EP3486193A1 - Umkehrbarer aerosolventilmechanismus und aerosolprodukt mit diesem umkehrbaren ventilmechanismus - Google Patents

Umkehrbarer aerosolventilmechanismus und aerosolprodukt mit diesem umkehrbaren ventilmechanismus Download PDF

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Publication number
EP3486193A1
EP3486193A1 EP17827264.7A EP17827264A EP3486193A1 EP 3486193 A1 EP3486193 A1 EP 3486193A1 EP 17827264 A EP17827264 A EP 17827264A EP 3486193 A1 EP3486193 A1 EP 3486193A1
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EP
European Patent Office
Prior art keywords
invertible
passage
contents
valve
upright
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
EP17827264.7A
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English (en)
French (fr)
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EP3486193B1 (de
EP3486193A4 (de
Inventor
Naoto Kawashima
Shin Matsumoto
Hiroshi Kanno
Yasuo Ohshima
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Mitani Valve Co Ltd
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Mitani Valve Co Ltd
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Publication date
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Publication of EP3486193A1 publication Critical patent/EP3486193A1/de
Publication of EP3486193A4 publication Critical patent/EP3486193A4/de
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B65—CONVEYING; PACKING; STORING; HANDLING THIN OR FILAMENTARY MATERIAL
    • B65D—CONTAINERS FOR STORAGE OR TRANSPORT OF ARTICLES OR MATERIALS, e.g. BAGS, BARRELS, BOTTLES, BOXES, CANS, CARTONS, CRATES, DRUMS, JARS, TANKS, HOPPERS, FORWARDING CONTAINERS; ACCESSORIES, CLOSURES, OR FITTINGS THEREFOR; PACKAGING ELEMENTS; PACKAGES
    • B65D83/00—Containers or packages with special means for dispensing contents
    • B65D83/14—Containers or packages with special means for dispensing contents for delivery of liquid or semi-liquid contents by internal gaseous pressure, i.e. aerosol containers comprising propellant for a product delivered by a propellant
    • B65D83/36—Containers or packages with special means for dispensing contents for delivery of liquid or semi-liquid contents by internal gaseous pressure, i.e. aerosol containers comprising propellant for a product delivered by a propellant allowing operation in any orientation, e.g. discharge in inverted position
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B65—CONVEYING; PACKING; STORING; HANDLING THIN OR FILAMENTARY MATERIAL
    • B65D—CONTAINERS FOR STORAGE OR TRANSPORT OF ARTICLES OR MATERIALS, e.g. BAGS, BARRELS, BOTTLES, BOXES, CANS, CARTONS, CRATES, DRUMS, JARS, TANKS, HOPPERS, FORWARDING CONTAINERS; ACCESSORIES, CLOSURES, OR FITTINGS THEREFOR; PACKAGING ELEMENTS; PACKAGES
    • B65D83/00—Containers or packages with special means for dispensing contents
    • B65D83/14—Containers or packages with special means for dispensing contents for delivery of liquid or semi-liquid contents by internal gaseous pressure, i.e. aerosol containers comprising propellant for a product delivered by a propellant
    • B65D83/44—Valves specially adapted therefor; Regulating devices
    • B65D83/48—Lift valves, e.g. operated by push action

Definitions

  • the present invention relates to a valve acting section (stem hole) by which an operation mode setting operation of an aerosol-type product is used to shift from the previous closed state to an open state to inject the contents in a container body to an outer space region and a contents passage section in an invertible use mode communicating with this.
  • the invention relates to an invertible valve mechanism in which the contents passage section is composed of an upright inflow passage and an inverted inflow passage that are continuous in a single straight line-form and a shared invertible passage providing the communication from these common outflow holes to a valve acting section and in which a free fall-type moving valve is provided at a predetermined position of the inverted inflow passage.
  • This moving valve is configured so that the inverted inflow passage is set in a shutoff state when the invertible valve mechanism is upright so as to prevent the vaporized gas flowing in the upper part of the container body from entering the upright inflow passage or the shared invertible passage.
  • the moving valve may be a ball valve for example.
  • the present invention provides an invertible valve mechanism for which the separation relation between this moving valve and the common outflow hole is considered for example to suppress the "gas entrainment" phenomenon of the vaporized gas in the contents to block the so-called intermittent injection of the contents caused by this so that the smooth and continuous injection state can be secured.
  • the "gas entrainment” phenomenon is caused, during the upright operation of the invertible valve mechanism, when the inverted inflow passage in the moving valve that should be shut off from the shared invertible passage is displaced in the "dancing" state in an up-and-down direction due to the strength of the contents flowing from the upright inflow passage.
  • the "upper” and “lower” directions around the respective components of the invertible valve mechanism show the upper and lower positions in the upright state in Fig. 1 to Fig. 2 .
  • the terms “upstream” and “downstream” are not included in the scope of the definitions of the upper and lower positions.
  • the up-and-down directions in the respective drawings are also denoted as a "longitudinal” direction and the left-and-right direction is denoted as a "lateral" direction as required.
  • the above-described aerosol-type invertible valve mechanism has been conventionally used that consists of the upright inflow passage, the inverted inflow passage, and the shared invertible passage, and this inverted inflow passage includes a free fall ball valve to switch the upright injection/inverted injection (see Patent Publication 1).
  • Patent Publication 1 Japanese unexamined patent application publication H6-199376
  • the upper end of the common outflow hole is separated from the lower end of the moving valve in the up-and-down direction by a distance of 1.2mm for example.
  • the moving valve has been provided in the very vicinity of the upper part of the common outflow hole in the inverted inflow passage that is shared by the upright inflow passage and the inverted inflow passage.
  • the moving valve tends to be in the "dancing" state due to the strength of the contents flowing from the upright inflow passage.
  • the invertible valve mechanism of the present invention pays attention on not the size or material of the moving valve but on the position of the moving valve in order to eliminate the intermittent injection state of the contents due to the "gas entrainment" in the invertible valve mechanism in which the moving valve is provided on the extended straight line at the contents outflow side of the upright inflow passage.
  • the moving valve that shuts off the inverted inflow passage from the downstream-side shared invertible passage in the upright operation mode is provided at a position separated from the upper end of the common outflow hole for the upright inflow passage and the inverted inflow passage by a distance of at least 3.5mm or more desirably a distance of 3.7mm or more.
  • This common outflow hole also functions as an inflow section to the shared invertible passage.
  • the moving valve to switch ON or OFF the inverted inflow passage is provided at a position upwardly separated from the common outflow hole for the upright inflow passage and the inverted inflow passage by a predetermined distance to thereby block the occurrence of the "dancing" state in which the moving valve in the upright operation mode is displaced by the strength of the upwardly-flowing contents.
  • This predetermined distance is "at least 3.5mm or more desirably a distance of 3.7mm or more" as described above.
  • the moving valve is provided at a position at the upper side of the common outflow hole separated by a distance about three times longer than the conventional distance of "1.2mm".
  • the present invention solves the above disadvantage using an invertible valve mechanism described below.
  • the present invention provides an invertible valve mechanism consisting of the above configuration and an aerosol-type product including this.
  • the present invention blocks the occurrence of the "dancing" state of the moving valve in the upright operation mode to prevent the "gas entrainment” of vaporized gas in the contents, thus stabilizing the continuous injection state of the contents.
  • the common outflow hole is separated, without requiring a particular change of the size of the moving valve itself or the material thereof, from the moving valve by such a distance that prevents the strength of the flowing injection contents from acting on the moving valve, thus providing the efficient use of the components of the invertible valve mechanism.
  • the letter A shows an upright inflow passage.
  • the letter B shows an inverted inflow passage.
  • the letter C shows a shared invertible passage starting from the common outflow hole for the upright inflow passage A and the inverted inflow passage B.
  • the letter L shows the interval in the up-and-down direction from the upper end of this common outflow hole to the lower end of the ball valve.
  • the reference numeral 1 denotes a depression-type button that can be moved in the up-and-down direction to operate the injection of the contents.
  • the reference numeral 1a denotes the well-known button interior passage reaching a contents injection opening.
  • the reference numeral 2 denotes a sheath-like stem integrated with the button 1.
  • the reference numeral 2a denotes a lateral hole functioning as an output valve with the stem gasket 3 (which will be described later).
  • the reference numeral 2b denotes a stem interior passage communicating with the lateral hole 2a and the button interior passage 1a.
  • the reference numeral 3 denotes a stem gasket for which the outer part is sandwiched between a housing body 4 and a mounting cup 9 (which will be described later) and the inner end functions as an output valve with the lateral hole 2a.
  • the reference numeral 4 denotes a housing body that is attached to the mounting cup 9 (which will be described later) to store the lower part of the stem 2 in the upright state and that defines the shared invertible passage C and the inverted inflow passage B for the contents in the container body.
  • the reference numeral 4a denotes an upper sheath-like section of an upper opening that stores a lower part of the stem 2 in the upright state (a substantially-lower part of the lateral hole 2a) and that functions as a space through which the contents are sent and in which the contents are stored.
  • the reference numeral 4b denotes a plurality of longitudinal rib-like sections that are provided on the inner circumferential face of an upper sheath-like section 4a and that have thereamong groove-like sections along which the contents are sent.
  • the reference numeral 4c denotes a lower sheath-like section of a lower opening that functions as the inverted inflow passage B or as a space region to store the ball valve 7 (which will be described later) in the inverted state.
  • the reference numeral 4d denotes the bottom face of the lower sheath-like section 4c in the inverted state that functions as a section to receive the ball valve 7 (which will be described later) in the inverted state.
  • the reference numeral 4e denotes the total of two peripheral face openings of the rectangular longitudinal cross section that are formed on the upper column of the lower sheath-like section 4c at an interval of 180 degrees in the circumferential direction and that function as the inflow side of the inverted inflow passage B, respectively.
  • the reference numeral 4f denotes the longitudinal space region having an upper opening in the inverted state and having a circular lateral cross section.
  • This longitudinal space region has a bottom face part 4d in the inverted state to communicate with a peripheral face opening 4e and guides the up-and-down motion of the ball valve 7 (which will be described later) and functions as a part of the inverted inflow passage B.
  • the reference numeral 4g denotes a longitudinal penetration section having a circular lateral cross section.
  • the total of 4 longitudinal penetration sections are formed with an interval of 60 degrees in the circumferential direction so as to penetrate, at the respective drum sections between a pair of the peripheral face openings 4e opposed to each other, through the interior of the upper sheath-like section 4a (contents passage groove-like section).
  • the reference numeral 4h denotes an annular space region that is set between the inner circumferential face of a lower sheath-like section 4c and the outer peripheral face of an upper cover body 6d (which will be described later) and that functions as an upstream part of the shared invertible passage C.
  • the reference numeral 5 denotes a coil spring that is provided between a lower face step of the stem 2 in the upright state and the bottom face part of the upper sheath-like section 4a to bias the stem in the upright state.
  • the reference numeral 6 denotes a cylindrical housing cover body having a circular lateral cross section that is engaged with the lower inner face of the housing body 4 in the upright state to define the upstream part of the shared invertible passage C.
  • the reference numeral 6a denotes an annular valve seat having a taper face at an inner end of the housing cover body 6 that is closely fitted (abutted) to the ball valve 7 (which will be described later) at the original lower motion position in the upright state.
  • the reference numeral 6b denotes an upper central cylindrical section that is continuously formed in the lower direction from the valve seat 6a in the upright state to receive the lower end side of the ball valve 7 in the upright state.
  • the reference numeral 6c denotes a cylindrical body that is continuously formed in the lower direction in a large diameter mode from the upper central cylindrical section 6b in the upright state.
  • the reference numeral 6d denotes an upper cover body at the upper side of the cylindrical body 6c that constitutes the downstream side of the inverted inflow passage B together with the upper central cylindrical section 6b so that the lower end thereof in the upright state constitutes the downstream end side (downstream side) of the upright inflow passage A.
  • the reference numeral 6e denotes a lower cover body at the lower part of the cylindrical body 6c that is attached with a dip tube 8 (which will be described later) to constitute the downstream side of the upright inflow passage A.
  • the reference numeral 6f denotes a common outflow hole.
  • the total of 2 common outflow holes are formed at the lower end side of the upper cover body 6d with an interval of 180 degrees in the circumferential direction to function as a starting part of the shared invertible passage C in the lateral penetration state.
  • the reference numeral 6g denotes an annular collar section that receives the lower end face of the lower sheath-like section 4c in the upright state.
  • the reference numeral 7 denotes a ball valve that is closely fitted (abutted) to the valve seat 6a at the lower motion positon in the upright state and that functions as a moving valve abutted to and retained by the bottom face part 4d at the lower motion position in the inverted state of the lower sheath-like section 4c.
  • the reference numeral 8 denotes a contents inflow dip tube that is attached to the lower inner circumferential face of the housing cover body 6.
  • the reference numeral 9 denotes a mounting cup that is engaged with the housing body 4 to sandwich the stem gasket 3.
  • the reference numeral 10 denotes a container body that is attached with the mounting cup 9 and that has an inner space region to store to-be-injected contents and vaporized injection gas.
  • the button 1, the stem 2, the housing body 4, the coil spring 5, and the housing cover body 6 are made of synthetic resin such as polypropylene, polyethylene, polyacetal, nylon, or polybutylene terephthalate or metal.
  • the stem gasket 3 is made of rubber or synthetic resin.
  • the ball valve 7, the mounting cup 9, and the container body 10 are made of metal (e.g., stainless).
  • the dip tube 8 is made of synthetic resin.
  • the aerosol-type invertible valve mechanism shown in Fig. 1 to Fig. 4 is basically characterized in that the vertical spacing L in the upright state between the upper end of the common outflow hole 6f of the upright inflow passage A and the inverted inflow passage B and the lower end of the ball valve 7 is set to at least 3.5mm or desirably 3.7mm or more.
  • this vertical spacing L is increased to have a value larger than a conventional value (e.g., 1.2mm) so as to reduce the influence on the ball valve 7 due to the strength of the contents upwardly flowing from the upright inflow passage A in the upright operation mode.
  • a conventional value e.g., 1.2mm
  • This reduction of the influence on the ball valve suppresses the vaporized gas in the upper part of the container body in the upright state from passing the ball valve to flow from the inverted inflow passage B to the shared invertible passage C. Specifically, this eliminates the "gas entrainment" of the vaporized gas in the contents in the shared invertible passage C.
  • the downward motion of the stem 2 changes the shape of the inner end of the stem gasket 3 to a "bow"-like shape, thereby cancelling the previous valve closed state to the lateral hole 2a.
  • This valve cancellation allows, as shown in the drawing, the contents in the lower space region of the container body 10 to pass through the upright inflow passage A and the shared invertible passage C to be injected to the outer space region through the well-known button injection opening.
  • the contents in the container body flow through the path composed of "the dip tube 8-the common outflow hole 6f-the annular space region 4h-the longitudinal penetration section 4g-the inner space region of the upper sheath-like section 4a-the lateral hole 2a-the button interior passage 1a".
  • the vertical spacing L extending from the upper end of the common outflow hole 6f to the lower end of the ball valve 7 is set to at least 3.5mm or more desirably 3.7mm or more.
  • the common outflow hole 6f separated from the ball valve 7 in the up-and-down direction as described above can substantially prevent the ball valve 7 in the upright operation mode from "dancing" due to the strength of the contents upwardly flowing from the upright inflow passage A.
  • this spacing can prevent a situation where the vaporized gas enters the shared invertible passage C via the ball valve 7 in the “dancing" state to cause the "gas entrainment" in the contents.
  • This suppression of the "gas entrainment" provides the contents injection to the outer space region not in a pulsating flow-like intermittent injection state but in a stable continuous injection state.
  • the following table 1 shows the result of the examination of this continuous injection. Specifically, the examination of the injection state was performed based on the total of 11 experimental models prepared to have the vertical spacing L between the upper end of the common outflow hole 6f and the lower end of the ball valve 7 so that the vertical spacing L is changed from 3.0mm to 4.0mm by an increment of 0.1mm.
  • L (mm) 3.0-3.4 3.5 3.6 3.7 3.8 3.9
  • the occurrence of the "gas entrainment” was examined by visually monitoring the flow of the contents injected to the outer space region via the valve acting section in the open state (the lateral hole 2a and the stem gasket 3). Specifically, the contents injected to the outer space region were visually monitored with regard to whether the contents formed a stable continuous flow or a pulsating flow-like intermittent flow.
  • the pulsating flow-like intermittent injection state of the "gas entrainment" may be sufficiently visually monitored by general users.
  • the examination result shows, as shown in the table 1, that the vertical spacing L having a different size shows the following different result.
  • the vertical spacing L from the upper end of the common outflow hole 6f to the lower end of the ball valve 7 is set to at least 3.5mm or more desirably 3.7mm or more.
  • the longitudinal space region 4f was used that had a height of 6.3mm in the up-and-down direction and a diameter of 3.4mm.
  • the upper central cylindrical section 6b was used that had a height of 1.0mm in the up-and-down direction and the inner diameter of 2.3mm.
  • the cylindrical body 6c was provided between the upper central cylindrical section 6b and the dip tube 8.
  • the cylindrical body 6c consisted of a pair of opposed flat surfaces having an interval of 2.8mm and a pair of opposed arc curved surfaces having an inner diameter of 3.3mm therebetween.
  • Each of the opposed flat surfaces included therein a common outflow hole 6f having a lateral length of 1.1mm and an inner diameter of 1.5mm.
  • the annular space region 4h had a lateral interval of 0.425mm.
  • the longitudinal penetration section 4g was used that had a height in the up-and-down direction of 6.7mm, the cross section width of 1.0mm, and a cross section having a depth of 0.6mm.
  • the cylindrical body 6c and the annular space region 4h have the direction in the up-and-down direction that is different depending on each experimental model set depending on the value of the vertical spacing L from the upper end of the common outflow hole 6f to the lower end of the ball valve 7.
  • This valve cancellation causes, as shown in the drawing, the contents in the upper space region of the container body 10 in the upright state to be sent through the inverted inflow passage B and the shared invertible passage C, thereby injecting the contents to the outer space region through the well-known button injection opening.
  • the contents in the container body are allowed to flow through the path of "the peripheral face opening 4e-the longitudinal space region 4f-the inner space region of the upper central cylindrical section 6b-the inner space region of the cylindrical body 6c-the common outflow hole 6f-the annular space region 4h-the longitudinal penetration section 4g-the inner space region of the upper sheath-like section 4a-the lateral hole 2a-the button interior passage 1a".
  • the present invention can be applied to aerosol-type products for various applications including cleaning agent, cleanup agent, antiperspirant, coolant, muscular antiphlogistic agent, hairstyling agent, hair treatment agent, hair dye, hair growth agent, cosmetics, shaving foam, foods, droplet-like products (e.g., vitamin), medical products, quasi-pharmaceutical products, paints, agricultural agent, repellents (pesticides), cleaner, deodorizer, laundry starch, urethane foam, fire extinguisher, adhesive agent, or lubricant.
  • cleaning agent cleanup agent, antiperspirant, coolant, muscular antiphlogistic agent, hairstyling agent, hair treatment agent, hair dye, hair growth agent, cosmetics, shaving foam, foods, droplet-like products (e.g., vitamin), medical products, quasi-pharmaceutical products, paints, agricultural agent, repellents (pesticides), cleaner, deodorizer, laundry starch, urethane foam, fire extinguisher, adhesive agent, or lubricant
  • the contents stored in the container body may be, for example, powder-like matters, oil components, alcohols, surfactant, high molecular compounds, or active ingredients depending on each application.
  • Powder-like matters include metal salts powders, inorganic substance powders, or resin powders such as talc, kaolin, aluminum hydroxychloride (aluminum salts), calcium alginate, gold powder, silver powder, mica, carbonate, barium sulfate, cellulose, or the mixtures thereof mixture for example.
  • metal salts powders such as talc, kaolin, aluminum hydroxychloride (aluminum salts), calcium alginate, gold powder, silver powder, mica, carbonate, barium sulfate, cellulose, or the mixtures thereof mixture for example.
  • Oil components include silicone oil, palm oil, eucalyptus oil, camellia oil, olive oil, jojoba oil, paraffin oil, myristic acid, palmitic acid, stearic acid, linoleic acid, or linolenic acid for example.
  • Alcohols include monohydric lower alcohol (e.g., ethanol), monohydric higher alcohol (e.g., lauryl alcohol), or polyalcohol (e.g., ethylene glycol).
  • monohydric lower alcohol e.g., ethanol
  • monohydric higher alcohol e.g., lauryl alcohol
  • polyalcohol e.g., ethylene glycol
  • Surfactants include anionic surfactant (e.g., sodium lauryl sulfate), nonionic surfactant (e.g., polyoxyethylene oleylether), amphoteric surfactant (e.g., lauryldimethylaminoacetic acid betaine), or cationic surfactant (e.g., alkyl trimethylammonium chloride) for example.
  • anionic surfactant e.g., sodium lauryl sulfate
  • nonionic surfactant e.g., polyoxyethylene oleylether
  • amphoteric surfactant e.g., lauryldimethylaminoacetic acid betaine
  • cationic surfactant e.g., alkyl trimethylammonium chloride
  • High molecular compounds include methyl cellulose, gelatin, starch, or casein for example.
  • Active ingredients depending on the respective applications include antiinflammatory agent (e.g., methyl salicylate, indomethacin), sterilization chemicals (e.g., sodium benzoate, cresol), insect pests repellents (e.g., pyrethroid, diethyltoluamide), antiperspirant (e.g., zinc oxide), refreshing medicine (e.g., camphor, menthol), antiasthmatic agent (e.g., ephedrine, adrenalin), sweetener (e.g., sucralose, aspartame), adhesive agent or paints (e.g., epoxy resin, urethane), dyes (e.g., paraphenylenediamine, aminophenol), extinguishing agent (e.g., ammonium dihydrogen phosphate, sodium bicarbonate, potassium) for example.
  • antiinflammatory agent e.g., methyl salicylate, indomethacin
  • sterilization chemicals e.g., sodium benzoate, cresol
  • agents other than the above contents can include suspension, ultraviolet absorber, emulsifier, moisturizing agent, antioxidant, or sequestering agent for example.
  • Contents pressurizing agent in an aerosol-type product includes carbon dioxide gas, nitrogen gas or the mixed gas thereof, compressed gas (e.g., compressed air), and LPG, DME, or liquefied gas (e.g., fluorohydrocarbon gas) for example.

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  • Chemical & Material Sciences (AREA)
  • Dispersion Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Mechanical Engineering (AREA)
  • Containers And Packaging Bodies Having A Special Means To Remove Contents (AREA)
  • Nozzles (AREA)
EP17827264.7A 2016-07-15 2017-05-30 Umkehrbarer aerosolventilmechanismus und aerosolprodukt mit diesem umkehrbaren ventilmechanismus Active EP3486193B1 (de)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2016140662 2016-07-15
PCT/JP2017/020088 WO2018012131A1 (ja) 2016-07-15 2017-05-30 エアゾールタイプの正倒立バルブ機構およびこの正倒立バルブ機構を備えたエアゾール式製品

Publications (3)

Publication Number Publication Date
EP3486193A1 true EP3486193A1 (de) 2019-05-22
EP3486193A4 EP3486193A4 (de) 2020-04-29
EP3486193B1 EP3486193B1 (de) 2021-08-11

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EP17827264.7A Active EP3486193B1 (de) 2016-07-15 2017-05-30 Umkehrbarer aerosolventilmechanismus und aerosolprodukt mit diesem umkehrbaren ventilmechanismus

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EP (1) EP3486193B1 (de)
JP (1) JPWO2018012131A1 (de)
CN (1) CN109476413B (de)
ES (1) ES2898378T3 (de)
TW (1) TWI633237B (de)
WO (1) WO2018012131A1 (de)

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Publication number Priority date Publication date Assignee Title
CN108380428B (zh) * 2018-05-15 2020-03-20 佛山安豪科技服务有限公司 一种喷枪的喷壶结构
KR20220062491A (ko) * 2019-09-13 2022-05-17 가부시키가이샤 미타니 밸브 내용물 분출 유닛 및 분출 용기
BE1027882B1 (nl) * 2020-05-15 2021-07-12 Altachem Steel van een ventiel

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CN205341105U (zh) * 2015-12-15 2016-06-29 上溢精密股份有限公司 可倒立使用的喷雾器

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Publication number Publication date
ES2898378T3 (es) 2022-03-07
EP3486193B1 (de) 2021-08-11
TWI633237B (zh) 2018-08-21
CN109476413A (zh) 2019-03-15
WO2018012131A1 (ja) 2018-01-18
TW201804082A (zh) 2018-02-01
EP3486193A4 (de) 2020-04-29
JPWO2018012131A1 (ja) 2019-05-23
CN109476413B (zh) 2020-01-03

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