KR970042908A - 전자부품용 액체 접착제 및 접착 테이프 - Google Patents

전자부품용 액체 접착제 및 접착 테이프 Download PDF

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Publication number
KR970042908A
KR970042908A KR1019960072505A KR19960072505A KR970042908A KR 970042908 A KR970042908 A KR 970042908A KR 1019960072505 A KR1019960072505 A KR 1019960072505A KR 19960072505 A KR19960072505 A KR 19960072505A KR 970042908 A KR970042908 A KR 970042908A
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South Korea
Prior art keywords
component
weight
liquid adhesive
formula
adhesive
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KR1019960072505A
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English (en)
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KR100403949B1 (ko
Inventor
다께시 하시모토
가쭈지 나까바
준 도찌하라
Original Assignee
호소이 소지로
도모에가와 페이퍼 캄파니 리미티드
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Priority claimed from JP07351086A external-priority patent/JP3118404B2/ja
Priority claimed from JP17294696A external-priority patent/JP3118420B2/ja
Application filed by 호소이 소지로, 도모에가와 페이퍼 캄파니 리미티드 filed Critical 호소이 소지로
Publication of KR970042908A publication Critical patent/KR970042908A/ko
Application granted granted Critical
Publication of KR100403949B1 publication Critical patent/KR100403949B1/ko

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    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F8/00—Chemical modification by after-treatment
    • C08F8/42—Introducing metal atoms or metal-containing groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F8/00—Chemical modification by after-treatment
    • C08F8/30—Introducing nitrogen atoms or nitrogen-containing groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/16—Nitrogen-containing compounds
    • C08K5/34—Heterocyclic compounds having nitrogen in the ring
    • C08K5/3412—Heterocyclic compounds having nitrogen in the ring having one nitrogen atom in the ring
    • C08K5/3415—Five-membered rings
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/54—Silicon-containing compounds
    • C08K5/544—Silicon-containing compounds containing nitrogen
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J109/00—Adhesives based on homopolymers or copolymers of conjugated diene hydrocarbons
    • C09J109/02—Copolymers with acrylonitrile
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J11/00—Features of adhesives not provided for in group C09J9/00, e.g. additives
    • C09J11/02—Non-macromolecular additives
    • C09J11/06—Non-macromolecular additives organic
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J161/00—Adhesives based on condensation polymers of aldehydes or ketones; Adhesives based on derivatives of such polymers
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J161/00—Adhesives based on condensation polymers of aldehydes or ketones; Adhesives based on derivatives of such polymers
    • C09J161/04—Condensation polymers of aldehydes or ketones with phenols only
    • C09J161/06—Condensation polymers of aldehydes or ketones with phenols only of aldehydes with phenols
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
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    • C09J163/00—Adhesives based on epoxy resins; Adhesives based on derivatives of epoxy resins
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J179/00—Adhesives based on macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing nitrogen, with or without oxygen, or carbon only, not provided for in groups C09J161/00 - C09J177/00
    • C09J179/02—Polyamines
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    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J183/00—Adhesives based on macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon, with or without sulfur, nitrogen, oxygen, or carbon only; Adhesives based on derivatives of such polymers
    • C09J183/04—Polysiloxanes
    • C09J183/08—Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen, and oxygen
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    • C09J7/00—Adhesives in the form of films or foils
    • C09J7/20—Adhesives in the form of films or foils characterised by their carriers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
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    • C08K5/17—Amines; Quaternary ammonium compounds
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    • C08K5/18—Amines; Quaternary ammonium compounds with aromatically bound amino groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L2666/00—Composition of polymers characterized by a further compound in the blend, being organic macromolecular compounds, natural resins, waxes or and bituminous materials, non-macromolecular organic substances, inorganic substances or characterized by their function in the composition
    • C08L2666/02—Organic macromolecular compounds, natural resins, waxes or and bituminous materials
    • C08L2666/14—Macromolecular compounds according to C08L59/00 - C08L87/00; Derivatives thereof
    • C08L2666/16—Addition or condensation polymers of aldehydes or ketones according to C08L59/00 - C08L61/00; Derivatives thereof
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L61/00—Compositions of condensation polymers of aldehydes or ketones; Compositions of derivatives of such polymers
    • C08L61/04—Condensation polymers of aldehydes or ketones with phenols only
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    • C09J2203/00—Applications of adhesives in processes or use of adhesives in the form of films or foils
    • C09J2203/326—Applications of adhesives in processes or use of adhesives in the form of films or foils for bonding electronic components such as wafers, chips or semiconductors
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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • General Chemical & Material Sciences (AREA)
  • Adhesives Or Adhesive Processes (AREA)

Abstract

비교적 낮은 온도에서 결합용으로 이용할 수 있으며 경화될 수 있고 충분한 내열성 및 신뢰도를 갖는 전자 부품용 접착제 및 상기 접착제를 이용한 전자 부품용 접착테이프에 관한 것으로 상기 접착제는 유기 용매에 성분(a)로서 아크릴로니트릴-부타디엔 공중합체, 성분(b)로서 페놀 수지,성분 (c)로서 최소 2개의 말레이미드기를 갖는 화합물 및 성분(d)로서 청구범위 제1항에서 일반식(1)의 디아민 화합물 및 또는 각 말단이 아미노기로 종결되고 중량 평균 분자량이 200∼7,000이며 청구범위 제1항에서 일반식(2)의 폴리실록산 화합물을 용해시켜 제조되며, 상기 성분(a) 100중량부당 성분(b),(c) 및 (d)의 총중량은 10-900 중량부 상기 성분 (b),(c) 및 (d)의 총중량을 기준으로 성분(b)의 양은 10∼90 중량%이며, 성분(c)의 말레이미드가 1몰당량 성분(d)의 아미노기의 양은 0.01∼2.0몰 당량인 액체 접착제가 제공된다.

Description

전자부품용 액체 접착제 및 접착 테이프
본 내용은 요부공개 건이므로 전문내용을 수록하지 않았음

Claims (13)

  1. 유기 용매에 성분(a)로서 아크릴로니트릴-부타디엔 공중합체, 성분(b)로서 페놀 수지, 성분(c)로서 최소 2개의 말레이미드기를 갖는 화합물 및 성분(d)로서 하기식(1)의 디아민 화합물 및 또는 각 말단이 아미노기로 종결되고 중량 평균 분자량이 200∼7,000이며 하기식(2)의 폴리실록산 화합물을 용해시켜 제조되며, 상기 성분(a) 100중량부당 성분(b).(c), 및 (d)의 총중량은 10-900 중량부 성분 b).(c), 및 (d)의 총중량을 기준으로 성분(b)의 양은 10∼90 중량%이며 성분(c)의 말레이미드가 1몰당량당 성분(d)의 아미노기의 양은 0.01∼2.0몰당량인 전자 부품용 액체 접착제
    [화학식 1]
    (단, 상기 식에서 R1은 2가 지방족,방향족 혹은 지방족 고리기이다.)
    [화학식 2]
    (단, 상기 식에서 R2은 2가 지방족,방향족 혹은 지방족 고리기이며, n은 0-7의 정수이다.)
  2. 제1항에 있어서, 상기 액체 접착제는 나이가 성분(e)로서 에폭시 수지를 함유하며, 성분(a) 100중량부당 성분(b),(c),(d) 및 (e)의 총중량은 10∼900중량부, 성분(b),(c),(d) 및 (e)의 총중량을 기준으로 성분(b)와 (e)의 총중량은 10∼90중량%이며, 성분(c)의 말레이미드가 1몰당량당 성분(d)의 아미노기의 양은 0.01∼2.0몰 당량임을 특징으로 하는 액체 접착제.
  3. 제1항에 있어서, 성분(a)로서 아크릴로니트릴-부타디엔 공중합체의 중량 평균 분자량은 50,000∼1,000,000이고 아크릴로니트릴의 함량은 5∼50중량%임을 특징으로 하는 액체 접착제.
  4. 제1항에 있어서, 성분(b)로서 페놀수지는 p-tert-부틸페놀형 페놀 수지,비스페놀 A형 페놀수지 혹은 크레졸형 페놀수지로부터 선택되며 상기 페놀수지의 페놀성분은 p-tert-부틸페놀, 비스페놀 A 및 크레졸 혹은 이들의 공-축합으로 제조된 레졸형 페놀수지로 구성되는 그룹으로부터 선택된 최소 일종임을 특징으로 하는 액체 접착제.
  5. 제1항에 있어서, 성분(c)로서 최소 2개의 말레이미드계를 갖는 화합물은 하기식 (3a) 내지 (3f)으로 부터 선택됨을 특징으로 하는 액체 접착제.
    [화학식 3a]
    [화학식 3b]
    [화학식 3c]
    [화학식 3d]
    (단, 상기식에서 p는 0-7의 정수이다.)
    [화학식 3e]
    [화학식 3f]
    (단, 상기식에서 MI= R = H 혹은 CH3 이고 r = 1-5이다)
  6. 제2항에 있어서, 성분(e)로서 에폭시 수지는 노볼락형 에폭시 수지, 비닐페놀형 에폭시 수지,비스페놀형 에폭시 수지와 비페닐형 에폭시 수지의 혼합물로 구성되는 그룹으로부터 선택된 최소 하나의 에폭시 수지임을 특징으로 하는 액체접착제.
  7. 제1항에 있어서, 상기 액체 접착제는 나아가 입자 직경이 1um 미만인 충진제를 총고형분의 함량을 기준으로 4∼40중량%를 함유하는 특징으로 하는 액체 접착제.
  8. 제1항의 액체 접착제를 내열성 피막의 최소 일면에 적용하고 상기 액체 접착제를 건조하여 형성된 접착층을 갖는 전자부품용 접착테이프로
  9. 제8항에 있어서, 상기 내열성 피막은 폴리아미드 피막임을 특징으로 하는 접착테이프
  10. 제1항의 액체 접착제를 분리형 피막의 최소 일면에 적용하고 상기 액체 접착제를 건조하여 형성된 접착층을 갖는 전자부품용 접착테이프
  11. 리드 프레임의 고정에 청구범위 제1항의 액체 접착제를 사용하는 방법.
  12. 리드 프레임의 고정에 청구범위 제8항의 접착 테이프를 사용하는 방법.
  13. 리드 프레임의 고정에 청구범위 제10항의 접착 테이프를 사용하는 방법.
KR1019960072505A 1995-12-25 1996-12-26 전자부품용액체접착제및접착테이프 KR100403949B1 (ko)

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JP351086/95 1995-12-25
JP07351086A JP3118404B2 (ja) 1995-12-25 1995-12-25 電子部品用液状接着剤および接着テープ
JP172946/96 1996-06-12
JP17294696A JP3118420B2 (ja) 1996-06-12 1996-06-12 電子部品用液状接着剤および接着テープ

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KR100625054B1 (ko) * 2000-05-04 2006-09-18 주식회사 코오롱 내열성 접착테이프
KR100642678B1 (ko) * 2004-07-13 2006-11-10 가부시키가이샤 도모에가와 세이시쇼 전자부품용 접착테이프 및 전자부품
KR100707732B1 (ko) * 2001-10-29 2007-04-16 주식회사 코오롱 전자부품용 접착액 및 접착테이프

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KR100613754B1 (ko) * 2000-01-18 2006-08-22 주식회사 코오롱 내열성 접착테이프
KR100625054B1 (ko) * 2000-05-04 2006-09-18 주식회사 코오롱 내열성 접착테이프
KR100707732B1 (ko) * 2001-10-29 2007-04-16 주식회사 코오롱 전자부품용 접착액 및 접착테이프
KR100642678B1 (ko) * 2004-07-13 2006-11-10 가부시키가이샤 도모에가와 세이시쇼 전자부품용 접착테이프 및 전자부품

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