BRPI1010725A2 - fluido tendo índice de viscosidade melhorado. - Google Patents
fluido tendo índice de viscosidade melhorado.Info
- Publication number
- BRPI1010725A2 BRPI1010725A2 BRPI1010725A BRPI1010725A BRPI1010725A2 BR PI1010725 A2 BRPI1010725 A2 BR PI1010725A2 BR PI1010725 A BRPI1010725 A BR PI1010725A BR PI1010725 A BRPI1010725 A BR PI1010725A BR PI1010725 A2 BRPI1010725 A2 BR PI1010725A2
- Authority
- BR
- Brazil
- Prior art keywords
- fluid
- viscosity index
- improved viscosity
- improved
- index
- Prior art date
Links
Classifications
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M169/00—Lubricating compositions characterised by containing as components a mixture of at least two types of ingredient selected from base-materials, thickeners or additives, covered by the preceding groups, each of these compounds being essential
- C10M169/04—Mixtures of base-materials and additives
- C10M169/041—Mixtures of base-materials and additives the additives being macromolecular compounds only
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M169/00—Lubricating compositions characterised by containing as components a mixture of at least two types of ingredient selected from base-materials, thickeners or additives, covered by the preceding groups, each of these compounds being essential
- C10M169/04—Mixtures of base-materials and additives
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M161/00—Lubricating compositions characterised by the additive being a mixture of a macromolecular compound and a non-macromolecular compound, each of these compounds being essential
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2203/00—Organic non-macromolecular hydrocarbon compounds and hydrocarbon fractions as ingredients in lubricant compositions
- C10M2203/10—Petroleum or coal fractions, e.g. tars, solvents, bitumen
- C10M2203/1006—Petroleum or coal fractions, e.g. tars, solvents, bitumen used as base material
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2203/00—Organic non-macromolecular hydrocarbon compounds and hydrocarbon fractions as ingredients in lubricant compositions
- C10M2203/10—Petroleum or coal fractions, e.g. tars, solvents, bitumen
- C10M2203/106—Naphthenic fractions
- C10M2203/1065—Naphthenic fractions used as base material
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2205/00—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
- C10M2205/02—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions containing acyclic monomers
- C10M2205/0206—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions containing acyclic monomers used as base material
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2207/00—Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
- C10M2207/28—Esters
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2207/00—Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
- C10M2207/28—Esters
- C10M2207/2805—Esters used as base material
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2207/00—Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
- C10M2207/28—Esters
- C10M2207/282—Esters of (cyclo)aliphatic oolycarboxylic acids
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2207/00—Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
- C10M2207/28—Esters
- C10M2207/282—Esters of (cyclo)aliphatic oolycarboxylic acids
- C10M2207/2825—Esters of (cyclo)aliphatic oolycarboxylic acids used as base material
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2209/00—Organic macromolecular compounds containing oxygen as ingredients in lubricant compositions
- C10M2209/02—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
- C10M2209/08—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds containing monomers having an unsaturated radical bound to a carboxyl radical, e.g. acrylate type
- C10M2209/084—Acrylate; Methacrylate
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2020/00—Specified physical or chemical properties or characteristics, i.e. function, of component of lubricating compositions
- C10N2020/01—Physico-chemical properties
- C10N2020/04—Molecular weight; Molecular weight distribution
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2030/00—Specified physical or chemical properties which is improved by the additive characterising the lubricating composition, e.g. multifunctional additives
- C10N2030/02—Pour-point; Viscosity index
Landscapes
- Chemical & Material Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- General Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Organic Chemistry (AREA)
- Lubricants (AREA)
- Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US18674409P | 2009-06-12 | 2009-06-12 | |
PCT/EP2010/058241 WO2010142789A1 (en) | 2009-06-12 | 2010-06-11 | A fluid having improved viscosity index |
Publications (1)
Publication Number | Publication Date |
---|---|
BRPI1010725A2 true BRPI1010725A2 (pt) | 2016-03-15 |
Family
ID=42313049
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
BRPI1010725A BRPI1010725A2 (pt) | 2009-06-12 | 2010-06-11 | fluido tendo índice de viscosidade melhorado. |
Country Status (10)
Country | Link |
---|---|
US (1) | US9175242B2 (pt) |
EP (1) | EP2440640A1 (pt) |
JP (1) | JP5591327B2 (pt) |
KR (1) | KR101676064B1 (pt) |
CN (2) | CN102459541A (pt) |
BR (1) | BRPI1010725A2 (pt) |
CA (1) | CA2765300A1 (pt) |
RU (1) | RU2576401C2 (pt) |
SG (1) | SG176054A1 (pt) |
WO (1) | WO2010142789A1 (pt) |
Families Citing this family (37)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE102010028195A1 (de) * | 2010-04-26 | 2011-10-27 | Evonik Rohmax Additives Gmbh | Schmiermittel für Getriebe |
WO2011134694A1 (en) | 2010-04-26 | 2011-11-03 | Evonik Rohmax Additives Gmbh | A polymer useful as viscosity index improver |
WO2012076285A1 (en) * | 2010-12-10 | 2012-06-14 | Evonik Rohmax Additives Gmbh | A lubricant composition |
CA2826120A1 (en) * | 2011-01-31 | 2012-08-09 | Rhodia Operations | Hydraulic fluids containing dibasic esters and methods for use |
CN104160002B (zh) | 2012-03-13 | 2016-03-30 | 吉坤日矿日石能源株式会社 | 变速机用润滑油组合物 |
US9534343B2 (en) * | 2012-10-18 | 2017-01-03 | The Chemours Company Fc, Llc | Partially fluorinated copolymer emulsions containing fatty acids and esters |
WO2014075993A1 (en) * | 2012-11-19 | 2014-05-22 | Basf Se | Use of polyesters as lubricants |
WO2014170169A1 (de) * | 2013-04-18 | 2014-10-23 | Evonik Industries Ag | Getriebeölformulierung zur verringerung des kraftstoffverbrauchs |
EP3215590A1 (en) * | 2014-11-04 | 2017-09-13 | Shell Internationale Research Maatschappij B.V. | Lubricating composition |
US10336961B2 (en) * | 2015-03-20 | 2019-07-02 | Sanyo Chemical Industries, Ltd. | Viscosity index improver, lubricant composition, and method for manufacturing lubricant composition |
EP3680313B1 (en) * | 2016-06-17 | 2022-03-23 | Total Marketing Services | Lubricant polymers |
RU2710192C1 (ru) * | 2016-06-17 | 2019-12-24 | Акцо Нобель Кемикалз Интернэшнл Б.В. | Полимеры распыляемых смазочных материалов |
US10544241B2 (en) | 2016-09-15 | 2020-01-28 | Fina Technology, Inc. | Farnesene-based macromonomers and methods of making and using the same |
US10982167B2 (en) | 2016-09-21 | 2021-04-20 | Nippon Shokubai Co., Ltd. | Viscosity index improver and lubricating oil composition |
JP7014552B2 (ja) * | 2016-09-21 | 2022-02-01 | 株式会社日本触媒 | 粘度指数向上剤および潤滑油組成物 |
EP3535357B1 (en) * | 2016-11-02 | 2020-12-16 | Evonik Operations GmbH | Lubricant composition with an improved viscosity characteristic at low operating temperature |
JP2018162433A (ja) * | 2017-03-27 | 2018-10-18 | 株式会社日本触媒 | 粘度指数向上剤および潤滑油組成物 |
EP3722395A4 (en) * | 2017-12-05 | 2021-08-04 | Adeka Corporation | Anti-friction compound and anti-friction compound with the anti-friction compound |
EP3498808B1 (en) | 2017-12-13 | 2020-05-13 | Evonik Operations GmbH | Viscosity index improver with improved shear-resistance and solubility after shear |
KR102587269B1 (ko) * | 2018-01-23 | 2023-10-11 | 에보닉 오퍼레이션스 게엠베하 | 중합체성-무기 나노입자 조성물, 이의 제조 방법 및 윤활제 첨가제로서의 이들의 용도 |
JP2019157047A (ja) * | 2018-03-15 | 2019-09-19 | 株式会社日本触媒 | (メタ)アクリレート系重合体の製造方法および粘度指数向上剤 |
FR3083244B1 (fr) | 2018-07-02 | 2020-07-17 | Total Marketing Services | Composition pour refroidir et lubrifier un systeme de propulsion d'un vehicule electrique ou hybride |
FR3088073B1 (fr) * | 2018-11-05 | 2021-07-23 | Total Marketing Services | Utilisation d'un diester pour ameliorer les proprietes anti-usure d'une composition lubrifiante |
WO2020099078A1 (en) * | 2018-11-13 | 2020-05-22 | Evonik Operations Gmbh | Random copolymers for use as base oils or lubricant additives |
SG11202110027XA (en) | 2019-03-20 | 2021-10-28 | Evonik Operations Gmbh | Polyalkyl(meth)acrylates for improving fuel economy, dispersancy and deposits performance |
EP3983507A1 (en) * | 2019-06-14 | 2022-04-20 | Basf Se | A lubricant with a polyacrylate based on c13/15 cacrylate |
US11085006B2 (en) * | 2019-07-12 | 2021-08-10 | Afton Chemical Corporation | Lubricants for electric and hybrid vehicle applications |
EP3778839B1 (en) | 2019-08-13 | 2021-08-04 | Evonik Operations GmbH | Viscosity index improver with improved shear-resistance |
US11384311B2 (en) * | 2019-12-16 | 2022-07-12 | Infineum International Limited | High viscosity index comb polymer viscosity modifiers and methods of modifying lubricant viscosity using same |
US11365273B2 (en) * | 2019-12-16 | 2022-06-21 | Infineum International Limited | High viscosity index comb polymer viscosity modifiers and methods of modifying lubricant viscosity using same |
US20210179961A1 (en) * | 2019-12-16 | 2021-06-17 | Infineum International Limited | High Viscosity Index Comb Copolymer Viscosity Modifiers and Methods of Modifying Lubricant Viscosity Using Same |
US11685874B2 (en) * | 2019-12-16 | 2023-06-27 | Infineum International Limited | High viscosity index comb polymer viscosity modifiers and methods of modifying lubricant viscosity using same |
EP3907269B1 (en) | 2020-05-05 | 2023-05-03 | Evonik Operations GmbH | Hydrogenated linear polydiene copolymers as base stock or lubricant additives for lubricant compositions |
KR20230036141A (ko) * | 2020-09-14 | 2023-03-14 | 산요가세이고교 가부시키가이샤 | 점도 지수 향상제 및 윤활유 조성물 |
KR20230037047A (ko) | 2020-09-14 | 2023-03-15 | 산요가세이고교 가부시키가이샤 | 점도 지수 향상제 및 윤활유 조성물 |
FR3115291B1 (fr) * | 2020-10-20 | 2023-11-17 | Total Marketing Services | Utilisation d’ester de dialkylène glycol pour diminuer le frottement dans les véhicules équipés de moteur hybride |
EP4060009B1 (en) | 2021-03-19 | 2023-05-03 | Evonik Operations GmbH | Viscosity index improver and lubricant compositions thereof |
Family Cites Families (28)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
NL241682A (pt) * | 1958-07-28 | |||
SU464127A3 (ru) | 1972-03-31 | 1975-03-15 | Стауффер Кемикал Компани (Фирма) | Смазочный материал дл газотурбинных двигателей |
US4956122A (en) * | 1982-03-10 | 1990-09-11 | Uniroyal Chemical Company, Inc. | Lubricating composition |
US4833184A (en) * | 1987-03-10 | 1989-05-23 | The Lubrizol Corporation | Acrylate polymer modified asphalt compositions |
US5047457A (en) | 1987-03-10 | 1991-09-10 | The Lubrizol Corporation | Acrylate polymer modified asphalt compositions |
US4941985A (en) * | 1989-12-01 | 1990-07-17 | Texaco Inc. | Dispersant/antioxidant VII lubricant additive |
JP2627725B2 (ja) | 1994-04-25 | 1997-07-09 | 三洋化成工業株式会社 | 粘度指数向上剤及び潤滑油 |
US6365558B2 (en) * | 1995-06-07 | 2002-04-02 | The Lubrizol Corporation | Vegetable oils containing styrene/butadiene copolymers in combination with additional commercial polymers that have good low temperature and high temperature viscometrics |
ZA97222B (en) * | 1996-01-16 | 1998-02-18 | Lubrizol Corp | Lubricating compositions. |
JP2000109876A (ja) | 1998-10-09 | 2000-04-18 | Tonen Corp | 緩衝器用油圧作動油組成物 |
US6090989A (en) * | 1997-10-20 | 2000-07-18 | Mobil Oil Corporation | Isoparaffinic lube basestock compositions |
US6303548B2 (en) | 1998-12-11 | 2001-10-16 | Exxon Research And Engineering Company | Partly synthetic multigrade crankcase lubricant |
DE10314776A1 (de) | 2003-03-31 | 2004-10-14 | Rohmax Additives Gmbh | Schmierölzusammensetzung mit guten Reibeigenschaften |
US7470381B2 (en) * | 2003-07-25 | 2008-12-30 | Rohmax Additives Gmbh | Functional fluid and the use thereof |
DE102004018094A1 (de) * | 2004-04-08 | 2005-11-03 | Rohmax Additives Gmbh | Polymere mit H-Brücken bildenden Funktionalitäten zur Verbesserung des Verschleißschutzes |
DE102004021778A1 (de) * | 2004-04-30 | 2005-12-08 | Rohmax Additives Gmbh | Verwendung von Polyalkyl(meth)acrylaten in Schmierölzusammensetzungen |
DE102004034618A1 (de) | 2004-07-16 | 2006-02-16 | Rohmax Additives Gmbh | Verwendung von Pfropfcopolymeren |
JP2006077119A (ja) | 2004-09-09 | 2006-03-23 | Nok Kluber Kk | 潤滑油組成物 |
JP4792216B2 (ja) | 2004-11-01 | 2011-10-12 | Jx日鉱日石エネルギー株式会社 | 極微量油剤供給式切削・研削加工用油剤組成物 |
DE102005015931A1 (de) | 2005-04-06 | 2006-10-12 | Rohmax Additives Gmbh | Polyalkyl(meth) acrylat-Copolymere mit hervorragenden Eigenschaften |
DE102005031244A1 (de) | 2005-07-01 | 2007-02-15 | Rohmax Additives Gmbh | Öllösliche Kammpolymere |
JP5069849B2 (ja) * | 2005-07-29 | 2012-11-07 | 三洋化成工業株式会社 | 潤滑油添加剤組成物およびエステル系合成潤滑油組成物 |
DE102005041528A1 (de) | 2005-08-31 | 2007-03-01 | Rohmax Additives Gmbh | Öllösliche Polymere |
DE102006016588A1 (de) | 2006-04-06 | 2007-10-18 | Rohmax Additives Gmbh | Kraftstoffzusammensetzungen umfassend nachwachsende Rohstoffe |
US9783630B2 (en) | 2007-07-09 | 2017-10-10 | Evonik Oil Additives Gmbh | Use of comb polymers for reducing fuel consumption |
JP2010532807A (ja) | 2007-07-12 | 2010-10-14 | エボニック ローマックス アディティヴス ゲゼルシャフト ミット ベシュレンクテル ハフツング | 連続的に変動性の組成のコポリマーを製造するための改善された方法 |
DE102007036856A1 (de) | 2007-08-06 | 2009-02-26 | Evonik Rohmax Additives Gmbh | Verwendung von Estergruppen-umfassenden Polymeren als Antifatigue-Additive |
CN103923726A (zh) * | 2007-12-05 | 2014-07-16 | 吉坤日矿日石能源株式会社 | 润滑油组合物 |
-
2010
- 2010-06-11 BR BRPI1010725A patent/BRPI1010725A2/pt not_active IP Right Cessation
- 2010-06-11 JP JP2012514482A patent/JP5591327B2/ja active Active
- 2010-06-11 WO PCT/EP2010/058241 patent/WO2010142789A1/en active Application Filing
- 2010-06-11 CN CN2010800248717A patent/CN102459541A/zh active Pending
- 2010-06-11 RU RU2012100237/04A patent/RU2576401C2/ru active
- 2010-06-11 CN CN201410226983.0A patent/CN104017633A/zh active Pending
- 2010-06-11 US US13/318,492 patent/US9175242B2/en active Active
- 2010-06-11 CA CA2765300A patent/CA2765300A1/en not_active Abandoned
- 2010-06-11 KR KR1020117029537A patent/KR101676064B1/ko active IP Right Grant
- 2010-06-11 EP EP10722717A patent/EP2440640A1/en not_active Withdrawn
- 2010-06-11 SG SG2011083755A patent/SG176054A1/en unknown
Also Published As
Publication number | Publication date |
---|---|
WO2010142789A1 (en) | 2010-12-16 |
SG176054A1 (en) | 2011-12-29 |
KR101676064B1 (ko) | 2016-11-14 |
CN104017633A (zh) | 2014-09-03 |
KR20120036835A (ko) | 2012-04-18 |
JP2012529550A (ja) | 2012-11-22 |
US9175242B2 (en) | 2015-11-03 |
JP5591327B2 (ja) | 2014-09-17 |
EP2440640A1 (en) | 2012-04-18 |
CN102459541A (zh) | 2012-05-16 |
RU2576401C2 (ru) | 2016-03-10 |
US20120053100A1 (en) | 2012-03-01 |
RU2012100237A (ru) | 2013-07-20 |
CA2765300A1 (en) | 2010-12-16 |
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Legal Events
Date | Code | Title | Description |
---|---|---|---|
B08F | Application fees: dismissal - article 86 of industrial property law |
Free format text: REFERENTE A 7A ANUIDADE. |
|
B08K | Lapse as no evidence of payment of the annual fee has been furnished to inpi (acc. art. 87) |