WO2008093731A1 - 燃料電池用電極触媒およびこれを用いた燃料電池 - Google Patents

燃料電池用電極触媒およびこれを用いた燃料電池 Download PDF

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Publication number
WO2008093731A1
WO2008093731A1 PCT/JP2008/051406 JP2008051406W WO2008093731A1 WO 2008093731 A1 WO2008093731 A1 WO 2008093731A1 JP 2008051406 W JP2008051406 W JP 2008051406W WO 2008093731 A1 WO2008093731 A1 WO 2008093731A1
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WIPO (PCT)
Prior art keywords
electrode
fuel cell
catalyst
fuel
electrode catalyst
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PCT/JP2008/051406
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English (en)
French (fr)
Inventor
Akari Hayashi
Ichizo Yagi
Ken'ichi Kimijima
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National Institute Of Advanced Industrial Science And Technology
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Publication date
Application filed by National Institute Of Advanced Industrial Science And Technology filed Critical National Institute Of Advanced Industrial Science And Technology
Priority to EP08704169A priority Critical patent/EP2117068A4/en
Priority to US12/525,627 priority patent/US20100092830A1/en
Priority to JP2008556149A priority patent/JPWO2008093731A1/ja
Publication of WO2008093731A1 publication Critical patent/WO2008093731A1/ja

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9075—Catalytic material supported on carriers, e.g. powder carriers
    • H01M4/9083—Catalytic material supported on carriers, e.g. powder carriers on carbon or graphite
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H01M4/925—Metals of platinum group supported on carriers, e.g. powder carriers
    • H01M4/926—Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M2008/1095—Fuel cells with polymeric electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Inert Electrodes (AREA)
  • Catalysts (AREA)

Abstract

　従来のようにシリカテンプレートを用いることなく簡便なプロセスで効率的に得られ、しかもメソ細孔径が比較的大きく（５nm以上）、かつその細孔内に安定に触媒粒子を担持でき、高度な三相界面状態が容易に発現し得る、燃料電池用電極触媒を提供する。 　このような燃料電池用電極触媒は、界面活性剤とカーボン前駆体の混合物を加熱・焼成炭化することにより得られるカーボンメソ多孔体担体と、該担体に担持された触媒粒子から構成される。また燃料極と、空気極と、この両極に介在する電解質膜とを備え、前記燃料極および空気極の少なくとも一つが上記電極触媒を含有する燃料電池を得ることもできる。
PCT/JP2008/051406 2007-02-01 2008-01-30 燃料電池用電極触媒およびこれを用いた燃料電池 WO2008093731A1 (ja)

Priority Applications (3)

Application Number Priority Date Filing Date Title
EP08704169A EP2117068A4 (en) 2007-02-01 2008-01-30 ELECTRODE CATALYST FOR FUEL CELL AND FUEL CELL USING THE ELECTRODE CATALYST
US12/525,627 US20100092830A1 (en) 2007-02-01 2008-01-30 Electrode catalyst for a fuel cell, and fuel cell using the same
JP2008556149A JPWO2008093731A1 (ja) 2007-02-01 2008-01-30 燃料電池用電極触媒およびこれを用いた燃料電池

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007023252 2007-02-01
JP2007-023252 2007-02-01

Publications (1)

Publication Number Publication Date
WO2008093731A1 true WO2008093731A1 (ja) 2008-08-07

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Family Applications (1)

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PCT/JP2008/051406 WO2008093731A1 (ja) 2007-02-01 2008-01-30 燃料電池用電極触媒およびこれを用いた燃料電池

Country Status (4)

Country Link
US (1) US20100092830A1 (ja)
EP (1) EP2117068A4 (ja)
JP (1) JPWO2008093731A1 (ja)
WO (1) WO2008093731A1 (ja)

Cited By (13)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2010084773A1 (ja) * 2009-01-23 2010-07-29 株式会社エクォス・リサーチ 燃料電池用触媒層及びそれに使用する触媒
JP2010167379A (ja) * 2009-01-23 2010-08-05 Equos Research Co Ltd 触媒及び燃料電池用触媒層
JP2010186678A (ja) * 2009-02-13 2010-08-26 Equos Research Co Ltd 燃料電池用触媒層
WO2012053638A1 (ja) * 2010-10-22 2012-04-26 日産自動車株式会社 固体高分子型燃料電池用電極触媒
JP2012096235A (ja) * 2012-02-08 2012-05-24 Toshiba Corp 静電霧化装置
JPWO2010131535A1 (ja) * 2009-05-13 2012-11-01 日本電気株式会社 触媒電極、燃料電池、空気電池および発電方法
WO2013073383A1 (ja) * 2011-11-17 2013-05-23 日産自動車株式会社 燃料電池用電極触媒層
JP2013178927A (ja) * 2012-02-28 2013-09-09 Nissan Motor Co Ltd 燃料電池
WO2014175106A1 (ja) * 2013-04-25 2014-10-30 日産自動車株式会社 電極、並びにこれを含む燃料電池用電極触媒層
WO2019017399A1 (ja) * 2017-07-19 2019-01-24 国立研究開発法人産業技術総合研究所 アンモニア合成触媒
JP2020517059A (ja) * 2017-04-13 2020-06-11 バラード パワー システムズ インコーポレイテッド 改善された結合力を有する膜電極アセンブリ
WO2022137985A1 (ja) 2020-12-24 2022-06-30 富士フイルム株式会社 内視鏡用可撓管、内視鏡型医療機器、及びこれらの製造方法
WO2022181261A1 (ja) * 2021-02-26 2022-09-01 三井金属鉱業株式会社 電極触媒及びその製造方法並びに燃料電池

Families Citing this family (33)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US7723262B2 (en) 2005-11-21 2010-05-25 Energ2, Llc Activated carbon cryogels and related methods
US7835136B2 (en) 2006-11-15 2010-11-16 Energ2, Inc. Electric double layer capacitance device
US8293818B2 (en) 2009-04-08 2012-10-23 Energ2 Technologies, Inc. Manufacturing methods for the production of carbon materials
CN105226284B (zh) 2009-07-01 2017-11-28 巴斯夫欧洲公司 超纯合成碳材料
US8916296B2 (en) 2010-03-12 2014-12-23 Energ2 Technologies, Inc. Mesoporous carbon materials comprising bifunctional catalysts
WO2012045002A1 (en) 2010-09-30 2012-04-05 Energ2 Technologies, Inc. Enhanced packing of energy storage particles
CN103370756B (zh) 2010-12-28 2018-05-11 巴斯福股份公司 包含增强的电化学特性的碳材料
US20120262127A1 (en) 2011-04-15 2012-10-18 Energ2 Technologies, Inc. Flow ultracapacitor
US20120286216A1 (en) * 2011-05-12 2012-11-15 Headwaters Technology Innovation, Llc Methods for mitigating agglomeration of carbon nanospheres using a long chain hydrocarbon surfactant
CN103947017B (zh) 2011-06-03 2017-11-17 巴斯福股份公司 用于混合能量存储装置中的碳‑铅共混物
US9409777B2 (en) 2012-02-09 2016-08-09 Basf Se Preparation of polymeric resins and carbon materials
JP2015513570A (ja) 2012-02-09 2015-05-14 ジョージア − パシフィック ケミカルズ エルエルシー ポリマ樹脂および炭素材料の調製
CN103682379B (zh) * 2012-09-07 2016-08-03 中国科学院大连化学物理研究所 一种燃料电池用金属掺杂的含氮炭基催化剂及其应用
US9714172B2 (en) 2012-11-26 2017-07-25 Georgia-Pacific Chemicals Llc Preparation of polymeric resins and carbon materials
KR20140085738A (ko) * 2012-12-27 2014-07-08 현대자동차주식회사 탄소가 포함된 막대형 실리카 미세입자의 제조방법
WO2014143213A1 (en) 2013-03-14 2014-09-18 Energ2 Technologies, Inc. Composite carbon materials comprising lithium alloying electrochemical modifiers
US10573901B2 (en) * 2013-04-25 2020-02-25 Tanaka Kikinzoku Kogyo K.K. Catalyst and manufacturing method thereof, and electrode catalyst layer using the catalyst
WO2014175098A1 (ja) 2013-04-25 2014-10-30 日産自動車株式会社 触媒ならびに当該触媒を用いる電極触媒層、膜電極接合体および燃料電池
US10195583B2 (en) 2013-11-05 2019-02-05 Group 14 Technologies, Inc. Carbon-based compositions with highly efficient volumetric gas sorption
WO2015137980A1 (en) 2014-03-14 2015-09-17 Energ2 Technologies, Inc. Novel methods for sol-gel polymerization in absence of solvent and creation of tunable carbon structure from same
JP6358680B2 (ja) * 2014-09-01 2018-07-18 国立大学法人 東京大学 共有結合性有機構造体を含む導電性ハイブリッド材料
EP3214679B1 (en) 2014-10-29 2019-12-25 Nissan Motor Co., Ltd Electrode catalyst layer for fuel cell, manufacturing method for same, and membrane electrode assembly and fuel cell using same
US10763501B2 (en) 2015-08-14 2020-09-01 Group14 Technologies, Inc. Nano-featured porous silicon materials
EP4286355A3 (en) 2015-08-28 2024-05-01 Group14 Technologies, Inc. Novel materials with extremely durable intercalation of lithium and manufacturing methods thereof
US20180222781A1 (en) * 2017-02-09 2018-08-09 California Institute Of Technology Water purification using porous carbon electrode
WO2018165610A1 (en) 2017-03-09 2018-09-13 Group 14 Technologies, Inc. Decomposition of silicon-containing precursors on porous scaffold materials
CA3167109A1 (en) * 2020-02-10 2021-08-19 Toshihiro Miyao Supported metal catalyst, method for producing same, and method for producing carrier
US11639292B2 (en) 2020-08-18 2023-05-02 Group14 Technologies, Inc. Particulate composite materials
US11335903B2 (en) 2020-08-18 2022-05-17 Group14 Technologies, Inc. Highly efficient manufacturing of silicon-carbon composites materials comprising ultra low z
US11174167B1 (en) 2020-08-18 2021-11-16 Group14 Technologies, Inc. Silicon carbon composites comprising ultra low Z
US11777107B2 (en) 2020-09-28 2023-10-03 Hyzon Motors Inc. Gas-solid reduction process for preparation of platinum-containing catalysts for fuel cells
CN112349918B (zh) * 2020-11-06 2023-03-10 昆明理工大学 一种热解壳聚糖制备氮掺杂铂碳催化剂的方法及应用
CN115925054B (zh) * 2022-10-31 2023-12-19 南京工业大学 一种膜泡相合成炭电极复合材料制备方法和应用

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2004071253A (ja) 2002-08-02 2004-03-04 Toyota Motor Corp 燃料電池用電極触媒及び燃料電池
JP2004178859A (ja) * 2002-11-25 2004-06-24 Aisin Seiki Co Ltd 触媒の製造方法および燃料電池
JP2006228502A (ja) * 2005-02-16 2006-08-31 Mitsui Chemicals Inc 燃料電池用電極触媒とその製造方法およびそれを用いた電極と燃料電池
JP2006321712A (ja) 2005-05-18 2006-11-30 Samsung Sdi Co Ltd メソ細孔性炭素体とその製造方法、担持触媒および燃料電池

Family Cites Families (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6248691B1 (en) * 1998-02-10 2001-06-19 Corning Incorporated Method of making mesoporous carbon
EP1109738A4 (en) * 1998-07-20 2010-08-11 Corning Inc PROCESS FOR MAKING MESOPOROUS CARBON USING POROGENIC COMPOUNDS
US6297293B1 (en) * 1999-09-15 2001-10-02 Tda Research, Inc. Mesoporous carbons and polymers

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2004071253A (ja) 2002-08-02 2004-03-04 Toyota Motor Corp 燃料電池用電極触媒及び燃料電池
JP2004178859A (ja) * 2002-11-25 2004-06-24 Aisin Seiki Co Ltd 触媒の製造方法および燃料電池
JP2006228502A (ja) * 2005-02-16 2006-08-31 Mitsui Chemicals Inc 燃料電池用電極触媒とその製造方法およびそれを用いた電極と燃料電池
JP2006321712A (ja) 2005-05-18 2006-11-30 Samsung Sdi Co Ltd メソ細孔性炭素体とその製造方法、担持触媒および燃料電池

Non-Patent Citations (3)

* Cited by examiner, † Cited by third party
Title
CHEM. COMMUN., 2005, pages 2125 - 2127
KONOSUKE IKEDA: "EVERYTHING IN FUEL CELLS", NIPPON JITSUGYO PUBLISHING, pages: 138 - 139
See also references of EP2117068A4

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JP2010167379A (ja) * 2009-01-23 2010-08-05 Equos Research Co Ltd 触媒及び燃料電池用触媒層
WO2010084773A1 (ja) * 2009-01-23 2010-07-29 株式会社エクォス・リサーチ 燃料電池用触媒層及びそれに使用する触媒
JP2010186678A (ja) * 2009-02-13 2010-08-26 Equos Research Co Ltd 燃料電池用触媒層
JPWO2010131535A1 (ja) * 2009-05-13 2012-11-01 日本電気株式会社 触媒電極、燃料電池、空気電池および発電方法
WO2012053638A1 (ja) * 2010-10-22 2012-04-26 日産自動車株式会社 固体高分子型燃料電池用電極触媒
WO2012053303A1 (ja) * 2010-10-22 2012-04-26 日産自動車株式会社 固体高分子型燃料電池用電極触媒
US9799903B2 (en) 2010-10-22 2017-10-24 Nissan Motor Co., Ltd. Electrocatalyst for solid polymer fuel cell
WO2013073383A1 (ja) * 2011-11-17 2013-05-23 日産自動車株式会社 燃料電池用電極触媒層
JP2013109856A (ja) * 2011-11-17 2013-06-06 Nissan Motor Co Ltd 燃料電池用電極触媒層
CN104094460A (zh) * 2011-11-17 2014-10-08 日产自动车株式会社 燃料电池用电极催化剂层
US10547075B2 (en) 2011-11-17 2020-01-28 Nissan Motor Co., Ltd. Electrode catalyst layer for fuel cell
JP2012096235A (ja) * 2012-02-08 2012-05-24 Toshiba Corp 静電霧化装置
JP2013178927A (ja) * 2012-02-28 2013-09-09 Nissan Motor Co Ltd 燃料電池
CN105163849A (zh) * 2013-04-25 2015-12-16 日产自动车株式会社 电极以及含有该电极的电极催化剂层
CN105163849B (zh) * 2013-04-25 2018-10-26 日产自动车株式会社 催化剂以及含有该催化剂的电极催化剂层
WO2014175106A1 (ja) * 2013-04-25 2014-10-30 日産自動車株式会社 電極、並びにこれを含む燃料電池用電極触媒層
JP2020517059A (ja) * 2017-04-13 2020-06-11 バラード パワー システムズ インコーポレイテッド 改善された結合力を有する膜電極アセンブリ
US11355759B2 (en) 2017-04-13 2022-06-07 Ballard Power Systems Inc. Membrane electrode assembly with improved cohesion
JP7203039B2 (ja) 2017-04-13 2023-01-12 バラード パワー システムズ インコーポレイテッド 改善された結合力を有する膜電極アセンブリ
WO2019017399A1 (ja) * 2017-07-19 2019-01-24 国立研究開発法人産業技術総合研究所 アンモニア合成触媒
JPWO2019017399A1 (ja) * 2017-07-19 2020-04-16 国立研究開発法人産業技術総合研究所 アンモニア合成触媒
WO2022137985A1 (ja) 2020-12-24 2022-06-30 富士フイルム株式会社 内視鏡用可撓管、内視鏡型医療機器、及びこれらの製造方法
WO2022181261A1 (ja) * 2021-02-26 2022-09-01 三井金属鉱業株式会社 電極触媒及びその製造方法並びに燃料電池
JPWO2022181261A1 (ja) * 2021-02-26 2022-09-01
JP7418656B2 (ja) 2021-02-26 2024-01-19 三井金属鉱業株式会社 電極触媒及びその製造方法並びに燃料電池

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EP2117068A4 (en) 2010-04-14
EP2117068A1 (en) 2009-11-11
JPWO2008093731A1 (ja) 2010-05-20
US20100092830A1 (en) 2010-04-15

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