KR102085903B1 - 스피넬 재료의 제조 - Google Patents

스피넬 재료의 제조 Download PDF

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KR102085903B1
KR102085903B1 KR1020157005781A KR20157005781A KR102085903B1 KR 102085903 B1 KR102085903 B1 KR 102085903B1 KR 1020157005781 A KR1020157005781 A KR 1020157005781A KR 20157005781 A KR20157005781 A KR 20157005781A KR 102085903 B1 KR102085903 B1 KR 102085903B1
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powder
lithium
manganese
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KR20150056542A (ko
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케니쓰 이케추쿠 오조에메나
찰 제레미 자프타
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씨에스아이알
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    • CCHEMISTRY; METALLURGY
    • C30CRYSTAL GROWTH
    • C30BSINGLE-CRYSTAL GROWTH; UNIDIRECTIONAL SOLIDIFICATION OF EUTECTIC MATERIAL OR UNIDIRECTIONAL DEMIXING OF EUTECTOID MATERIAL; REFINING BY ZONE-MELTING OF MATERIAL; PRODUCTION OF A HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; SINGLE CRYSTALS OR HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; AFTER-TREATMENT OF SINGLE CRYSTALS OR A HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; APPARATUS THEREFOR
    • C30B1/00Single-crystal growth directly from the solid state
    • C30B1/02Single-crystal growth directly from the solid state by thermal treatment, e.g. strain annealing
    • C30B1/04Isothermal recrystallisation
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01GCOMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
    • C01G53/00Compounds of nickel
    • C01G53/40Complex oxides containing nickel and at least one other metal element
    • C01G53/42Complex oxides containing nickel and at least one other metal element containing alkali metals, e.g. LiNiO2
    • C01G53/44Complex oxides containing nickel and at least one other metal element containing alkali metals, e.g. LiNiO2 containing manganese
    • C01G53/54Complex oxides containing nickel and at least one other metal element containing alkali metals, e.g. LiNiO2 containing manganese of the type (Mn2O4)-, e.g. Li(NixMn2-x)O4 or Li(MyNixMn2-x-y)O4
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    • C30CRYSTAL GROWTH
    • C30BSINGLE-CRYSTAL GROWTH; UNIDIRECTIONAL SOLIDIFICATION OF EUTECTIC MATERIAL OR UNIDIRECTIONAL DEMIXING OF EUTECTOID MATERIAL; REFINING BY ZONE-MELTING OF MATERIAL; PRODUCTION OF A HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; SINGLE CRYSTALS OR HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; AFTER-TREATMENT OF SINGLE CRYSTALS OR A HOMOGENEOUS POLYCRYSTALLINE MATERIAL WITH DEFINED STRUCTURE; APPARATUS THEREFOR
    • C30B29/00Single crystals or homogeneous polycrystalline material with defined structure characterised by the material or by their shape
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    • C30B30/00Production of single crystals or homogeneous polycrystalline material with defined structure characterised by the action of electric or magnetic fields, wave energy or other specific physical conditions
    • C30B30/02Production of single crystals or homogeneous polycrystalline material with defined structure characterised by the action of electric or magnetic fields, wave energy or other specific physical conditions using electric fields, e.g. electrolysis
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M4/36Selection of substances as active materials, active masses, active liquids
    • H01M4/48Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/50Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese
    • H01M4/505Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese of mixed oxides or hydroxides containing manganese for inserting or intercalating light metals, e.g. LiMn2O4 or LiMn2OxFy
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M4/36Selection of substances as active materials, active masses, active liquids
    • H01M4/48Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/52Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron
    • H01M4/525Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron of mixed oxides or hydroxides containing iron, cobalt or nickel for inserting or intercalating light metals, e.g. LiNiO2, LiCoO2 or LiCoOxFy
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    • C01INORGANIC CHEMISTRY
    • C01PINDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00Crystal-structural characteristics
    • C01P2002/30Three-dimensional structures
    • C01P2002/32Three-dimensional structures spinel-type (AB2O4)
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    • C01P2002/00Crystal-structural characteristics
    • C01P2002/50Solid solutions
    • C01P2002/52Solid solutions containing elements as dopants
    • C01P2002/54Solid solutions containing elements as dopants one element only
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    • C01P2002/70Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data
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    • C01P2002/70Crystal-structural characteristics defined by measured X-ray, neutron or electron diffraction data
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    • C01PINDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2002/00Crystal-structural characteristics
    • C01P2002/80Crystal-structural characteristics defined by measured data other than those specified in group C01P2002/70
    • C01P2002/85Crystal-structural characteristics defined by measured data other than those specified in group C01P2002/70 by XPS, EDX or EDAX data
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    • C01INORGANIC CHEMISTRY
    • C01PINDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
    • C01P2004/00Particle morphology
    • C01P2004/01Particle morphology depicted by an image
    • C01P2004/03Particle morphology depicted by an image obtained by SEM
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    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
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    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M2004/026Electrodes composed of, or comprising, active material characterised by the polarity
    • H01M2004/028Positive electrodes
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10Energy storage using batteries

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • General Chemical & Material Sciences (AREA)
  • Physics & Mathematics (AREA)
  • Thermal Sciences (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Inorganic Compounds Of Heavy Metals (AREA)
KR1020157005781A 2012-08-10 2013-07-25 스피넬 재료의 제조 Active KR102085903B1 (ko)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
ZA2012/06016 2012-08-10
ZA201206016 2012-08-10
PCT/IB2013/056103 WO2014024075A1 (en) 2012-08-10 2013-07-25 Production of a spinel material

Publications (2)

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KR20150056542A KR20150056542A (ko) 2015-05-26
KR102085903B1 true KR102085903B1 (ko) 2020-03-06

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US (1) US9834854B2 (enExample)
EP (1) EP2882690B1 (enExample)
JP (1) JP6316812B2 (enExample)
KR (1) KR102085903B1 (enExample)
CN (1) CN104703920A (enExample)
AR (1) AR092069A1 (enExample)
BR (1) BR112015002884B1 (enExample)
CA (1) CA2880876C (enExample)
WO (1) WO2014024075A1 (enExample)
ZA (1) ZA201501121B (enExample)

Families Citing this family (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
BR112017000017A2 (pt) * 2014-07-03 2018-11-06 Csir produção de material óxido de lítio, manganês, níquel e cobalto, em camadas
US9979011B2 (en) * 2014-09-26 2018-05-22 The United States Of America As Represented By The Secretary Of The Army LixMn2O4-y(C1z) spinal cathode material, method of preparing the same, and rechargeable lithium and li-ion electrochemical systems containing the same
US20180277844A1 (en) * 2014-10-31 2018-09-27 Csir Production of a Spinel Material
US10505188B2 (en) * 2015-03-03 2019-12-10 The Government Of The United States As Represented By The Secretary Of The Army “B” and “O” site doped AB2O4 spinel cathode material, method of preparing the same, and rechargeable lithium and Li-ion electrochemical systems containing the same
US20180375097A1 (en) * 2015-12-22 2018-12-27 Csir Spinel material
CN105576231A (zh) * 2016-02-25 2016-05-11 江南大学 一种具有尖晶石结构的高电压锂离子电池正极材料及其制备方法
WO2017163922A1 (ja) 2016-03-24 2017-09-28 富士フイルム株式会社 感活性光線性又は感放射線性組成物、感活性光線性又は感放射線性組成物の精製方法、パターン形成方法、及び電子デバイスの製造方法
JPWO2017164018A1 (ja) 2016-03-24 2018-11-08 富士フイルム株式会社 感活性光線性又は感放射線性組成物、感活性光線性又は感放射線性組成物の精製方法、感活性光線性又は感放射線性組成物の製造方法、パターン形成方法、及び電子デバイスの製造方法
JPWO2017163816A1 (ja) 2016-03-24 2018-12-13 富士フイルム株式会社 感活性光線性又は感放射線性組成物、感活性光線性又は感放射線性組成物の製造方法、パターン形成方法、及び電子デバイスの製造方法
US10516156B2 (en) * 2016-05-25 2019-12-24 The Government Of The United States As Represented By The Secretary Of The Army Chlorinated lithium manganese oxide spinel cathode material with charge transfer catalyst coating, method of preparing the same, and Li electrochemical cell containing the same
KR101963251B1 (ko) * 2017-10-17 2019-03-29 한국과학기술연구원 양극 활물질 제조방법 및 이를 이용한 이차전지
CN114369863B (zh) * 2021-12-08 2023-02-14 中国科学院地球化学研究所 一种高温高压下制备锰铝榴石单晶的方法

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2000281355A (ja) 1999-03-29 2000-10-10 Nippon Chem Ind Co Ltd リチウム複合酸化物の製造方法
JP2011210463A (ja) * 2010-03-29 2011-10-20 Jx Nippon Mining & Metals Corp リチウムイオン電池用正極活物質の製造方法

Family Cites Families (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CA1331506C (en) * 1988-07-12 1994-08-23 Michael Makepeace Thackeray Method of synthesizing a lithium manganese oxide
CN1042377C (zh) * 1996-05-10 1999-03-03 中国科学院物理研究所 一种合成锂离子电池中正极材料的方法
JP2973299B2 (ja) * 1996-06-27 1999-11-08 本荘ケミカル株式会社 スピネル型構造を有するリチウム−マンガン複合酸化物の製造方法
US6348182B1 (en) * 1996-06-27 2002-02-19 The Honjo Chemical Corporation Process for producing lithium manganese oxide with spinel structure
JP3411488B2 (ja) * 1997-12-01 2003-06-03 本荘ケミカル株式会社 リチウムイオン二次電池用正極活物質の製造方法
JP4726896B2 (ja) * 2005-04-28 2011-07-20 日産自動車株式会社 非水電解質リチウムイオン電池用正極材料およびこれを用いた電池
US8496855B2 (en) * 2009-07-27 2013-07-30 Samsung Electronics Co., Ltd. Cathode active material, cathode including cathode active material, and lithium battery including cathode

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2000281355A (ja) 1999-03-29 2000-10-10 Nippon Chem Ind Co Ltd リチウム複合酸化物の製造方法
JP2011210463A (ja) * 2010-03-29 2011-10-20 Jx Nippon Mining & Metals Corp リチウムイオン電池用正極活物質の製造方法

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CA2880876C (en) 2020-07-07
JP6316812B2 (ja) 2018-04-25
US9834854B2 (en) 2017-12-05
JP2015525734A (ja) 2015-09-07
KR20150056542A (ko) 2015-05-26
ZA201501121B (en) 2016-01-27
EP2882690B1 (en) 2016-10-12
CA2880876A1 (en) 2014-02-13
CN104703920A (zh) 2015-06-10
BR112015002884A2 (pt) 2019-10-08
AR092069A1 (es) 2015-03-18
BR112015002884B1 (pt) 2021-06-08
WO2014024075A1 (en) 2014-02-13
US20150197872A1 (en) 2015-07-16
EP2882690A1 (en) 2015-06-17

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