AU2016305184B2 - Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts - Google Patents

Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts Download PDF

Info

Publication number
AU2016305184B2
AU2016305184B2 AU2016305184A AU2016305184A AU2016305184B2 AU 2016305184 B2 AU2016305184 B2 AU 2016305184B2 AU 2016305184 A AU2016305184 A AU 2016305184A AU 2016305184 A AU2016305184 A AU 2016305184A AU 2016305184 B2 AU2016305184 B2 AU 2016305184B2
Authority
AU
Australia
Prior art keywords
copper
layer
binder
mixture
weight
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Active
Application number
AU2016305184A
Other languages
English (en)
Other versions
AU2016305184A1 (en
Inventor
Ralf Krause
Anna Maltenberger
Christian Reller
Bernhard Schmid
Günter Schmid
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Siemens Energy Global GmbH and Co KG
Original Assignee
Siemens Energy Global GmbH and Co KG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Siemens Energy Global GmbH and Co KG filed Critical Siemens Energy Global GmbH and Co KG
Publication of AU2016305184A1 publication Critical patent/AU2016305184A1/en
Application granted granted Critical
Publication of AU2016305184B2 publication Critical patent/AU2016305184B2/en
Assigned to Siemens Energy Global GmbH & Co. KG reassignment Siemens Energy Global GmbH & Co. KG Request for Assignment Assignors: SIEMENS AKTIENGESELLSCHAFT
Active legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/02—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form
    • C25B11/03—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form perforated or foraminous
    • C25B11/031—Porous electrodes
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
    • C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
    • C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
    • C25B11/055—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the substrate or carrier material
    • C25B11/057—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the substrate or carrier material consisting of a single element or compound
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
    • C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
    • C25B11/073—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material
    • C25B11/091—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of at least one catalytic element and at least one catalytic compound; consisting of two or more catalytic elements or catalytic compounds
    • C25B11/095—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of at least one catalytic element and at least one catalytic compound; consisting of two or more catalytic elements or catalytic compounds at least one of the compounds being organic
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/20—Processes
    • C25B3/25—Reduction

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)
  • Electrodes For Compound Or Non-Metal Manufacture (AREA)
  • Catalysts (AREA)
AU2016305184A 2015-08-11 2016-07-19 Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts Active AU2016305184B2 (en)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE102015215309.6A DE102015215309A1 (de) 2015-08-11 2015-08-11 Präparationstechnik von kohlenwasserstoffselektiven Gasdiffusionselektroden basierend auf Cu-haltigen-Katalysatoren
DE102015215309.6 2015-08-11
PCT/EP2016/067165 WO2017025285A1 (de) 2015-08-11 2016-07-19 Präparationstechnik von kohlenwasserstoffselektiven gasdiffusionselektroden basierend auf cu-haltigen-katalysatoren

Publications (2)

Publication Number Publication Date
AU2016305184A1 AU2016305184A1 (en) 2018-02-01
AU2016305184B2 true AU2016305184B2 (en) 2019-02-28

Family

ID=56511563

Family Applications (1)

Application Number Title Priority Date Filing Date
AU2016305184A Active AU2016305184B2 (en) 2015-08-11 2016-07-19 Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts

Country Status (10)

Country Link
US (1) US20180230612A1 (zh)
EP (1) EP3307924B1 (zh)
CN (1) CN107923052B (zh)
AU (1) AU2016305184B2 (zh)
DE (1) DE102015215309A1 (zh)
DK (1) DK3307924T3 (zh)
ES (1) ES2746118T3 (zh)
PL (1) PL3307924T3 (zh)
SA (1) SA518390888B1 (zh)
WO (1) WO2017025285A1 (zh)

Families Citing this family (26)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102017203900A1 (de) 2017-03-09 2018-09-13 Siemens Aktiengesellschaft Elektroden umfassend in Festkörperelektrolyten eingebrachtes Metall
DE102017203903A1 (de) * 2017-03-09 2018-09-13 Siemens Aktiengesellschaft Schwerlösliche Salze als Zuschlag zu Gasdiffusionselektroden zur Erhöhung der CO2-Selektivität bei hohen Stromdichten
DE102017204096A1 (de) 2017-03-13 2018-09-13 Siemens Aktiengesellschaft Herstellung von Gasdiffusionselektroden mit Ionentransport-Harzen zur elektrochemischen Reduktion von CO2 zu chemischen Wertstoffen
JP6622237B2 (ja) 2017-03-14 2019-12-18 株式会社東芝 二酸化炭素電解装置
JP6672211B2 (ja) * 2017-03-21 2020-03-25 株式会社東芝 二酸化炭素電解装置および二酸化炭素電解方法
DE102017208518A1 (de) 2017-05-19 2018-11-22 Siemens Aktiengesellschaft Herstellung von dendritischen Elektrokatalysatoren zur Reduktion von CO2 und/oder CO
DE102017208610A1 (de) * 2017-05-22 2018-11-22 Siemens Aktiengesellschaft Zwei-Membran-Aufbau zur elektrochemischen Reduktion von CO2
DE102017212278A1 (de) * 2017-07-18 2019-01-24 Siemens Aktiengesellschaft CO2-Elektrolyseur
DE102017118118A1 (de) * 2017-08-09 2019-02-14 Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. Elektrode für eine insbesondere bioelektrochemische Zelle
DE102017219766A1 (de) * 2017-11-07 2019-05-09 Siemens Aktiengesellschaft Anordnung für die Kohlendioxid-Elektrolyse
DE102018212409A1 (de) 2017-11-16 2019-05-16 Siemens Aktiengesellschaft Kohlenwasserstoff-selektive Elektrode
US11299811B2 (en) * 2018-01-29 2022-04-12 Board Of Regents, The University Of Texas System Continuous flow reactor and hybrid electro-catalyst for high selectivity production of C2H4 from CO2 and water via electrolysis
DE102018202184A1 (de) 2018-02-13 2019-08-14 Siemens Aktiengesellschaft Separatorlose Doppel-GDE-Zelle zur elektrochemischen Umsetzung
DE102018105115A1 (de) * 2018-03-06 2019-09-12 Deutsches Zentrum für Luft- und Raumfahrt e.V. Elektrode, Zelleneinheit und Elektrolyseur
DE102018205571A1 (de) * 2018-03-29 2019-10-02 Siemens Aktiengesellschaft Gasdiffusionselektrode, eine Elektrolyseanordnung sowie ein Verfahren zum Betreiben einer Elektrolyseanlage
DE102018210457A1 (de) * 2018-06-27 2020-01-02 Siemens Aktiengesellschaft Gasdiffusionselektrode zur Kohlendioxid-Verwertung, Verfahren zu deren Herstellung sowie Elektrolysezelle mit Gasdiffusionselektrode
DE102018210458A1 (de) 2018-06-27 2020-01-02 Siemens Aktiengesellschaft Gasdiffusionselektrode zur Kohlendioxid-Verwertung, Verfahren zu deren Herstellung sowie Elektrolysezelle mit Gasdiffusionselektrode
FI3827114T3 (fi) * 2018-07-23 2023-06-30 Governing Council Univ Toronto Katalyyttejä co2:n elektrokemialliseksi pelkistämiseksi ja siihen liittyviä menetelmiä
CN109695048B (zh) * 2019-02-28 2020-08-07 武汉大学 自支撑碳基体表面原位电化学生长纳米碳化物基电催化膜层的方法及应用
CN111074294B (zh) * 2019-12-12 2021-12-14 中国科学技术大学 一种铜合金材料电催化二氧化碳制备含碳化合物的方法
DE102020205393A1 (de) 2020-04-29 2021-11-04 Siemens Aktiengesellschaft Bimetallische und multimetallische Katalysatoren zur selektiven Elektroreduzierung von CO2 und/oder CO zu Kohlenwasserstoffen und Oxygenaten
DE102020206448A1 (de) 2020-05-25 2021-11-25 Siemens Aktiengesellschaft Vorrichtung zum Befestigen einer Elektrode
DE102020206449A1 (de) 2020-05-25 2021-11-25 Siemens Aktiengesellschaft Verfahren zum Befestigen einer Elektrode
CN114574889A (zh) * 2021-12-13 2022-06-03 中国科学技术大学 一种气体扩散电极及其制备方法和应用
CN114481184A (zh) * 2021-12-21 2022-05-13 上海交通大学 一种用于二氧化碳电化学还原的气体扩散层及其制备方法
CN114908375A (zh) * 2022-05-25 2022-08-16 中国科学技术大学 电催化co2还原中具有稳定活性位点的铜催化剂及其制备方法与应用

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3710168A1 (de) * 1987-03-27 1988-10-13 Varta Batterie Verfahren zur herstellung einer kunststoffgebundenen gasdiffusionselektrode mit metallischen elektrokatalysatoren
DE102005023615A1 (de) * 2005-05-21 2006-11-23 Bayer Materialscience Ag Verfahren zur Herstellung von Gasdiffusionselektroden

Family Cites Families (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3303779A1 (de) 1983-02-04 1984-08-16 Hoechst Ag, 6230 Frankfurt Verfahren zur herstellung eines katalytisch wirksamen elektrodenmaterials fuer sauerstoffverzehr-elektroden
DE3722019A1 (de) 1987-07-03 1989-01-12 Varta Batterie Verfahren zur herstellung einer kunststoffgebundenen gasdiffusionselektrode, die einen manganoxidkatalysator der ueberwiegenden zusammensetzung mno(pfeil abwaerts)2(pfeil abwaerts)o(pfeil abwaerts)3(pfeil abwaerts)* x mn(pfeil abwaerts)5(pfeil abwaerts)o(pfeil abwaerts)8(pfeil abwaerts) enthaelt
DE10130441B4 (de) * 2001-06-23 2005-01-05 Uhde Gmbh Verfahren zum Herstellen von Gasdiffusionselektroden
DE10148599A1 (de) 2001-10-02 2003-04-10 Bayer Ag Verfahren zur Herstellung von Gasdiffusionselektroden aus trockenen Pulvermischungen mittels Walzen
DE10335184A1 (de) 2003-07-30 2005-03-03 Bayer Materialscience Ag Elektrochemische Zelle
DE102005003612B3 (de) 2005-01-26 2006-06-14 Forschungszentrum Jülich GmbH Verfahren zur Herstellung einer dünnen, gasdichten und Protonen leitenden Keramikschicht sowie Verwendung derselben
DE102010031571A1 (de) 2010-07-20 2012-01-26 Bayer Materialscience Ag Sauerstoffverzehrelektrode
DE102010042729A1 (de) 2010-10-21 2012-04-26 Bayer Materialscience Aktiengesellschaft Sauerstoffverzehrkathode und Verfahren zu ihrer Herstellung
CN103299463B (zh) * 2010-12-29 2016-09-28 帕马斯坎德公司 气体扩散电极

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3710168A1 (de) * 1987-03-27 1988-10-13 Varta Batterie Verfahren zur herstellung einer kunststoffgebundenen gasdiffusionselektrode mit metallischen elektrokatalysatoren
DE102005023615A1 (de) * 2005-05-21 2006-11-23 Bayer Materialscience Ag Verfahren zur Herstellung von Gasdiffusionselektroden

Also Published As

Publication number Publication date
EP3307924A1 (de) 2018-04-18
CN107923052A (zh) 2018-04-17
PL3307924T3 (pl) 2020-01-31
CN107923052B (zh) 2020-06-19
SA518390888B1 (ar) 2021-10-10
DK3307924T3 (da) 2019-09-02
ES2746118T3 (es) 2020-03-04
EP3307924B1 (de) 2019-06-19
AU2016305184A1 (en) 2018-02-01
WO2017025285A1 (de) 2017-02-16
US20180230612A1 (en) 2018-08-16
DE102015215309A1 (de) 2017-02-16

Similar Documents

Publication Publication Date Title
AU2016305184B2 (en) Method for preparing hydrocarbon-selective gas diffusion electrodes based on copper-containing catalysts
Merino-Garcia et al. Cu oxide/ZnO-based surfaces for a selective ethylene production from gas-phase CO2 electroconversion
AU2018233505B2 (en) Production of gas diffusion electrodes comprising ion transport resins for elctrochemical reduction of CO2 to afford chemical products
Peng et al. Separated growth of Bi-Cu bimetallic electrocatalysts on defective copper foam for highly converting CO2 to formate with alkaline anion-exchange membrane beyond KHCO3 electrolyte
AU2017329370B2 (en) Selective electrochemical hydrogenation of alkynes to alkenes
EP2659536B1 (en) Gas diffusion electrode and method for preparing the same
US20200208280A1 (en) Production of Dendritic Electrocatalysts for the Reduction Of CO2 and/or CO
Díaz-Sainz et al. Catalyst coated membrane electrodes for the gas phase CO2 electroreduction to formate
Liu et al. Design and engineering of urchin-like nanostructured SnO2 catalysts via controlled facial hydrothermal synthesis for efficient electro-reduction of CO2
AU2018232301A1 (en) Electrodes comprising metal introduced into a solid-state electrolyte
CN111373076A (zh) 具有混合价Cu4O3催化剂的乙烯选择性电极
Rhimi et al. Cu-based materials for enhanced C2+ product selectivity in photo-/electro-catalytic CO2 reduction: challenges and prospects
Yuda et al. Review of electrocatalytic reduction of CO2 on carbon supported films
US20210207277A1 (en) Gas diffusion electrode for carbon dioxide treatment, method for production thereof, and electrolysis cell having a gas diffusion electrode
Stamatelos et al. Exploring heterostructures of d-block metal oxides coupled to ZnO for the Electrochemical Reduction of CO2
Mezzapesa et al. Development of In–Cu binary oxide catalysts for hydrogenating CO 2 via thermocatalytic and electrocatalytic routes
US20230304175A1 (en) Catalyst for an electrochemical cell, and methods of making and using the catalyst
이기백 Design and Implementation of Binary Metal System for Understanding of Electrochemical CO2 Reduction Catalyst Stability
GB2619688A (en) Copper catalysts for the electrochemical conversion of carbon dioxide or carbon monoxide to C2+ products
Wan et al. CO2 Electrochemical Reduction to CO: From Catalysts, Electrodes to Electrolytic Cells and Effect of Operating Conditions
Ng et al. Elevating the prospects of green hydrogen (H2) production through solar-powered water splitting devices: A systematic review
Siracusano Development and characterization of catalysts for electrolytic hydrogen production and chlor–alkali electrolysis cells
WO2022153236A1 (en) Use of semiconductors to control the selectivity of eletrochemical reduction of carbon dioxide

Legal Events

Date Code Title Description
FGA Letters patent sealed or granted (standard patent)
PC Assignment registered

Owner name: SIEMENS ENERGY GLOBAL GMBH & CO. KG

Free format text: FORMER OWNER(S): SIEMENS AKTIENGESELLSCHAFT