JP5650403B2 - プロトン伝導性電解質用の、スルホニルがグラフト化された複素環材料 - Google Patents

プロトン伝導性電解質用の、スルホニルがグラフト化された複素環材料 Download PDF

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JP5650403B2
JP5650403B2 JP2009543293A JP2009543293A JP5650403B2 JP 5650403 B2 JP5650403 B2 JP 5650403B2 JP 2009543293 A JP2009543293 A JP 2009543293A JP 2009543293 A JP2009543293 A JP 2009543293A JP 5650403 B2 JP5650403 B2 JP 5650403B2
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polymer
proton
heterocyclic compound
proton conducting
sulfonated
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JP2011507979A5 (enExample
JP2011507979A (ja
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リ,シウェン
チョウ,チェン
チャン,ユエラン
リュー,メイリン
リ,ウェン
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トヨタ モーター エンジニアリング アンド マニュファクチャリング ノース アメリカ,インコーポレイティド
トヨタ モーター エンジニアリング アンド マニュファクチャリング ノース アメリカ,インコーポレイティド
ジョージア テク リサーチ コーポレイション
ジョージア テク リサーチ コーポレイション
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    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/103Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having nitrogen, e.g. sulfonated polybenzimidazoles [S-PBI], polybenzimidazoles with phosphoric acid, sulfonated polyamides [S-PA] or sulfonated polyphosphazenes [S-PPh]
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G59/00Polycondensates containing more than one epoxy group per molecule; Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups
    • C08G59/18Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing
    • C08G59/20Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing characterised by the epoxy compounds used
    • C08G59/22Di-epoxy compounds
    • C08G59/30Di-epoxy compounds containing atoms other than carbon, hydrogen, oxygen and nitrogen
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G61/00Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
    • C08G61/02Macromolecular compounds containing only carbon atoms in the main chain of the macromolecule, e.g. polyxylylenes
    • C08G61/10Macromolecular compounds containing only carbon atoms in the main chain of the macromolecule, e.g. polyxylylenes only aromatic carbon atoms, e.g. polyphenylenes
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G73/00Macromolecular compounds obtained by reactions forming a linkage containing nitrogen with or without oxygen or carbon in the main chain of the macromolecule, not provided for in groups C08G12/00 - C08G71/00
    • C08G73/06Polycondensates having nitrogen-containing heterocyclic rings in the main chain of the macromolecule
    • C08G73/18Polybenzimidazoles
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04Polysiloxanes
    • C08G77/22Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen
    • C08G77/28Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen sulfur-containing groups
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20Manufacture of shaped structures of ion-exchange resins
    • C08J5/22Films, membranes or diaphragms
    • C08J5/2206Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218Synthetic macromolecular compounds
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1037Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having silicon, e.g. sulfonated crosslinked polydimethylsiloxanes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00Electrolytes
    • H01M2300/0017Non-aqueous electrolytes
    • H01M2300/0065Solid electrolytes
    • H01M2300/0082Organic polymers
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Manufacturing & Machinery (AREA)
  • Electrochemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Conductive Materials (AREA)
  • Fuel Cell (AREA)
  • Polyethers (AREA)
  • Polymers With Sulfur, Phosphorus Or Metals In The Main Chain (AREA)
  • Epoxy Resins (AREA)
  • Macromolecular Compounds Obtained By Forming Nitrogen-Containing Linkages In General (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Silicon Polymers (AREA)
JP2009543293A 2006-12-21 2007-12-28 プロトン伝導性電解質用の、スルホニルがグラフト化された複素環材料 Expired - Fee Related JP5650403B2 (ja)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US11/614,198 US7964651B2 (en) 2006-12-21 2006-12-21 Sulfonyl grafted heterocycle materials for proton conducting electrolytes
PCT/US2007/089056 WO2008091475A1 (en) 2006-12-21 2007-12-28 Sulfonyl grafted heterocycle materials for proton conducting electrolytes

Publications (3)

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JP2011507979A JP2011507979A (ja) 2011-03-10
JP2011507979A5 JP2011507979A5 (enExample) 2011-04-21
JP5650403B2 true JP5650403B2 (ja) 2015-01-07

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JP2009543293A Expired - Fee Related JP5650403B2 (ja) 2006-12-21 2007-12-28 プロトン伝導性電解質用の、スルホニルがグラフト化された複素環材料

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US (1) US7964651B2 (enExample)
JP (1) JP5650403B2 (enExample)
CN (1) CN101230113B (enExample)
DE (1) DE102007060692B4 (enExample)
WO (1) WO2008091475A1 (enExample)

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US8519074B2 (en) * 2010-01-15 2013-08-27 The University of Massachusettes Comb polymers for supramolecular nanoconfinement
JP2014009190A (ja) * 2012-06-29 2014-01-20 Shikoku Chem Corp イミダゾールシラン化合物、合成方法及びその利用
CN103467991A (zh) * 2013-09-23 2013-12-25 上海大学 双草酸硼酸盐离子液体掺杂磺化聚苯硫醚质子交换膜材料及其制备方法
CN107033350B (zh) * 2017-03-31 2019-07-23 上海大学 质子交换膜用膦酸和1,2,3-三唑功能化聚醚砜及其制备方法
CN115873150B (zh) * 2021-09-27 2024-10-22 山东东岳未来氢能材料股份有限公司 一类带有吡啶侧基的全氟离子聚合物及其合成方法与应用
CN119264301A (zh) * 2021-09-27 2025-01-07 山东东岳未来氢能材料股份有限公司 带有联吡啶侧基的长寿命质子交换膜及制备方法
CN115873154B (zh) * 2021-09-27 2024-10-22 山东东岳未来氢能材料股份有限公司 带有三联吡啶侧基的全氟离子聚合物及合成方法与应用

Family Cites Families (16)

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US3574593A (en) 1967-07-21 1971-04-13 American Cyanamid Co Herbicidal method using substituted alkylsulfonylimidazoles
EP0532408A1 (fr) * 1991-09-13 1993-03-17 Saint-Gobain Vitrage International Polymère conducteur protonique, application en tant qu'électrolyte dans des dispositifs électrochimiques
US5525436A (en) 1994-11-01 1996-06-11 Case Western Reserve University Proton conducting polymers used as membranes
US5827602A (en) 1995-06-30 1998-10-27 Covalent Associates Incorporated Hydrophobic ionic liquids
US6248469B1 (en) 1997-08-29 2001-06-19 Foster-Miller, Inc. Composite solid polymer electrolyte membranes
US6310110B1 (en) 1999-07-30 2001-10-30 Michael A. Markowitz Molecularly-imprinted material made by template-directed synthesis
DE10017654A1 (de) 2000-04-08 2001-10-18 Degussa Organosiliciumverbindungen
US20040122256A1 (en) * 2001-02-01 2004-06-24 Masanori Ikeda Perfluorvinyl ether monomer having sulfonamide group
WO2002062749A1 (fr) * 2001-02-01 2002-08-15 Asahi Kasei Kabushiki Kaisha Monomere d'ether perfluorovinylique ayant un groupe sulfonamide
DE10163518A1 (de) 2001-12-21 2003-07-10 Fraunhofer Ges Forschung Protonenleitfähige Membranen/Schichten und Verfahren zu deren Herstellung
US6987163B2 (en) 2002-08-07 2006-01-17 Research Foundation Of The State University Of New York Modified polybenzimidazole (PBI) membranes for enhanced polymer electrochemical cells
US6878475B2 (en) 2002-11-22 2005-04-12 T/J Technologies, Inc. Membrane for fuel cell, and fuel cell incorporating that membrane
JP5085132B2 (ja) * 2003-05-28 2012-11-28 トヨタ モーター エンジニアリング アンド マニュファクチャリング ノース アメリカ,インコーポレイティド イミダゾール環末端可撓性分岐をグラフトしたハイブリッド無機−有機ポリマーを基剤とするポリマー電解質膜(pem)
JP3904083B2 (ja) * 2003-07-10 2007-04-11 株式会社豊田中央研究所 高分子電解質組成物
JP3896105B2 (ja) * 2003-08-28 2007-03-22 株式会社東芝 燃料電池用電解質膜、及び燃料電池
US7576165B2 (en) * 2004-01-27 2009-08-18 Georgia Institute Of Technology Heterocycle grafted monomers and related polymers and hybrid inorganic-organic polymer membranes

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Publication number Publication date
CN101230113B (zh) 2013-05-22
US7964651B2 (en) 2011-06-21
DE102007060692A1 (de) 2008-09-11
DE102007060692B4 (de) 2021-05-27
US20080152985A1 (en) 2008-06-26
WO2008091475A1 (en) 2008-07-31
JP2011507979A (ja) 2011-03-10
CN101230113A (zh) 2008-07-30

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