CN101536115B - 固体高分子电解质及其制造方法，以及使用了该电解质的燃料电池用膜·电极接合体 - Google Patents

固体高分子电解质及其制造方法，以及使用了该电解质的燃料电池用膜·电极接合体 Download PDF

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CN101536115B
CN101536115B CN2007800408540A CN200780040854A CN101536115B CN 101536115 B CN101536115 B CN 101536115B CN 2007800408540 A CN2007800408540 A CN 2007800408540A CN 200780040854 A CN200780040854 A CN 200780040854A CN 101536115 B CN101536115 B CN 101536115B
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polymer electrolyte
solid polymer
membrane
electrode
formula
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CN101536115A (zh
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高见昌宜
吉田利彦
植田昌宏
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Toyota Motor Corp
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    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20—Manufacture of shaped structures of ion-exchange resins
    • C08J5/22—Films, membranes or diaphragms
    • C08J5/2206—Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218—Synthetic macromolecular compounds
    • C08J5/2256—Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F8/00—Chemical modification by after-treatment
    • C08F8/12—Hydrolysis
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
    • H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
    • H01B1/06—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances
    • H01B1/12—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances organic substances
    • H01B1/122—Ionic conductors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1025—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having only carbon and oxygen, e.g. polyethers, sulfonated polyetheretherketones [S-PEEK], sulfonated polysaccharides, sulfonated celluloses or sulfonated polyesters
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/1069—Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1072—Polymeric electrolyte materials characterised by the manufacturing processes by chemical reactions, e.g. in situ polymerisation or in situ crosslinking
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F2810/00—Chemical modification of a polymer
    • C08F2810/50—Chemical modification of a polymer wherein the polymer is a copolymer and the modification is taking place only on one or more of the monomers present in minority
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2371/00—Characterised by the use of polyethers obtained by reactions forming an ether link in the main chain; Derivatives of such polymers
    • C08J2371/08—Polyethers derived from hydroxy compounds or from their metallic derivatives
    • C08J2371/10—Polyethers derived from hydroxy compounds or from their metallic derivatives from phenols
    • C08J2371/12—Polyphenylene oxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0082—Organic polymers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Sustainable Energy (AREA)
  • Polymers & Plastics (AREA)
  • Sustainable Development (AREA)
  • Electrochemistry (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Physics & Mathematics (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Inert Electrodes (AREA)
CN2007800408540A 2006-11-07 2007-11-07 固体高分子电解质及其制造方法，以及使用了该电解质的燃料电池用膜·电极接合体 Expired - Fee Related CN101536115B (zh)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
JP301513/2006 2006-11-07
JP2006301513A JP4586794B2 (ja) 2006-11-07 2006-11-07 固体高分子電解質並びにその製造方法及びこれを用いた燃料電池用膜・電極接合体
PCT/JP2007/071644 WO2008056704A1 (en) 2006-11-07 2007-11-07 Solid polyelectrolyte, process for production thereof, and membrane/electrode assemly for fuel cells made by using the polyelectrolyte

Publications (2)

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CN101536115A CN101536115A (zh) 2009-09-16
CN101536115B true CN101536115B (zh) 2011-11-23

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CN2007800408540A Expired - Fee Related CN101536115B (zh) 2006-11-07 2007-11-07 固体高分子电解质及其制造方法，以及使用了该电解质的燃料电池用膜·电极接合体

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US (1) US20100104917A1 (enExample)
EP (1) EP2081195B1 (enExample)
JP (1) JP4586794B2 (enExample)
CN (1) CN101536115B (enExample)
AT (1) ATE531051T1 (enExample)
WO (1) WO2008056704A1 (enExample)

Families Citing this family (7)

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Publication number Priority date Publication date Assignee Title
JP6822101B2 (ja) 2016-11-29 2021-01-27 セイコーエプソン株式会社 高分子電解質、電池、および電子機器
JP6801446B2 (ja) * 2016-12-27 2020-12-16 セイコーエプソン株式会社 電池および電子機器
WO2024232344A1 (ja) * 2023-05-08 2024-11-14 住友化学株式会社 重合体、電解質組成物、及び電池
CN118970072B (zh) * 2024-10-10 2025-03-04 杭州德海艾科能源科技有限公司 一种钒电池用一体化膜电极及其制备方法
WO2026105789A1 (ja) * 2024-11-12 2026-05-21 Ａｇｃ株式会社 固体高分子電解質膜、膜電極接合体、水電解装置、電解水素化装置及び水素の製造方法
WO2026105788A1 (ja) * 2024-11-12 2026-05-21 Ａｇｃ株式会社 固体高分子電解質膜、膜電極接合体、水電解装置、電解水素化装置及び水素の製造方法
WO2026105790A1 (ja) * 2024-11-12 2026-05-21 Ａｇｃ株式会社 固体高分子電解質膜、膜電極接合体、水電解装置、電解水素化装置及び水素の製造方法

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB796199A (en) * 1955-02-11 1958-06-04 Bayer Ag Process for the production of moulded articles by a dipping process
US5741611A (en) * 1996-08-28 1998-04-21 E.C.R. - Electro-Chemical Research Ltd. Method of preparing an electrochemical system operated at ambient temperatures

Family Cites Families (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2450670A1 (de) * 1974-10-25 1976-04-29 Benckiser Gmbh Joh A Verfahren zur abtrennung von citrat oder citronensaeure aus fermentationsloesungen
JPS5258785A (en) * 1975-11-07 1977-05-14 Japan Exlan Co Ltd Process for preparing acrylonitrile polymer melts
DE19754305A1 (de) 1997-12-08 1999-06-10 Hoechst Ag Verfahren zur Herstellung einer Membran zum Betrieb von Brennstoffzellen und Elektrolyseuren
JPH11302410A (ja) * 1998-04-24 1999-11-02 Nissan Motor Co Ltd イオン交換膜およびその製造方法
JP3735516B2 (ja) * 2000-03-31 2006-01-18 株式会社東芝 燃料電池
JP2003535940A (ja) * 2000-06-02 2003-12-02 エスアールアイ インターナショナル 高分子組成物
US7318972B2 (en) * 2001-09-07 2008-01-15 Itm Power Ltd. Hydrophilic polymers and their use in electrochemical cells
CA2473907A1 (en) * 2002-01-23 2003-07-31 Polyfuel, Inc. Acid-base proton conducting polymer blend membrane
JP2005048088A (ja) 2003-07-30 2005-02-24 Toyota Motor Corp 分枝化された高分子化合物及びその製造方法、高耐久性固体高分子電解質膜及びその製造方法、並びに燃料電池
JP2005310389A (ja) * 2004-04-16 2005-11-04 Toyota Motor Corp 電解質膜およびそれを用いた燃料電池

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB796199A (en) * 1955-02-11 1958-06-04 Bayer Ag Process for the production of moulded articles by a dipping process
US5741611A (en) * 1996-08-28 1998-04-21 E.C.R. - Electro-Chemical Research Ltd. Method of preparing an electrochemical system operated at ambient temperatures

Non-Patent Citations (3)

* Cited by examiner, † Cited by third party
Title
JP特开2001-283635A 2001.12.12
JP特开2005-310389A 2005.11.04
JP特开平11-302410A 1999.11.02

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Publication number Publication date
CN101536115A (zh) 2009-09-16
EP2081195A1 (en) 2009-07-22
WO2008056704A1 (en) 2008-05-15
JP2008117694A (ja) 2008-05-22
US20100104917A1 (en) 2010-04-29
EP2081195B1 (en) 2011-10-26
JP4586794B2 (ja) 2010-11-24
ATE531051T1 (de) 2011-11-15
EP2081195A4 (en) 2010-05-05

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