200230586A1 (en) | 2020-07-23 |
EP3666377B1 (en) | 2021-11-10 |
WO2019031080A1 (ja) | 2019-02-14 |
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US11135577B2 (en) | 2021-10-05 |
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