CN104685682B - 燃料电池用催化剂的制造方法和含有利用该制造方法制造的燃料电池用催化剂的燃料电池 - Google Patents

燃料电池用催化剂的制造方法和含有利用该制造方法制造的燃料电池用催化剂的燃料电池 Download PDF

Info

Publication number
CN104685682B
CN104685682B CN201380025115.XA CN201380025115A CN104685682B CN 104685682 B CN104685682 B CN 104685682B CN 201380025115 A CN201380025115 A CN 201380025115A CN 104685682 B CN104685682 B CN 104685682B
Authority
CN
China
Prior art keywords
catalyst
fuel cell
palladium
carbon
supported
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
CN201380025115.XA
Other languages
English (en)
Chinese (zh)
Other versions
CN104685682A (zh
Inventor
木村纮子
竹广直树
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Audi AG
Toyota Motor Corp
Original Assignee
Audi AG
Toyota Motor Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Audi AG, Toyota Motor Corp filed Critical Audi AG
Publication of CN104685682A publication Critical patent/CN104685682A/zh
Application granted granted Critical
Publication of CN104685682B publication Critical patent/CN104685682B/zh
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8817—Treatment of supports before application of the catalytic active composition
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8825—Methods for deposition of the catalytic active composition
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H01M4/921—Alloys or mixtures with metallic elements
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H01M4/925—Metals of platinum group supported on carriers, e.g. powder carriers
    • H01M4/926—Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M2008/1095—Fuel cells with polymeric electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Composite Materials (AREA)
  • Inert Electrodes (AREA)
  • Catalysts (AREA)
  • Fuel Cell (AREA)
CN201380025115.XA 2012-05-15 2013-01-21 燃料电池用催化剂的制造方法和含有利用该制造方法制造的燃料电池用催化剂的燃料电池 Expired - Fee Related CN104685682B (zh)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
JP2012111402A JP5829973B2 (ja) 2012-05-15 2012-05-15 燃料電池用触媒の製造方法
JP2012-111402 2012-05-15
PCT/JP2013/051083 WO2013172050A1 (ja) 2012-05-15 2013-01-21 燃料電池用触媒の製造方法、及び当該製造方法により製造される燃料電池用触媒を含む燃料電池

Publications (2)

Publication Number Publication Date
CN104685682A CN104685682A (zh) 2015-06-03
CN104685682B true CN104685682B (zh) 2017-10-13

Family

ID=49583476

Family Applications (1)

Application Number Title Priority Date Filing Date
CN201380025115.XA Expired - Fee Related CN104685682B (zh) 2012-05-15 2013-01-21 燃料电池用催化剂的制造方法和含有利用该制造方法制造的燃料电池用催化剂的燃料电池

Country Status (7)

Country Link
US (1) US11239474B2 (enExample)
EP (1) EP2854207B1 (enExample)
JP (1) JP5829973B2 (enExample)
KR (1) KR101651344B1 (enExample)
CN (1) CN104685682B (enExample)
IN (1) IN2014DN09536A (enExample)
WO (1) WO2013172050A1 (enExample)

Families Citing this family (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6403046B2 (ja) * 2014-05-07 2018-10-10 学校法人同志社 燃料電池用触媒の製造方法、それを用いた触媒及び燃料電池
JP6168009B2 (ja) 2014-07-31 2017-07-26 トヨタ自動車株式会社 コアシェル触媒の製造方法
JP6308090B2 (ja) 2014-10-02 2018-04-11 トヨタ自動車株式会社 コアシェル触媒の製造方法
JP6248957B2 (ja) * 2015-01-26 2017-12-20 トヨタ自動車株式会社 コアシェル触媒の製造方法
JP6653875B2 (ja) * 2015-03-10 2020-02-26 学校法人同志社 白金触媒の製造方法及びそれを用いた燃料電池
JP6269581B2 (ja) * 2015-06-02 2018-01-31 トヨタ自動車株式会社 燃料電池電極用コアシェル触媒の製造方法
CN107910566B (zh) * 2017-11-10 2021-02-05 北京工业大学 一种三元核壳结构纳米电催化剂及制备方法
KR102398409B1 (ko) 2020-09-07 2022-05-17 한국에너지기술연구원 일산화탄소를 이용한 코어-쉘 입자의 제조방법
KR102841625B1 (ko) 2020-09-07 2025-08-06 한국에너지기술연구원 연속 반응기 타입의 일산화탄소를 이용한 코어-쉘 입자의 시트 제조장치
KR102893825B1 (ko) 2020-09-07 2025-12-05 한국에너지기술연구원 레이저 어블레이션 연계 일산화탄소 활용 코어-쉘 입자의 제조장치 및 방법
KR102841624B1 (ko) 2020-09-07 2025-08-05 한국에너지기술연구원 롤투롤 공정 기반의 일산화탄소를 이용한 코어-쉘 입자의 시트 제조장치

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20040038808A1 (en) * 1998-08-27 2004-02-26 Hampden-Smith Mark J. Method of producing membrane electrode assemblies for use in proton exchange membrane and direct methanol fuel cells
US20070031722A1 (en) * 2004-12-22 2007-02-08 Radoslav Adzic Electrocatalysts having platinum monolayers on palladium, palladium alloy, and gold alloy nanoparticle cores, and uses thereof
CN101516550A (zh) * 2006-08-30 2009-08-26 尤米科尔股份公司及两合公司 核/壳型催化剂颗粒及它们的制备方法
JP2011218278A (ja) * 2010-04-07 2011-11-04 Toyota Motor Corp カーボン担持コアシェル型触媒微粒子の製造方法、当該製造方法により得られるコアシェル型触媒微粒子を用いた触媒インクの製造方法、及び、当該製造方法により得られる触媒インクを含む触媒層

Family Cites Families (17)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS60133662A (ja) * 1983-12-21 1985-07-16 Fuji Electric Corp Res & Dev Ltd 燃料電池のガス拡散電極の製造方法
US6103393A (en) * 1998-02-24 2000-08-15 Superior Micropowders Llc Metal-carbon composite powders, methods for producing powders and devices fabricated from same
US7066976B2 (en) * 1998-02-24 2006-06-27 Cabot Corporation Method for the production of electrocatalyst powders
JP3869568B2 (ja) * 1998-11-30 2007-01-17 本田技研工業株式会社 燃料電池用電極
AU2003217382A1 (en) * 2002-02-12 2003-09-04 Honda Giken Kogyo Kabushiki Kaisha FUEL CELL ELECTROCATALYST OF Pt-Rh-Mo-Ni/Fe
JP5082187B2 (ja) * 2003-10-06 2012-11-28 日産自動車株式会社 固体高分子型燃料電池用電極触媒粒子の製造方法
JP4506740B2 (ja) * 2006-09-14 2010-07-21 トヨタ自動車株式会社 燃料電池用触媒構造体、膜電極接合体、燃料電池、燃料電池用触媒構造体の製造方法
JP5092381B2 (ja) * 2006-12-08 2012-12-05 株式会社Ｇｓユアサ 燃料電池用触媒粉末、燃料電池用触媒粉末の製造方法および燃料電池
JP2009217975A (ja) * 2008-03-07 2009-09-24 Hitachi Ltd 燃料極触媒、膜電極接合体及び燃料電池
JP2009245932A (ja) 2008-03-13 2009-10-22 Toppan Printing Co Ltd 燃料電池用電極触媒インク、電極触媒層、膜電極接合体および固体高分子型燃料電池
JP5736306B2 (ja) * 2008-06-23 2015-06-17 ブルックヘイヴン サイエンス アソシエイツ， エルエルシー アンダーポテンシャル析出で媒介される薄膜の逐次積層成長
US8168561B2 (en) * 2008-07-31 2012-05-01 University Of Utah Research Foundation Core shell catalyst
US20100035124A1 (en) * 2008-08-11 2010-02-11 Gm Clobal Technology Operations, Inc. Hybrid particle and core-shell electrode structure
JP5660603B2 (ja) 2010-03-19 2015-01-28 学校法人同志社 白金コアシェル触媒の製造方法
JP5573438B2 (ja) * 2010-07-09 2014-08-20 トヨタ自動車株式会社 コアシェル型触媒微粒子の製造方法
JP2012074347A (ja) * 2010-08-31 2012-04-12 Equos Research Co Ltd 触媒ペーストの製造方法及びその装置
JP5675255B2 (ja) * 2010-10-08 2015-02-25 国立大学法人 宮崎大学 燃料電池用触媒の製造方法

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20040038808A1 (en) * 1998-08-27 2004-02-26 Hampden-Smith Mark J. Method of producing membrane electrode assemblies for use in proton exchange membrane and direct methanol fuel cells
US20070031722A1 (en) * 2004-12-22 2007-02-08 Radoslav Adzic Electrocatalysts having platinum monolayers on palladium, palladium alloy, and gold alloy nanoparticle cores, and uses thereof
CN101516550A (zh) * 2006-08-30 2009-08-26 尤米科尔股份公司及两合公司 核/壳型催化剂颗粒及它们的制备方法
JP2011218278A (ja) * 2010-04-07 2011-11-04 Toyota Motor Corp カーボン担持コアシェル型触媒微粒子の製造方法、当該製造方法により得られるコアシェル型触媒微粒子を用いた触媒インクの製造方法、及び、当該製造方法により得られる触媒インクを含む触媒層

Also Published As

Publication number Publication date
EP2854207A4 (en) 2015-09-02
EP2854207B1 (en) 2019-06-05
CN104685682A (zh) 2015-06-03
JP5829973B2 (ja) 2015-12-09
KR20150008104A (ko) 2015-01-21
JP2013239331A (ja) 2013-11-28
US20150093682A1 (en) 2015-04-02
IN2014DN09536A (enExample) 2015-07-17
US11239474B2 (en) 2022-02-01
KR101651344B1 (ko) 2016-08-25
EP2854207A1 (en) 2015-04-01
WO2013172050A1 (ja) 2013-11-21

Similar Documents

Publication Publication Date Title
CN104685682B (zh) 燃料电池用催化剂的制造方法和含有利用该制造方法制造的燃料电池用催化剂的燃料电池
CN105209169B (zh) 催化剂微粒的制造方法、和包含采用该制造方法制造的催化剂微粒的燃料电池
JP5699287B2 (ja) 触媒微粒子、カーボン担持触媒微粒子、触媒合剤、及び電極の各製造方法
CN102820475B (zh) 三元铂合金催化剂
CN106605325B (zh) 燃料电池用电极催化剂及其制造方法
EP3446781A1 (en) Electrocatalyst, membrane electrode assembly using said electrocatalyst, and fuel cell
CN106058268B (zh) 燃料电池用电极的制造方法
CN102823039B (zh) 燃料电池
US10090530B2 (en) Non-carbon mixed-metal oxide electrocatalysts
CN103079696A (zh) 催化剂微粒及催化剂微粒的制造方法
JP2013215701A (ja) コアシェル触媒の製造方法、及び、膜電極接合体の製造方法
CN105992645B (zh) 碳负载催化剂
Lu et al. Phosphotungstic acid-assisted preparation of carbon nanotubes-supported uniform Pt and Pt bimetallic nanoparticles, and their enhanced catalytic activity on methanol electro-oxidation
JP5488486B2 (ja) 触媒合剤の製造方法
JP2006253042A (ja) 固体高分子形燃料電池用触媒の製造方法
JP2006209999A (ja) 固体高分子形燃料電池用電極およびその製造方法
JP2014117652A (ja) 触媒微粒子の製造方法、及び当該製造方法により製造される触媒微粒子を含む燃料電池

Legal Events

Date Code Title Description
C06 Publication
PB01 Publication
C10 Entry into substantive examination
SE01 Entry into force of request for substantive examination
C41 Transfer of patent application or patent right or utility model
TA01 Transfer of patent application right

Effective date of registration: 20160222

Address after: Aichi Prefecture, Japan

Applicant after: Toyota Motor Corp.

Applicant after: AUDI AG

Address before: Aichi Prefecture, Japan

Applicant before: Toyota Motor Corp.

Applicant before: Ballard Power Systems

GR01 Patent grant
GR01 Patent grant
CF01 Termination of patent right due to non-payment of annual fee

Granted publication date: 20171013

CF01 Termination of patent right due to non-payment of annual fee