DE2119702C3 - Verwendung einer Substanz mit Perowskitstruktur als Katalysator für elektrochemische Verfahren und heterogene Gasphasen-Reaktionen - Google Patents
Verwendung einer Substanz mit Perowskitstruktur als Katalysator für elektrochemische Verfahren und heterogene Gasphasen-ReaktionenInfo
- Publication number
- DE2119702C3 DE2119702C3 DE2119702A DE2119702A DE2119702C3 DE 2119702 C3 DE2119702 C3 DE 2119702C3 DE 2119702 A DE2119702 A DE 2119702A DE 2119702 A DE2119702 A DE 2119702A DE 2119702 C3 DE2119702 C3 DE 2119702C3
- Authority
- DE
- Germany
- Prior art keywords
- oxygen
- catalyst
- gas phase
- substance
- electrode
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired
Links
- 239000000126 substance Substances 0.000 title claims description 15
- 239000003054 catalyst Substances 0.000 title claims description 13
- 238000000034 method Methods 0.000 title claims description 12
- 230000008569 process Effects 0.000 title claims description 11
- 238000010574 gas phase reaction Methods 0.000 title claims description 3
- PXHVJJICTQNCMI-UHFFFAOYSA-N Nickel Chemical compound [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 claims description 7
- 229910017052 cobalt Inorganic materials 0.000 claims description 6
- 239000010941 cobalt Substances 0.000 claims description 6
- GUTLYIVDDKVIGB-UHFFFAOYSA-N cobalt atom Chemical compound [Co] GUTLYIVDDKVIGB-UHFFFAOYSA-N 0.000 claims description 6
- 229910052759 nickel Inorganic materials 0.000 claims description 4
- 229910052712 strontium Inorganic materials 0.000 claims description 4
- OYPRJOBELJOOCE-UHFFFAOYSA-N Calcium Chemical compound [Ca] OYPRJOBELJOOCE-UHFFFAOYSA-N 0.000 claims description 2
- 229910052788 barium Inorganic materials 0.000 claims description 2
- DSAJWYNOEDNPEQ-UHFFFAOYSA-N barium atom Chemical compound [Ba] DSAJWYNOEDNPEQ-UHFFFAOYSA-N 0.000 claims description 2
- 229910052791 calcium Inorganic materials 0.000 claims description 2
- 239000011575 calcium Substances 0.000 claims description 2
- CIOAGBVUUVVLOB-UHFFFAOYSA-N strontium atom Chemical compound [Sr] CIOAGBVUUVVLOB-UHFFFAOYSA-N 0.000 claims description 2
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 description 27
- 239000001301 oxygen Substances 0.000 description 27
- 229910052760 oxygen Inorganic materials 0.000 description 27
- 150000002500 ions Chemical class 0.000 description 7
- BASFCYQUMIYNBI-UHFFFAOYSA-N platinum Chemical compound [Pt] BASFCYQUMIYNBI-UHFFFAOYSA-N 0.000 description 6
- 238000006243 chemical reaction Methods 0.000 description 5
- 238000010586 diagram Methods 0.000 description 5
- 238000007254 oxidation reaction Methods 0.000 description 5
- 239000000243 solution Substances 0.000 description 5
- 239000007789 gas Substances 0.000 description 4
- 230000003647 oxidation Effects 0.000 description 4
- 230000005298 paramagnetic effect Effects 0.000 description 4
- 230000009467 reduction Effects 0.000 description 4
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 description 3
- 239000012670 alkaline solution Substances 0.000 description 3
- 230000003197 catalytic effect Effects 0.000 description 3
- 238000005260 corrosion Methods 0.000 description 3
- 230000007797 corrosion Effects 0.000 description 3
- 239000001257 hydrogen Substances 0.000 description 3
- 229910052739 hydrogen Inorganic materials 0.000 description 3
- 230000005291 magnetic effect Effects 0.000 description 3
- 229910052697 platinum Inorganic materials 0.000 description 3
- -1 polytetrafluoroethylene Polymers 0.000 description 3
- 229920001343 polytetrafluoroethylene Polymers 0.000 description 3
- 239000004810 polytetrafluoroethylene Substances 0.000 description 3
- 230000002441 reversible effect Effects 0.000 description 3
- IJGRMHOSHXDMSA-UHFFFAOYSA-N Atomic nitrogen Chemical compound N#N IJGRMHOSHXDMSA-UHFFFAOYSA-N 0.000 description 2
- MYMOFIZGZYHOMD-UHFFFAOYSA-N Dioxygen Chemical compound O=O MYMOFIZGZYHOMD-UHFFFAOYSA-N 0.000 description 2
- 238000006555 catalytic reaction Methods 0.000 description 2
- 150000001875 compounds Chemical class 0.000 description 2
- 239000013078 crystal Substances 0.000 description 2
- 239000006185 dispersion Substances 0.000 description 2
- 239000012153 distilled water Substances 0.000 description 2
- 239000003792 electrolyte Substances 0.000 description 2
- 239000000446 fuel Substances 0.000 description 2
- 229910052746 lanthanum Inorganic materials 0.000 description 2
- 239000000463 material Substances 0.000 description 2
- 125000004430 oxygen atom Chemical group O* 0.000 description 2
- 238000001179 sorption measurement Methods 0.000 description 2
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Chemical compound O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 2
- 238000004438 BET method Methods 0.000 description 1
- BVKZGUZCCUSVTD-UHFFFAOYSA-L Carbonate Chemical compound [O-]C([O-])=O BVKZGUZCCUSVTD-UHFFFAOYSA-L 0.000 description 1
- VGGSQFUCUMXWEO-UHFFFAOYSA-N Ethene Chemical compound C=C VGGSQFUCUMXWEO-UHFFFAOYSA-N 0.000 description 1
- 239000005977 Ethylene Substances 0.000 description 1
- IAYPIBMASNFSPL-UHFFFAOYSA-N Ethylene oxide Chemical compound C1CO1 IAYPIBMASNFSPL-UHFFFAOYSA-N 0.000 description 1
- 229910002254 LaCoO3 Inorganic materials 0.000 description 1
- 229910018068 Li 2 O Inorganic materials 0.000 description 1
- WHXSMMKQMYFTQS-UHFFFAOYSA-N Lithium Chemical compound [Li] WHXSMMKQMYFTQS-UHFFFAOYSA-N 0.000 description 1
- GOOHAUXETOMSMM-UHFFFAOYSA-N Propylene oxide Chemical compound CC1CO1 GOOHAUXETOMSMM-UHFFFAOYSA-N 0.000 description 1
- BAPRMBRFVUJBEI-UHFFFAOYSA-N [O].[O].[Ni] Chemical compound [O].[O].[Ni] BAPRMBRFVUJBEI-UHFFFAOYSA-N 0.000 description 1
- 239000000654 additive Substances 0.000 description 1
- 230000000996 additive effect Effects 0.000 description 1
- 230000005290 antiferromagnetic effect Effects 0.000 description 1
- 230000005303 antiferromagnetism Effects 0.000 description 1
- 230000009286 beneficial effect Effects 0.000 description 1
- 230000008901 benefit Effects 0.000 description 1
- 230000015572 biosynthetic process Effects 0.000 description 1
- 230000008859 change Effects 0.000 description 1
- 238000000576 coating method Methods 0.000 description 1
- 229910001429 cobalt ion Inorganic materials 0.000 description 1
- XLJKHNWPARRRJB-UHFFFAOYSA-N cobalt(2+) Chemical compound [Co+2] XLJKHNWPARRRJB-UHFFFAOYSA-N 0.000 description 1
- 238000002485 combustion reaction Methods 0.000 description 1
- 239000012141 concentrate Substances 0.000 description 1
- 238000012937 correction Methods 0.000 description 1
- 238000005090 crystal field Methods 0.000 description 1
- 230000005292 diamagnetic effect Effects 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 238000001704 evaporation Methods 0.000 description 1
- 230000008020 evaporation Effects 0.000 description 1
- 230000005294 ferromagnetic effect Effects 0.000 description 1
- 239000000295 fuel oil Substances 0.000 description 1
- PCHJSUWPFVWCPO-UHFFFAOYSA-N gold Chemical compound [Au] PCHJSUWPFVWCPO-UHFFFAOYSA-N 0.000 description 1
- 239000010931 gold Substances 0.000 description 1
- 229910052737 gold Inorganic materials 0.000 description 1
- 238000010438 heat treatment Methods 0.000 description 1
- 229930195733 hydrocarbon Natural products 0.000 description 1
- 150000002430 hydrocarbons Chemical class 0.000 description 1
- 230000006872 improvement Effects 0.000 description 1
- 230000003993 interaction Effects 0.000 description 1
- 238000011835 investigation Methods 0.000 description 1
- FZLIPJUXYLNCLC-UHFFFAOYSA-N lanthanum atom Chemical compound [La] FZLIPJUXYLNCLC-UHFFFAOYSA-N 0.000 description 1
- 239000007788 liquid Substances 0.000 description 1
- 229910001947 lithium oxide Inorganic materials 0.000 description 1
- 238000011068 loading method Methods 0.000 description 1
- 238000005259 measurement Methods 0.000 description 1
- 230000007246 mechanism Effects 0.000 description 1
- 229910052751 metal Inorganic materials 0.000 description 1
- 239000002184 metal Substances 0.000 description 1
- 238000002156 mixing Methods 0.000 description 1
- 229910000480 nickel oxide Inorganic materials 0.000 description 1
- 229910052757 nitrogen Inorganic materials 0.000 description 1
- GNRSAWUEBMWBQH-UHFFFAOYSA-N oxonickel Chemical compound [Ni]=O GNRSAWUEBMWBQH-UHFFFAOYSA-N 0.000 description 1
- 150000002978 peroxides Chemical class 0.000 description 1
- 230000010287 polarization Effects 0.000 description 1
- 239000000843 powder Substances 0.000 description 1
- QQONPFPTGQHPMA-UHFFFAOYSA-N propylene Natural products CC=C QQONPFPTGQHPMA-UHFFFAOYSA-N 0.000 description 1
- 125000004805 propylene group Chemical group [H]C([H])([H])C([H])([*:1])C([H])([H])[*:2] 0.000 description 1
- 238000010791 quenching Methods 0.000 description 1
- 230000000171 quenching effect Effects 0.000 description 1
- 238000010405 reoxidation reaction Methods 0.000 description 1
- 230000027756 respiratory electron transport chain Effects 0.000 description 1
- 239000007787 solid Substances 0.000 description 1
- 230000003068 static effect Effects 0.000 description 1
- 238000003756 stirring Methods 0.000 description 1
- 238000012360 testing method Methods 0.000 description 1
- 238000002604 ultrasonography Methods 0.000 description 1
Classifications
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
- B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
- B01J23/83—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with rare earths or actinides
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/10—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of rare earths
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
- B01J23/16—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M4/00—Electrodes
- H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
- H01M4/90—Selection of catalytic material
- H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10S—TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10S502/00—Catalyst, solid sorbent, or support therefor: product or process of making
- Y10S502/525—Perovskite
Landscapes
- Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Organic Chemistry (AREA)
- Electrochemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Catalysts (AREA)
- Inert Electrodes (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
- Inorganic Compounds Of Heavy Metals (AREA)
- Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
- Electrodes For Compound Or Non-Metal Manufacture (AREA)
- Investigating Or Analyzing Materials By The Use Of Electric Means (AREA)
- Gas Burners (AREA)
- Exhaust Gas Treatment By Means Of Catalyst (AREA)
Applications Claiming Priority (1)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| GB1929270 | 1970-04-22 |
Publications (3)
| Publication Number | Publication Date |
|---|---|
| DE2119702A1 DE2119702A1 (de) | 1971-11-04 |
| DE2119702B2 DE2119702B2 (de) | 1979-06-13 |
| DE2119702C3 true DE2119702C3 (de) | 1980-02-21 |
Family
ID=10126975
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| DE2119702A Expired DE2119702C3 (de) | 1970-04-22 | 1971-04-22 | Verwendung einer Substanz mit Perowskitstruktur als Katalysator für elektrochemische Verfahren und heterogene Gasphasen-Reaktionen |
Country Status (4)
| Country | Link |
|---|---|
| US (1) | US3922204A (OSRAM) |
| JP (1) | JPS525472B1 (OSRAM) |
| DE (1) | DE2119702C3 (OSRAM) |
| GB (1) | GB1352995A (OSRAM) |
Families Citing this family (29)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US3951603A (en) * | 1972-07-08 | 1976-04-20 | Hitachi, Ltd. | Gas-sensor element and method for detecting reducing gas or oxygen gas |
| US3972837A (en) * | 1973-07-03 | 1976-08-03 | Johnson Matthey & Co., Limited | Catalyst for purifying automotive exhaust gases |
| US4001143A (en) * | 1975-04-08 | 1977-01-04 | E. I. Du Pont De Nemours And Company | Catalyst preparation |
| US3935027A (en) * | 1975-04-09 | 1976-01-27 | Westinghouse Electric Corporation | Oxygen-reduction electrocatalysts for electrodes |
| US4102777A (en) * | 1976-04-13 | 1978-07-25 | Exxon Research & Engineering Co. | Hydrocarbon conversion processes employing perovskite catalysts |
| US4162235A (en) * | 1976-06-17 | 1979-07-24 | Johnson, Matthey & Co., Limited | Catalysts |
| US4186072A (en) * | 1976-06-28 | 1980-01-29 | Blumenthal Robert N | Hot gas measuring device |
| DE2735934C3 (de) * | 1977-08-10 | 1980-07-31 | Dornier System Gmbh, 7990 Friedrichshafen | Verbindungsmaterial zur elektrischen Serienschaltung von elektrochemischen ZeUen |
| DE2738755C3 (de) * | 1977-08-27 | 1980-03-06 | Brown, Boveri & Cie Ag, 6800 Mannheim | Elektrochemische Meßzelle |
| US4221827A (en) * | 1978-12-19 | 1980-09-09 | The United States Of America As Represented By The Secretary Of The Interior | Method of manufacturing a gas sensor |
| US4314996A (en) | 1979-04-04 | 1982-02-09 | Matsushita Electric Industrial Company, Limited | Oxygen sensor |
| US4537674A (en) * | 1982-07-19 | 1985-08-27 | Energy Conversion Devices, Inc. | Electrolytic cell anode |
| US4545883A (en) * | 1982-07-19 | 1985-10-08 | Energy Conversion Devices, Inc. | Electrolytic cell cathode |
| US4484172A (en) * | 1983-04-01 | 1984-11-20 | Arthur D. Little, Inc. | Humidity sensor, comprised of compound metal oxides with perovskite structure |
| JPH0649146B2 (ja) * | 1985-06-07 | 1994-06-29 | 松下電器産業株式会社 | 酸化触媒 |
| US5021137A (en) * | 1986-07-25 | 1991-06-04 | Ceramatec, Inc. | Ceramic solid electrolyte based electrochemical oxygen concentrator cell |
| US5378345A (en) * | 1986-07-25 | 1995-01-03 | Ceramatec, Inc. | Ceramic solid electrolyte-based electrochemical oxygen concentrator cell |
| EP0271917B1 (en) * | 1986-12-19 | 1991-09-25 | Matsushita Electric Industrial Co., Ltd. | Air/fuel ratio sensor |
| EP0348162A3 (en) * | 1988-06-21 | 1991-02-13 | Victor Company Of Japan, Limited | Method and apparatus of repeatedly recording optical image information and image pickup device |
| JP2520297B2 (ja) * | 1989-02-21 | 1996-07-31 | 堺化学工業株式会社 | α―オレフイン重合触媒、及びこれを用いる重合体・ペロブスカイト型化合物複合体とその製造方法 |
| US5028404A (en) * | 1989-04-25 | 1991-07-02 | University Of Notre Dame Du Lac | Metal oxide catalysts |
| US5286698A (en) * | 1989-04-25 | 1994-02-15 | University Of Notre Dame Du Lac | Metal oxide catalysts |
| US7303606B2 (en) * | 2002-01-08 | 2007-12-04 | The Boc Group, Inc. | Oxy-fuel combustion process |
| US20030138747A1 (en) * | 2002-01-08 | 2003-07-24 | Yongxian Zeng | Oxy-fuel combustion process |
| US7259126B2 (en) * | 2004-03-11 | 2007-08-21 | Ceramatec, Inc. | Gas diffusion electrode and catalyst for electrochemical oxygen reduction and method of dispersing the catalyst |
| JP2009544843A (ja) * | 2006-07-22 | 2009-12-17 | セラマテック・インク | 固体酸化物電解槽セル用の効率的な可逆電極 |
| US8354011B2 (en) * | 2006-07-22 | 2013-01-15 | Ceramatec, Inc. | Efficient reversible electrodes for solid oxide electrolyzer cells |
| US9688647B2 (en) | 2013-11-15 | 2017-06-27 | Corning Incorporated | Alkylene oxide synthesis |
| JP5869169B1 (ja) * | 2015-06-01 | 2016-02-24 | 公立大学法人大阪府立大学 | 酸素発生反応用ペロブスカイト酸化物触媒 |
Family Cites Families (5)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US3644147A (en) * | 1969-04-24 | 1972-02-22 | Exxon Research Engineering Co | Mixed valency transition metal perovskites as cathodic reduction catalysts |
| US3595809A (en) * | 1969-06-27 | 1971-07-27 | Gulf Research Development Co | Lanthanum chromium ferrite catalyst |
| BE755982A (fr) * | 1969-09-16 | 1971-03-10 | Petro Tex Chem Corp | Catalyseurs de deshydrogenation oxydante |
| JPS4810773B1 (OSRAM) * | 1970-03-17 | 1973-04-07 | ||
| US3780126A (en) * | 1971-03-26 | 1973-12-18 | Petro Tex Chem Corp | Oxidative dehydrogenation in the presence of crystalline,provoskite type manganese compounds |
-
1970
- 1970-04-22 GB GB1929270A patent/GB1352995A/en not_active Expired
-
1971
- 1971-04-19 US US134988A patent/US3922204A/en not_active Expired - Lifetime
- 1971-04-22 JP JP46026415A patent/JPS525472B1/ja active Pending
- 1971-04-22 DE DE2119702A patent/DE2119702C3/de not_active Expired
Also Published As
| Publication number | Publication date |
|---|---|
| GB1352995A (en) | 1974-05-15 |
| DE2119702A1 (de) | 1971-11-04 |
| US3922204A (en) | 1975-11-25 |
| DE2119702B2 (de) | 1979-06-13 |
| JPS525472B1 (OSRAM) | 1977-02-14 |
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Legal Events
| Date | Code | Title | Description |
|---|---|---|---|
| OD | Request for examination | ||
| C3 | Grant after two publication steps (3rd publication) | ||
| 8339 | Ceased/non-payment of the annual fee |