MX9708142A - Copolimeros de oligourea polidiorganosiloxano, segmentados, y proceso para su fabricacion. - Google Patents
Copolimeros de oligourea polidiorganosiloxano, segmentados, y proceso para su fabricacion.Info
- Publication number
- MX9708142A MX9708142A MX9708142A MX9708142A MX9708142A MX 9708142 A MX9708142 A MX 9708142A MX 9708142 A MX9708142 A MX 9708142A MX 9708142 A MX9708142 A MX 9708142A MX 9708142 A MX9708142 A MX 9708142A
- Authority
- MX
- Mexico
- Prior art keywords
- copolymers
- segmented copolymers
- making same
- oligourea segmented
- polydiorganosiloxane oligourea
- Prior art date
Links
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/2805—Compounds having only one group containing active hydrogen
- C08G18/288—Compounds containing at least one heteroatom other than oxygen or nitrogen
- C08G18/289—Compounds containing at least one heteroatom other than oxygen or nitrogen containing silicon
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/40—High-molecular-weight compounds
- C08G18/61—Polysiloxanes
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/71—Monoisocyanates or monoisothiocyanates
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/71—Monoisocyanates or monoisothiocyanates
- C08G18/718—Monoisocyanates or monoisothiocyanates containing silicon
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/81—Unsaturated isocyanates or isothiocyanates
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/81—Unsaturated isocyanates or isothiocyanates
- C08G18/8108—Unsaturated isocyanates or isothiocyanates having only one isocyanate or isothiocyanate group
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/83—Chemically modified polymers
- C08G18/833—Chemically modified polymers by nitrogen containing compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G77/00—Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
- C08G77/42—Block-or graft-polymers containing polysiloxane sequences
- C08G77/458—Block-or graft-polymers containing polysiloxane sequences containing polyurethane sequences
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G2190/00—Compositions for sealing or packing joints
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Polyurethanes Or Polyureas (AREA)
- Silicon Polymers (AREA)
Abstract
La presente invencion proporciona copolímeros de oligoureas polidiorganosiloxanos segmentados. Los copolímeros contienen unidades de polidiorganosiloxano blandas, segmentos duros que son residuos de diisocianato, las unidades de polidiorganosiloxano y los residuos de diisocianato están conectados por enlace urea, y grupos terminales que no son reactivos, reactivos bajo radicales libres o condiciones de curado humedas, o aminas. La invencion también proporciona los métodos para preparar los copolímeros.
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US42837695A | 1995-04-25 | 1995-04-25 | |
PCT/US1996/005870 WO1996034030A1 (en) | 1995-04-25 | 1996-04-25 | Polydiorganosiloxane oligourea segmented copolymers and a process for making same |
Publications (1)
Publication Number | Publication Date |
---|---|
MX9708142A true MX9708142A (es) | 1997-12-31 |
Family
ID=23698634
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
MX9708142A MX9708142A (es) | 1995-04-25 | 1996-04-25 | Copolimeros de oligourea polidiorganosiloxano, segmentados, y proceso para su fabricacion. |
Country Status (11)
Country | Link |
---|---|
EP (1) | EP0822952B1 (es) |
JP (2) | JPH11504373A (es) |
KR (1) | KR100427675B1 (es) |
CN (1) | CN1186505A (es) |
AU (1) | AU5668396A (es) |
BR (1) | BR9608034A (es) |
CA (1) | CA2218363A1 (es) |
DE (1) | DE69629189T2 (es) |
ES (1) | ES2199288T3 (es) |
MX (1) | MX9708142A (es) |
WO (1) | WO1996034030A1 (es) |
Families Citing this family (65)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
WO1998012075A1 (en) | 1996-09-18 | 1998-03-26 | Minnessota Mining And Manufacturing Company | Adhesively-bonded inflatable restraint and method of making |
US6846893B1 (en) * | 1996-10-23 | 2005-01-25 | Minnesota Mining And Manufacturing Company | Polymer mixtures containing polydiorganosiloxane urea-containing components |
US6083856A (en) * | 1997-12-01 | 2000-07-04 | 3M Innovative Properties Company | Acrylate copolymeric fibers |
US6007914A (en) * | 1997-12-01 | 1999-12-28 | 3M Innovative Properties Company | Fibers of polydiorganosiloxane polyurea copolymers |
US6107222A (en) * | 1997-12-01 | 2000-08-22 | 3M Innovative Properties Company | Repositionable sheets with a nonwoven web of pressure-sensitive adhesive fibers |
FR2809726A1 (fr) | 2000-05-31 | 2001-12-07 | Corning Sa | Monomeres monofonctionnels, compositions polymerisables les renfermant, resines et articles ophtalmiques obtenus a partir de ceux-ci |
FR2809736A1 (fr) * | 2000-05-31 | 2001-12-07 | Corning Sa | Preparation d'une composition stable de monomeres copolymerisables radicalairement, renfermant au moins un monomere a fonction(s) uree |
DE10113980A1 (de) * | 2001-03-22 | 2002-10-02 | Consortium Elektrochem Ind | Silanterminiertes Polydiorganosiloxan-Urethan-Copolymer |
DE10137855A1 (de) * | 2001-08-02 | 2003-02-27 | Consortium Elektrochem Ind | Organopolysiloxan/Polyharnstoff/ Polyurethan-Blockcopolymere |
DE10141235A1 (de) | 2001-08-23 | 2003-03-27 | Consortium Elektrochem Ind | Feuchtigkeitsvernetzende elastische Zusammensetzung |
US7012110B2 (en) | 2001-12-18 | 2006-03-14 | 3M Innovative Properties Company | Silicone pressure sensitive adhesives prepared using processing aids, articles, and methods |
US6730397B2 (en) | 2001-12-18 | 2004-05-04 | 3M Innovative Properties Company | Silicone pressure sensitive adhesives, articles and methods |
US7090922B2 (en) | 2001-12-18 | 2006-08-15 | 3M Innovative Properties Company | Silicone priming compositions, articles, and methods |
DE10201703A1 (de) | 2002-01-17 | 2003-08-07 | Consortium Elektrochem Ind | Alkoxysilanterminierte Polymere enthaltende vernetzbare Polymerabmischungen |
DE10241148A1 (de) * | 2002-09-05 | 2004-03-18 | Wacker-Chemie Gmbh | Siliconölpasten |
US7189781B2 (en) * | 2003-03-13 | 2007-03-13 | H.B. Fuller Licensing & Finance Inc. | Moisture curable, radiation curable sealant composition |
DE10313936A1 (de) * | 2003-03-27 | 2004-10-14 | Consortium für elektrochemische Industrie GmbH | Organopolysiloxan/Polyharnstoff/Polyurethan-Blockcopolymere |
EP1496079B1 (de) * | 2003-07-10 | 2005-07-06 | Wacker-Chemie GmbH | Vernetzbare Siloxan-Harnstoff-Copolymere |
DE102004035710A1 (de) | 2004-07-23 | 2006-03-16 | Wacker Chemie Ag | Vernetzbares Siloxan-Harnstoff-Copolymere |
DE102004041379A1 (de) * | 2004-08-26 | 2006-03-02 | Wacker-Chemie Gmbh | Vernetzbare Siloxan-Harnstoff-Copolymere |
DE102005026085A1 (de) * | 2005-06-07 | 2006-12-14 | Construction Research & Technology Gmbh | Silan-modifizierte Harnstoff-Derivate, Verfahren zu ihrer Herstellung und deren Verwendung als Rheologiehilfsmittel |
DE102005029282A1 (de) * | 2005-06-23 | 2006-12-28 | Henkel Kgaa | Silanvernetzende Kleb- und Dichtstoffmassen, Verfahren zu ihrer Herstellung und ihre Verwendung |
ATE540065T1 (de) * | 2006-04-18 | 2012-01-15 | Henkel Ag & Co Kgaa | Organosilikon-polyharnstoff basierte polymere, daraus hergestellte elastomere und deren verwendung |
DE102006022095A1 (de) | 2006-05-11 | 2007-11-15 | Wacker Chemie Ag | Alkoxysilanterminierte Polymere enthaltende transparente Polymerabmischungen |
DE102006054155A1 (de) | 2006-11-16 | 2008-05-21 | Wacker Chemie Ag | Schäumbare Mischungen enthaltend alkoxysilanterminierte Prepolymere |
US8334037B2 (en) | 2007-05-11 | 2012-12-18 | 3M Innovative Properties Company | Multi-layer assembly, multi-layer stretch releasing pressure-sensitive adhesive assembly, and methods of making and using the same |
US7705101B2 (en) | 2007-06-22 | 2010-04-27 | 3M Innovative Properties Company | Branched polydiorganosiloxane polyamide copolymers |
US20080318065A1 (en) | 2007-06-22 | 2008-12-25 | Sherman Audrey A | Mixtures of polydiorganosiloxane polyamide-containing components and organic polymers |
KR20160008653A (ko) | 2008-01-11 | 2016-01-22 | 쓰리엠 이노베이티브 프로퍼티즈 컴파니 | 광학적으로 투명한 연신 해제 감압 접착제 |
DE102008002075A1 (de) * | 2008-05-29 | 2009-12-03 | Wacker Chemie Ag | Mischungen von Organopolysiloxan-Copolymeren |
DE102008043218A1 (de) | 2008-09-24 | 2010-04-01 | Evonik Goldschmidt Gmbh | Polymere Werkstoffe sowie daraus bestehende Kleber- und Beschichtungsmittel auf Basis multialkoxysilylfunktioneller Präpolymerer |
BRPI0919628A2 (pt) * | 2008-10-29 | 2015-12-01 | 3M Innovative Proferties Company | materiais de liberação de silicone curado com feixe de elétrons |
DE102009022628A1 (de) | 2008-12-05 | 2010-06-10 | Evonik Goldschmidt Gmbh | Verfahren zur Modifizierung von Oberflächen |
TWI396702B (zh) | 2009-05-08 | 2013-05-21 | Yun Liang Ouyang | 生醫材料之預聚物 |
DE102009022631A1 (de) | 2009-05-25 | 2010-12-16 | Evonik Goldschmidt Gmbh | Härtbare Silylgruppen enthaltende Zusammensetzungen und deren Verwendung |
DE102009022630A1 (de) | 2009-05-25 | 2010-12-02 | Evonik Goldschmidt Gmbh | Emulsionen auf Basis Silylgruppen tragender Hydroxylverbindungen |
DE102009034607A1 (de) | 2009-07-24 | 2011-01-27 | Evonik Goldschmidt Gmbh | Neuartige Siliconpolyethercopolymere und Verfahren zu deren Herstellung |
DE102009046850A1 (de) * | 2009-11-18 | 2011-05-19 | Wacker Chemie Ag | Siloxan-Copolymere enthaltende Zusammensetzungen |
CN102712750B (zh) | 2009-12-30 | 2014-06-25 | 3M创新有限公司 | 具有乙二酰胺基团的含全氟聚醚化合物 |
CN102695745B (zh) | 2009-12-30 | 2013-11-13 | 3M创新有限公司 | 具有全氟聚醚链段和聚二有机硅氧烷链段的共聚物 |
JP5777635B2 (ja) | 2009-12-30 | 2015-09-09 | スリーエム イノベイティブ プロパティズ カンパニー | ペルフルオロポリエーテルセグメント及び複数のアミノオキサリルアミノ基を有するコポリマー |
KR101820979B1 (ko) | 2009-12-30 | 2018-01-22 | 쓰리엠 이노베이티브 프로퍼티즈 컴파니 | 폴리다이오르가노실록산 폴리옥사미드 공중합체의 제조 방법 |
US10456499B2 (en) | 2012-05-18 | 2019-10-29 | 3M Innovative Properties Company | Adhesive articles for medical applications |
AU2013286932B2 (en) | 2012-07-03 | 2016-04-28 | 3M Innovative Properties Company | Siloxane-based pipe coatings |
CN104411791B (zh) | 2012-07-03 | 2017-06-09 | 3M创新有限公司 | 可热活化的硅氧烷基粘合剂 |
DE102013213655A1 (de) | 2013-07-12 | 2015-01-15 | Evonik Industries Ag | Härtbare Silylgruppen enthaltende Zusammensetzungen mit verbesserter Lagerstabilität |
WO2015167870A1 (en) | 2014-04-29 | 2015-11-05 | 3M Innovative Properties Company | Copolymers of poly(ethylene-co-acrylic acid) and polydiorganosiloxanes |
WO2016106040A1 (en) | 2014-12-23 | 2016-06-30 | 3M Innovative Properties Company | Dual-sided multi-layer adhesive |
US10723894B2 (en) | 2014-12-23 | 2020-07-28 | 3M Innovative Properties Company | Tie layers prepared from particle-containing waterborne suspensions |
BR112017021396A2 (pt) | 2015-04-06 | 2018-07-03 | 3M Innovative Properties Company | composição em gel, filme e método para aplicação de uma composição em gel |
EP3487949A1 (en) | 2016-07-22 | 2019-05-29 | 3M Innovative Properties Company | Siloxane-based adhesive layers as ceramic precursors |
KR102203508B1 (ko) * | 2016-10-07 | 2021-01-15 | 와커 헤미 아게 | 실록산-유기-공중합체를 함유하는 중합체 조성물 |
US20190381208A1 (en) | 2016-10-13 | 2019-12-19 | 3M Innovative Properties Company | Removable Film Forming Gel Compositions Featuring Adhesion Promoters |
WO2019082023A1 (en) | 2017-10-26 | 2019-05-02 | 3M Innovative Properties Company | COMPOSITION CONTAINING SILICONE ADHESIVE AND CELLULOSE NANOCRYSTALS, METHODS AND ARTICLES |
GB201811834D0 (en) * | 2018-07-19 | 2018-09-05 | Medherant Ltd | Patch |
WO2020243506A1 (en) | 2019-05-31 | 2020-12-03 | Kindeva Drug Delivery | Removable film-forming gel compositions featuring adhesion promoters |
US20220257424A1 (en) | 2019-07-25 | 2022-08-18 | 3M Innovative Properties Company | Fluid-managing medical adhesive articles with microstructured surfaces |
WO2021099997A1 (en) | 2019-11-20 | 2021-05-27 | 3M Innovative Properties Company | Medical tapes with high optical clarity when over-taped |
JP2023520808A (ja) | 2020-04-13 | 2023-05-19 | スリーエム イノベイティブ プロパティズ カンパニー | 有効弾性係数が小さい医療用接着剤物品 |
WO2022084888A1 (en) | 2020-10-21 | 2022-04-28 | 3M Innovative Properties Company | Packaged medical articles with reduced packaging |
JP2023552590A (ja) | 2020-12-11 | 2023-12-18 | スリーエム イノベイティブ プロパティズ カンパニー | 医療用途のための有孔テープ |
JP2024501930A (ja) | 2020-12-21 | 2024-01-17 | スリーエム イノベイティブ プロパティズ カンパニー | オンデマンド接着による両面接着テープ |
CN112680167A (zh) * | 2020-12-25 | 2021-04-20 | 成都硅宝科技股份有限公司 | 一种耐候性高强度聚氨酯密封胶及其制备方法 |
CN117750951A (zh) | 2021-07-29 | 2024-03-22 | 3M创新有限公司 | 包含水杨酸的成膜组合物和使用方法 |
WO2024009810A1 (ja) * | 2022-07-06 | 2024-01-11 | 信越化学工業株式会社 | 二官能性オルガノポリシロキサン、二重硬化性オルガノポリシロキサン組成物及び硬化物並びに電子機器 |
Family Cites Families (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4563539A (en) * | 1984-12-18 | 1986-01-07 | Dow Corning Corporation | Acrylofunctional silicones |
ES2110391T3 (es) * | 1986-06-20 | 1998-02-16 | Minnesota Mining & Mfg | Copolimero de bloques, metodo para preparar el mismo, precursores de diamina del mismo metodo, metodo para preparar tales diaminas y productos finales que comprenden el copolimero de bloques. |
EP0455585B1 (en) * | 1990-04-26 | 1994-03-23 | Ciba-Geigy Ag | Unsaturated urea polysiloxanes |
JP3708983B2 (ja) * | 1994-06-24 | 2005-10-19 | 大日本印刷株式会社 | 含液晶/高分子マイクロカプセル及び液晶電気光学素子 |
-
1996
- 1996-04-25 KR KR1019970707545A patent/KR100427675B1/ko not_active IP Right Cessation
- 1996-04-25 CN CN96194351A patent/CN1186505A/zh active Pending
- 1996-04-25 EP EP96913846A patent/EP0822952B1/en not_active Expired - Lifetime
- 1996-04-25 ES ES96913846T patent/ES2199288T3/es not_active Expired - Lifetime
- 1996-04-25 JP JP8532764A patent/JPH11504373A/ja not_active Withdrawn
- 1996-04-25 BR BR9608034A patent/BR9608034A/pt not_active IP Right Cessation
- 1996-04-25 AU AU56683/96A patent/AU5668396A/en not_active Abandoned
- 1996-04-25 CA CA002218363A patent/CA2218363A1/en not_active Abandoned
- 1996-04-25 DE DE69629189T patent/DE69629189T2/de not_active Expired - Lifetime
- 1996-04-25 WO PCT/US1996/005870 patent/WO1996034030A1/en active IP Right Grant
- 1996-04-25 MX MX9708142A patent/MX9708142A/es unknown
-
2006
- 2006-11-16 JP JP2006310569A patent/JP5122792B2/ja not_active Expired - Lifetime
Also Published As
Publication number | Publication date |
---|---|
EP0822952B1 (en) | 2003-07-23 |
AU5668396A (en) | 1996-11-18 |
CN1186505A (zh) | 1998-07-01 |
JPH11504373A (ja) | 1999-04-20 |
KR100427675B1 (ko) | 2004-07-27 |
JP5122792B2 (ja) | 2013-01-16 |
BR9608034A (pt) | 1999-01-12 |
WO1996034030A1 (en) | 1996-10-31 |
KR19990008021A (ko) | 1999-01-25 |
DE69629189D1 (de) | 2003-08-28 |
JP2007051302A (ja) | 2007-03-01 |
EP0822952A1 (en) | 1998-02-11 |
CA2218363A1 (en) | 1996-10-31 |
DE69629189T2 (de) | 2004-06-03 |
ES2199288T3 (es) | 2004-02-16 |
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