KR880006050A - 적층물 - Google Patents

적층물 Download PDF

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Publication number
KR880006050A
KR880006050A KR870012568A KR870012568A KR880006050A KR 880006050 A KR880006050 A KR 880006050A KR 870012568 A KR870012568 A KR 870012568A KR 870012568 A KR870012568 A KR 870012568A KR 880006050 A KR880006050 A KR 880006050A
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South Korea
Prior art keywords
flame retardant
containing flame
monomer
iii
monomers
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KR870012568A
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English (en)
Inventor
후미오 마쯔이
노보루 스즈끼
미노루 다까이시
류우시 오구라
노리아끼 하리가이
타다요시 하시모또
도모에 우에마투
Original Assignee
무라다 가즈
쇼와덴꼬 가부시끼가이샤
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Priority claimed from JP26612986A external-priority patent/JPS63120713A/ja
Priority claimed from JP26612186A external-priority patent/JPS63118311A/ja
Priority claimed from JP27007186A external-priority patent/JPS63122719A/ja
Priority claimed from JP27006986A external-priority patent/JPS63124494A/ja
Priority claimed from JP27244186A external-priority patent/JPS63125503A/ja
Priority claimed from JP4890287A external-priority patent/JPS63218722A/ja
Priority claimed from JP4890487A external-priority patent/JPS63218721A/ja
Priority claimed from JP4890387A external-priority patent/JPS63218720A/ja
Priority claimed from JP9203687A external-priority patent/JPS63258916A/ja
Priority claimed from JP9203587A external-priority patent/JPS63258915A/ja
Priority claimed from JP20089887A external-priority patent/JPS6445418A/ja
Priority claimed from JP20089787A external-priority patent/JPS6445417A/ja
Priority claimed from JP20089587A external-priority patent/JPS6445415A/ja
Priority claimed from JP20089687A external-priority patent/JPS6445416A/ja
Application filed by 무라다 가즈, 쇼와덴꼬 가부시끼가이샤 filed Critical 무라다 가즈
Publication of KR880006050A publication Critical patent/KR880006050A/ko

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    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • C08F299/00—Macromolecular compounds obtained by interreacting polymers involving only carbon-to-carbon unsaturated bond reactions, in the absence of non-macromolecular monomers
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    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/24—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/24—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs
    • C08J5/247—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs using fibres of at least two types
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    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/24—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs
    • C08J5/249—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs characterised by the additives used in the prepolymer mixture
    • H—ELECTRICITY
    • H05—ELECTRIC TECHNIQUES NOT OTHERWISE PROVIDED FOR
    • H05K—PRINTED CIRCUITS; CASINGS OR CONSTRUCTIONAL DETAILS OF ELECTRIC APPARATUS; MANUFACTURE OF ASSEMBLAGES OF ELECTRICAL COMPONENTS
    • H05K1/00—Printed circuits
    • H05K1/02—Details
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B32—LAYERED PRODUCTS
    • B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B2260/00—Layered product comprising an impregnated, embedded, or bonded layer wherein the layer comprises an impregnation, embedding, or binder material
    • B32B2260/02—Composition of the impregnated, bonded or embedded layer
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B32—LAYERED PRODUCTS
    • B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B2260/00—Layered product comprising an impregnated, embedded, or bonded layer wherein the layer comprises an impregnation, embedding, or binder material
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    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B32B2305/00—Condition, form or state of the layers or laminate
    • B32B2305/72—Cured, e.g. vulcanised, cross-linked
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    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
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    • C08J2333/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Derivatives of such polymers
    • C08J2333/04—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Derivatives of such polymers esters
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    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
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    • Y10T428/31504—Composite [nonstructural laminate]
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    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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    • Y10T428/31551—Of polyamidoester [polyurethane, polyisocyanate, polycarbamate, etc.]
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Abstract

내용 없음

Description

적층물
본 내용은 요부공개 건이므로 전문내용을 수록하지 않았음

Claims (21)

  1. (i) 주성분으로서, 필수적으로 비닐 단량체와 아크릴 도는 메타크릴 단량체의 랜덤 공중합체로 구성되는 주쇄, 및 말단에 아크릴로일 또는 메타크릴로일 그룹을 함유하는 측쇄를 갖는 경화성 프레폴리머(prepolymer), 및 (ii) 교차 결합성 비닐 단량체로 이루어진 경화성 조성물로 함침되고, 적층되고 경화된 기판으로 이루어지는 적층물(laminate).
  2. 제1항에 있어서, 경화성 프레폴리머가 다음 일반식(I)로 표시되는 적층물.
    상기식에서, A는 비닐 단량체와 아크릴로일 도는 메타크릴로일 단량체의 랜덤 공중합체로 구성된 주쇄를 나타내며, R1내지 R3는 각각 수소원자 또는 메틸그룹을 나타내고, n은 0 또는 1내지 5의 정수이다.
  3. 제1항에 있어서, 경화성 프레폴리머가 다음 일반식(Ⅱ)로 표시되는 적층물.
    상기식에서 A는 비닐 단량체와 아크릴로일 또는 메타크릴로일 단량체의 램덤 공중합체로 구성된 주쇄를 나타내며, X1및 X2는 각각 탄소수 1 내지 16의 탄화수소 그룹 또는 에테르 결합을 통해 연결되고 총 탄소수가 1 내지 16인 탄화수소 그룹을 나타내고, B는 탄소수 20이하의 지방족, 지환족 또는 방향족 탄화수소 그룹을 나타내며, L1및 L2는 각각 -O- 또는 -NH-를 나타내고, R4는 수소원자 또는 메틸그룹을 나타낸다.
  4. 제1항에 있어서, 경화성 프레폴리머가 다음 일반식(Ⅲ)으로 표시되는 적층물.
    상기식에서 A는 비닐 단량체와 아크릴로일 또는 메타크릴로일 단량체의 랜덤 공중합체로 구성된 주쇄를 나타내며, R5는 수소원자 또는 메틸 그룹을 나타낸다.
  5. 제1항에 있어서, 경화성 조성물중의 경화성 프레폴리머의 비율이 10 내지 60중량%인 적층물.
  6. 제2항에 있어서, 경화성 조성물중의 경화성 프레폴리머의 비율이 10 내지 60중량%인 적층물.
  7. 제3항에 있어서, 경화성 조성물중의 경화성 프레폴리머의 비율이 10 내지 60중량%인 적층물.
  8. 제4항에 있어서, 경화성 조성물중의 경화성 프레폴리머의 비율이 10 내지 60중량%인 적층물.
  9. 제5항에 있어서, 교차 결합성 비닐 단량체가 일작용성 단량체와 다작용성 단량체의 혼합물이며, 일작용성 단량체에 대한 다작용성 단량체의 중량비가 1/20 내지 1/2인 적층물.
  10. 제6항에 있어서, 교차 결합성 비닐 단량체가 일작용성 단량체와 다작용성 단량체의 혼합물이며, 일작용성 단량체에 대한 다작용성 단량체의 중량비가 1/20 내지 1/2인 적층물.
  11. 제7항에 있어서, 교차 결합성 비닐 단량체가 일작용성 단량체와 다작용성 단량체의 혼합물이며, 일작용성 단량체에 대한 다작용성 단량체의 중량비가 1/20 내지 1/2인 적층물.
  12. 제8항에 있어서, 교차 결합성 비닐 단량체가 일작용성 단량체와 다작용성 단량체의 혼합물이며, 일작용성 단량체에 대한 다작용성 단량체의 중량비가 1/20 내지 1/2인 적층물.
  13. 제5항에 있어서, 경화성 조성물이 추가로(i)포화 다염기산과, 탄소수 1 내지 18의 브롬 또는 염소-함유 지방족 또는 지환족 포화탄화수소 그룹을 갖는 다가 알콜과의 에스테르에 모노글리시딜 메타크릴레이트 또는 모노글리시딜 아크릴레이트를 부가반응시켜 생성된 할로겐-함유 난연성 단량체, (ii) 일반식(Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (iii) 일반식(ⅩI)의 염소-함유 난연성 단량체로 구성된 그룹중에서 선택된 할로겐-함유 난연성 단량체 5 내지 70중량%를 함유하는 적층물.
    상기식에서 R11, R12, R13및 R15는 각각 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  14. 제6항에 있어서, 경화성 조성물이 추가로(i) 포화 다염기산과, 탄소수 1 내지 18의 브롬 또는 염소-함유 지방족 또는 지환족 포화탄화수소 그룹을 갖는 다가 알콜과의 에스테르에 모노글리시딜 메타크릴레이트 또는 모노글리시딜 아크릴레이트를 부가반응시켜 생성된 할로겐-함유 난연성 단량체, (ii) 일반식 (Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (iii) 일반식(ⅩI)의 염소-함유 난연성 단량체로 구성된 그룹중에서 선택된 할로겐-함유 난연성 단량체 5 내지 70중량%를 함유하는 적층물.
    상기식에서 R11, R12, R13및 R15는 각각 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  15. 제7항에 있어서, 경화성 조성물이 추가로(i)포화 다염기산과, 탄소수 1 내지 18의 브롬 또는 염소-함유 지방족 또는 지환족 포화탄화수소 그룹을 갖는 다가 알콜과의 에스테르에 모노글리시딜 메타크릴레이트 또는 모노글리시딜 아크릴레이트를 부가반응시켜 생성된 할로겐-함유 난연성 단량체, (ii) 일반식(Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (iii) 일반식(ⅩI)의 염소-함유 난연성 단량체로 구성된 그룹중에서 선택된 할로겐-함유 난연성 단량체 5 내지 70중량%를 함유하는 적층물.
    상기식에서 R11, R12, R13및 R15는 각각 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  16. 제8항에 있어서, 경화성 조성물이 추가로(i)포화 다염기산과, 탄소수 1 내지 18의 브롬 또는 염소-함유 지방족 또는 지환족 포화탄화수소 그룹을 갖는 다가 알콜과의 에스테르에 모노글리시딜 메타크릴레이트 또는 모노글리시딜 아크릴레이트를 부가반응시켜 생성된 할로겐-함유 난연성 단량체, (ii) 일반식(Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (iii) 일반식(ⅩI)의 염소-함유 난연성 단량체로 구성된 그룹중에서 선택된 할로겐-함유 난연성 단량체 5 내지 70중량%를 함유하는 적층물.
    상기식에서 R11, R12, R13및 R15는 각각 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  17. 제5항에 있어서, 할로겐-함유 난연성 단량체가 (i)적어도 하나의 (Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (ii) 일반식(ⅩI)의 염소-함유 난연성 단량체의 혼합물이며, 염소-함유 난연성 단량체의 양은 브롬-함유 난연성 단량체의 총량을 기준으로 하여 50 내지 200중량%인 적층물.
    상기식에서 R11, R12, 및 R13은 각각 수소원자 또는 메틸 그룹을 나타내고, R15는 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  18. 제6항에 있어서, 할로겐-함유 난연성 단량체가 (i)적어도 하나의 (Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (ii) 일반식(ⅩI)의 염소-함유 난연성 단량체의 혼합물이며, 염소-함유 난연성 단량체의 양은 브롬-함유 난연성 단량체의 총량을 기준으로 하여 50 내지 200중량%인 적층물.
    상기식에서 R11, R12, 및 R13은 각각 수소원자 또는 메틸 그룹을 나타내고, R15는 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  19. 제7항에 있어서, 할로겐-함유 난연성 단량체가 (i)적어도 하나의 (Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (ii) 일반식(ⅩI)의 염소-함유 난연성 단량체의 혼합물이며, 염소-함유 난연성 단량체의 양은 브롬-함유 난연성 단량체의 총량을 기준으로 하여 50 내지 200중량%인 적층물.
    상기식에서 R11, R12, 및 R13은 각각 수소원자 또는 메틸 그룹을 나타내고, R15는 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  20. 제8항에 있어서, 할로겐-함유 난연성 단량체가 (i)적어도 하나의 (Ⅷ) 및 (Ⅸ)의 브롬-함유 난연성 단량체, 및 (ii) 일반식(ⅩI)의 염소-함유 난연성 단량체의 혼합물이며, 염소-함유 난연성 단량체의 양은 브롬-함유 난연성 단량체의 총량을 기준으로 하여 50 내지 200중량%인 적층물.
    상기식에서 R11, R12, 및 R13은 각각 수소원자 또는 메틸 그룹을 나타내고, R15는 수소원자 또는 메틸 그룹을 나타내고, n2는 1 내지 10의 정수를 나타낸다.
  21. 제5항에 있어서, 교차 결합성 단량체로서 일반식(ⅩⅡ)의 유연성-부여 단량체를 교차결합성 단량체를 총중량을 기준으로 하여 0.1 내지 40중량%의 양으로 함유하는 적층물.
    상기식에서, R16은 수소원자 또는 메틸그룹을 나타내고, R17은 탄소수 2 내지 5의 2가 지방족 탄화수소 그룹을 나타내며, R18은 수소원자 또는 탄소수 1 내지 10의 탄화수소 그룹을 나타내고, n3는 1 내지 20의 정수를 나타낸다.
    ※ 참고사항 : 최초출원 내용에 의하여 공개하는 것임.
KR870012568A 1986-11-07 1987-11-07 적층물 KR880006050A (ko)

Applications Claiming Priority (28)

Application Number Priority Date Filing Date Title
JP26612986A JPS63120713A (ja) 1986-11-07 1986-11-07 電気用積層板用樹脂組成物
JP266129 1986-11-07
JP266121 1986-11-07
JP26612186A JPS63118311A (ja) 1986-11-07 1986-11-07 電気用積層板用樹脂組成物
JP270069 1986-11-13
JP270071 1986-11-13
JP27006986A JPS63124494A (ja) 1986-11-13 1986-11-13 電気回路用積層板及びその製造方法
JP27007186A JPS63122719A (ja) 1986-11-13 1986-11-13 ラジカル硬化可能な樹脂組成物及び積層板
JP272441 1986-11-14
JP27244186A JPS63125503A (ja) 1986-11-14 1986-11-14 ラジカル硬化可能な共重合体樹脂およびその組成物と製造方法
JP48903 1987-03-05
JP48902 1987-03-05
JP4890487A JPS63218721A (ja) 1987-03-05 1987-03-05 積層板用樹脂組成物
JP48904 1987-03-05
JP4890287A JPS63218722A (ja) 1987-03-05 1987-03-05 積層板用樹脂組成物
JP4890387A JPS63218720A (ja) 1987-03-05 1987-03-05 積層板用樹脂組成物
JP92035 1987-04-16
JP9203687A JPS63258916A (ja) 1987-04-16 1987-04-16 電気用積層板用樹脂組成物
JP9203587A JPS63258915A (ja) 1987-04-16 1987-04-16 電気用積層板用樹脂組成物
JP92036 1987-04-16
JP20089887A JPS6445418A (en) 1987-08-13 1987-08-13 Polymer composition for laminated board for electrical use
JP200896 1987-08-13
JP200897 1987-08-13
JP20089787A JPS6445417A (en) 1987-08-13 1987-08-13 Polymer composition for laminated board for electrical use
JP20089587A JPS6445415A (en) 1987-08-13 1987-08-13 Polymer composition for laminated board for electrical use
JP20089687A JPS6445416A (en) 1987-08-13 1987-08-13 Polymer composition for laminated board for electrical use
JP200898 1987-08-13
JP200895 1988-08-11

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