WO2009005003A1 - 遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法 - Google Patents

遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法 Download PDF

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Publication number
WO2009005003A1
WO2009005003A1 PCT/JP2008/061740 JP2008061740W WO2009005003A1 WO 2009005003 A1 WO2009005003 A1 WO 2009005003A1 JP 2008061740 W JP2008061740 W JP 2008061740W WO 2009005003 A1 WO2009005003 A1 WO 2009005003A1
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WIPO (PCT)
Prior art keywords
transition metal
metal complex
compound
complex compound
polymerization catalyst
Prior art date
Application number
PCT/JP2008/061740
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English (en)
French (fr)
Inventor
Yasuhiko Suzuki
Shinsuke Kinoshita
Atsushi Shibahara
Naritoshi Yoshimura
Isao Hara
Tetsuya Hamada
Kazumori Kawamura
Kou Tsurugi
Yasunori Saito
Seiichi Ishii
Yasushi Nakayama
Naoto Matsukawa
Susumu Murata
Original Assignee
Mitsui Chemicals, Inc.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Publication date
Application filed by Mitsui Chemicals, Inc. filed Critical Mitsui Chemicals, Inc.
Priority to KR1020107002504A priority Critical patent/KR101143713B1/ko
Priority to CN200880022637.3A priority patent/CN101687776B/zh
Priority to US12/452,438 priority patent/US8258361B2/en
Priority to JP2009521612A priority patent/JP5126993B2/ja
Priority to EP08790705.1A priority patent/EP2174928B1/en
Publication of WO2009005003A1 publication Critical patent/WO2009005003A1/ja
Priority to ZA2010/00020A priority patent/ZA201000020B/en

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F10/00—Homopolymers and copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/02—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides
    • B01J31/12—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing organo-metallic compounds or metal hydrides
    • B01J31/14—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing organo-metallic compounds or metal hydrides of aluminium or boron
    • B01J31/143—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing organo-metallic compounds or metal hydrides of aluminium or boron of aluminium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/1616—Coordination complexes, e.g. organometallic complexes, immobilised on an inorganic support, e.g. ship-in-a-bottle type catalysts
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/22—Organic complexes
    • B01J31/2204—Organic complexes the ligands containing oxygen or sulfur as complexing atoms
    • B01J31/2208—Oxygen, e.g. acetylacetonates
    • B01J31/2226—Anionic ligands, i.e. the overall ligand carries at least one formal negative charge
    • B01J31/2243—At least one oxygen and one nitrogen atom present as complexing atoms in an at least bidentate or bridging ligand
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
    • C07C2/02—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by addition between unsaturated hydrocarbons
    • C07C2/04—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by addition between unsaturated hydrocarbons by oligomerisation of well-defined unsaturated hydrocarbons without ring formation
    • C07C2/06—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by addition between unsaturated hydrocarbons by oligomerisation of well-defined unsaturated hydrocarbons without ring formation of alkenes, i.e. acyclic hydrocarbons having only one carbon-to-carbon double bond
    • C07C2/08—Catalytic processes
    • C07C2/26—Catalytic processes with hydrides or organic compounds
    • C07C2/32—Catalytic processes with hydrides or organic compounds as complexes, e.g. acetyl-acetonates
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C251/00—Compounds containing nitrogen atoms doubly-bound to a carbon skeleton
    • C07C251/02—Compounds containing nitrogen atoms doubly-bound to a carbon skeleton containing imino groups
    • C07C251/24—Compounds containing nitrogen atoms doubly-bound to a carbon skeleton containing imino groups having carbon atoms of imino groups bound to carbon atoms of six-membered aromatic rings
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F7/00—Compounds containing elements of Groups 4 or 14 of the Periodic Table
    • C07F7/003—Compounds containing elements of Groups 4 or 14 of the Periodic Table without C-Metal linkages
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
    • B01J2231/10—Polymerisation reactions involving at least dual use catalysts, e.g. for both oligomerisation and polymerisation
    • B01J2231/12—Olefin polymerisation or copolymerisation
    • B01J2231/122—Cationic (co)polymerisation, e.g. single-site or Ziegler-Natta type
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
    • B01J2231/20—Olefin oligomerisation or telomerisation
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/40—Complexes comprising metals of Group IV (IVA or IVB) as the central metal
    • B01J2531/46—Titanium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/60—Complexes comprising metals of Group VI (VIA or VIB) as the central metal
    • B01J2531/62—Chromium
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2521/00—Catalysts comprising the elements, oxides or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium or hafnium
    • C07C2521/06—Silicon, titanium, zirconium or hafnium; Oxides or hydroxides thereof
    • C07C2521/08—Silica
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2521/00—Catalysts comprising the elements, oxides or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium or hafnium
    • C07C2521/16—Clays or other mineral silicates
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2531/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • C07C2531/02—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides
    • C07C2531/12—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing organo-metallic compounds or metal hydrides
    • C07C2531/14—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing organo-metallic compounds or metal hydrides of aluminium or boron
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2531/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • C07C2531/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • C07C2531/22—Organic complexes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F110/00—Homopolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F110/02—Ethene

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Materials Engineering (AREA)
  • Engineering & Computer Science (AREA)
  • Inorganic Chemistry (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Health & Medical Sciences (AREA)
  • Catalysts (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Transition And Organic Metals Composition Catalysts For Addition Polymerization (AREA)
  • Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)

Abstract

　本発明は遷移金属錯体化合物、および該化合物を含有する、優れた活性を有するオレフィン多量化用触媒を提供することと、該オレフィン多量化用触媒存在下で行うオレフィン多量体の製造方法を提供することを目的する。 　本発明の[Ａ]遷移金属錯体化合物は下記一般式（Ｉ）または（Ｉ’）で表される。本発明のオレフィン多量化用触媒は、[Ａ]遷移金属化合物を含んでおり、本発明のオレフィン多量体の製造方法は、該触媒の存在下でオレフィンの多量化を行うことを特徴とする。
PCT/JP2008/061740 2007-07-04 2008-06-27 遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法 WO2009005003A1 (ja)

Priority Applications (6)

Application Number Priority Date Filing Date Title
KR1020107002504A KR101143713B1 (ko) 2007-07-04 2008-06-27 전이금속 착체 화합물, 이 화합물을 포함하는 올레핀 다량화용 촉매 및 이 촉매 존재 하에서 실시하는 올레핀 다량체의 제조 방법
CN200880022637.3A CN101687776B (zh) 2007-07-04 2008-06-27 过渡金属配位化合物、含有该化合物的烯烃聚合用催化剂以及在该催化剂存在下进行的烯烃聚合物的制造方法
US12/452,438 US8258361B2 (en) 2007-07-04 2008-06-27 Transition metal complex compounds, olefin oligomerization catalysts including the compounds, and processes for producing olefin oligomers using the catalysts
JP2009521612A JP5126993B2 (ja) 2007-07-04 2008-06-27 遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
EP08790705.1A EP2174928B1 (en) 2007-07-04 2008-06-27 Transition metal complex compound, olefin oligomerization catalyst containing the compound, and method for producing olefin oligomer performed in the presence of the catalyst
ZA2010/00020A ZA201000020B (en) 2007-07-04 2010-01-04 Transition metal complex compounds,olefin oligomerization catalysts including the compounds,and processes for producing olefin oligomers using the catalysts

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007-176026 2007-07-04
JP2007176026 2007-07-04

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Country Status (9)

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US (1) US8258361B2 (ja)
EP (1) EP2174928B1 (ja)
JP (1) JP5126993B2 (ja)
KR (1) KR101143713B1 (ja)
CN (1) CN101687776B (ja)
MY (1) MY152879A (ja)
TW (1) TWI433727B (ja)
WO (1) WO2009005003A1 (ja)
ZA (1) ZA201000020B (ja)

Cited By (22)

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JP2009072666A (ja) * 2007-09-19 2009-04-09 Mitsui Chemicals Inc オレフィン多量化用触媒およびエチレン多量体の製造方法
US20100227990A1 (en) * 2009-03-06 2010-09-09 Dow Global Technologies Inc. Catalysts, processes for making catalysts, processes for making polyolefin compositions, and polyolefin compositions
JP2011016789A (ja) * 2009-06-08 2011-01-27 Mitsui Chemicals Inc 遷移金属化合物、オレフィン重合用触媒およびポリオレフィンの製造方法
JP2011195583A (ja) * 2010-02-26 2011-10-06 Mitsui Chemicals Inc 遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
JP2011195584A (ja) * 2010-02-26 2011-10-06 Mitsui Chemicals Inc 遷移金属錯体化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
WO2012133919A1 (en) * 2011-03-30 2012-10-04 Sumitomo Chemical Company, Limited Process for producing catalyst for producing ethylenic polymer, catalyst for producing ethylenic polymer and process for producing ethylenic polymer
WO2012133928A1 (en) * 2011-03-30 2012-10-04 Sumitomo Chemical Company, Limited Trimerization catalyst and method for producing 1-hexene
WO2012133936A1 (en) * 2011-03-30 2012-10-04 Sumitomo Chemical Company, Limited Catalyst for producing ethylene-based polymer and method for producing the same
JP2013060400A (ja) * 2011-09-14 2013-04-04 Mitsui Chemicals Inc オレフィンの製造方法
JP2013095671A (ja) * 2011-10-28 2013-05-20 Mitsui Chemicals Inc オレフィンの製造方法
WO2014123212A1 (ja) 2013-02-08 2014-08-14 三井化学株式会社 固体状ポリアルミノキサン組成物、オレフィン重合用触媒、オレフィン重合体の製造方法、および固体状ポリアルミノキサン組成物の製造方法
WO2014133005A1 (ja) 2013-02-27 2014-09-04 三井化学株式会社 オレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
JP2014224053A (ja) * 2013-05-15 2014-12-04 三井化学株式会社 遷移金属化合物、オレフィン重合用触媒およびオレフィン系重合体の製造方法
US20150259361A1 (en) * 2012-09-30 2015-09-17 Bridgestone Corporation Organometallic Catalyst Complex And Polymerization Method Employing Same
JP2016182554A (ja) * 2015-03-26 2016-10-20 東京応化工業株式会社 濾過材料、濾過フィルター、濾過方法、フェニルイミン化合物の製造方法、アルコキシフェニルイミン化合物の製造方法、化合物
JP2016188204A (ja) * 2015-03-27 2016-11-04 三井化学株式会社 遷移金属化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
JP2017095359A (ja) * 2015-11-18 2017-06-01 三井化学株式会社 遷移金属化合物、該化合物を含むオレフィン多量化用触媒および該触媒存在下で行うオレフィン多量体の製造方法
JP2018162229A (ja) * 2017-03-27 2018-10-18 三井化学株式会社 遷移金属化合物、オレフィン多量化用触媒およびオレフィン多量体の製造方法
JP2018162230A (ja) * 2017-03-27 2018-10-18 三井化学株式会社 遷移金属化合物、オレフィン多量化用触媒およびオレフィン多量体の製造方法
US10124326B2 (en) 2014-09-30 2018-11-13 Sumitomo Chemical Company, Limited Modified solid polyalkylaluminoxane and catalyst for olefin oligomerization reaction
WO2019009390A1 (ja) 2017-07-06 2019-01-10 三井化学株式会社 オレフィン多量化用触媒およびその触媒存在下で行うオレフィン多量体の製造方法
JP2021066675A (ja) * 2019-10-18 2021-04-30 三井化学株式会社 遷移金属化合物、オレフィン重合用触媒およびオレフィン重合体の製造方法

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KR101513145B1 (ko) 2012-05-10 2015-04-17 주식회사 엘지화학 리간드 화합물, 크롬 화합물 및 이를 포함하는 촉매계
CN102838637B (zh) * 2012-09-18 2015-08-19 华东理工大学 亚胺酚氧基镁化合物及其制备方法和应用
US9969828B2 (en) * 2016-01-21 2018-05-15 California Institute Of Technology Co-supported catalysts for the tandem trimerization and polymerization of ethylene to produce linear low density polyethylene
CN116669852A (zh) * 2020-12-24 2023-08-29 浙江大学 共价有机框架材料、催化剂、其制备方法及应用

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