JP2012506357A - カーボンナノチューブ、フラーレン及び/又はグラフェン含有コーティングの製造方法 - Google Patents
カーボンナノチューブ、フラーレン及び/又はグラフェン含有コーティングの製造方法 Download PDFInfo
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- JP2012506357A JP2012506357A JP2011532491A JP2011532491A JP2012506357A JP 2012506357 A JP2012506357 A JP 2012506357A JP 2011532491 A JP2011532491 A JP 2011532491A JP 2011532491 A JP2011532491 A JP 2011532491A JP 2012506357 A JP2012506357 A JP 2012506357A
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- carbon nanotubes
- fullerenes
- graphene
- graphenes
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- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 title claims abstract description 122
- 239000002041 carbon nanotube Substances 0.000 title claims abstract description 69
- 229910021393 carbon nanotube Inorganic materials 0.000 title claims abstract description 69
- 238000000576 coating method Methods 0.000 title claims abstract description 69
- 239000011248 coating agent Substances 0.000 title claims abstract description 66
- XMWRBQBLMFGWIX-UHFFFAOYSA-N C60 fullerene Chemical compound C12=C3C(C4=C56)=C7C8=C5C5=C9C%10=C6C6=C4C1=C1C4=C6C6=C%10C%10=C9C9=C%11C5=C8C5=C8C7=C3C3=C7C2=C1C1=C2C4=C6C4=C%10C6=C9C9=C%11C5=C5C8=C3C3=C7C1=C1C2=C4C6=C2C9=C5C3=C12 XMWRBQBLMFGWIX-UHFFFAOYSA-N 0.000 title claims abstract description 63
- 229910003472 fullerene Inorganic materials 0.000 title claims abstract description 62
- 229910021389 graphene Inorganic materials 0.000 title claims abstract description 62
- 238000004519 manufacturing process Methods 0.000 title claims abstract description 6
- 238000000034 method Methods 0.000 claims abstract description 23
- ATJFFYVFTNAWJD-UHFFFAOYSA-N Tin Chemical compound [Sn] ATJFFYVFTNAWJD-UHFFFAOYSA-N 0.000 claims abstract description 21
- 239000000758 substrate Substances 0.000 claims abstract description 21
- 238000007669 thermal treatment Methods 0.000 claims abstract description 7
- 238000002844 melting Methods 0.000 claims description 12
- 230000008018 melting Effects 0.000 claims description 12
- 239000002184 metal Substances 0.000 claims description 11
- 229910052751 metal Inorganic materials 0.000 claims description 11
- RYGMFSIKBFXOCR-UHFFFAOYSA-N Copper Chemical compound [Cu] RYGMFSIKBFXOCR-UHFFFAOYSA-N 0.000 claims description 9
- 239000007788 liquid Substances 0.000 claims description 9
- 239000007787 solid Substances 0.000 claims description 9
- 229910045601 alloy Inorganic materials 0.000 claims description 8
- 239000000956 alloy Substances 0.000 claims description 8
- 229910052802 copper Inorganic materials 0.000 claims description 8
- 239000010949 copper Substances 0.000 claims description 8
- 229910001128 Sn alloy Inorganic materials 0.000 claims description 6
- 238000010438 heat treatment Methods 0.000 claims description 5
- 238000007664 blowing Methods 0.000 claims description 4
- 239000002048 multi walled nanotube Substances 0.000 claims description 4
- 230000001681 protective effect Effects 0.000 claims description 4
- 239000002109 single walled nanotube Substances 0.000 claims description 4
- 238000005507 spraying Methods 0.000 claims description 4
- 229910052782 aluminium Inorganic materials 0.000 claims description 3
- 229910052742 iron Inorganic materials 0.000 claims description 3
- 238000004898 kneading Methods 0.000 claims description 3
- 235000011837 pasties Nutrition 0.000 claims description 2
- 239000000126 substance Substances 0.000 claims description 2
- XEEYBQQBJWHFJM-UHFFFAOYSA-N Iron Chemical compound [Fe] XEEYBQQBJWHFJM-UHFFFAOYSA-N 0.000 claims 4
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 claims 2
- 229910002804 graphite Inorganic materials 0.000 description 6
- 239000010439 graphite Substances 0.000 description 6
- 239000010410 layer Substances 0.000 description 6
- 229910052799 carbon Inorganic materials 0.000 description 5
- 125000004432 carbon atom Chemical group C* 0.000 description 5
- 239000007789 gas Substances 0.000 description 5
- 239000000463 material Substances 0.000 description 5
- XKRFYHLGVUSROY-UHFFFAOYSA-N Argon Chemical compound [Ar] XKRFYHLGVUSROY-UHFFFAOYSA-N 0.000 description 4
- 239000002071 nanotube Substances 0.000 description 3
- 239000004033 plastic Substances 0.000 description 3
- 229920003023 plastic Polymers 0.000 description 3
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- XUIMIQQOPSSXEZ-UHFFFAOYSA-N Silicon Chemical compound [Si] XUIMIQQOPSSXEZ-UHFFFAOYSA-N 0.000 description 2
- 229910052786 argon Inorganic materials 0.000 description 2
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 2
- 239000004020 conductor Substances 0.000 description 2
- 238000005260 corrosion Methods 0.000 description 2
- 230000007797 corrosion Effects 0.000 description 2
- 229910003460 diamond Inorganic materials 0.000 description 2
- 239000010432 diamond Substances 0.000 description 2
- 239000001301 oxygen Substances 0.000 description 2
- 229910052760 oxygen Inorganic materials 0.000 description 2
- 239000004065 semiconductor Substances 0.000 description 2
- 239000002356 single layer Substances 0.000 description 2
- 229910000838 Al alloy Inorganic materials 0.000 description 1
- 229910000640 Fe alloy Inorganic materials 0.000 description 1
- 229910000831 Steel Inorganic materials 0.000 description 1
- 230000015572 biosynthetic process Effects 0.000 description 1
- 239000006227 byproduct Substances 0.000 description 1
- 238000006243 chemical reaction Methods 0.000 description 1
- 150000001875 compounds Chemical class 0.000 description 1
- 238000001816 cooling Methods 0.000 description 1
- 239000013078 crystal Substances 0.000 description 1
- 238000000151 deposition Methods 0.000 description 1
- 238000010891 electric arc Methods 0.000 description 1
- 238000001704 evaporation Methods 0.000 description 1
- -1 for example Substances 0.000 description 1
- 238000009396 hybridization Methods 0.000 description 1
- 229910044991 metal oxide Inorganic materials 0.000 description 1
- 150000004706 metal oxides Chemical class 0.000 description 1
- 229910052757 nitrogen Inorganic materials 0.000 description 1
- 230000000149 penetrating effect Effects 0.000 description 1
- 229920000642 polymer Polymers 0.000 description 1
- 239000000843 powder Substances 0.000 description 1
- 239000012266 salt solution Substances 0.000 description 1
- 229910052710 silicon Inorganic materials 0.000 description 1
- 239000010703 silicon Substances 0.000 description 1
- HBMJWWWQQXIZIP-UHFFFAOYSA-N silicon carbide Chemical compound [Si+]#[C-] HBMJWWWQQXIZIP-UHFFFAOYSA-N 0.000 description 1
- 229910010271 silicon carbide Inorganic materials 0.000 description 1
- 238000005476 soldering Methods 0.000 description 1
- 239000010959 steel Substances 0.000 description 1
- 239000002887 superconductor Substances 0.000 description 1
- 239000000725 suspension Substances 0.000 description 1
- 238000003786 synthesis reaction Methods 0.000 description 1
- 238000005496 tempering Methods 0.000 description 1
Classifications
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D1/00—Processes for applying liquids or other fluent materials
- B05D1/36—Successively applying liquids or other fluent materials, e.g. without intermediate treatment
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
- H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
- H01B1/04—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of carbon-silicon compounds, carbon or silicon
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B05—SPRAYING OR ATOMISING IN GENERAL; APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D—PROCESSES FOR APPLYING FLUENT MATERIALS TO SURFACES, IN GENERAL
- B05D3/00—Pretreatment of surfaces to which liquids or other fluent materials are to be applied; After-treatment of applied coatings, e.g. intermediate treating of an applied coating preparatory to subsequent applications of liquids or other fluent materials
- B05D3/12—Pretreatment of surfaces to which liquids or other fluent materials are to be applied; After-treatment of applied coatings, e.g. intermediate treating of an applied coating preparatory to subsequent applications of liquids or other fluent materials by mechanical means
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
- C01G19/00—Compounds of tin
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C24/00—Coating starting from inorganic powder
- C23C24/02—Coating starting from inorganic powder by application of pressure only
- C23C24/04—Impact or kinetic deposition of particles
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C24/00—Coating starting from inorganic powder
- C23C24/02—Coating starting from inorganic powder by application of pressure only
- C23C24/06—Compressing powdered coating material, e.g. by milling
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C26/00—Coating not provided for in groups C23C2/00 - C23C24/00
-
- C—CHEMISTRY; METALLURGY
- C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
- C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
- C23C8/00—Solid state diffusion of only non-metal elements into metallic material surfaces; Chemical surface treatment of metallic material by reaction of the surface with a reactive gas, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals
- C23C8/02—Pretreatment of the material to be coated
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
- Y10T428/00—Stock material or miscellaneous articles
- Y10T428/12—All metal or with adjacent metals
- Y10T428/12493—Composite; i.e., plural, adjacent, spatially distinct metal components [e.g., layers, joint, etc.]
- Y10T428/12708—Sn-base component
Abstract
Description
Claims (20)
- 基体上にカーボンナノチューブ、フラーレン、及び/又はグラフェン含有のコーティングを製造する方法であり、カーボンナノチューブ、フラーレン及び/又はグラフェンを、スズ含有コーティング上に供すること、及び該カーボンナノチューブ、フラーレン及び/又はグラフェンを、機械的処理及び/又は熱的処理によってそのコーティング中に導入することを含む、上記方法。
- スズ含有コーティングとして、スズ又はスズ合金が使用されることを特徴とする、請求項1に記載の方法。
- 前記コーティングが、前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際に、固体状、液状又はペースト状であることを特徴とする、請求項1又は2に記載の方法。
- 前記機械的処理が、前記カーボンナノチューブ、フラーレン及び/又はグラフェンに対して機械的圧力を及ぼすことを含むことを特徴とする、請求項1〜3のいずれか一つに記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンに対して機械的圧力を及ぼすことが、ローラー、スタンプ、機械ブラシを使って、あるいは吹き付け又は吹き込みによって行われることを特徴とする、請求項4に記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際に、前記コーティングが固体状で存在し、そして、ローラー、スタンプ又は機械ブラシを使って前記カーボンナノチューブ、フラーレン及び/又はグラフェンに対して機械的圧力を及ぼすことによって、前記カーボンナノチューブ、フラーレン及び/又はグラフェンを該コーティング中に導入することを特徴とする、請求項3〜5のいずれか一つに記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際に、前記コーティングが液状又はペースト状で存在し、そして、ローラー、スタンプ又は機械ブラシを使って、吹き付け又は吹き込みによって前記カーボンナノチューブ、フラーレン及び/又はグラフェンに対して機械的圧力を及ぼすことにより、前記カーボンナノチューブ、フラーレン及び/又はグラフェンを該コーティング中に導入することを特徴とする、請求項3〜5のいずれか一つに記載の方法。
- 前記熱的処理が、前記コーティングの融点を上回るか又は下回る温度への該コーティングの加熱を含むことを特徴とする、請求項1〜3のいずれか一つに記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際に、前記コーティングが固体状で存在していて、そのあと、該コーティングの融点を上回る温度に加熱されることを特徴とする、請求項8に記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際に、前記コーティングが液状で存在していて、そのあと該コーティングの融点を下回る温度にされることを特徴とする、請求項8に記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを供する際、前記コーティングが固体状で存在していて、そのあと該コーティングの融点を下回る温度に加熱されることを特徴とする、請求項8に記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンを前記コーティング上への施与、及び/又は前記カーボンナノチューブ、フラーレン及び/又はグラフェンの前記コーティング中への導入が、標準大気下又は保護ガス下で遂行されることを特徴とする、請求項1〜11のいずれか一つに記載の方法。
- カーボンナノチューブとして、単層又は多層カーボンナノチューブが使用されることを特徴とする、請求項1〜12のいずれか一つに記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンが前記コーティング上へ供される前に、それらに金属からなるシェルが供されることを特徴とする、請求項1〜13のいずれか一つに記載の方法。
- 前記シェルの付与が、前記カーボンナノチューブ、フラーレン及び/又はグラフェンと、金属との機械的混練を使って、又は化学的手段によって行われることを特徴とする、請求項14に記載の方法。
- 前記カーボンナノチューブ、フラーレン及び/又はグラフェンが、金属テープ上に供される前に、超音波によってスズ含有金属溶融物中に分散され、そして波状に供され、その後、所定の層厚を調節するために機械的ストリッピングを行うことを特徴とする、請求項1〜15のいずれか一つに記載の方法。
- 請求項1〜16に記載の方法に従って製造されたコーティングされた基体。
- 前記基体が、銅又は銅含有合金、アルミニウム又はアルミニウム含有合金、あるいは鉄又は鉄含有合金からなることを特徴とする、コーティングされた基体。
- 前記基体が、更に、該基体とスズ含有コーティングとの間に配置される、少なくとも一つの中間層を含むことを特徴とする、請求項17又は18に記載のコーティングされた基体。
- 請求項17〜19のいずれか一つに記載の、又は請求項1〜16のいずれか一つに記載の方法に従って製造されたコーティングされた基体の、電機機械部材又はリードフレームとしての使用。
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE102008053027.1 | 2008-10-24 | ||
DE102008053027A DE102008053027A1 (de) | 2008-10-24 | 2008-10-24 | Verfahren zum Herstellen einer Kohlenstoff-Nanoröhren,Fullerene und/oder Graphene enthaltenden Beschichtung |
PCT/DE2009/001237 WO2010045905A1 (de) | 2008-10-24 | 2009-09-03 | Verfahren zum herstellen einer kohlenstoff-nanoröhren, fullerene und/oder graphene enthaltenden beschichtung |
Publications (2)
Publication Number | Publication Date |
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JP2012506357A true JP2012506357A (ja) | 2012-03-15 |
JP5542829B2 JP5542829B2 (ja) | 2014-07-09 |
Family
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Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
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JP2011532491A Expired - Fee Related JP5542829B2 (ja) | 2008-10-24 | 2009-09-03 | カーボンナノチューブ、フラーレン及び/又はグラフェン含有コーティングの製造方法 |
Country Status (11)
Country | Link |
---|---|
US (1) | US20110206946A1 (ja) |
EP (1) | EP2340229A1 (ja) |
JP (1) | JP5542829B2 (ja) |
KR (1) | KR101283275B1 (ja) |
CN (1) | CN102105396A (ja) |
BR (1) | BRPI0920915A2 (ja) |
CA (1) | CA2731963C (ja) |
DE (1) | DE102008053027A1 (ja) |
MX (1) | MX2011003398A (ja) |
RU (1) | RU2483021C2 (ja) |
WO (1) | WO2010045905A1 (ja) |
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WO2012017117A1 (es) * | 2010-07-23 | 2012-02-09 | Baolab Microsystems Sl | Antenas vibrantes de mems cmos y aplicaciones de las mismas |
DE102011009469B4 (de) | 2011-01-21 | 2013-04-18 | Innovent E.V. | Verfahren zur Herstellung von polymerfunktionalisierten Kohlenstoffnanoröhren |
DE102011000395A1 (de) * | 2011-01-28 | 2012-08-02 | Hydro Aluminium Rolled Products Gmbh | Thermisch und elektrisch hochleitfähiges Aluminiumband |
US20120273255A1 (en) * | 2011-04-26 | 2012-11-01 | Tyco Electronics Corporation | Electrical Conductors Having Organic Compound Coatings |
CN102324497A (zh) * | 2011-09-21 | 2012-01-18 | 上海大学 | 一种石墨烯负载碳包覆锡锑的锂电池负极材料的制备方法 |
CN102646575A (zh) * | 2012-04-17 | 2012-08-22 | 北京大学 | 一种二氧化硅图形加工的方法 |
US8889997B2 (en) * | 2012-05-01 | 2014-11-18 | Tyco Electronics Corporation | Methods for improving corrosion resistance and applications in electrical connectors |
CN104037393B (zh) * | 2013-03-06 | 2019-03-26 | 佛山市顺德宇红纳米科技有限公司 | 一种锡/石墨烯/碳纤维复合锂电池负极材料制备方法 |
AU2013396770C1 (en) * | 2013-06-24 | 2017-06-01 | Hitachi Energy Ltd | A material comprising reduced graphene oxide, a device comprising the material and a method of producing the material |
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EP2958110B1 (de) * | 2014-06-16 | 2018-09-26 | Siemens Aktiengesellschaft | Messwandlerwicklung und Messwandler |
GB201604341D0 (en) * | 2016-03-14 | 2016-04-27 | Aurubis Belgium Nv Sa | Composition |
CN106048285B (zh) * | 2016-06-20 | 2017-10-13 | 山东建筑大学 | 一种制备碳纳米管‑石墨烯粉末复合增强锡铅合金的方法 |
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CA2731963C (en) | 2013-11-05 |
DE102008053027A1 (de) | 2010-04-29 |
CA2731963A1 (en) | 2010-04-29 |
EP2340229A1 (de) | 2011-07-06 |
BRPI0920915A2 (pt) | 2015-12-29 |
US20110206946A1 (en) | 2011-08-25 |
KR101283275B1 (ko) | 2013-07-11 |
CN102105396A (zh) | 2011-06-22 |
JP5542829B2 (ja) | 2014-07-09 |
RU2483021C2 (ru) | 2013-05-27 |
MX2011003398A (es) | 2012-09-07 |
WO2010045905A1 (de) | 2010-04-29 |
KR20110055653A (ko) | 2011-05-25 |
RU2011120826A (ru) | 2012-11-27 |
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