JP4630064B2 - 運転停止した燃料電池発電設備内のガス組成を決定するシステムおよび作動方法 - Google Patents
運転停止した燃料電池発電設備内のガス組成を決定するシステムおよび作動方法 Download PDFInfo
- Publication number
- JP4630064B2 JP4630064B2 JP2004536614A JP2004536614A JP4630064B2 JP 4630064 B2 JP4630064 B2 JP 4630064B2 JP 2004536614 A JP2004536614 A JP 2004536614A JP 2004536614 A JP2004536614 A JP 2004536614A JP 4630064 B2 JP4630064 B2 JP 4630064B2
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- Prior art keywords
- fuel cell
- anode
- flow
- hydrogen
- voltage
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- Expired - Lifetime
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- 239000000446 fuel Substances 0.000 title claims description 149
- 239000000203 mixture Substances 0.000 title claims description 47
- 238000000034 method Methods 0.000 title claims description 33
- 239000001257 hydrogen Substances 0.000 claims description 71
- 229910052739 hydrogen Inorganic materials 0.000 claims description 71
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 claims description 69
- 239000007789 gas Substances 0.000 claims description 48
- 230000001590 oxidative effect Effects 0.000 claims description 31
- 239000007800 oxidant agent Substances 0.000 claims description 24
- 238000001514 detection method Methods 0.000 claims description 23
- 239000012530 fluid Substances 0.000 claims description 23
- 239000003792 electrolyte Substances 0.000 claims description 16
- 239000000376 reactant Substances 0.000 claims description 16
- 238000004891 communication Methods 0.000 claims description 9
- 238000010248 power generation Methods 0.000 claims description 8
- 230000001568 sexual effect Effects 0.000 claims 1
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 27
- 239000001301 oxygen Substances 0.000 description 27
- 229910052760 oxygen Inorganic materials 0.000 description 27
- 239000003570 air Substances 0.000 description 19
- 239000011261 inert gas Substances 0.000 description 8
- 238000005260 corrosion Methods 0.000 description 7
- 230000007797 corrosion Effects 0.000 description 7
- 239000000758 substrate Substances 0.000 description 6
- 239000003054 catalyst Substances 0.000 description 5
- 238000012544 monitoring process Methods 0.000 description 5
- 238000010926 purge Methods 0.000 description 5
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 4
- 230000015556 catabolic process Effects 0.000 description 4
- 238000006731 degradation reaction Methods 0.000 description 4
- 238000012360 testing method Methods 0.000 description 4
- 229910019142 PO4 Inorganic materials 0.000 description 3
- 238000006243 chemical reaction Methods 0.000 description 3
- 230000005611 electricity Effects 0.000 description 3
- 125000004435 hydrogen atom Chemical group [H]* 0.000 description 3
- 239000012528 membrane Substances 0.000 description 3
- NBIIXXVUZAFLBC-UHFFFAOYSA-K phosphate Chemical compound [O-]P([O-])([O-])=O NBIIXXVUZAFLBC-UHFFFAOYSA-K 0.000 description 3
- 239000010452 phosphate Substances 0.000 description 3
- MYMOFIZGZYHOMD-UHFFFAOYSA-N Dioxygen Chemical compound O=O MYMOFIZGZYHOMD-UHFFFAOYSA-N 0.000 description 2
- 230000007423 decrease Effects 0.000 description 2
- 229910001882 dioxygen Inorganic materials 0.000 description 2
- 238000004519 manufacturing process Methods 0.000 description 2
- 239000011159 matrix material Substances 0.000 description 2
- VNWKTOKETHGBQD-UHFFFAOYSA-N methane Chemical compound C VNWKTOKETHGBQD-UHFFFAOYSA-N 0.000 description 2
- 229910052757 nitrogen Inorganic materials 0.000 description 2
- 230000003134 recirculating effect Effects 0.000 description 2
- 230000002378 acidificating effect Effects 0.000 description 1
- 239000012080 ambient air Substances 0.000 description 1
- 230000000712 assembly Effects 0.000 description 1
- 238000000429 assembly Methods 0.000 description 1
- 239000000919 ceramic Substances 0.000 description 1
- 238000010586 diagram Methods 0.000 description 1
- 238000009792 diffusion process Methods 0.000 description 1
- 239000003502 gasoline Substances 0.000 description 1
- 150000002431 hydrogen Chemical class 0.000 description 1
- -1 hydrogen ions Chemical class 0.000 description 1
- 239000007788 liquid Substances 0.000 description 1
- 239000000463 material Substances 0.000 description 1
- 238000005259 measurement Methods 0.000 description 1
- 239000003345 natural gas Substances 0.000 description 1
- 239000003758 nuclear fuel Substances 0.000 description 1
- 230000003647 oxidation Effects 0.000 description 1
- 238000007254 oxidation reaction Methods 0.000 description 1
- 230000033116 oxidation-reduction process Effects 0.000 description 1
- 239000005518 polymer electrolyte Substances 0.000 description 1
- 239000011148 porous material Substances 0.000 description 1
- 229910021426 porous silicon Inorganic materials 0.000 description 1
- 230000036647 reaction Effects 0.000 description 1
- 238000006479 redox reaction Methods 0.000 description 1
- 230000001105 regulatory effect Effects 0.000 description 1
- 230000000717 retained effect Effects 0.000 description 1
- 230000002441 reversible effect Effects 0.000 description 1
- HBMJWWWQQXIZIP-UHFFFAOYSA-N silicon carbide Chemical compound [Si+]#[C-] HBMJWWWQQXIZIP-UHFFFAOYSA-N 0.000 description 1
- 239000007787 solid Substances 0.000 description 1
- 238000011895 specific detection Methods 0.000 description 1
- 239000000126 substance Substances 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Chemical compound O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 1
Images
Classifications
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
- H01M8/241—Grouping of fuel cells, e.g. stacking of fuel cells with solid or matrix-supported electrolytes
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
- H01M8/0258—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/02—Details
- H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
- H01M8/0267—Collectors; Separators, e.g. bipolar separators; Interconnectors having heating or cooling means, e.g. heaters or coolant flow channels
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
- H01M8/04223—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids during start-up or shut-down; Depolarisation or activation, e.g. purging; Means for short-circuiting defective fuel cells
- H01M8/04228—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids during start-up or shut-down; Depolarisation or activation, e.g. purging; Means for short-circuiting defective fuel cells during shut-down
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
- H01M8/04298—Processes for controlling fuel cells or fuel cell systems
- H01M8/043—Processes for controlling fuel cells or fuel cell systems applied during specific periods
- H01M8/04303—Processes for controlling fuel cells or fuel cell systems applied during specific periods applied during shut-down
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
- H01M8/2457—Grouping of fuel cells, e.g. stacking of fuel cells with both reactants being gaseous or vaporised
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
- H01M8/2465—Details of groupings of fuel cells
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
Description
Claims (3)
- a. 水素含有還元性流体流れおよびプロセス酸化剤反応物流れから電流を生成するための燃料電池12であって、電解質18の両側にアノード電極14およびカソード電極16と、アノード電極14に隣接して流れるように還元性流体流れを導くための、アノード電極14に隣接するアノード流れ区域28と、カソード電極16に隣接して流れるようにプロセス酸化剤流れを導くための、カソード電極16に隣接するカソード流れ区域30と、アノード流れ区域28内へ還元性流体を選択的に導入するための、アノード流れ区域28と流体連通するように取り付けられたアノード入口弁62とを含む、少なくとも一つの燃料電池12と、
b. 電源88と、燃料電池12の電圧を測定するための電圧測定装置90と、検出器回路スイッチ92とを含み、燃料電池12と電気的に接続するように取り付けられた検出器回路86であって、電源88が所定の検出継続時間の間、燃料電池12に所定の検出電流を供給することができるように電源88が検出器回路スイッチ92を介して燃料電池12に取り付けられている、検出器回路86と、
を備えることを特徴とする、運転停止した燃料電池発電設備の燃料電池12内のガス組成を決定するためのシステム。 - 検出器回路86が、燃料電池12の運転停止モニタ電圧が燃料電池12発電設備の検出器電圧限界とほぼ同じかまたはそれを超えることを検出するときは必ず、アノード流れ区域28内へ水素含有還元性流体を選択的に導入するように、検出器回路86およびアノード入口弁62と電気的に連通するように取り付けられたアノード入口弁62制御手段をさらに備えることを特徴とする請求項1記載の運転停止した燃料電池発電設備の燃料電池12内のガス組成を決定するためのシステム。
- アノード出口42とアノード入口40との間に流体連通するように取り付けられたアノード再循環ライン66と、アノード排気の流れの少なくとも一部をアノード出口42からアノード入口40へ導くための、アノード再循環ライン66に取り付けられたアノード再循環送風機68とをさらに備えることを特徴とする請求項2記載の運転停止した燃料電池発電設備の燃料電池12内のガス組成を決定するためのシステム。
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US10/244,495 US7147945B2 (en) | 2002-09-16 | 2002-09-16 | System for determining a gas composition within a shut down fuel cell power plant and method of operation |
PCT/US2003/029338 WO2004025269A2 (en) | 2002-09-16 | 2003-09-15 | System for determining a gas composition within a shut down fuel cell power plant and method of operation |
Publications (2)
Publication Number | Publication Date |
---|---|
JP2005539353A JP2005539353A (ja) | 2005-12-22 |
JP4630064B2 true JP4630064B2 (ja) | 2011-02-09 |
Family
ID=31991904
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
JP2004536614A Expired - Lifetime JP4630064B2 (ja) | 2002-09-16 | 2003-09-15 | 運転停止した燃料電池発電設備内のガス組成を決定するシステムおよび作動方法 |
Country Status (5)
Country | Link |
---|---|
US (1) | US7147945B2 (ja) |
JP (1) | JP4630064B2 (ja) |
AU (1) | AU2003270743A1 (ja) |
DE (1) | DE10393322T5 (ja) |
WO (1) | WO2004025269A2 (ja) |
Families Citing this family (32)
Publication number | Priority date | Publication date | Assignee | Title |
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US6774637B2 (en) * | 2000-11-30 | 2004-08-10 | Plug Power, Inc. | Method of qualifying at least a portion of a fuel cell system and an apparatus employing same |
DE10358933A1 (de) * | 2003-12-12 | 2005-07-28 | Webasto Ag | Bestimmung des Lambdawertes von Reformat |
JP4507584B2 (ja) * | 2003-12-15 | 2010-07-21 | トヨタ自動車株式会社 | 燃料電池システム |
JP4633354B2 (ja) * | 2003-12-19 | 2011-02-16 | 本田技研工業株式会社 | 燃料電池の停止方法 |
US7651806B2 (en) * | 2004-03-26 | 2010-01-26 | Gm Global Technology Operations, Inc. | Non-flammable exhaust enabler for hydrogen powered fuel cells |
JP4702592B2 (ja) * | 2004-04-28 | 2011-06-15 | トヨタ自動車株式会社 | 燃料電池システム及びその運転方法 |
US8606516B2 (en) * | 2004-11-30 | 2013-12-10 | Dash Navigation, Inc. | User interface system and method for a vehicle navigation device |
EP1902486B1 (en) * | 2005-07-14 | 2011-10-19 | Nissan Motor Company Limited | Fuel cell power plant and control method thereof |
US8715872B2 (en) | 2005-12-27 | 2014-05-06 | Nissan Motor Co., Ltd. | Fuel cell system having decreased deterioration during initiation |
US7976995B2 (en) * | 2005-12-27 | 2011-07-12 | Nissan Motor Co., Ltd. | Fuel cell system comprising a voltage limit device |
JP5070700B2 (ja) * | 2005-12-28 | 2012-11-14 | 日産自動車株式会社 | 燃料電池システム |
JP5168828B2 (ja) * | 2006-06-27 | 2013-03-27 | 日産自動車株式会社 | 燃料電池システム |
DE102006043349A1 (de) * | 2006-09-15 | 2008-03-27 | Enerday Gmbh | Brennstoffzellensystem und Verfahren zum Starten eines Brennstoffzellensystems |
KR100805445B1 (ko) | 2006-12-04 | 2008-02-20 | 현대자동차주식회사 | 연료전지 차량의 셧 다운시의 수소 공급 시스템 |
ATE556455T1 (de) * | 2006-12-27 | 2012-05-15 | Nissan Motor | Brennstoffzellensystem |
US7841228B2 (en) * | 2007-02-05 | 2010-11-30 | Toyota Motor Engineering & Manufacturing North America, Inc. | Method of detecting hydrogen sensor saturation in a hydrogen powered fuel cell |
US8920984B2 (en) * | 2008-02-19 | 2014-12-30 | Ford Motor Company | System and method for purging water from a fuel cell stack |
EP2351134A1 (en) * | 2008-10-03 | 2011-08-03 | UTC Power Corporation | Low power control of fuel cell open circuit voltage |
US8338044B2 (en) * | 2009-01-15 | 2012-12-25 | Ford Motor Company | System and method for detecting a fuel cell anode gas composition |
JP5364492B2 (ja) * | 2009-01-23 | 2013-12-11 | 株式会社東芝 | 燃料電池発電システム |
US8177884B2 (en) * | 2009-05-20 | 2012-05-15 | United Technologies Corporation | Fuel deoxygenator with porous support plate |
US8195407B2 (en) * | 2009-10-09 | 2012-06-05 | GM Global Technology Operations LLC | Online method to estimate hydrogen concentration estimation in fuel cell systems at shutdown and startup |
JP5592657B2 (ja) * | 2010-01-13 | 2014-09-17 | 大阪瓦斯株式会社 | コージェネレーションシステム |
JP5592656B2 (ja) * | 2010-01-13 | 2014-09-17 | 大阪瓦斯株式会社 | 燃料電池用の運転制御装置 |
US9947948B2 (en) * | 2012-06-01 | 2018-04-17 | Nissan Motor Co., Ltd. | Fuel cell system |
CN103647092B (zh) * | 2013-10-30 | 2016-02-03 | 张勇 | 延长燃料电池寿命的方法和装置 |
JP6218114B2 (ja) * | 2013-12-27 | 2017-10-25 | Toto株式会社 | 固体酸化物型燃料電池 |
CN104064787B (zh) * | 2014-06-17 | 2016-06-15 | 苏州弗尔赛能源科技股份有限公司 | 一种燃料电池备用电源系统用氢气压力控制方法 |
JP6447838B2 (ja) * | 2016-11-21 | 2019-01-09 | トヨタ自動車株式会社 | 燃料電池車両 |
JP7067402B2 (ja) * | 2018-10-05 | 2022-05-16 | トヨタ自動車株式会社 | 燃料電池システム |
CN109253850B (zh) * | 2018-11-27 | 2023-09-19 | 安徽明天氢能科技股份有限公司 | 一种燃料电池双极板水腔密封性检测装置 |
CN113029900B (zh) * | 2021-02-26 | 2024-02-13 | 武汉理工大学 | 氢能与燃料电池中多孔输运层传质性能的测量系统及方法 |
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-
2002
- 2002-09-16 US US10/244,495 patent/US7147945B2/en not_active Expired - Lifetime
-
2003
- 2003-09-15 JP JP2004536614A patent/JP4630064B2/ja not_active Expired - Lifetime
- 2003-09-15 DE DE10393322T patent/DE10393322T5/de not_active Withdrawn
- 2003-09-15 WO PCT/US2003/029338 patent/WO2004025269A2/en active Application Filing
- 2003-09-15 AU AU2003270743A patent/AU2003270743A1/en not_active Abandoned
Also Published As
Publication number | Publication date |
---|---|
JP2005539353A (ja) | 2005-12-22 |
US7147945B2 (en) | 2006-12-12 |
AU2003270743A8 (en) | 2004-04-30 |
US20040053089A1 (en) | 2004-03-18 |
DE10393322T5 (de) | 2005-09-01 |
AU2003270743A1 (en) | 2004-04-30 |
WO2004025269A2 (en) | 2004-03-25 |
WO2004025269A3 (en) | 2004-05-13 |
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