WO2011016668A3 - 메탄의 열분해 및 이산화탄소 전환 반응을 포함하는 탄소 함유 물질의 가스화 방법 - Google Patents

메탄의 열분해 및 이산화탄소 전환 반응을 포함하는 탄소 함유 물질의 가스화 방법 Download PDF

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Publication number
WO2011016668A3
WO2011016668A3 PCT/KR2010/005101 KR2010005101W WO2011016668A3 WO 2011016668 A3 WO2011016668 A3 WO 2011016668A3 KR 2010005101 W KR2010005101 W KR 2010005101W WO 2011016668 A3 WO2011016668 A3 WO 2011016668A3
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WO
WIPO (PCT)
Prior art keywords
carbon
gasification
containing materials
methane
conversion
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PCT/KR2010/005101
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English (en)
French (fr)
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WO2011016668A2 (ko
Inventor
김진홍
이상호
김경록
정일용
최선
오승훈
김규태
이용일
Original Assignee
에스케이이노베이션 주식회사
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Priority to AU2010279831A priority Critical patent/AU2010279831B2/en
Priority to CN201080034787.3A priority patent/CN102597182B/zh
Priority to CA2770290A priority patent/CA2770290C/en
Priority to US13/388,702 priority patent/US8663504B2/en
Priority to DE112010003184T priority patent/DE112010003184T5/de
Priority to JP2012523562A priority patent/JP5686803B2/ja
Publication of WO2011016668A2 publication Critical patent/WO2011016668A2/ko
Publication of WO2011016668A3 publication Critical patent/WO2011016668A3/ko

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    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/22—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds
    • C01B3/24—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds of hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C10J3/02—Fixed-bed gasification of lump fuel
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10K—PURIFYING OR MODIFYING THE CHEMICAL COMPOSITION OF COMBUSTIBLE GASES CONTAINING CARBON MONOXIDE
    • C10K1/00—Purifying combustible gases containing carbon monoxide
    • C10K1/002—Removal of contaminants
    • C10K1/003—Removal of contaminants of acid contaminants, e.g. acid gas removal
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10K—PURIFYING OR MODIFYING THE CHEMICAL COMPOSITION OF COMBUSTIBLE GASES CONTAINING CARBON MONOXIDE
    • C10K3/00—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide
    • C10K3/06—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide by mixing with gases
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0266—Processes for making hydrogen or synthesis gas containing a decomposition step
    • C01B2203/0272—Processes for making hydrogen or synthesis gas containing a decomposition step containing a non-catalytic decomposition step
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0913—Carbonaceous raw material
    • C10J2300/093—Coal
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0953—Gasifying agents
    • C10J2300/0966—Hydrogen
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0953—Gasifying agents
    • C10J2300/0973—Water
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0983—Additives
    • C10J2300/0986—Catalysts
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/16—Integration of gasification processes with another plant or parts within the plant
    • C10J2300/164—Integration of gasification processes with another plant or parts within the plant with conversion of synthesis gas
    • C10J2300/1656—Conversion of synthesis gas to chemicals
    • C10J2300/1659—Conversion of synthesis gas to chemicals to liquid hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/16—Integration of gasification processes with another plant or parts within the plant
    • C10J2300/164—Integration of gasification processes with another plant or parts within the plant with conversion of synthesis gas
    • C10J2300/1656—Conversion of synthesis gas to chemicals
    • C10J2300/1665—Conversion of synthesis gas to chemicals to alcohols, e.g. methanol or ethanol
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/18—Details of the gasification process, e.g. loops, autothermal operation
    • C10J2300/1807—Recycle loops, e.g. gas, solids, heating medium, water

Abstract

본 발명은 탄소 함유 물질의 가스화에 관한 것으로, 보다 상세하게는 탄소 효율을 높이고 이산화탄소의 발생을 감소시킬 수 있는 탄소 함유 물질의 가스화 방법에 관한 것으로서, 가스화단계를 통하여 산출된 CH4를 C 및 H2로 분해하여 생성된 탄소 등을 재순환시키고, 공정 중의 생성물을 이용하여, CO2를 CO로 전환시키는 단계를 포함함으로써, 높은 탄소효율을 달성하고 이산화탄소의 발생량을 줄일 수 있는 효과를 지닌다.
PCT/KR2010/005101 2009-08-04 2010-08-03 메탄의 열분해 및 이산화탄소 전환 반응을 포함하는 탄소 함유 물질의 가스화 방법 WO2011016668A2 (ko)

Priority Applications (6)

Application Number Priority Date Filing Date Title
AU2010279831A AU2010279831B2 (en) 2009-08-04 2010-08-03 Method for gasification of carbon-containing materials by thermal decomposition of methane and conversion of carbon dioxide
CN201080034787.3A CN102597182B (zh) 2009-08-04 2010-08-03 通过甲烷热分解和二氧化碳转化将含碳材料气化的方法
CA2770290A CA2770290C (en) 2009-08-04 2010-08-03 Method for gasification of carbon-containing materials by thermal decomposition of methane and conversion of carbon dioxide
US13/388,702 US8663504B2 (en) 2009-08-04 2010-08-03 Method for gasification of carbon-containing materials by thermal decomposition of methane and conversion of carbon dioxide
DE112010003184T DE112010003184T5 (de) 2009-08-04 2010-08-03 Verfahren zur Vergasung von kohlenstoffhaltigen Material ien mittels thermischer Zersetzung von Methan und Umwandlung von Kohlendioxid
JP2012523562A JP5686803B2 (ja) 2009-08-04 2010-08-03 メタン熱分解及び二酸化炭素転換反応を含む炭素含有物質のガス化方法

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
KR1020090071688A KR101570882B1 (ko) 2009-08-04 2009-08-04 메탄의 열분해 및 이산화탄소 전환 반응을 포함하는 탄소 함유 물질의 가스화 방법
KR10-2009-0071688 2009-08-04

Publications (2)

Publication Number Publication Date
WO2011016668A2 WO2011016668A2 (ko) 2011-02-10
WO2011016668A3 true WO2011016668A3 (ko) 2011-06-30

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PCT/KR2010/005101 WO2011016668A2 (ko) 2009-08-04 2010-08-03 메탄의 열분해 및 이산화탄소 전환 반응을 포함하는 탄소 함유 물질의 가스화 방법

Country Status (8)

Country Link
US (1) US8663504B2 (ko)
JP (1) JP5686803B2 (ko)
KR (1) KR101570882B1 (ko)
CN (1) CN102597182B (ko)
AU (1) AU2010279831B2 (ko)
CA (1) CA2770290C (ko)
DE (1) DE112010003184T5 (ko)
WO (1) WO2011016668A2 (ko)

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CN102597182A (zh) 2012-07-18
CA2770290A1 (en) 2011-02-10
JP2013501123A (ja) 2013-01-10
CN102597182B (zh) 2014-08-20
WO2011016668A2 (ko) 2011-02-10
DE112010003184T5 (de) 2012-06-28
US20120241676A1 (en) 2012-09-27
KR20110013968A (ko) 2011-02-10
KR101570882B1 (ko) 2015-11-23
AU2010279831A1 (en) 2012-02-23
JP5686803B2 (ja) 2015-03-18
AU2010279831B2 (en) 2016-02-25
US8663504B2 (en) 2014-03-04
CA2770290C (en) 2017-01-24

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