GB2517928B - Metal supported solid oxide fuel cell - Google Patents

Metal supported solid oxide fuel cell

Info

Publication number
GB2517928B
GB2517928B GB1315746.6A GB201315746A GB2517928B GB 2517928 B GB2517928 B GB 2517928B GB 201315746 A GB201315746 A GB 201315746A GB 2517928 B GB2517928 B GB 2517928B
Authority
GB
United Kingdom
Prior art keywords
fuel cell
solid oxide
oxide fuel
metal supported
supported solid
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Active
Application number
GB1315746.6A
Other languages
English (en)
Other versions
GB2517928A (en
GB201315746D0 (en
Inventor
Leah Robert
Lankin Mike
Pierce Robin
Bone Adam
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Ceres Intellectual Property Co Ltd
Original Assignee
Ceres Intellectual Property Co Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ceres Intellectual Property Co Ltd filed Critical Ceres Intellectual Property Co Ltd
Priority to GB1315746.6A priority Critical patent/GB2517928B/en
Priority to US14/053,301 priority patent/US9236614B2/en
Publication of GB201315746D0 publication Critical patent/GB201315746D0/en
Priority to RU2016105830A priority patent/RU2672093C2/ru
Priority to CN201480048581.4A priority patent/CN105531861B/zh
Priority to JP2016539627A priority patent/JP2016533017A/ja
Priority to ES14756116T priority patent/ES2868189T3/es
Priority to DK14756116.1T priority patent/DK3042411T3/da
Priority to HUE14756116A priority patent/HUE055456T2/hu
Priority to EP14756116.1A priority patent/EP3042411B1/en
Priority to MX2016002173A priority patent/MX382669B/es
Priority to PCT/GB2014/052549 priority patent/WO2015033104A1/en
Priority to SG11201601152YA priority patent/SG11201601152YA/en
Priority to CA2922744A priority patent/CA2922744C/en
Priority to KR1020167005821A priority patent/KR102256568B1/ko
Publication of GB2517928A publication Critical patent/GB2517928A/en
Priority to HK15104425.0A priority patent/HK1204151B/xx
Priority to US14/992,531 priority patent/US10008726B2/en
Application granted granted Critical
Publication of GB2517928B publication Critical patent/GB2517928B/en
Priority to JP2019149074A priority patent/JP7089494B2/ja
Active legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647—Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8652—Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites as mixture
    • C—CHEMISTRY; METALLURGY
    • C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C18/00—Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating
    • C23C18/02—Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating by thermal decomposition
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8605—Porous electrodes
    • H01M4/8621—Porous electrodes containing only metallic or ceramic material, e.g. made by sintering or sputtering
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8647—Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites
    • H01M4/8657—Inert electrodes with catalytic activity, e.g. for fuel cells consisting of more than one material, e.g. consisting of composites layered
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8803—Supports for the deposition of the catalytic active composition
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8825—Methods for deposition of the catalytic active composition
    • H01M4/8828—Coating with slurry or ink
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8825—Methods for deposition of the catalytic active composition
    • H01M4/8828—Coating with slurry or ink
    • H01M4/8832—Ink jet printing
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8878—Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8882—Heat treatment, e.g. drying, baking
    • H01M4/8885—Sintering or firing
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8878—Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8896—Pressing, rolling, calendering
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9033—Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9041—Metals or alloys
    • H01M4/905—Metals or alloys specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9066—Metals or alloys specially used in fuel cell operating at high temperature, e.g. SOFC of metal-ceramic composites or mixtures, e.g. cermets
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204—Non-porous and characterised by the material
    • H01M8/0206—Metals or alloys
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
    • H01M8/1226—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material characterised by the supporting layer
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
    • H01M8/241—Grouping of fuel cells, e.g. stacking of fuel cells with solid or matrix-supported electrolytes
    • H01M8/2425—High-temperature cells with solid electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
    • H01M8/241—Grouping of fuel cells, e.g. stacking of fuel cells with solid or matrix-supported electrolytes
    • H01M8/2425—High-temperature cells with solid electrolytes
    • H01M8/2432—Grouping of unit cells of planar configuration
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M2004/8678—Inert electrodes with catalytic activity, e.g. for fuel cells characterised by the polarity
    • H01M2004/8684—Negative electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8878—Treatment steps after deposition of the catalytic active composition or after shaping of the electrode being free-standing body
    • H01M4/8882—Heat treatment, e.g. drying, baking
    • H01M4/8885—Sintering or firing
    • H01M4/8889—Cosintering or cofiring of a catalytic active layer with another type of layer
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Electrochemistry (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Physics & Mathematics (AREA)
  • Thermal Sciences (AREA)
  • Composite Materials (AREA)
  • Ceramic Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Inert Electrodes (AREA)
  • Fuel Cell (AREA)
GB1315746.6A 2013-09-04 2013-09-04 Metal supported solid oxide fuel cell Active GB2517928B (en)

Priority Applications (17)

Application Number Priority Date Filing Date Title
GB1315746.6A GB2517928B (en) 2013-09-04 2013-09-04 Metal supported solid oxide fuel cell
US14/053,301 US9236614B2 (en) 2013-09-04 2013-10-14 Metal supported solid oxide fuel cell
PCT/GB2014/052549 WO2015033104A1 (en) 2013-09-04 2014-08-20 Metal supported solid oxide fuel cell
SG11201601152YA SG11201601152YA (en) 2013-09-04 2014-08-20 Metal supported solid oxide fuel cell
JP2016539627A JP2016533017A (ja) 2013-09-04 2014-08-20 金属支持固体酸化物燃料電池
ES14756116T ES2868189T3 (es) 2013-09-04 2014-08-20 Celda de combustible de óxido sólido con soporte metálico
DK14756116.1T DK3042411T3 (da) 2013-09-04 2014-08-20 Metalunderstøttet fastoxidbrændselscelle
HUE14756116A HUE055456T2 (hu) 2013-09-04 2014-08-20 Fémtartalmú szilárd oxid tûzelõanyag-cella
EP14756116.1A EP3042411B1 (en) 2013-09-04 2014-08-20 Metal supported solid oxide fuel cell
MX2016002173A MX382669B (es) 2013-09-04 2014-08-20 Celda de combustible de oxido solido soportado en metal.
RU2016105830A RU2672093C2 (ru) 2013-09-04 2014-08-20 Твердооксидный топливный элемент с металлической опорой
CN201480048581.4A CN105531861B (zh) 2013-09-04 2014-08-20 金属支撑型固体氧化物燃料电池
CA2922744A CA2922744C (en) 2013-09-04 2014-08-20 Metal supported solid oxide fuel cell
KR1020167005821A KR102256568B1 (ko) 2013-09-04 2014-08-20 금속지지체형 고체산화물 연료전지
HK15104425.0A HK1204151B (en) 2015-05-11 Metal supported solid oxide fuel cell
US14/992,531 US10008726B2 (en) 2013-09-04 2016-01-11 Metal supported solid oxide fuel cell
JP2019149074A JP7089494B2 (ja) 2013-09-04 2019-08-15 金属支持固体酸化物燃料電池

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
GB1315746.6A GB2517928B (en) 2013-09-04 2013-09-04 Metal supported solid oxide fuel cell

Publications (3)

Publication Number Publication Date
GB201315746D0 GB201315746D0 (en) 2013-10-16
GB2517928A GB2517928A (en) 2015-03-11
GB2517928B true GB2517928B (en) 2018-02-28

Family

ID=49397283

Family Applications (1)

Application Number Title Priority Date Filing Date
GB1315746.6A Active GB2517928B (en) 2013-09-04 2013-09-04 Metal supported solid oxide fuel cell

Country Status (14)

Country Link
US (2) US9236614B2 (enExample)
EP (1) EP3042411B1 (enExample)
JP (2) JP2016533017A (enExample)
KR (1) KR102256568B1 (enExample)
CN (1) CN105531861B (enExample)
CA (1) CA2922744C (enExample)
DK (1) DK3042411T3 (enExample)
ES (1) ES2868189T3 (enExample)
GB (1) GB2517928B (enExample)
HU (1) HUE055456T2 (enExample)
MX (1) MX382669B (enExample)
RU (1) RU2672093C2 (enExample)
SG (1) SG11201601152YA (enExample)
WO (1) WO2015033104A1 (enExample)

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JP6581836B2 (ja) * 2015-08-03 2019-09-25 本田技研工業株式会社 メタルサポートセル
CN105206855B (zh) * 2015-09-10 2018-03-30 刘备之 一种用于制氧的复合电解质膜
TWI558568B (zh) * 2015-11-03 2016-11-21 行政院原子能委員會核能研究所 透氣金屬基板、金屬支撐固態氧化物燃料電池及其製作方法
GB2550317B (en) 2016-03-09 2021-12-15 Ceres Ip Co Ltd Fuel cell
JP7175759B2 (ja) * 2016-03-18 2022-11-21 大阪瓦斯株式会社 電気化学素子、電気化学モジュール、電気化学装置およびエネルギーシステム
EP3488482B1 (en) * 2016-07-19 2021-05-05 Georgia Tech Research Corporation Intermediate-temperature fuel cell tailored for efficient utilization of methane
CN108145144B (zh) * 2017-12-27 2023-08-15 武汉科技大学 一种控制钢液卷渣的钢包工作衬
CA3107244A1 (en) 2018-03-30 2019-10-03 Osaka Gas Co., Ltd. Metal support for electrochemical element, electrochemical element, electrochemical module, electrochemical device, energy system, solid oxide fuel cell, solid oxide electrolytic cell, and method for manufacturing metal support
CA3107254A1 (en) * 2018-03-30 2019-10-03 Osaka Gas Co., Ltd. Metal support for electrochemical element, electrochemical element, electrochemical module, electrochemical device, energy system, solid oxide fuel cell, solid oxide electrolytic cell, and method for manufacturing metal support
JP7300672B2 (ja) * 2018-09-21 2023-06-30 パナソニックＩｐマネジメント株式会社 燃料電池システムおよびその運転方法
US11239470B2 (en) 2018-12-17 2022-02-01 General Electric Company Integrated fuel cell and combustion system
JP7301768B2 (ja) * 2020-03-18 2023-07-03 東芝エネルギーシステムズ株式会社 電気化学セル、電気化学セルスタックおよび電気化学セル用電解質
JP7561511B2 (ja) * 2020-03-27 2024-10-04 大阪瓦斯株式会社 電気化学素子の金属支持体、電気化学素子、電気化学モジュール、電気化学装置、エネルギーシステム、固体酸化物形燃料電池、および固体酸化物形電解セル
CN111584910B (zh) * 2020-04-24 2022-11-01 合肥学院 一种CeO2基复合固体电解质材料及其制备方法
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