JP2011518659A - モリブデン、ビスマスおよび鉄を含有する多金属酸化物を含むシェル触媒 - Google Patents

モリブデン、ビスマスおよび鉄を含有する多金属酸化物を含むシェル触媒 Download PDF

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JP2011518659A
JP2011518659A JP2011503423A JP2011503423A JP2011518659A JP 2011518659 A JP2011518659 A JP 2011518659A JP 2011503423 A JP2011503423 A JP 2011503423A JP 2011503423 A JP2011503423 A JP 2011503423A JP 2011518659 A JP2011518659 A JP 2011518659A
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molybdenum
oxide
shell
shell catalyst
catalyst
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チャヤ アレクサンダー
クラウス マーティン
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BASF SE
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BASF SE
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
    • B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/84—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B01J23/85—Chromium, molybdenum or tungsten
    • B01J23/88—Molybdenum
    • B01J23/887—Molybdenum containing in addition other metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/8878—Chromium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/002—Mixed oxides other than spinels, e.g. perovskite
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/30—Catalysts, in general, characterised by their form or physical properties characterised by their physical properties
    • B01J35/396—Distribution of the active metal ingredient
    • B01J35/397—Egg shell like
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0215—Coating
    • B01J37/0219—Coating the coating containing organic compounds
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0215—Coating
    • B01J37/0221—Coating of particles
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07B—GENERAL METHODS OF ORGANIC CHEMISTRY; APPARATUS THEREFOR
    • C07B33/00—Oxidation in general
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07B—GENERAL METHODS OF ORGANIC CHEMISTRY; APPARATUS THEREFOR
    • C07B35/00—Reactions without formation or introduction of functional groups containing hetero atoms, involving a change in the type of bonding between two carbon atoms already directly linked
    • C07B35/04—Dehydrogenation
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C5/00—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms
    • C07C5/32—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms by dehydrogenation with formation of free hydrogen
    • C07C5/327—Formation of non-aromatic carbon-to-carbon double bonds only
    • C07C5/333—Catalytic processes
    • C07C5/3332—Catalytic processes with metal oxides or metal sulfides
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C5/00—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms
    • C07C5/42—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms by dehydrogenation with a hydrogen acceptor
    • C07C5/48—Preparation of hydrocarbons from hydrocarbons containing the same number of carbon atoms by dehydrogenation with a hydrogen acceptor with oxygen as an acceptor
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2523/00—Constitutive chemical elements of heterogeneous catalysts
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/0009—Use of binding agents; Moulding; Pressing; Powdering; Granulating; Addition of materials ameliorating the mechanical properties of the product catalyst
    • B01J37/0018—Addition of a binding agent or of material, later completely removed among others as result of heat treatment, leaching or washing,(e.g. forming of pores; protective layer, desintegrating by heat)
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/0009—Use of binding agents; Moulding; Pressing; Powdering; Granulating; Addition of materials ameliorating the mechanical properties of the product catalyst
    • B01J37/0027—Powdering
    • B01J37/0045—Drying a slurry, e.g. spray drying
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/03—Precipitation; Co-precipitation
    • B01J37/031—Precipitation
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/02—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the alkali- or alkaline earth metals or beryllium
    • C07C2523/04—Alkali metals
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/16—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • C07C2523/18—Arsenic, antimony or bismuth
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/16—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • C07C2523/24—Chromium, molybdenum or tungsten
    • C07C2523/26—Chromium
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/16—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • C07C2523/24—Chromium, molybdenum or tungsten
    • C07C2523/28—Molybdenum
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the iron group metals or copper
    • C07C2523/74—Iron group metals
    • C07C2523/745—Iron
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the iron group metals or copper
    • C07C2523/74—Iron group metals
    • C07C2523/75—Cobalt
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2523/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00
    • C07C2523/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the iron group metals or copper
    • C07C2523/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups C07C2523/02 - C07C2523/36
    • C07C2523/84—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group C07C2521/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups C07C2523/02 - C07C2523/36 with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • C07C2523/85—Chromium, molybdenum or tungsten
    • C07C2523/88—Molybdenum
    • C07C2523/887—Molybdenum containing in addition other metals, oxides or hydroxides provided for in groups C07C2523/02 - C07C2523/36

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Catalysts (AREA)
  • Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
JP2011503423A 2008-04-09 2009-04-07 モリブデン、ビスマスおよび鉄を含有する多金属酸化物を含むシェル触媒 Pending JP2011518659A (ja)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
EP08154235 2008-04-09
EP08154235.9 2008-04-09
PCT/EP2009/054167 WO2009124945A2 (de) 2008-04-09 2009-04-07 Schalenkatalysatoren enthaltend ein molybdän, bismut und eisen enthaltendes multimetalloxid

Publications (2)

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JP2011518659A true JP2011518659A (ja) 2011-06-30
JP2011518659A5 JP2011518659A5 (https=) 2012-06-07

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JP2011503423A Pending JP2011518659A (ja) 2008-04-09 2009-04-07 モリブデン、ビスマスおよび鉄を含有する多金属酸化物を含むシェル触媒

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US (1) US20110034330A1 (https=)
EP (1) EP2265371A2 (https=)
JP (1) JP2011518659A (https=)
CN (1) CN101990460A (https=)
CA (1) CA2719157A1 (https=)
TW (1) TW200950880A (https=)
WO (1) WO2009124945A2 (https=)

Cited By (6)

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WO2013161703A1 (ja) 2012-04-23 2013-10-31 日本化薬株式会社 成型触媒の製造方法および該成型触媒を用いるジエンまたは不飽和アルデヒドおよび／または不飽和カルボン酸の製造方法
WO2013161702A1 (ja) 2012-04-23 2013-10-31 日本化薬株式会社 ブタジエンの製造用触媒、その触媒の製造方法およびその触媒を用いたブタジエンの製造方法
JP2014198334A (ja) * 2013-03-13 2014-10-23 三菱化学株式会社 複合金属酸化物触媒及び共役ジエンの製造方法
WO2018043007A1 (ja) * 2016-08-31 2018-03-08 旭化成株式会社 触媒の製造方法、及びアクリロニトリルの製造方法
JPWO2018043007A1 (ja) * 2016-08-31 2018-12-20 旭化成株式会社 触媒の製造方法、及びアクリロニトリルの製造方法
JP2019005701A (ja) * 2017-06-23 2019-01-17 旭化成株式会社 金属酸化物触媒及びその製造方法ならびにそれを用いたアクリロニトリルの製造方法

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CN103796752A (zh) * 2011-07-12 2014-05-14 巴斯夫欧洲公司 含Mo、Bi和Fe的多金属氧化物物质
JP6138161B2 (ja) 2012-01-30 2017-05-31 ビーエーエスエフ ソシエタス・ヨーロピアＢａｓｆ Ｓｅ ｎ−ブタンからのブタジエンおよび／またはブテン類の製造方法
PL2826764T3 (pl) * 2012-03-13 2016-12-30 Sposób wytwarzania wsprzężonej diolefiny
EP2897927B1 (de) 2012-09-20 2016-06-22 Basf Se Verfahren zur herstellung von butadien mit entfernung von sauerstoff aus c4-kohlenwasserstoffströmen
KR20150091387A (ko) * 2012-12-06 2015-08-10 바스프 에스이 n-부텐의 부타디엔으로의 산화성 탈수소화 방법
US20140163290A1 (en) * 2012-12-06 2014-06-12 Basf Se Process for the Oxidative Dehydrogenation of N-Butenes to Butadiene
EA201591089A1 (ru) 2012-12-06 2016-01-29 Басф Се Катализатор и способ окислительного дегидрирования н-бутенов в бутадиен
EP2928602A1 (de) * 2012-12-06 2015-10-14 Basf Se Schalenkatalysator zur oxidativen dehydrierung von n-butenen zu butadien
US9399606B2 (en) 2012-12-06 2016-07-26 Basf Se Catalyst and process for the oxidative dehydrogenation of N-butenes to butadiene
EA201591040A1 (ru) 2012-12-06 2015-11-30 Басф Се Способ окислительного дегидрирования н-бутенов в бутадиен
US20140163292A1 (en) * 2012-12-06 2014-06-12 Basf Se Process for the Oxidative Dehydrogenation of N-Butenes to Butadiene
CN104837795B (zh) * 2012-12-06 2017-08-29 巴斯夫欧洲公司 用于将正丁烯氧化脱氢成丁二烯的方法
US10144681B2 (en) 2013-01-15 2018-12-04 Basf Se Process for the oxidative dehydrogenation of N-butenes to butadiene
EP3019458B1 (de) * 2013-07-10 2017-04-05 Basf Se Verfahren zur oxidativen dehydrierung von n-butenen zu butadien
DE102013226370A1 (de) * 2013-12-18 2015-06-18 Evonik Industries Ag Herstellung von Butadien durch oxidative Dehydrierung von n-Buten nach vorhergehender Isomerisierung
DE102014203725A1 (de) 2014-02-28 2015-09-03 Basf Se Oxidationskatalysator mit sattelförmigem Trägerformkörper
WO2016177764A1 (de) 2015-05-06 2016-11-10 Basf Se Verfahren zur herstellung chrom enthaltender katalysatoren für die oxidehydrierung von n-butenen zu butadien unter vermeidung von cr(vi)-intermediaten
RU2674762C1 (ru) * 2015-08-29 2018-12-13 Юоп Ллк Ступенчатое давление в реакторах получения бутадиена для улучшения рекуперации энергии
US10232357B2 (en) 2015-12-15 2019-03-19 Uop Llc Crystalline ammonia transition metal molybdate
US10053637B2 (en) 2015-12-15 2018-08-21 Uop Llc Transition metal tungsten oxy-hydroxide
US10052616B2 (en) 2015-12-15 2018-08-21 Uop Llc Crystalline ammonia transition metal molybdotungstate
US10322404B2 (en) 2015-12-15 2019-06-18 Uop Llc Crystalline transition metal oxy-hydroxide molybdate
US10005812B2 (en) * 2015-12-15 2018-06-26 Uop Llc Transition metal molybdotungsten oxy-hydroxide
US10052614B2 (en) 2015-12-15 2018-08-21 Uop Llc Mixed metal oxides
US10399065B2 (en) 2015-12-15 2019-09-03 Uop Llc Crystalline transition metal tungstate
US10233398B2 (en) 2015-12-15 2019-03-19 Uop Llc Crystalline transition metal oxy-hydroxide molybdotungstate
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US10046315B2 (en) 2015-12-15 2018-08-14 Uop Llc Crystalline transition metal molybdotungstate
FI3408023T3 (fi) * 2016-01-29 2024-04-26 Totalenergies Onetech Homogeenisesti dispergoituneita monimetallisia oksihydroksidikatalyyttejä
US10773245B2 (en) 2017-08-25 2020-09-15 Uop Llc Crystalline transition metal molybdotungstate
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US11117811B2 (en) 2017-12-20 2021-09-14 Uop Llc Highly active quaternary metallic materials using short-chain alkyl quaternary ammonium compounds
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US11426711B2 (en) 2019-05-22 2022-08-30 Uop Llc Method of making highly active metal oxide and metal sulfide materials
JP7371986B2 (ja) * 2020-07-29 2023-10-31 エルジー・ケム・リミテッド プロピレンのアンモ酸化用触媒、その製造方法、これを用いたプロピレンのアンモ酸化方法
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JPH1170333A (ja) * 1997-06-26 1999-03-16 Consortium Elektrochem Ind Gmbh Ｃ−原子数４の炭化水素を気相酸化して無水マレイン酸にするためのシェル型触媒、その製法及びｃ−原子数４の炭化水素の気相酸化法
WO2005063658A1 (de) * 2003-12-30 2005-07-14 Basf Aktiengesellschaft Verfahren zur herstellung von butadien
JP2006015330A (ja) * 2004-06-02 2006-01-19 Nippon Shokubai Co Ltd アクリル酸製造用触媒とこれを用いるアクリル酸製造方法
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