JP5775930B2 - 石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 - Google Patents
石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 Download PDFInfo
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Description
ガスタービンへの燃料ガス(H2)を精製するためのガス化炉および水性ガスシフト反応炉においては、反応後の燃料ガスには、水素(H2)以外にも二酸化炭素(CO2)が等モル分含まれている。
反応後の燃料ガスには、水素(H2)以外にも二酸化炭素(CO2)が等モル分含まれている。
本発明の二酸化炭素膜分離システムのゼオライト膜モジュールに用いる複合ゼオライト膜は、酸素12員環構造を有するゼオライト膜が、FAU型ゼオライト膜により構成され、酸素8員環を有するゼオライト膜が、CHA型ゼオライトまたはMER型ゼオライト膜、好ましくはCHA型ゼオライトにより構成されることが好ましい。
まず、微粉砕した石炭は熱分解反応炉(図示略)に導入される。熱分解反応炉では、高温ガス発生炉において発生する高温ガスに石炭を混合し、熱分解することによって、熱分解反応生成物として熱分解ガス、オイル、チャーが発生する。発生したチャーは、サイクロンによってガス、オイルから分離される。
この実施例の石炭ガス化プロセスにおける二酸化炭素膜分離システムでは、上記実施例1の水性ガスシフト反応炉と、二酸化炭素除去用ゼオライト膜を具備するゼオライト膜モジュールとの組み合わせよりなる燃料ガス生成・二酸化炭素分離ユニットを、順に3個連続して組み合わせ、各ユニットから生じる水素に富む燃料ガス中に含まれる未反応原料ガスを、次段のユニットの水性ガスシフト反応炉において反応させるとともに、各ユニットで生じる二酸化炭素を回収した。
Claims (2)
- 水性ガスシフト反応炉からの水性ガスシフト反応により発生する高温・高圧状態の二酸化炭素(CO 2 )と水素(H 2 )の混合ガスを、そのままの温度・圧力状態で二酸化炭素除去用ゼオライト膜を具備するゼオライト膜モジュールに導入し、二酸化炭素を除去するとともに、水素に富む燃料ガスを生成する石炭ガス化プロセスにおける二酸化炭素膜分離システムにおいて、
上記水性ガスシフト反応炉と、上記ゼオライト膜モジュールとの組み合わせよりなる燃料ガス生成・二酸化炭素分離ユニットを、順に複数個連続して組み合わせ、各ユニットから生じる水素に富む燃料ガス中に含まれる未反応原料ガスを、次段のユニットの水性ガスシフト反応炉において反応させるとともに、各ユニットで生じる二酸化炭素を回収することを特徴とする、二酸化炭素の膜分離システム。 - 上記燃料ガス生成・二酸化炭素分離ユニットを複数備える請求項1に記載の二酸化炭素の膜分離システムを用い、最終段の燃料ガス生成・二酸化炭素分離ユニットのゼオライト膜モジュールから排出される高温・高圧状態の水素に富む燃料ガスを、そのままの温度・圧力状態で発電設備のガスタービンへ供給することを特徴とする石炭ガス化複合発電設備。
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JP2013512308A JP5775930B2 (ja) | 2011-04-28 | 2012-04-19 | 石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 |
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JP2011101729 | 2011-04-28 | ||
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PCT/JP2012/060608 WO2012147618A1 (ja) | 2011-04-28 | 2012-04-19 | 石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 |
JP2013512308A JP5775930B2 (ja) | 2011-04-28 | 2012-04-19 | 石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 |
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US (1) | US9863314B2 (ja) |
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JP5779397B2 (ja) * | 2011-05-11 | 2015-09-16 | 日立造船株式会社 | 石炭ガス化プロセスにおける二酸化炭素膜分離システム、およびこれを用いた石炭ガス化複合発電設備 |
EP3132842A4 (en) * | 2014-04-18 | 2017-04-05 | Mitsubishi Chemical Corporation | (porous support)-(zeolite film) complex, and method for producing (porous support)-(zeolite film) complex |
WO2017150737A1 (ja) | 2016-03-04 | 2017-09-08 | 三菱ケミカル株式会社 | 二酸化炭素の分離方法、及び二酸化炭素の分離装置 |
CN107201251B (zh) * | 2017-06-23 | 2023-08-22 | 西安热工研究院有限公司 | 一种基于煤气化的太阳能储能和利用系统及方法 |
CN108313980A (zh) * | 2018-02-06 | 2018-07-24 | 吴波挺 | 一种水煤气制氢装置 |
WO2020071107A1 (ja) | 2018-10-04 | 2020-04-09 | 日本碍子株式会社 | ガス分離方法およびガス分離装置 |
JP2022543628A (ja) * | 2019-08-07 | 2022-10-13 | シェブロン ユー.エス.エー. インコーポレイテッド | カリウム-メリノイトゼオライト、その合成及び使用 |
Citations (4)
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JPH05322112A (ja) * | 1992-05-20 | 1993-12-07 | Ishikawajima Harima Heavy Ind Co Ltd | 二酸化炭素抑制燃焼設備 |
JPH09279163A (ja) * | 1996-04-11 | 1997-10-28 | Ishikawajima Harima Heavy Ind Co Ltd | Co2除去石炭ガス化複合発電システム |
JP2009029676A (ja) * | 2007-07-27 | 2009-02-12 | Nippon Oil Corp | 水素製造および二酸化炭素回収方法ならびに装置 |
JP2009536260A (ja) * | 2006-05-05 | 2009-10-08 | プラスコエナジー アイピー ホールディングス、エス.エル.、ビルバオ シャフハウゼン ブランチ | 炭素質原料のガスへの変換のための制御システム |
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CN103687932B (zh) | 2015-11-25 |
US9863314B2 (en) | 2018-01-09 |
JPWO2012147618A1 (ja) | 2014-07-28 |
US20140190146A1 (en) | 2014-07-10 |
CN103687932A (zh) | 2014-03-26 |
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