JP4843024B2 - 触媒支持体 - Google Patents
触媒支持体 Download PDFInfo
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- JP4843024B2 JP4843024B2 JP2008508162A JP2008508162A JP4843024B2 JP 4843024 B2 JP4843024 B2 JP 4843024B2 JP 2008508162 A JP2008508162 A JP 2008508162A JP 2008508162 A JP2008508162 A JP 2008508162A JP 4843024 B2 JP4843024 B2 JP 4843024B2
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- Prior art keywords
- catalyst body
- catalyst
- passage
- body according
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- Prior art date
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- 239000003054 catalyst Substances 0.000 title claims description 130
- 229930195733 hydrocarbon Natural products 0.000 claims description 6
- 150000002430 hydrocarbons Chemical class 0.000 claims description 6
- 238000000034 method Methods 0.000 claims description 5
- 230000002093 peripheral effect Effects 0.000 claims description 5
- 238000000629 steam reforming Methods 0.000 claims description 5
- 229910044991 metal oxide Inorganic materials 0.000 claims description 3
- 150000004706 metal oxides Chemical class 0.000 claims description 3
- 229910018072 Al 2 O 3 Inorganic materials 0.000 claims description 2
- 239000004215 Carbon black (E152) Substances 0.000 claims description 2
- 229910004298 SiO 2 Inorganic materials 0.000 claims description 2
- 238000006243 chemical reaction Methods 0.000 description 6
- 239000000945 filler Substances 0.000 description 6
- 239000007789 gas Substances 0.000 description 5
- 238000004519 manufacturing process Methods 0.000 description 5
- 238000006555 catalytic reaction Methods 0.000 description 4
- 239000000463 material Substances 0.000 description 3
- 230000003197 catalytic effect Effects 0.000 description 2
- 239000000919 ceramic Substances 0.000 description 2
- 239000008187 granular material Substances 0.000 description 2
- 239000005022 packaging material Substances 0.000 description 2
- 239000000376 reactant Substances 0.000 description 2
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 1
- 239000012190 activator Substances 0.000 description 1
- 239000011149 active material Substances 0.000 description 1
- 230000037237 body shape Effects 0.000 description 1
- 229910010293 ceramic material Inorganic materials 0.000 description 1
- 150000001875 compounds Chemical class 0.000 description 1
- 230000006835 compression Effects 0.000 description 1
- 238000007906 compression Methods 0.000 description 1
- 238000005336 cracking Methods 0.000 description 1
- 230000006378 damage Effects 0.000 description 1
- 230000018044 dehydration Effects 0.000 description 1
- 238000006297 dehydration reaction Methods 0.000 description 1
- 230000001419 dependent effect Effects 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 238000001125 extrusion Methods 0.000 description 1
- 238000007429 general method Methods 0.000 description 1
- 229910002804 graphite Inorganic materials 0.000 description 1
- 239000010439 graphite Substances 0.000 description 1
- 239000012535 impurity Substances 0.000 description 1
- 239000007788 liquid Substances 0.000 description 1
- 150000004668 long chain fatty acids Chemical class 0.000 description 1
- 239000000314 lubricant Substances 0.000 description 1
- FPYJFEHAWHCUMM-UHFFFAOYSA-N maleic anhydride Chemical compound O=C1OC(=O)C=C1 FPYJFEHAWHCUMM-UHFFFAOYSA-N 0.000 description 1
- IJDNQMDRQITEOD-UHFFFAOYSA-N n-butane Chemical compound CCCC IJDNQMDRQITEOD-UHFFFAOYSA-N 0.000 description 1
- 230000003647 oxidation Effects 0.000 description 1
- 238000007254 oxidation reaction Methods 0.000 description 1
- 238000004806 packaging method and process Methods 0.000 description 1
- 239000002245 particle Substances 0.000 description 1
- 238000005192 partition Methods 0.000 description 1
- 239000000843 powder Substances 0.000 description 1
- 239000012495 reaction gas Substances 0.000 description 1
- 239000011949 solid catalyst Substances 0.000 description 1
- 235000013619 trace mineral Nutrition 0.000 description 1
- 239000011573 trace mineral Substances 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 1
Images
Classifications
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
- B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
- B01J23/78—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with alkali- or alkaline earth metals
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J19/30—Loose or shaped packing elements, e.g. Raschig rings or Berl saddles, for pouring into the apparatus for mass or heat transfer
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J35/00—Catalysts, in general, characterised by their form or physical properties
- B01J35/50—Catalysts, in general, characterised by their form or physical properties characterised by their shape or configuration
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
- C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
- C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
- C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
- C01B3/38—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts
- C01B3/40—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using catalysts characterised by the catalyst
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/302—Basic shape of the elements
- B01J2219/30223—Cylinder
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/304—Composition or microstructure of the elements
- B01J2219/30416—Ceramic
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/304—Composition or microstructure of the elements
- B01J2219/30416—Ceramic
- B01J2219/30425—Carbon
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/304—Composition or microstructure of the elements
- B01J2219/30475—Composition or microstructure of the elements comprising catalytically active material
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/308—Details relating to random packing elements filling or discharging the elements into or from packed columns
- B01J2219/3081—Orientation of the packing elements within the column or vessel
- B01J2219/3083—Random or dumped packing elements
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/308—Details relating to random packing elements filling or discharging the elements into or from packed columns
- B01J2219/3086—Filling of the packing elements into the column or vessel, e.g. using a tube
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/31—Size details
- B01J2219/312—Sizes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
- B01J2219/30—Details relating to random packing elements
- B01J2219/318—Manufacturing aspects
- B01J2219/3188—Extruding
-
- C—CHEMISTRY; METALLURGY
- C01—INORGANIC CHEMISTRY
- C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
- C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
- C01B2203/10—Catalysts for performing the hydrogen forming reactions
- C01B2203/1005—Arrangement or shape of catalyst
- C01B2203/1011—Packed bed of catalytic structures, e.g. particles, packing elements
- C01B2203/1017—Packed bed of catalytic structures, e.g. particles, packing elements characterised by the form of the structure
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- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P20/00—Technologies relating to chemical industry
- Y02P20/50—Improvements relating to the production of bulk chemicals
- Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts
Landscapes
- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Organic Chemistry (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- General Health & Medical Sciences (AREA)
- Physics & Mathematics (AREA)
- Health & Medical Sciences (AREA)
- Combustion & Propulsion (AREA)
- Inorganic Chemistry (AREA)
- Thermal Sciences (AREA)
- Catalysts (AREA)
- Hydrogen, Water And Hydrids (AREA)
- Exhaust Gas After Treatment (AREA)
Description
(a) 歯先円直径(d2):歯元円直径(d1)が約1.2ないし2.5:1;
(b) 歯元の隙間幅(b1):歯幅(b2)の比が0.1ないし0.9:1;
(c) 歯元の隙間幅(b1)が少なくとも0.1mmとなる。
NiO 10−20重量%
CaO 10−20重量%
Al2O3 100重量%までの残余分
から形成することが好適である。
2 縦軸
3 外周面
4 溝部
5 ブリッジ部
6 半径
7 半径
8 中央通路
9 円
10 副通路
11 直径
12 直径
13 縦軸
14 ブリッジ部
15 ブリッジ部
16 ブリッジ部
17 直径
Claims (12)
- 触媒体(1)の縦軸(2)に平行に延在する溝部(4)群とそれらの溝部(4)の間に延在するブリッジ部(5)群を外周面(3)上に備えた円筒形状の触媒体であり、前記溝部(4)およびそれらの溝部(4)の間に延在しているブリッジ部(5)がその断面において部分円の形状を有しており、ブリッジ部(5)の部分円の半径(7)が溝部(4)の部分円の半径(6)よりも大きく選択され、前記触媒体(1)がさらにこの触媒体(1)の縦軸(2)に沿って延在する中央通路(8)を有し、触媒体(1)はこの触媒体(1)の縦軸(2)に平行であるがそれに対して偏心である副通路(10)を有し、前記副通路(10)の縦軸(13)は、その円心が触媒体(1)の縦軸(2)によって形成されるものである円(9)上に配置され、前記ブリッジ部(5)の部分円の中心点を副通路(10)の縦軸(13)上に配置することを特徴とする触媒体。
- 中央通路(8)は円形の断面を有することを特徴とする請求項1記載の触媒体。
- 副通路(10)は円形の断面を有することを特徴とする請求項1または2記載の触媒体。
- 副通路(10)の数は7本超に選択することを特徴とする請求項1ないし3のいずれかに記載の触媒体。
- 副通路(10)は中央通路(8)に比べてより小さな直径を有することを特徴とする請求項1ないし4のいずれかに記載の触媒体。
- 中央通路(8)の直径を4ないし8mmに選択することを特徴とする請求項1ないし5のいずれかに記載の触媒体。
- 副通路(10)の直径を1.5ないし3mmに選択することを特徴とする請求項1ないし6のいずれかに記載の触媒体。
- 触媒体の直径(17)と縦軸方向の長さの比は0.9ないし1.5となるように選択することを特徴とする請求項1ないし7のいずれかに記載の触媒体。
- 触媒体(1)は700N超の耐側圧強度を有することを特徴とする請求項1ないし8のいずれかに記載の触媒体。
- 触媒体(1)はいずれも酸化金属で計算して実質的に:
NiO 10−20重量%と
CaO 10−20重量%と
Al2O3 100重量%までの残余分
から形成することを特徴とする請求項1ないし9のいずれかに記載の触媒体。 - 触媒体(1)中のNaならびにSiO2の含有率は0.05重量%未満とすることを特徴とする請求項1ないし10のいずれかに記載の触媒体。
- 炭化水素の水蒸気改質への請求項10または11記載の触媒体の適用方法。
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE102005019596.2 | 2005-04-27 | ||
DE102005019596A DE102005019596A1 (de) | 2005-04-27 | 2005-04-27 | Katalysatorträger |
PCT/EP2006/003939 WO2006114320A1 (de) | 2005-04-27 | 2006-04-27 | Katalysatorträger |
Publications (2)
Publication Number | Publication Date |
---|---|
JP2008539060A JP2008539060A (ja) | 2008-11-13 |
JP4843024B2 true JP4843024B2 (ja) | 2011-12-21 |
Family
ID=36734515
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
JP2008508162A Expired - Fee Related JP4843024B2 (ja) | 2005-04-27 | 2006-04-27 | 触媒支持体 |
Country Status (8)
Country | Link |
---|---|
US (1) | US7799730B2 (ja) |
EP (1) | EP1874465B1 (ja) |
JP (1) | JP4843024B2 (ja) |
CN (1) | CN101227976B (ja) |
DE (1) | DE102005019596A1 (ja) |
DK (1) | DK1874465T3 (ja) |
EA (1) | EA011759B1 (ja) |
WO (1) | WO2006114320A1 (ja) |
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US9510559B2 (en) | 2011-11-16 | 2016-12-06 | Eatron, Inc. | Cage for breeding small animals |
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DE102007045106A1 (de) * | 2007-09-20 | 2009-04-02 | Refractory Intellectual Property Gmbh & Co. Kg | Basisches feuerfestes Bauteil |
DE102007046297B4 (de) | 2007-09-27 | 2016-12-22 | Süd-Chemie Ip Gmbh & Co. Kg | Neues Katalysatordesign und Herstellungsmethode für Dampfreformierungskatalysatoren |
GB0816705D0 (en) | 2008-09-12 | 2008-10-22 | Johnson Matthey Plc | Shaped heterogeneous catalysts |
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GB0816703D0 (en) | 2008-09-12 | 2008-10-22 | Johnson Matthey Plc | Shaped heterogeneous catalysts |
DE102009051462B4 (de) | 2009-10-30 | 2015-02-05 | Clariant International Ag | Verfahren zur Herstellung eines Kompositmaterials, Kompositmaterial und dessen Verwendung |
DE102010052126A1 (de) * | 2010-11-22 | 2012-05-24 | Süd-Chemie AG | Katalysatorformkörper für durchströmte Festbettreaktoren |
JP2014509556A (ja) | 2011-03-01 | 2014-04-21 | エクソンモービル リサーチ アンド エンジニアリング カンパニー | ガスを分離するための急速温度スイング吸着接触器 |
US9133079B2 (en) | 2012-01-13 | 2015-09-15 | Siluria Technologies, Inc. | Process for separating hydrocarbon compounds |
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US8808426B2 (en) | 2012-09-04 | 2014-08-19 | Exxonmobil Research And Engineering Company | Increasing scales, capacities, and/or efficiencies in swing adsorption processes with hydrocarbon gas feeds |
CN102921476A (zh) * | 2012-10-15 | 2013-02-13 | 安徽工程大学 | 一种甲醇催化剂颗粒 |
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WO2017065970A1 (en) * | 2015-10-15 | 2017-04-20 | Saint-Gobain Ceramics & Plastics, Inc. | Catalyst carrier |
WO2017065947A1 (en) | 2015-10-16 | 2017-04-20 | Siluria Technologies, Inc. | Separation methods and systems for oxidative coupling of methane |
US9944573B2 (en) | 2016-04-13 | 2018-04-17 | Siluria Technologies, Inc. | Oxidative coupling of methane for olefin production |
WO2018026517A1 (en) | 2016-08-04 | 2018-02-08 | Exxonmobil Research And Engineering Company | Increasing scales, capacities, and/or efficiencies in swing adsorption processes with hydrocarbon gas feeds |
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JP2020521811A (ja) | 2017-05-23 | 2020-07-27 | ラマス テクノロジー リミテッド ライアビリティ カンパニー | メタン酸化カップリングプロセスの統合 |
KR20200051583A (ko) | 2017-07-07 | 2020-05-13 | 루머스 테크놀로지 엘엘씨 | 메탄의 산화적 커플링를 위한 시스템 및 방법 |
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EP3569308A1 (de) * | 2018-05-18 | 2019-11-20 | Basf Se | Formkörper in form von multiloben |
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EP3659703A1 (en) | 2018-11-28 | 2020-06-03 | Basf Se | Catalyst for producing ethylene oxide by gas-phase oxidation |
EA202191639A1 (ru) | 2018-12-12 | 2021-09-23 | Хальдор Топсёэ А/С | Форма частиц катализатора |
WO2021038027A1 (en) | 2019-08-28 | 2021-03-04 | Basf Se | Process for preparing an epoxidation catalyst |
US20230278021A1 (en) | 2020-07-29 | 2023-09-07 | Basf Se | Solid shaped body and use of the solid shaped body |
EP4188597A1 (en) | 2020-07-29 | 2023-06-07 | Basf Se | Solid shaped body and use of the solid shaped body |
RU2753669C1 (ru) * | 2020-11-17 | 2021-08-19 | Акционерное общество "Специальное конструкторско-технологическое бюро "Катализатор" | Катализатор для гетерогенных реакций с пониженным гидравлическим сопротивлением слоя |
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2006
- 2006-04-27 DK DK06753436.2T patent/DK1874465T3/da active
- 2006-04-27 EA EA200702343A patent/EA011759B1/ru not_active IP Right Cessation
- 2006-04-27 JP JP2008508162A patent/JP4843024B2/ja not_active Expired - Fee Related
- 2006-04-27 WO PCT/EP2006/003939 patent/WO2006114320A1/de active Search and Examination
- 2006-04-27 EP EP06753436A patent/EP1874465B1/de active Active
- 2006-04-27 US US11/912,308 patent/US7799730B2/en active Active
- 2006-04-27 CN CN2006800142839A patent/CN101227976B/zh active Active
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JPS5419487A (en) * | 1977-07-13 | 1979-02-14 | Nippon Steel Corp | Method of producing catalyst carrier |
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US9510559B2 (en) | 2011-11-16 | 2016-12-06 | Eatron, Inc. | Cage for breeding small animals |
Also Published As
Publication number | Publication date |
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US20080277315A1 (en) | 2008-11-13 |
US7799730B2 (en) | 2010-09-21 |
JP2008539060A (ja) | 2008-11-13 |
WO2006114320A1 (de) | 2006-11-02 |
EP1874465B1 (de) | 2012-12-19 |
CN101227976A (zh) | 2008-07-23 |
DE102005019596A1 (de) | 2006-11-02 |
DK1874465T3 (da) | 2013-01-14 |
EP1874465A1 (de) | 2008-01-09 |
EA011759B1 (ru) | 2009-06-30 |
CN101227976B (zh) | 2011-11-23 |
EA200702343A1 (ru) | 2008-04-28 |
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