JP4102299B2 - 燃料電池に用いるイオノマー及びその製造方法 - Google Patents

燃料電池に用いるイオノマー及びその製造方法 Download PDF

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Publication number
JP4102299B2
JP4102299B2 JP2003511332A JP2003511332A JP4102299B2 JP 4102299 B2 JP4102299 B2 JP 4102299B2 JP 2003511332 A JP2003511332 A JP 2003511332A JP 2003511332 A JP2003511332 A JP 2003511332A JP 4102299 B2 JP4102299 B2 JP 4102299B2
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Japan
Prior art keywords
monomer
ionomer
fuel cell
polymer electrolyte
anode
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Expired - Fee Related
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JP2003511332A
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Japanese (ja)
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JP2004534890A (ja
JP2004534890A5 (enExample
Inventor
シャオ，グユ
ソン，グオミン
ヤン，ダユエ
ダブリュ． マーチン，チャールズ
ウ，フェイ
グラティ，カリン
アルベルト カバルカ，カルロス
チウ，シンユアン
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WL Gore and Associates Inc
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WL Gore and Associates Inc
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Priority claimed from CNB011132574A external-priority patent/CN1161397C/zh
Priority claimed from CN 02111491 external-priority patent/CN1200029C/zh
Application filed by WL Gore and Associates Inc filed Critical WL Gore and Associates Inc
Publication of JP2004534890A publication Critical patent/JP2004534890A/ja
Publication of JP2004534890A5 publication Critical patent/JP2004534890A5/ja
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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C08J5/2256—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2275—Heterogeneous membranes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1027—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having carbon, oxygen and other atoms, e.g. sulfonated polyethersulfones [S-PES]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/103—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having nitrogen, e.g. sulfonated polybenzimidazoles [S-PBI], polybenzimidazoles with phosphoric acid, sulfonated polyamides [S-PA] or sulfonated polyphosphazenes [S-PPh]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1032—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having sulfur, e.g. sulfonated-polyethersulfones [S-PES]
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2379/00—Characterised by the use of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing nitrogen with or without oxygen, or carbon only, not provided for in groups C08J2361/00 - C08J2377/00
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8605—Porous electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Materials Engineering (AREA)
  • Medicinal Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Polyethers (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Polymers With Sulfur, Phosphorus Or Metals In The Main Chain (AREA)
  • Macromolecular Compounds Obtained By Forming Nitrogen-Containing Linkages In General (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
JP2003511332A 2001-07-05 2002-07-05 燃料電池に用いるイオノマー及びその製造方法 Expired - Fee Related JP4102299B2 (ja)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
CNB011132574A CN1161397C (zh) 2001-07-05 2001-07-05 带磺酸盐侧基的聚二氮杂萘酮醚酮及制备方法
CN 02111491 CN1200029C (zh) 2002-04-25 2002-04-25 带磺酸盐侧基的聚二氮杂萘酮醚砜及制备方法
PCT/US2002/021346 WO2003005474A2 (en) 2001-07-05 2002-07-05 Ionomer for use in fuel cells and method of making same

Publications (3)

Publication Number Publication Date
JP2004534890A JP2004534890A (ja) 2004-11-18
JP2004534890A5 JP2004534890A5 (enExample) 2006-01-05
JP4102299B2 true JP4102299B2 (ja) 2008-06-18

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JP2003511332A Expired - Fee Related JP4102299B2 (ja) 2001-07-05 2002-07-05 燃料電池に用いるイオノマー及びその製造方法

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Country Link
US (1) US7405015B2 (enExample)
EP (1) EP1402590B1 (enExample)
JP (1) JP4102299B2 (enExample)
KR (1) KR100817691B1 (enExample)
AU (1) AU2002354786B2 (enExample)
BR (1) BR0210803B1 (enExample)
CA (1) CA2451896C (enExample)
DE (1) DE60223539T2 (enExample)
RU (1) RU2004103077A (enExample)
WO (1) WO2003005474A2 (enExample)

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CA2485971A1 (en) 2002-05-13 2004-05-21 Polyfuel, Inc. Ion conductive block copolymers
US7297429B2 (en) * 2002-07-05 2007-11-20 Gore Enterprise Holdings, Inc. Ionomer for use in fuel cells and method of making same
JP2005133092A (ja) * 2003-10-10 2005-05-26 Hitachi Chem Co Ltd 複素環を有する高分子電解質化合物、高分子電解質膜、それを用いた触媒層形成電解質膜及びそれを用いた電気化学素子
JP2006135022A (ja) * 2004-11-04 2006-05-25 Nitto Denko Corp 配線回路基板
KR100614100B1 (ko) * 2005-01-14 2006-08-22 한국과학기술연구원 나피온 이오노머 용액의 완전 건조전 전극상막 방법을이용하는 연료 전지용 막전극접합체의 제조 방법 및 그에의해 제조되는 연료 전지용 막전극접합체
CN101120419B (zh) * 2005-02-15 2011-02-16 东丽株式会社 高分子电解质成型体的制造方法、高分子电解质材料、高分子电解质膜和高分子电解质型燃料电池
US20060199059A1 (en) * 2005-03-01 2006-09-07 Xu Helen X Ion conductive polymer electrolyte and its membrane electrode assembly
EP2355218B1 (en) * 2005-03-04 2012-10-03 Ube Industries, Ltd. Novel polymer electrolyte, polymer electrolyte composition, electrolyte membrane, and production method and use thereof
JP2006338928A (ja) * 2005-05-31 2006-12-14 Hitachi Chem Co Ltd 補強高分子電解質、電極−高分子電解質膜接合体、燃料電池並びにそれらの製造方法
KR100833056B1 (ko) * 2006-03-31 2008-05-27 주식회사 엘지화학 연료전지용 강화-복합 전해질막
KR100897104B1 (ko) 2006-11-02 2009-05-14 현대자동차주식회사 다층구조를 가진 전해질 강화막의 제조 방법
KR100851924B1 (ko) 2007-02-01 2008-08-12 충주대학교 산학협력단 다중 술폰화된 폴리 아릴에테르케톤 공중합체 및 이를포함하는 전해질막
DE102007008268B4 (de) * 2007-02-20 2009-02-19 Staxera Gmbh Prüfstand und Prüfverfahren für einen Brennstoffzellenstapel
US20100159298A1 (en) * 2008-12-22 2010-06-24 3M Innovative Properties Company Fuel cell membrane electrode assembly with multilayer cathode
KR101651093B1 (ko) * 2009-12-11 2016-08-26 건국대학교 글로컬산학협력단 다중황산기를 포함하는 다중페닐 단위체를 지닌 양이온 교환 고분자
US9005841B2 (en) * 2009-12-18 2015-04-14 Lg Chem, Ltd. Polymer electrolyte membrane for fuel cell, membrane electrode assembly and fuel cell including the same
US20110274990A1 (en) * 2010-05-07 2011-11-10 Yang G Xu Methanol and Hydrogen Peroxide Fuel Cell with Hydroxyl Ion Exchange Membrane
JP5725685B2 (ja) * 2011-06-16 2015-05-27 エルジー ケム． エルティーディ． 燃料電池用高分子電解質膜、それを含む膜電極接合体及び燃料電池
US10603639B2 (en) 2016-09-02 2020-03-31 Hossein Beydaghi Nanocomposite blend membrane
EP4466742A1 (en) 2022-01-21 2024-11-27 Basf Se Mixed platinum ruthenium oxide and electrodes for the oxygen evolution reaction

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Publication number Publication date
US20050079399A1 (en) 2005-04-14
WO2003005474A9 (en) 2004-07-01
WO2003005474A2 (en) 2003-01-16
DE60223539D1 (de) 2007-12-27
BR0210803A (pt) 2004-06-29
KR20040013094A (ko) 2004-02-11
KR100817691B1 (ko) 2008-03-27
EP1402590B1 (en) 2007-11-14
WO2003005474A3 (en) 2003-08-28
DE60223539T2 (de) 2008-09-25
CA2451896C (en) 2009-09-08
AU2002354786B2 (en) 2005-08-18
BR0210803B1 (pt) 2011-11-29
US7405015B2 (en) 2008-07-29
JP2004534890A (ja) 2004-11-18
EP1402590A2 (en) 2004-03-31
RU2004103077A (ru) 2005-03-27
CA2451896A1 (en) 2003-01-16

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