BR112013016686A2 - composição de resina epóxi, processo para a preparação de uma composição, composição curável, material de poliisocianurato e poliuretano, processo para frabricar um material de poliisocianurato e poliuretano, e, uso de um composto - Google Patents
composição de resina epóxi, processo para a preparação de uma composição, composição curável, material de poliisocianurato e poliuretano, processo para frabricar um material de poliisocianurato e poliuretano, e, uso de um compostoInfo
- Publication number
- BR112013016686A2 BR112013016686A2 BR112013016686A BR112013016686A BR112013016686A2 BR 112013016686 A2 BR112013016686 A2 BR 112013016686A2 BR 112013016686 A BR112013016686 A BR 112013016686A BR 112013016686 A BR112013016686 A BR 112013016686A BR 112013016686 A2 BR112013016686 A2 BR 112013016686A2
- Authority
- BR
- Brazil
- Prior art keywords
- composition
- polyisocyanurate
- polyurethane material
- epoxy resin
- compound
- Prior art date
Links
- 239000000203 mixture Substances 0.000 title abstract 10
- 239000003822 epoxy resin Substances 0.000 title abstract 5
- 229920000647 polyepoxide Polymers 0.000 title abstract 5
- 238000004519 manufacturing process Methods 0.000 title abstract 4
- 239000000463 material Substances 0.000 title abstract 4
- 239000011495 polyisocyanurate Substances 0.000 title abstract 4
- 229920000582 polyisocyanurate Polymers 0.000 title abstract 4
- 239000004814 polyurethane Substances 0.000 title abstract 4
- 229920002635 polyurethane Polymers 0.000 title abstract 4
- 150000001875 compounds Chemical class 0.000 title abstract 3
- 238000000034 method Methods 0.000 title abstract 2
- -1 lithium halide Chemical class 0.000 abstract 3
- 239000004202 carbamide Substances 0.000 abstract 2
- 239000012948 isocyanate Substances 0.000 abstract 2
- 150000002513 isocyanates Chemical class 0.000 abstract 2
- 229910052744 lithium Inorganic materials 0.000 abstract 2
- 239000005056 polyisocyanate Substances 0.000 abstract 2
- 229920001228 polyisocyanate Polymers 0.000 abstract 2
- XSQUKJJJFZCRTK-UHFFFAOYSA-N Urea Chemical compound NC(N)=O XSQUKJJJFZCRTK-UHFFFAOYSA-N 0.000 abstract 1
- OHJMTUPIZMNBFR-UHFFFAOYSA-N biuret Chemical compound NC(=O)NC(N)=O OHJMTUPIZMNBFR-UHFFFAOYSA-N 0.000 abstract 1
- 125000005392 carboxamide group Chemical group NC(=O)* 0.000 abstract 1
- 229920005862 polyol Polymers 0.000 abstract 1
- 150000003077 polyols Chemical class 0.000 abstract 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/16—Nitrogen-containing compounds
- C08K5/20—Carboxylic acid amides
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/08—Processes
- C08G18/09—Processes comprising oligomerisation of isocyanates or isothiocyanates involving reaction of a part of the isocyanate or isothiocyanate groups with each other in the reaction mixture
- C08G18/092—Processes comprising oligomerisation of isocyanates or isothiocyanates involving reaction of a part of the isocyanate or isothiocyanate groups with each other in the reaction mixture oligomerisation to isocyanurate groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/08—Processes
- C08G18/16—Catalysts
- C08G18/22—Catalysts containing metal compounds
- C08G18/225—Catalysts containing metal compounds of alkali or alkaline earth metals
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/30—Low-molecular-weight compounds
- C08G18/38—Low-molecular-weight compounds having heteroatoms other than oxygen
- C08G18/3819—Low-molecular-weight compounds having heteroatoms other than oxygen having nitrogen
- C08G18/3823—Low-molecular-weight compounds having heteroatoms other than oxygen having nitrogen containing -N-C=O groups
- C08G18/3829—Low-molecular-weight compounds having heteroatoms other than oxygen having nitrogen containing -N-C=O groups containing ureum groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/40—High-molecular-weight compounds
- C08G18/4009—Two or more macromolecular compounds not provided for in one single group of groups C08G18/42 - C08G18/64
- C08G18/4045—Mixtures of compounds of group C08G18/58 with other macromolecular compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/40—High-molecular-weight compounds
- C08G18/48—Polyethers
- C08G18/4804—Two or more polyethers of different physical or chemical nature
- C08G18/4812—Mixtures of polyetherdiols with polyetherpolyols having at least three hydroxy groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/72—Polyisocyanates or polyisothiocyanates
- C08G18/77—Polyisocyanates or polyisothiocyanates having heteroatoms in addition to the isocyanate or isothiocyanate nitrogen and oxygen or sulfur
- C08G18/78—Nitrogen
- C08G18/7806—Nitrogen containing -N-C=0 groups
- C08G18/7818—Nitrogen containing -N-C=0 groups containing ureum or ureum derivative groups
- C08G18/7825—Nitrogen containing -N-C=0 groups containing ureum or ureum derivative groups containing ureum groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/72—Polyisocyanates or polyisothiocyanates
- C08G18/77—Polyisocyanates or polyisothiocyanates having heteroatoms in addition to the isocyanate or isothiocyanate nitrogen and oxygen or sulfur
- C08G18/78—Nitrogen
- C08G18/7806—Nitrogen containing -N-C=0 groups
- C08G18/7818—Nitrogen containing -N-C=0 groups containing ureum or ureum derivative groups
- C08G18/7831—Nitrogen containing -N-C=0 groups containing ureum or ureum derivative groups containing biuret groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
- C08G18/72—Polyisocyanates or polyisothiocyanates
- C08G18/77—Polyisocyanates or polyisothiocyanates having heteroatoms in addition to the isocyanate or isothiocyanate nitrogen and oxygen or sulfur
- C08G18/78—Nitrogen
- C08G18/79—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates
- C08G18/791—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates containing isocyanurate groups
- C08G18/792—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates containing isocyanurate groups formed by oligomerisation of aliphatic and/or cycloaliphatic isocyanates or isothiocyanates
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L63/00—Compositions of epoxy resins; Compositions of derivatives of epoxy resins
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L75/00—Compositions of polyureas or polyurethanes; Compositions of derivatives of such polymers
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G2115/00—Oligomerisation
- C08G2115/02—Oligomerisation to isocyanurate groups
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- Polyurethanes Or Polyureas (AREA)
- Epoxy Resins (AREA)
Abstract
composição de resina epóxi, processo para a preparação de uma composição, composição curável, material de poliisocianurato e poliuretano, processo para frabricar um material de poliisocianurato e poliuretano, e, uso de um composto composição curável, obtida por combinação e mistura de uma composição de resina epóxi compreendendo uma resina epóxi, um monool e/ou poliol e um composto compreendendo um grupo carboxamida, e uma composição de poliisocianato compreendendo um poliisocianato, um halogeneto de lítio e um composto de ureia, em que o número de moles de halogeneto de lítio por equivalentes de isocianato varia de 0,0001 a 0,04 e o número de equivalentes de ureia + biureto por equivalente de isocianato varia de 0,0001 a 0,4. a composição de resina epóxi é também reivindicada.
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
EP11152720.6 | 2011-01-31 | ||
EP11152720 | 2011-01-31 | ||
PCT/EP2011/069562 WO2012103965A1 (en) | 2011-01-31 | 2011-11-07 | Epoxy resin composition |
Publications (2)
Publication Number | Publication Date |
---|---|
BR112013016686A2 true BR112013016686A2 (pt) | 2016-10-04 |
BR112013016686B1 BR112013016686B1 (pt) | 2020-07-07 |
Family
ID=44315244
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
BR112013016686-0A BR112013016686B1 (pt) | 2011-01-31 | 2011-11-07 | composição de resina epóxi, processo para a preparação de uma composição, composição curável, material de poliisocianurato-poliuretano, processo para fabricar um material de poliisocianurato- poliuretano, e, uso de um composto |
Country Status (11)
Country | Link |
---|---|
US (2) | US20130303694A1 (pt) |
EP (1) | EP2670784B1 (pt) |
JP (1) | JP2014503668A (pt) |
KR (1) | KR20140012987A (pt) |
CN (1) | CN103391953B (pt) |
BR (1) | BR112013016686B1 (pt) |
CA (1) | CA2820786C (pt) |
PL (1) | PL2670784T3 (pt) |
RU (1) | RU2560434C2 (pt) |
TW (1) | TWI509016B (pt) |
WO (1) | WO2012103965A1 (pt) |
Families Citing this family (9)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US9926447B2 (en) * | 2011-11-22 | 2018-03-27 | Huntsman International Llc | Curable polyisocyanate composition comprising an epoxy |
EP2687551A1 (en) * | 2012-07-17 | 2014-01-22 | Huntsman International Llc | Intermediate polyisocyanurate comprising materials |
EP2805976A1 (en) * | 2013-05-24 | 2014-11-26 | Huntsman International Llc | Aldehyde comprising compositions suitable for making curable polyisocyanate compositions |
ES2860673T3 (es) * | 2013-11-29 | 2021-10-05 | Basf Se | Sistema de poliuretano con un largo tiempo de tratamiento y un curado rápido. |
WO2016188774A1 (en) * | 2015-05-27 | 2016-12-01 | Basf Se | Use of a composition for stabilizing a geological formation in oil fields, gas fields, water pumping fields, mining or tunnel constructions |
US10781284B2 (en) | 2015-05-28 | 2020-09-22 | Basf Se | Polyurethane-polyisocyanurate compound comprising outstanding mechanical properties |
CN107683297B (zh) * | 2015-05-29 | 2020-09-08 | 巴斯夫欧洲公司 | 用于纤维复合材料的具有较长开放时间的聚氨酯-聚异氰脲酸酯树脂 |
WO2020165135A1 (en) | 2019-02-11 | 2020-08-20 | Basf Se | Acrylic copolymer capsule designed to open up at < 90°c for controlled release of in-situ forming pu/pir catalyst |
KR20220049564A (ko) | 2019-08-19 | 2022-04-21 | 바스프 에스이 | 기계적 성질이 우수한 폴리우레탄-폴리이소시아누레이트 화합물 |
Family Cites Families (28)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE1230778B (de) | 1965-05-24 | 1966-12-22 | Bayer Ag | Verfahren zur Herstellung von acylierten Harnstoffpolyisocyanaten |
GB1340068A (en) | 1970-09-22 | 1973-12-05 | Insituform Pipes & Structures | Lining of surfaces defining passageways |
DE2403858A1 (de) | 1974-01-28 | 1975-08-21 | Basf Ag | Stabile, fluessige amid- und/oder acylharnstoffgruppenhaltige isocyanurat-polyisocyanatloesungen |
GB1463809A (en) * | 1974-04-25 | 1977-02-09 | Ici Ltd | Polymeric materials |
US4002598A (en) * | 1975-03-06 | 1977-01-11 | Texaco Development Corporation | Polyether urea epoxy curing agent |
DE2843739C3 (de) * | 1978-10-06 | 1982-04-22 | Bayer Ag, 5090 Leverkusen | Verfahren zur Herstellung von im wesentlichen homogenen Polyurethan-Elastomeren |
SU887595A1 (ru) * | 1980-02-07 | 1981-12-07 | Ленинградская Ордена Ленина Лесотехническая Академия Им.С.М.Кирова | Препрег |
JPS56133856A (en) * | 1980-03-21 | 1981-10-20 | Nitto Electric Ind Co Ltd | Epoxy resin composition for sealing semiconductor |
US4366012A (en) | 1981-02-05 | 1982-12-28 | Insituform International Inc. | Impregnation process |
DE3151591A1 (de) * | 1981-12-28 | 1983-07-14 | Lechler Chemie Gmbh, 7000 Stuttgart | Haertbare kunstharzmischungen und mittel fuer haertbare kunstharzmischungen auf basis von praepolymeren polyaetherurethanharnstoffaminen und epoxidharzen und/oder aromatischen carbamidsaeurearylestern |
JPS58145721A (ja) * | 1982-02-24 | 1983-08-30 | Hitachi Ltd | 樹脂組成物の硬化方法 |
GB8400365D0 (en) | 1984-01-07 | 1984-02-08 | Edgealpha Ltd | Lining of pipelines and passageways |
US4658007A (en) | 1985-05-07 | 1987-04-14 | The Dow Chemical Company | Polyisocyanurate-based polyoxazolidone polymers and process for their preparation |
JPS62161817A (ja) * | 1986-01-10 | 1987-07-17 | Hitachi Chem Co Ltd | エポキシ樹脂組成物 |
JPH02110123A (ja) | 1988-10-19 | 1990-04-23 | Asahi Chem Ind Co Ltd | ポリイソシアナートの製法 |
DE3932958A1 (de) | 1989-10-03 | 1991-04-11 | Bayer Ag | Verfahren zur herstellung licht- und abgasbestaendiger puh-elastomerfaeden und -folien und elastomerfaeden entsprechender zusammensetzung |
IT1252690B (it) | 1991-11-26 | 1995-06-23 | Donegani Guido Ist | Composizioni reattive liquide comprendenti poliisocianati, epossidi e soluzioni di alogenuri di metalli alcalini in composti poliossialchilenici |
DE4229183A1 (de) | 1992-09-02 | 1994-03-03 | Basf Ag | Verfahren zur Herstellung von niedrigviskosen Isocyanurat- und Urethangruppen enthaltenden Polyisocyanatmischungen |
JPH08157569A (ja) * | 1994-10-06 | 1996-06-18 | Hitachi Chem Co Ltd | 印刷配線板用エポキシ樹脂組成物 |
US20030134971A1 (en) * | 1996-09-30 | 2003-07-17 | Blount David H. | Amino catalyst for polyurethane products |
US5854309A (en) * | 1996-09-30 | 1998-12-29 | Blount; David H. | Flame retardant compositions utilizing amino condensation compounds |
GB2332202A (en) * | 1997-12-09 | 1999-06-16 | Courtaulds Coatings | Curable epoxy resin compositions |
EP1989242B1 (en) | 2006-02-21 | 2010-07-21 | Huntsman International Llc | Process for making a polyisocyanurate composite |
EP2045278A1 (de) * | 2007-10-05 | 2009-04-08 | Bayer MaterialScience AG | Verfahren zur Herstellung von Polyurethan-Schäumen |
JP5268934B2 (ja) | 2006-12-04 | 2013-08-21 | ビーエーエスエフ ソシエタス・ヨーロピア | ポリイソシアネートを製造するための方法 |
HUE041930T2 (hu) | 2007-03-27 | 2019-06-28 | Basf Se | Eljárás diizocianátok színtelen izocianurátjainak elõállítására |
WO2010121898A1 (en) * | 2009-04-21 | 2010-10-28 | Huntsman International Llc | Polyisocyanate composition |
JP2013506745A (ja) * | 2009-10-05 | 2013-02-28 | コンストラクション リサーチ アンド テクノロジー ゲーエムベーハー | 高い生強度およびガンアビリティを有するポリウレタン配合物 |
-
2011
- 2011-11-07 KR KR1020137023104A patent/KR20140012987A/ko not_active Application Discontinuation
- 2011-11-07 CA CA2820786A patent/CA2820786C/en active Active
- 2011-11-07 JP JP2013550779A patent/JP2014503668A/ja active Pending
- 2011-11-07 RU RU2013140400/05A patent/RU2560434C2/ru active
- 2011-11-07 BR BR112013016686-0A patent/BR112013016686B1/pt not_active IP Right Cessation
- 2011-11-07 PL PL11778926T patent/PL2670784T3/pl unknown
- 2011-11-07 WO PCT/EP2011/069562 patent/WO2012103965A1/en active Application Filing
- 2011-11-07 CN CN201180066372.9A patent/CN103391953B/zh active Active
- 2011-11-07 US US13/979,156 patent/US20130303694A1/en not_active Abandoned
- 2011-11-07 EP EP11778926.3A patent/EP2670784B1/en active Active
- 2011-11-10 TW TW100141101A patent/TWI509016B/zh not_active IP Right Cessation
-
2018
- 2018-10-10 US US16/156,086 patent/US10689503B2/en active Active
Also Published As
Publication number | Publication date |
---|---|
PL2670784T3 (pl) | 2015-11-30 |
EP2670784A1 (en) | 2013-12-11 |
CA2820786A1 (en) | 2012-08-09 |
US20130303694A1 (en) | 2013-11-14 |
US10689503B2 (en) | 2020-06-23 |
CN103391953A (zh) | 2013-11-13 |
JP2014503668A (ja) | 2014-02-13 |
EP2670784B1 (en) | 2015-06-17 |
RU2560434C2 (ru) | 2015-08-20 |
CA2820786C (en) | 2015-11-03 |
BR112013016686B1 (pt) | 2020-07-07 |
RU2013140400A (ru) | 2015-03-10 |
CN103391953B (zh) | 2016-06-01 |
KR20140012987A (ko) | 2014-02-04 |
US20190040230A1 (en) | 2019-02-07 |
WO2012103965A1 (en) | 2012-08-09 |
TWI509016B (zh) | 2015-11-21 |
TW201231543A (en) | 2012-08-01 |
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