JP6162179B2 - 陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜 - Google Patents

陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜 Download PDF

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JP6162179B2
JP6162179B2 JP2015134000A JP2015134000A JP6162179B2 JP 6162179 B2 JP6162179 B2 JP 6162179B2 JP 2015134000 A JP2015134000 A JP 2015134000A JP 2015134000 A JP2015134000 A JP 2015134000A JP 6162179 B2 JP6162179 B2 JP 6162179B2
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group
cation exchange
divalent
formula
carbon
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JP2017014423A (ja
JP2017014423A5 (enExample
Inventor
宮武　健治
健治 宮武
内田　誠
誠 内田
純平 三宅
純平 三宅
崇史 望月
崇史 望月
小野　英明
英明 小野
愛生 島田
愛生 島田
尚樹 横田
尚樹 横田
菜摘 吉村
菜摘 吉村
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Takahata Precision Japan Co Ltd
University of Yamanashi NUC
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Takahata Precision Japan Co Ltd
University of Yamanashi NUC
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Priority to JP2015134000A priority Critical patent/JP6162179B2/ja
Priority to PCT/JP2016/069364 priority patent/WO2017006831A1/ja
Priority to US15/738,270 priority patent/US10471420B2/en
Publication of JP2017014423A publication Critical patent/JP2017014423A/ja
Publication of JP2017014423A5 publication Critical patent/JP2017014423A5/ja
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J39/00—Cation exchange; Use of material as cation exchangers; Treatment of material for improving the cation exchange properties
    • B01J39/08—Use of material as cation exchangers; Treatment of material for improving the cation exchange properties
    • B01J39/16—Organic material
    • B01J39/18—Macromolecular compounds
    • B01J39/19—Macromolecular compounds obtained otherwise than by reactions only involving unsaturated carbon-to-carbon bonds
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J47/00—Ion-exchange processes in general; Apparatus therefor
    • B01J47/12—Ion-exchange processes in general; Apparatus therefor characterised by the use of ion-exchange material in the form of ribbons, filaments, fibres or sheets, e.g. membranes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G61/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
    • C08G61/02—Macromolecular compounds containing only carbon atoms in the main chain of the macromolecule, e.g. polyxylylenes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G61/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
    • C08G61/02—Macromolecular compounds containing only carbon atoms in the main chain of the macromolecule, e.g. polyxylylenes
    • C08G61/10—Macromolecular compounds containing only carbon atoms in the main chain of the macromolecule, e.g. polyxylylenes only aromatic carbon atoms, e.g. polyphenylenes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C08J5/2256—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • C08J5/2262—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation containing fluorine
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1023—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon, e.g. polyarylenes, polystyrenes or polybutadiene-styrenes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1039—Polymeric electrolyte materials halogenated, e.g. sulfonated polyvinylidene fluorides
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
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    • C08G2261/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
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    • C08G2261/122—Copolymers statistical
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    • C08G2261/10—Definition of the polymer structure
    • C08G2261/14—Side-groups
    • C08G2261/145—Side-chains containing sulfur
    • C08G2261/1452—Side-chains containing sulfur containing sulfonyl or sulfonate-groups
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    • C08G2261/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
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    • C08G2261/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
    • C08G2261/30—Monomer units or repeat units incorporating structural elements in the main chain
    • C08G2261/31—Monomer units or repeat units incorporating structural elements in the main chain incorporating aromatic structural elements in the main chain
    • C08G2261/312—Non-condensed aromatic systems, e.g. benzene
    • C—CHEMISTRY; METALLURGY
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    • C08G2261/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
    • C08G2261/30—Monomer units or repeat units incorporating structural elements in the main chain
    • C08G2261/34—Monomer units or repeat units incorporating structural elements in the main chain incorporating partially-aromatic structural elements in the main chain
    • C08G2261/342—Monomer units or repeat units incorporating structural elements in the main chain incorporating partially-aromatic structural elements in the main chain containing only carbon atoms
    • C08G2261/3424—Monomer units or repeat units incorporating structural elements in the main chain incorporating partially-aromatic structural elements in the main chain containing only carbon atoms non-conjugated, e.g. paracyclophanes or xylenes
    • C—CHEMISTRY; METALLURGY
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    • C08G2261/00—Macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain of the macromolecule
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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
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    • C08J2365/00—Characterised by the use of macromolecular compounds obtained by reactions forming a carbon-to-carbon link in the main chain; Derivatives of such polymers
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    • H01M8/00—Fuel cells; Manufacture thereof
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    • H01M8/00—Fuel cells; Manufacture thereof
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    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1037—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having silicon, e.g. sulfonated crosslinked polydimethylsiloxanes
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  • Inorganic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Fuel Cell (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Polyoxymethylene Polymers And Polymers With Carbon-To-Carbon Bonds (AREA)
  • Conductive Materials (AREA)
JP2015134000A 2015-07-03 2015-07-03 陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜 Active JP6162179B2 (ja)

Priority Applications (3)

Application Number Priority Date Filing Date Title
JP2015134000A JP6162179B2 (ja) 2015-07-03 2015-07-03 陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜
PCT/JP2016/069364 WO2017006831A1 (ja) 2015-07-03 2016-06-29 陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜
US15/738,270 US10471420B2 (en) 2015-07-03 2016-06-29 Cation exchange resin, and cation exchange membrane and fuel cell electrolyte membrane using same

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JP2015134000A JP6162179B2 (ja) 2015-07-03 2015-07-03 陽イオン交換樹脂、ならびにそれを用いた陽イオン交換膜および燃料電池用電解質膜

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JP2017014423A5 JP2017014423A5 (enExample) 2017-02-23
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Families Citing this family (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6888778B2 (ja) * 2017-02-22 2021-06-16 国立大学法人山梨大学 陰イオン交換樹脂、電解質膜、電極触媒層形成用バインダー、電池電極触媒層および燃料電池
KR102642656B1 (ko) * 2018-05-18 2024-02-29 에이지씨 가부시키가이샤 함불소 폴리머의 제조 방법 및 함불소 이온 교환 폴리머의 제조 방법
JP7513970B2 (ja) * 2020-07-16 2024-07-10 国立大学法人山梨大学 陰イオン交換樹脂の製造方法および電解質膜の製造方法
JP7513971B2 (ja) * 2020-07-16 2024-07-10 国立大学法人山梨大学 陰イオン交換樹脂の製造方法および電解質膜の製造方法
JP7767190B2 (ja) * 2022-03-15 2025-11-11 株式会社小松製作所 オイルフィルタ装置
US20260001983A1 (en) 2022-07-15 2026-01-01 University Of Yamanashi Cation exchange resin, cation exchange membrane, electrolyte membrane, binder for forming electrode catalyst layer, and battery electrode catalyst layer

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US4029783A (en) 1973-08-03 1977-06-14 Boehringer Mannheim G.M.B.H. N-substituted 1-amino-3-phenoxy-propan-2-ol compounds and therapeutic compositions containing them
US3969285A (en) 1973-12-17 1976-07-13 E. I. Du Pont De Nemours And Company Heat-treated fluorocarbon sulfonylamine cation permselectivity
US4030988A (en) 1973-12-17 1977-06-21 E. I. Du Pont De Nemours And Company Process for producing halogen and metal hydroxides with cation exchange membranes of improved permselectivity
US4026785A (en) 1975-12-22 1977-05-31 Olin Corporation Adjustable electrode
JP2006045512A (ja) * 2004-06-29 2006-02-16 Sumitomo Chemical Co Ltd 高分子電解質膜及びそれを用いた燃料電池
EP1944820A4 (en) * 2005-09-16 2010-02-03 Sumitomo Chemical Co POLYMER ELECTROLYTE, POLYMER ELECTROLYTE MEMBRANE THEREOF, MEMBRANE ELECTRODE ASSEMBLY AND FUEL CELL
US8492460B2 (en) * 2006-07-28 2013-07-23 GM Global Technology Operations LLC Fluorinated polymer blocks for PEM applications
US7973088B2 (en) * 2006-08-25 2011-07-05 Sumitomo Chemical Company, Limited Polymer electrolyte membrane, method for producing the same, and proton conductivity evaluation method for polymer electrolyte membrane
JP2013505825A (ja) * 2009-09-24 2013-02-21 ジョージア・テック・リサーチ・コーポレイション 陰イオン交換高分子電解質
FR2963621B1 (fr) * 2010-08-04 2012-08-17 Soc Tech Michelin Monomere perfluoroalcane aromatique
JP5827077B2 (ja) 2011-08-29 2015-12-02 ダイハツ工業株式会社 陰イオン交換樹脂、燃料電池用電解質層、電極触媒層形成用バインダー、電池電極触媒層および燃料電池
US9102789B2 (en) * 2011-10-28 2015-08-11 Daimler Ag Sulfonated poly(phenylene) copolymer electrolyte for fuel cells
JP2013209457A (ja) * 2012-03-30 2013-10-10 Sumitomo Chemical Co Ltd ポリアリーレン及びその製造方法

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JP2017014423A (ja) 2017-01-19
US20180178210A1 (en) 2018-06-28
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