CA2544728A1 - Cathode material for a high-temperature fuel cell (sofc) and a cathode that can be produced therefrom - Google Patents

Cathode material for a high-temperature fuel cell (sofc) and a cathode that can be produced therefrom Download PDF

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Publication number
CA2544728A1
CA2544728A1 CA002544728A CA2544728A CA2544728A1 CA 2544728 A1 CA2544728 A1 CA 2544728A1 CA 002544728 A CA002544728 A CA 002544728A CA 2544728 A CA2544728 A CA 2544728A CA 2544728 A1 CA2544728 A1 CA 2544728A1
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CA
Canada
Prior art keywords
cathode
delta
fuel cell
grain size
cathode material
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Abandoned
Application number
CA002544728A
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English (en)
French (fr)
Inventor
Hans Peter Buchkremer
Frank Tietz
Andreas Mai
Detlev Stoever
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Forschungszentrum Jülich
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Individual
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Filing date
Publication date
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Publication of CA2544728A1 publication Critical patent/CA2544728A1/en
Abandoned legal-status Critical Current

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    • H—ELECTRICITY
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    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8878—Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8882—Heat treatment, e.g. drying, baking
    • H01M4/8885—Sintering or firing
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • C—CHEMISTRY; METALLURGY
    • C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
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    • C04B35/00—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/01—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics
    • C04B35/26—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics based on ferrites
    • C04B35/2608—Compositions containing one or more ferrites of the group comprising manganese, zinc, nickel, copper or cobalt and one or more ferrites of the group comprising rare earth metals, alkali metals, alkaline earth metals or lead
    • C04B35/2633—Compositions containing one or more ferrites of the group comprising manganese, zinc, nickel, copper or cobalt and one or more ferrites of the group comprising rare earth metals, alkali metals, alkaline earth metals or lead containing barium, strontium or calcium
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    • C04B35/00—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/01—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics
    • C04B35/26—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics based on ferrites
    • C04B35/2641—Compositions containing one or more ferrites of the group comprising rare earth metals and one or more ferrites of the group comprising alkali metals, alkaline earth metals or lead
    • C—CHEMISTRY; METALLURGY
    • C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
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    • C04B35/00—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/50—Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on rare-earth compounds
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    • C04B38/00—Porous mortars, concrete, artificial stone or ceramic ware; Preparation thereof
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9033—Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
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    • C04B2111/00—Mortars, concrete or artificial stone or mixtures to prepare them, characterised by specific function, property or use
    • C04B2111/00241—Physical properties of the materials not provided for elsewhere in C04B2111/00
    • C04B2111/00413—Materials having an inhomogeneous concentration of ingredients or irregular properties in different layers
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    • C04B2111/00—Mortars, concrete or artificial stone or mixtures to prepare them, characterised by specific function, property or use
    • C04B2111/00474—Uses not provided for elsewhere in C04B2111/00
    • C04B2111/00853—Uses not provided for elsewhere in C04B2111/00 in electrochemical cells or batteries, e.g. fuel cells
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3205—Alkaline earth oxides or oxide forming salts thereof, e.g. beryllium oxide
    • C04B2235/3208—Calcium oxide or oxide-forming salts thereof, e.g. lime
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3205—Alkaline earth oxides or oxide forming salts thereof, e.g. beryllium oxide
    • C04B2235/3213—Strontium oxides or oxide-forming salts thereof
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3224—Rare earth oxide or oxide forming salts thereof, e.g. scandium oxide
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3224—Rare earth oxide or oxide forming salts thereof, e.g. scandium oxide
    • C04B2235/3229—Cerium oxides or oxide-forming salts thereof
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    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/327—Iron group oxides, their mixed metal oxides, or oxide-forming salts thereof
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    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/327—Iron group oxides, their mixed metal oxides, or oxide-forming salts thereof
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    • C04B2235/00—Aspects relating to ceramic starting mixtures or sintered ceramic products
    • C04B2235/02—Composition of constituents of the starting material or of secondary phases of the final product
    • C04B2235/30—Constituents and secondary phases not being of a fibrous nature
    • C04B2235/32—Metal oxides, mixed metal oxides, or oxide-forming salts thereof, e.g. carbonates, nitrates, (oxy)hydroxides, chlorides
    • C04B2235/3281—Copper oxides, cuprates or oxide-forming salts thereof, e.g. CuO or Cu2O
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    • H—ELECTRICITY
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    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M2004/8678—Inert electrodes with catalytic activity, e.g. for fuel cells characterised by the polarity
    • H01M2004/8689—Positive electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Ceramic Engineering (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Organic Chemistry (AREA)
  • Structural Engineering (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Physics & Mathematics (AREA)
  • Thermal Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Inert Electrodes (AREA)
CA002544728A 2003-11-07 2004-11-04 Cathode material for a high-temperature fuel cell (sofc) and a cathode that can be produced therefrom Abandoned CA2544728A1 (en)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE10351955.6 2003-11-07
DE10351955A DE10351955A1 (de) 2003-11-07 2003-11-07 Kathodenwerkstoff für eine Hochtemperatur-Brennstoffzelle (SOFC) sowie eine daraus herstellbare Kathode
PCT/DE2004/002443 WO2005045979A2 (de) 2003-11-07 2004-11-04 Kathodenwerkstoff für eine hochtemperatur-brennstoffzelle (sofc) sowie eine daraus herstellbare kathode

Publications (1)

Publication Number Publication Date
CA2544728A1 true CA2544728A1 (en) 2005-05-19

Family

ID=34559436

Family Applications (1)

Application Number Title Priority Date Filing Date
CA002544728A Abandoned CA2544728A1 (en) 2003-11-07 2004-11-04 Cathode material for a high-temperature fuel cell (sofc) and a cathode that can be produced therefrom

Country Status (9)

Country Link
US (1) US20070148529A1 (cg-RX-API-DMAC7.html)
EP (1) EP1680832A2 (cg-RX-API-DMAC7.html)
JP (1) JP2007538354A (cg-RX-API-DMAC7.html)
KR (1) KR20060120675A (cg-RX-API-DMAC7.html)
CN (1) CN1902778A (cg-RX-API-DMAC7.html)
AU (1) AU2004307760A1 (cg-RX-API-DMAC7.html)
CA (1) CA2544728A1 (cg-RX-API-DMAC7.html)
DE (1) DE10351955A1 (cg-RX-API-DMAC7.html)
WO (1) WO2005045979A2 (cg-RX-API-DMAC7.html)

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JP2010536146A (ja) * 2007-08-08 2010-11-25 コーニング インコーポレイテッド 固体酸化物型燃料電池装置用の複合空気極
JP5133787B2 (ja) * 2008-06-09 2013-01-30 日本電信電話株式会社 固体酸化物形燃料電池
ES2331828B2 (es) 2008-06-27 2011-08-08 Universidad Politecnica De Valencia Capa catalitica para la activacion de oxigeno sobre electrolitos solidos ionicos a alta temperatura.
US8124037B2 (en) * 2009-12-11 2012-02-28 Delphi Technologies, Inc. Perovskite materials for solid oxide fuel cell cathodes
KR101177621B1 (ko) * 2010-06-25 2012-08-27 한국생산기술연구원 고체산화물 연료전지 단위셀의 제조방법
WO2012144785A2 (ko) 2011-04-18 2012-10-26 주식회사 엘지화학 양극 활물질 및 그것을 포함한 리튬 이차전지
JP4962640B1 (ja) * 2011-07-22 2012-06-27 大日本印刷株式会社 固体酸化物形燃料電池
JP5882857B2 (ja) * 2012-07-30 2016-03-09 京セラ株式会社 固体酸化物形燃料電池セルおよびセルスタック装置ならびに燃料電池モジュール
JP6780920B2 (ja) * 2015-06-19 2020-11-04 森村Ｓｏｆｃテクノロジー株式会社 燃料電池単セルおよび燃料電池スタック
JP6110524B2 (ja) * 2016-01-27 2017-04-05 京セラ株式会社 固体酸化物形燃料電池セルおよびセルスタック装置ならびに燃料電池モジュール
JP6356852B2 (ja) * 2017-03-08 2018-07-11 京セラ株式会社 固体酸化物形燃料電池セルおよびセルスタック装置ならびに燃料電池モジュール
JP7134646B2 (ja) * 2018-02-28 2022-09-12 株式会社ノリタケカンパニーリミテド 固体酸化物形燃料電池とこれに用いる電極材料
JP7115873B2 (ja) * 2018-02-28 2022-08-09 株式会社ノリタケカンパニーリミテド 固体酸化物形燃料電池とこれに用いる電極材料
JP6585774B2 (ja) * 2018-06-12 2019-10-02 京セラ株式会社 固体酸化物形燃料電池セルおよびセルスタック装置ならびに燃料電池モジュール
CN113302771A (zh) * 2018-11-17 2021-08-24 环球公用事业公司 制备电化学反应器的方法
US20200388854A1 (en) * 2019-05-28 2020-12-10 The Regents Of The University Of Michigan Cermet electrode for solid state and lithium ion batteries
KR102376399B1 (ko) 2020-07-30 2022-03-18 울산과학기술원 페로브스카이트 물질로 구성된 전극 소재, 그를 포함하는 고체 산화물 연료전지, 금속공기전지, 및 고체 산화물 수전해 셀

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US6632554B2 (en) * 2001-04-10 2003-10-14 Hybrid Power Generation Systems, Llc High performance cathodes for solid oxide fuel cells
JP3661676B2 (ja) * 2001-11-07 2005-06-15 東陶機器株式会社 固体電解質型燃料電池
JP3827209B2 (ja) * 2001-12-19 2006-09-27 日本電信電話株式会社 固体電解質型燃料電池用複合型空気極の作製方法

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CN1902778A (zh) 2007-01-24
AU2004307760A1 (en) 2005-05-19
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WO2005045979A3 (de) 2006-06-22
EP1680832A2 (de) 2006-07-19

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