BR112017016522A2 - polímero com base em dieno conjugado modificado, método de fabricação do mesmo, e composição de polímero com base em dieno conjugado modificado - Google Patents
polímero com base em dieno conjugado modificado, método de fabricação do mesmo, e composição de polímero com base em dieno conjugado modificadoInfo
- Publication number
- BR112017016522A2 BR112017016522A2 BR112017016522-8A BR112017016522A BR112017016522A2 BR 112017016522 A2 BR112017016522 A2 BR 112017016522A2 BR 112017016522 A BR112017016522 A BR 112017016522A BR 112017016522 A2 BR112017016522 A2 BR 112017016522A2
- Authority
- BR
- Brazil
- Prior art keywords
- denaturation
- conjugate diene
- system polymer
- diene system
- manufacturing
- Prior art date
Links
- 150000001993 dienes Chemical class 0.000 title abstract 3
- 229920000642 polymer Polymers 0.000 title abstract 3
- 238000004925 denaturation Methods 0.000 title 2
- 230000036425 denaturation Effects 0.000 title 2
- 239000000470 constituent Substances 0.000 title 1
- 238000004519 manufacturing process Methods 0.000 title 1
- 241001441571 Hiodontidae Species 0.000 abstract 1
- 230000004048 modification Effects 0.000 abstract 1
- 238000012986 modification Methods 0.000 abstract 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F8/00—Chemical modification by after-treatment
- C08F8/30—Introducing nitrogen atoms or nitrogen-containing groups
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08C—TREATMENT OR CHEMICAL MODIFICATION OF RUBBERS
- C08C19/00—Chemical modification of rubber
- C08C19/25—Incorporating silicon atoms into the molecule
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F236/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds
- C08F236/02—Copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds
- C08F236/04—Copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds conjugated
- C08F236/06—Butadiene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F2/00—Processes of polymerisation
- C08F2/38—Polymerisation using regulators, e.g. chain terminating agents, e.g. telomerisation
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F36/00—Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds
- C08F36/02—Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds
- C08F36/04—Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds conjugated
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F8/00—Chemical modification by after-treatment
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/34—Silicon-containing compounds
- C08K3/36—Silica
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
- C08K5/544—Silicon-containing compounds containing nitrogen
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
- C08K5/544—Silicon-containing compounds containing nitrogen
- C08K5/5445—Silicon-containing compounds containing nitrogen containing at least one Si-N bond
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
- C08K5/544—Silicon-containing compounds containing nitrogen
- C08K5/5477—Silicon-containing compounds containing nitrogen containing nitrogen in a heterocyclic ring
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L15/00—Compositions of rubber derivatives
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L47/00—Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds; Compositions of derivatives of such polymers
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
- C08L9/06—Copolymers with styrene
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Tires In General (AREA)
- Polymerization Catalysts (AREA)
Applications Claiming Priority (3)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| JP2015-031082 | 2015-02-19 | ||
| JP2015031082 | 2015-02-19 | ||
| PCT/JP2016/054869 WO2016133202A1 (ja) | 2015-02-19 | 2016-02-19 | 変性共役ジエン系重合体及びその製造方法、並びに変性共役ジエン系重合体組成物 |
Publications (1)
| Publication Number | Publication Date |
|---|---|
| BR112017016522A2 true BR112017016522A2 (pt) | 2018-04-10 |
Family
ID=56692204
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| BR112017016522-8A BR112017016522A2 (pt) | 2015-02-19 | 2016-02-19 | polímero com base em dieno conjugado modificado, método de fabricação do mesmo, e composição de polímero com base em dieno conjugado modificado |
Country Status (10)
| Country | Link |
|---|---|
| US (1) | US10766972B2 (https=) |
| EP (1) | EP3260476B1 (https=) |
| JP (2) | JP6607916B2 (https=) |
| KR (2) | KR102160548B1 (https=) |
| CN (1) | CN107250172B (https=) |
| BR (1) | BR112017016522A2 (https=) |
| HU (1) | HUE044416T2 (https=) |
| SG (1) | SG11201706426YA (https=) |
| TW (1) | TWI607026B (https=) |
| WO (1) | WO2016133202A1 (https=) |
Families Citing this family (42)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JP6480820B2 (ja) * | 2015-06-29 | 2019-03-13 | 旭化成株式会社 | タイヤ用ゴム組成物及びその製造方法 |
| JPWO2017038001A1 (ja) * | 2015-08-31 | 2018-06-14 | 株式会社ブリヂストン | 変性ジエン系ゴムの製造方法、ゴム組成物及びタイヤ |
| WO2018034217A1 (ja) * | 2016-08-19 | 2018-02-22 | 旭化成株式会社 | 変性共役ジエン系重合体、その製造方法、ゴム組成物、タイヤ |
| JP2018048234A (ja) * | 2016-09-20 | 2018-03-29 | 旭化成株式会社 | 変性共役ジエン系重合体組成物及びタイヤ |
| JP2018062566A (ja) * | 2016-10-12 | 2018-04-19 | 旭化成株式会社 | 変性共役ジエン系重合体組成物 |
| JP7387247B2 (ja) * | 2016-12-07 | 2023-11-28 | 旭化成株式会社 | 変性共役ジエン系重合体、変性共役ジエン系重合体組成物、及びタイヤ |
| JP2018123225A (ja) * | 2017-01-31 | 2018-08-09 | 旭化成株式会社 | ヒステリシスロスが改良されたゴム組成物、加硫物、及びゴム組成物の製造方法 |
| EP3594251A4 (en) * | 2017-03-07 | 2020-06-03 | Asahi Kasei Kabushiki Kaisha | MODIFIED CONJUGATED DIENE POLYMER, POLYMER COMPOSITION AND RUBBER COMPOSITION |
| WO2018199267A1 (ja) | 2017-04-28 | 2018-11-01 | 旭化成株式会社 | 変性共役ジエン系重合体、重合体組成物、及びゴム組成物 |
| WO2019008727A1 (ja) * | 2017-07-06 | 2019-01-10 | 三菱重工機械システム株式会社 | 混練機制御装置、混練機制御方法、プログラム |
| KR102328792B1 (ko) * | 2017-09-18 | 2021-11-22 | 주식회사 엘지화학 | 연속식 중합에 의한 공액디엔계 중합체의 제조방법 |
| KR102323810B1 (ko) * | 2017-12-05 | 2021-11-10 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| KR102122471B1 (ko) | 2017-12-05 | 2020-06-26 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| WO2019112261A1 (ko) * | 2017-12-05 | 2019-06-13 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| KR102167122B1 (ko) * | 2017-12-05 | 2020-10-16 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| KR102179487B1 (ko) * | 2017-12-05 | 2020-11-16 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| WO2019112263A1 (ko) * | 2017-12-05 | 2019-06-13 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| WO2019225824A1 (ko) * | 2018-05-25 | 2019-11-28 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| KR102288852B1 (ko) * | 2018-05-25 | 2021-08-12 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| JP7280115B2 (ja) * | 2018-06-28 | 2023-05-23 | 旭化成株式会社 | 変性共役ジエン系重合体混合物の製造方法 |
| CN110684154B (zh) * | 2018-07-04 | 2022-05-17 | 旭化成株式会社 | 改性共轭二烯系聚合物、改性共轭二烯系聚合物组合物以及橡胶组合物 |
| KR102035177B1 (ko) * | 2018-07-11 | 2019-11-08 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| JP7161883B2 (ja) * | 2018-07-27 | 2022-10-27 | 旭化成株式会社 | 変性共役ジエン系重合体、その製造方法、変性共役ジエン系組成物、及びタイヤ |
| JP7385394B2 (ja) * | 2018-08-30 | 2023-11-22 | 旭化成株式会社 | 変性共役ジエン系重合体組成物、ゴム組成物、ゴム組成物の製造方法、及びタイヤ |
| US11993620B2 (en) * | 2018-09-03 | 2024-05-28 | Synthos S.A. | Aminosilyl-functionalized conjugated dienes, their preparation and their use in the production of rubbers |
| US11780994B2 (en) * | 2018-10-04 | 2023-10-10 | Bridgestone Corporation | Rubber composition, tread rubber, and tire |
| EP4026704B1 (en) * | 2019-09-05 | 2024-09-04 | Asahi Kasei Kabushiki Kaisha | Conjugated diene polymer, method for producing conjugated diene polymer, conjugated diene polymer composition, and rubber composition |
| KR102604539B1 (ko) * | 2019-09-11 | 2023-11-22 | 주식회사 엘지화학 | 변성 공액디엔계 중합체, 이의 제조방법 및 이를 포함하는 고무 조성물 |
| WO2021049916A1 (ko) | 2019-09-11 | 2021-03-18 | 주식회사 엘지화학 | 변성 공액디엔계 중합체, 이의 제조방법 및 이를 포함하는 고무 조성물 |
| JP7280972B2 (ja) | 2019-09-11 | 2023-05-24 | エルジー・ケム・リミテッド | 変性共役ジエン系重合体、その製造方法、およびそれを含むゴム組成物 |
| KR102800784B1 (ko) * | 2019-09-27 | 2025-04-29 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| US12522720B2 (en) | 2019-09-30 | 2026-01-13 | Lg Chem, Ltd. | Modified conjugated diene-based polymer, method for preparing the same and rubber composition including the same |
| KR102585915B1 (ko) * | 2019-10-30 | 2023-10-10 | 주식회사 엘지화학 | 변성 공액디엔계 중합체 및 이를 포함하는 고무 조성물 |
| CN115298859A (zh) * | 2020-03-17 | 2022-11-04 | 株式会社引能仕材料 | 全固体二次电池用粘结剂、全固体二次电池用粘结剂组合物、全固体二次电池用浆料、全固体二次电池用固体电解质片及其制造方法、以及全固体二次电池及其制造方法 |
| BR112022026866A2 (pt) | 2020-08-11 | 2023-02-23 | Asahi Chemical Ind | Artigo moldado embalado, composição de borracha reticulada, método para produção de artigo moldado embalado, método para produção da composição de borracha reticulada e banda de rodagem para pneu |
| JPWO2022163387A1 (https=) * | 2021-01-29 | 2022-08-04 | ||
| WO2023104783A1 (en) | 2021-12-07 | 2023-06-15 | Arlanxeo Deutschland Gmbh | Functionalized diene rubbers prepared with unsaturated siloxane-based coupling agents |
| US20260055216A1 (en) * | 2022-08-12 | 2026-02-26 | Asahi Kasei Kabushiki Kaisha | Conjugated Diene-Based Polymer, Formed Body, Production Method for Conjugated Diene-Based Polymer, Rubber Composition, and Tire |
| JP7581541B2 (ja) * | 2022-08-24 | 2024-11-12 | 旭化成株式会社 | ゴム改質用マスターバッチ、及び分岐共役ジエン系重合体組成物 |
| CN121568972A (zh) * | 2023-08-02 | 2026-02-24 | 旭化成株式会社 | 改性共轭二烯系聚合物、压块、改性共轭二烯系聚合物的制造方法、橡胶组合物和轮胎 |
| WO2025150432A1 (ja) * | 2024-01-12 | 2025-07-17 | 旭化成株式会社 | 変性共役ジエン系重合体、及び変性共役ジエン系重合体の製造方法 |
| IT202400004015A1 (it) | 2024-02-26 | 2025-08-26 | Versalis Spa | Copolimeri random stirene-butadiene funzionalizzati e procedimento per la loro preparazione. |
Family Cites Families (17)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JP3441201B2 (ja) | 1993-12-29 | 2003-08-25 | 株式会社ブリヂストン | 重合体及びその重合体組成物 |
| EP1153972B2 (en) | 1999-09-27 | 2012-01-11 | Asahi Kasei Kabushiki Kaisha | Rubber composition |
| JP4598909B2 (ja) | 1999-12-02 | 2010-12-15 | 株式会社ブリヂストン | ゴム組成物及びそれを用いた空気入りタイヤ |
| JP4129619B2 (ja) | 2001-09-27 | 2008-08-06 | Ｊｓｒ株式会社 | 共役ジオレフィン（共）重合ゴム、該（共）重合ゴムの製造方法、ゴム組成物およびタイヤ |
| CN101268107B (zh) * | 2005-09-22 | 2012-10-10 | 旭化成化学株式会社 | 共轭二烯系聚合物及其制造方法 |
| JP5568860B2 (ja) | 2006-03-31 | 2014-08-13 | 日本ゼオン株式会社 | タイヤ用ゴム組成物の製造方法、タイヤ用ゴム組成物、及びタイヤ |
| JP5127521B2 (ja) * | 2008-03-24 | 2013-01-23 | 旭化成ケミカルズ株式会社 | 変性共役ジエン系重合体及びその製造方法、並びに重合体組成物 |
| CN102177185A (zh) | 2008-10-14 | 2011-09-07 | 旭化成化学株式会社 | 改性共轭二烯系聚合物、其制造方法、改性共轭二烯系聚合物组合物及轮胎 |
| JP5584288B2 (ja) * | 2010-04-16 | 2014-09-03 | 旭化成ケミカルズ株式会社 | 変性共役ジエン系重合体の製造方法、及び変性共役ジエン系重合体組成物 |
| EA201490496A1 (ru) | 2011-08-26 | 2014-08-29 | Асахи Касеи Кемикалз Корпорейшн | Способ получения модифицированных полимеров сопряженных диенов, модифицированные полимеры сопряженных диенов, композиции модифицированных полимеров сопряженных диенов, композиции каучука и автомобильные шины |
| PL2754674T3 (pl) * | 2011-09-08 | 2015-08-31 | Asahi Kasei Chemicals Corp | Sposób wytwarzania zmodyfikowanego polimeru na bazie sprzężonego dienu, zmodyfikowany polimer na bazie sprzężonego dienu, kompozycja zmodyfikowanego polimeru na bazie sprzężonego dienu oraz kompozycja kauczuku i opony |
| JP5971915B2 (ja) * | 2011-10-11 | 2016-08-17 | 旭化成株式会社 | 変性共役ジエン系重合体組成物及びその製造方法 |
| JP5964571B2 (ja) * | 2011-10-12 | 2016-08-03 | 旭化成株式会社 | 変性共役ジエン系重合体の製造方法、変性共役ジエン系重合体、及び変性共役ジエン系重合体組成物、及びタイヤ |
| JP6032882B2 (ja) * | 2011-10-19 | 2016-11-30 | 旭化成株式会社 | サイドウォール用ゴム組成物 |
| JP2013129693A (ja) | 2011-12-20 | 2013-07-04 | Asahi Kasei Chemicals Corp | 変性共役ジエン重合体の製造方法及び変性共役ジエン重合体の組成物 |
| JP6106476B2 (ja) * | 2013-03-13 | 2017-03-29 | 旭化成株式会社 | 変性共役ジエン系重合体組成物、トレッド、サイドウォール及びタイヤ |
| JP2015113437A (ja) * | 2013-12-13 | 2015-06-22 | 旭化成ケミカルズ株式会社 | 変性共役ジエン系重合体組成物の製造方法 |
-
2016
- 2016-02-19 BR BR112017016522-8A patent/BR112017016522A2/pt not_active Application Discontinuation
- 2016-02-19 SG SG11201706426YA patent/SG11201706426YA/en unknown
- 2016-02-19 KR KR1020197015111A patent/KR102160548B1/ko not_active Ceased
- 2016-02-19 WO PCT/JP2016/054869 patent/WO2016133202A1/ja not_active Ceased
- 2016-02-19 US US15/551,548 patent/US10766972B2/en active Active
- 2016-02-19 CN CN201680010344.8A patent/CN107250172B/zh active Active
- 2016-02-19 TW TW105105015A patent/TWI607026B/zh not_active IP Right Cessation
- 2016-02-19 HU HUE16752588 patent/HUE044416T2/hu unknown
- 2016-02-19 JP JP2017500757A patent/JP6607916B2/ja active Active
- 2016-02-19 EP EP16752588.0A patent/EP3260476B1/en active Active
- 2016-02-19 KR KR1020177021439A patent/KR20170102320A/ko not_active Ceased
-
2019
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| Publication number | Publication date |
|---|---|
| KR20170102320A (ko) | 2017-09-08 |
| JP6908662B2 (ja) | 2021-07-28 |
| TWI607026B (zh) | 2017-12-01 |
| EP3260476B1 (en) | 2019-05-08 |
| HUE044416T2 (hu) | 2019-10-28 |
| CN107250172B (zh) | 2021-04-09 |
| SG11201706426YA (en) | 2017-09-28 |
| TW201708272A (zh) | 2017-03-01 |
| KR102160548B9 (ko) | 2022-02-18 |
| KR102160548B1 (ko) | 2020-09-28 |
| CN107250172A (zh) | 2017-10-13 |
| US10766972B2 (en) | 2020-09-08 |
| WO2016133202A1 (ja) | 2016-08-25 |
| JP6607916B2 (ja) | 2019-11-20 |
| EP3260476A1 (en) | 2017-12-27 |
| JPWO2016133202A1 (ja) | 2017-11-02 |
| KR20190060893A (ko) | 2019-06-03 |
| JP2019206723A (ja) | 2019-12-05 |
| US20180037674A1 (en) | 2018-02-08 |
| EP3260476A4 (en) | 2018-01-03 |
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