BRPI0718191A2 - Materiais de coordenação de metal e de formação de filme - Google Patents

Materiais de coordenação de metal e de formação de filme Download PDF

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BRPI0718191A2
BRPI0718191A2 BRPI0718191-4A BRPI0718191A BRPI0718191A2 BR PI0718191 A2 BRPI0718191 A2 BR PI0718191A2 BR PI0718191 A BRPI0718191 A BR PI0718191A BR PI0718191 A2 BRPI0718191 A2 BR PI0718191A2
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group
film
forming material
material according
metal
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BRPI0718191-4A
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Timothy December
Sergio Gonzales
Guenther Ott
Karl-Heinz Grosse-Brinkhaus
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Basf Corp
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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L101/00—Compositions of unspecified macromolecular compounds
    • C08L101/02—Compositions of unspecified macromolecular compounds characterised by the presence of specified groups, e.g. terminal or pendant functional groups
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
    • C09D5/44—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes for electrophoretic applications
    • C09D5/4419—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes for electrophoretic applications with polymers obtained otherwise than by polymerisation reactions only involving carbon-to-carbon unsaturated bonds
    • C09D5/4465—Polyurethanes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/4009—Two or more macromolecular compounds not provided for in one single group of groups C08G18/42 - C08G18/64
    • C08G18/4081—Mixtures of compounds of group C08G18/64 with other macromolecular compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/62—Polymers of compounds having carbon-to-carbon double bonds
    • C08G18/6216—Polymers of alpha-beta ethylenically unsaturated carboxylic acids or of derivatives thereof
    • C08G18/622—Polymers of esters of alpha-beta ethylenically unsaturated carboxylic acids
    • C08G18/6225—Polymers of esters of acrylic or methacrylic acid
    • C08G18/6229—Polymers of hydroxy groups containing esters of acrylic or methacrylic acid with aliphatic polyalcohols
    • C08G18/6233—Polymers of hydroxy groups containing esters of acrylic or methacrylic acid with aliphatic polyalcohols the monomers or polymers being esterified with carboxylic acids or lactones
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/62—Polymers of compounds having carbon-to-carbon double bonds
    • C08G18/6283—Polymers of nitrogen containing compounds having carbon-to-carbon double bonds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/64—Macromolecular compounds not provided for by groups C08G18/42 - C08G18/63
    • C08G18/6415—Macromolecular compounds not provided for by groups C08G18/42 - C08G18/63 having nitrogen
    • C08G18/643—Reaction products of epoxy resins with at least equivalent amounts of amines
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/80—Masked polyisocyanates
    • C08G18/8061—Masked polyisocyanates masked with compounds having only one group containing active hydrogen
    • C08G18/8064—Masked polyisocyanates masked with compounds having only one group containing active hydrogen with monohydroxy compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G59/00—Polycondensates containing more than one epoxy group per molecule; Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups
    • C08G59/18—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing
    • C08G59/182—Macromolecules obtained by polymerising compounds containing more than one epoxy group per molecule using curing agents or catalysts which react with the epoxy groups ; e.g. general methods of curing using pre-adducts of epoxy compounds with curing agents
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09D—COATING COMPOSITIONS, e.g. PAINTS, VARNISHES OR LACQUERS; FILLING PASTES; CHEMICAL PAINT OR INK REMOVERS; INKS; CORRECTING FLUIDS; WOODSTAINS; PASTES OR SOLIDS FOR COLOURING OR PRINTING; USE OF MATERIALS THEREFOR
    • C09D5/00—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes
    • C09D5/44—Coating compositions, e.g. paints, varnishes or lacquers, characterised by their physical nature or the effects produced; Filling pastes for electrophoretic applications
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2150/00—Compositions for coatings
    • C08G2150/90—Compositions for anticorrosive coatings

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Molecular Biology (AREA)
  • Wood Science & Technology (AREA)
  • Manufacturing & Machinery (AREA)
  • Paints Or Removers (AREA)
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Description

RESUMO Patente de Invenção: "MATERIAIS DE COORDENAÇÃO DE METAL E DE FORMAÇÃO DE FILME".
Materiais formadores de filme incluem estruturas de coordena- ção de metal não-iônico. Estruturas de coordenação de metal não-iônico po- dem coordenar metais, tais como catalisadores de metal e substratos de me- tal. Materiais formadores de filme exemplares podem ser o produto de um epóxido polifuncional e um Iigante nucleofílico tendo uma estrutura de coor- denação de metal não-iônico, ou o produto de um álcool polifuncional e um Iigante eletrofílico tendo uma estrutura de coordenação de metal não-iônico.

Claims (15)

REIVINDICAÇÕES
1. Material de formação de filme caracterizado pelo fato de que compreende: uma resina, em que a resina inclui pelo menos um grupo pen- dente compreendendo uma estrutura de coordenação de metal não-iônico e pelo menos um grupo reativo com um reticulador, estrutura de coordenação de metal não-iônico compreendendo pelo menos dois grupos funcionais ri- cos em elétrons, independentemente selecionados do grupo que consiste em: nitrogênio, oxigênio, fósforo, enxofre, silício, carbono insaturado, éster, cetona, éter e hidroxila; e um reticulador compreendendo pelo menos dois grupos funcio- nais reativos com a resina.
2. Material de formação de filme de acordo com a reivindicação 1, caracterizado pelo fato de que a resina é uma resina epóxi, acrílica, poliu- retano, policarbonato, polissiloxano, aminoplástico, ou poliéster.
3. Material de formação de filme de acordo com a reivindicação 1 ou 2, caracterizado pelo fato de que pelo menos um grupo reativo com um reticulador é um grupo epóxido, hidroxila, carboxila, carbamato, ou amina.
4. Material de formação de filme de acordo com qualquer uma das reivindicações 1 a 3, caracterizado pelo fato de que a resina compreen- de a fórmula: <formula>formula see original document page 58</formula> em que, X1 e X2 são independentemente radicais monovalentes funcionais de hidrogênio, hidroxila, epóxido, ou amina; cada R1 e R2 é independentemente radicais divalentes de alqui- Ieno ou arileno; R3 é um radical divalente de alquileno ou arileno compreenden- do uma estrutura de coordenação de metal não-iônico, compreendendo pelo menos dois grupos funcionais ricos em elétrons, independentemente sele- cionados do grupo que consiste em: nitrogênio, oxigênio, fósforo, enxofre, silício, carbono insaturado, éster, cetona, éter e hidroxila; η é um número de 1 a cerca de 12; m é um número de 0 a cerca de 12; e ρ é um número de 1 a cerca de 12.
5. Material de formação de filme de acordo com a reivindicação4, caracterizado pelo fato de que R1 e R2 são radicais divalentes de 2,2- difenilpropano.
6. Material de formação de filme de acordo com qualquer um das reivindicações 1 a 5, caracterizado pelo fato de que dois dos grupos funcio- nais ricos em elétrons, estão em uma posição alfa ou beta um em relação ao outro.
7. Material de formação de filme de acordo com qualquer um das reivindicações 1 a 6,caracterizado pelo fato de que adicionalmente compre- ende um metal ou um composto de metal coordenado pela estrutura de co- ordenação de metal não-iônico.
8. Material de formação de filme de acordo com a reivindicação7, caracterizado pelo fato de que o metal ou composto de metal é seleciona- do de um grupo que consiste em M, MO, M2O3, M(OH)n, RxMO, e combina- ções dos mesmos; em que, M é um metal selecionado do grupo que consis- te em Al, Bi, Ce, Cu, Fe, Pb, Sn, Sb, Ti, Y, Zn, e Zr; η é um número inteiro satisfazendo a valência de M; R é um grupo alquila ou aromático; e χ é um número inteiro de 1 a 6.
9. Material de formação de filme de acordo com a reivindicação7, caracterizado pelo fato de que o metal ou composto de metal compreende um catalisador de metal selecionado de um grupo que consiste em óxido de dibutilestanho, dilaurato de dibutilestanho, óxido de zinco, óxido de bismuto, óxido de estanho, óxido de ítrio, óxido de cobre, e combinações dos mes- mos.
10. Material de formação de filme de acordo com qualquer um das reivindicações 1 a 9, caracterizado pelo fato de que a resina compreen- de pelo menos: (a) um produto de uma reação de: uma resina, em que a resina tem pelo menos um grupo reativo com um nucleófilo, e - um Iigante nucleofílico, em que o Iigante nucleofílico tem a fórmula:X3-R4-X4 em que,X3 é um radical monovalente de hidroxila ou carbo- xila; R4 é um radical divalente de alquileno ou arileno tendo um peso molecu- lar de cerca de 90 g/mol a cerca de 5000 g/mol e uma estrutura de coorde- nação de metal não-iônico compreendendo pelo menos dois grupos funcio- nais ricos em elétrons, independentemente selecionados do grupo que con- siste em: nitrogênio, oxigênio, fósforo, enxofre, silício, carbono insaturado, éster, cetona, éter e hidroxila; e X4 é um radical monovalente de hidrogênio, hidroxila, ou carboxila; (b) um produto de uma reação de: - uma resina que tem pelo menos um grupo reativo com um eletrófilo, e um Iigante eletrofílico, em que o Iigante eletrofílico tem a fórmula:X5-R5-X6 em que, X5 é um radical monovalente de epóxido ou haleto; R5 é um radical divalente de alquileno ou arileno tendo um peso molecular de cerca de 90 g/mol a cerca de 5000 g/mol e uma estrutura de coordenação de metal não-iônico compreendendo pelo menos dois grupos funcionais ri- cos em elétrons, independentemente selecionados do grupo que consiste em: nitrogênio, oxigênio, fósforo, enxofre, silício, carbono insaturado, éster, cetona, éter e hidroxila; e X6 é um radical monovalente de hidrogênio, epóxi- do, ou haleto.
11. Material de formação de filme de acordo com a reivindicação 10, caracterizado pelo fato de que pelo menos um grupo reativo com um nu- cleófilo é um grupo epóxido.
12. Material de formação de filme de acordo com a reivindicação 10 ou 11, caracterizado pelo fato de que o Iigante nucleofílico é selecionado de um grupo que consiste em etil-2-hidroxibenzoato, etil-4-hidroxibenzoato, 4-hidróxi-1-(4-hidroxifenil)pentan-2-ona, 1-(2- hidróxi-6-metoxifenil)etanona, e combinações dos mesmos.
13. Material de formação de filme de acordo com a reivindicação10, caracterizado pelo fato de que o pelo menos um grupo reativo com um eletrófilo é um grupo hidroxila.
14. Material de formação de filme de acordo com a reivindicação ou 13, caracterizado pelo fato de que o Iigante eletrofílico é selecionado de um grupo que consiste em 3-metil-1-(oxiran-2-il)but-3-en-2-ona, etilfenil- glicidato, e combinações dos mesmos.
15. Composição de revestimento, caracterizada pelo fato de que compreende um material de formação de filme como definido em qualquer uma das reivindicações 1 a 14. ι
BRPI0718191-4A 2006-10-26 2007-08-13 Materiais de coordenação de metal e de formação de filme BRPI0718191A2 (pt)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US11/553,185 2006-10-26
US11/553,185 US7759436B2 (en) 2006-10-26 2006-10-26 Film-former of resin with nonionic metal coordinating structure and crosslinker-reactive group
PCT/US2007/075764 WO2008051648A1 (en) 2006-10-26 2007-08-13 Metal coordinating and film-forming materials

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BRPI0718191A2 true BRPI0718191A2 (pt) 2013-11-05

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US (1) US7759436B2 (pt)
EP (1) EP2076555B1 (pt)
JP (1) JP5383494B2 (pt)
KR (1) KR20090080099A (pt)
CN (1) CN101528795B (pt)
AT (1) ATE494317T1 (pt)
BR (1) BRPI0718191A2 (pt)
CA (1) CA2629072A1 (pt)
DE (1) DE602007011794D1 (pt)
WO (1) WO2008051648A1 (pt)

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KR102072223B1 (ko) 2016-10-20 2020-01-31 주식회사 엘지화학 코폴리카보네이트 및 이를 포함하는 수지 조성물
CN109749103B (zh) * 2018-12-13 2021-11-19 东华大学 一种不溶不熔的金属改性十字型酯化物及其制备方法
CN111978513A (zh) * 2019-06-14 2020-11-24 上海雄润树脂有限公司 一种高压电开关浇注用环氧树脂及其制备方法
CN110256678A (zh) * 2019-06-24 2019-09-20 界首万昌新材料技术有限公司 一种成膜时间短的改性硅油的制备方法
CN111909336B (zh) * 2020-07-15 2022-11-04 芦娜 一种聚氨酯固体废弃物的降解方法
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CN101528795B (zh) 2012-02-29
EP2076555B1 (en) 2011-01-05
CN101528795A (zh) 2009-09-09
US20080103268A1 (en) 2008-05-01
KR20090080099A (ko) 2009-07-23
DE602007011794D1 (pt) 2011-02-17
EP2076555A1 (en) 2009-07-08
CA2629072A1 (en) 2008-05-02
ATE494317T1 (de) 2011-01-15
US7759436B2 (en) 2010-07-20
WO2008051648A1 (en) 2008-05-02
JP5383494B2 (ja) 2014-01-08
JP2010508396A (ja) 2010-03-18

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