WO2005016524A3 - Immobilisierte immidazole und ruthenium-katalysatoren - Google Patents
Immobilisierte immidazole und ruthenium-katalysatoren Download PDFInfo
- Publication number
- WO2005016524A3 WO2005016524A3 PCT/EP2004/007939 EP2004007939W WO2005016524A3 WO 2005016524 A3 WO2005016524 A3 WO 2005016524A3 EP 2004007939 W EP2004007939 W EP 2004007939W WO 2005016524 A3 WO2005016524 A3 WO 2005016524A3
- Authority
- WO
- WIPO (PCT)
- Prior art keywords
- compounds
- general formulae
- immobilised
- imidazoles
- ruthenium catalysts
- Prior art date
Links
- 239000003054 catalyst Substances 0.000 title abstract 3
- KJTLSVCANCCWHF-UHFFFAOYSA-N Ruthenium Chemical compound [Ru] KJTLSVCANCCWHF-UHFFFAOYSA-N 0.000 title abstract 2
- 229910052707 ruthenium Inorganic materials 0.000 title abstract 2
- 150000002460 imidazoles Chemical class 0.000 title 1
- 150000001875 compounds Chemical class 0.000 abstract 5
- ADLVDYMTBOSDFE-UHFFFAOYSA-N 5-chloro-6-nitroisoindole-1,3-dione Chemical compound C1=C(Cl)C([N+](=O)[O-])=CC2=C1C(=O)NC2=O ADLVDYMTBOSDFE-UHFFFAOYSA-N 0.000 abstract 2
- 230000015572 biosynthetic process Effects 0.000 abstract 2
- 239000003446 ligand Substances 0.000 abstract 2
- 238000003786 synthesis reaction Methods 0.000 abstract 2
- -1 N,N-disubstituted imidazolium Chemical class 0.000 abstract 1
- 150000001336 alkenes Chemical class 0.000 abstract 1
- 238000005859 coupling reaction Methods 0.000 abstract 1
- 229910052809 inorganic oxide Inorganic materials 0.000 abstract 1
- 238000004519 manufacturing process Methods 0.000 abstract 1
- 238000000034 method Methods 0.000 abstract 1
- JRZJOMJEPLMPRA-UHFFFAOYSA-N olefin Natural products CCCCCCCC=C JRZJOMJEPLMPRA-UHFFFAOYSA-N 0.000 abstract 1
- 229910052723 transition metal Inorganic materials 0.000 abstract 1
- 150000003624 transition metals Chemical class 0.000 abstract 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
- C07F15/00—Compounds containing elements of Groups 8, 9, 10 or 18 of the Periodic Table
- C07F15/0006—Compounds containing elements of Groups 8, 9, 10 or 18 of the Periodic Table compounds of the platinum group
- C07F15/0046—Ruthenium compounds
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
- B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
- B01J31/1616—Coordination complexes, e.g. organometallic complexes, immobilised on an inorganic support, e.g. ship-in-a-bottle type catalysts
- B01J31/1625—Coordination complexes, e.g. organometallic complexes, immobilised on an inorganic support, e.g. ship-in-a-bottle type catalysts immobilised by covalent linkages, i.e. pendant complexes with optional linking groups
- B01J31/1633—Coordination complexes, e.g. organometallic complexes, immobilised on an inorganic support, e.g. ship-in-a-bottle type catalysts immobilised by covalent linkages, i.e. pendant complexes with optional linking groups covalent linkages via silicon containing groups
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
- B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
- B01J31/22—Organic complexes
- B01J31/2265—Carbenes or carbynes, i.e.(image)
- B01J31/2269—Heterocyclic carbenes
- B01J31/2273—Heterocyclic carbenes with only nitrogen as heteroatomic ring members, e.g. 1,3-diarylimidazoline-2-ylidenes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
- B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
- B01J31/24—Phosphines, i.e. phosphorus bonded to only carbon atoms, or to both carbon and hydrogen atoms, including e.g. sp2-hybridised phosphorus compounds such as phosphabenzene, phosphole or anionic phospholide ligands
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
- B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
- B01J31/24—Phosphines, i.e. phosphorus bonded to only carbon atoms, or to both carbon and hydrogen atoms, including e.g. sp2-hybridised phosphorus compounds such as phosphabenzene, phosphole or anionic phospholide ligands
- B01J31/2404—Cyclic ligands, including e.g. non-condensed polycyclic ligands, the phosphine-P atom being a ring member or a substituent on the ring
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
- C07C6/00—Preparation of hydrocarbons from hydrocarbons containing a different number of carbon atoms by redistribution reactions
- C07C6/02—Metathesis reactions at an unsaturated carbon-to-carbon bond
- C07C6/04—Metathesis reactions at an unsaturated carbon-to-carbon bond at a carbon-to-carbon double bond
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/30—Addition reactions at carbon centres, i.e. to either C-C or C-X multiple bonds
- B01J2231/32—Addition reactions to C=C or C-C triple bonds
- B01J2231/321—Hydroformylation, metalformylation, carbonylation or hydroaminomethylation
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/40—Substitution reactions at carbon centres, e.g. C-C or C-X, i.e. carbon-hetero atom, cross-coupling, C-H activation or ring-opening reactions
- B01J2231/42—Catalytic cross-coupling, i.e. connection of previously not connected C-atoms or C- and X-atoms without rearrangement
- B01J2231/4205—C-C cross-coupling, e.g. metal catalyzed or Friedel-Crafts type
- B01J2231/4211—Suzuki-type, i.e. RY + R'B(OR)2, in which R, R' are optionally substituted alkyl, alkenyl, aryl, acyl and Y is the leaving group
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/40—Substitution reactions at carbon centres, e.g. C-C or C-X, i.e. carbon-hetero atom, cross-coupling, C-H activation or ring-opening reactions
- B01J2231/42—Catalytic cross-coupling, i.e. connection of previously not connected C-atoms or C- and X-atoms without rearrangement
- B01J2231/4205—C-C cross-coupling, e.g. metal catalyzed or Friedel-Crafts type
- B01J2231/4261—Heck-type, i.e. RY + C=C, in which R is aryl
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/50—Redistribution or isomerisation reactions of C-C, C=C or C-C triple bonds
- B01J2231/52—Isomerisation reactions
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/50—Redistribution or isomerisation reactions of C-C, C=C or C-C triple bonds
- B01J2231/54—Metathesis reactions, e.g. olefin metathesis
- B01J2231/543—Metathesis reactions, e.g. olefin metathesis alkene metathesis
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
- B01J2231/60—Reduction reactions, e.g. hydrogenation
- B01J2231/64—Reductions in general of organic substrates, e.g. hydride reductions or hydrogenations
- B01J2231/641—Hydrogenation of organic substrates, i.e. H2 or H-transfer hydrogenations, e.g. Fischer-Tropsch processes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
- B01J2531/80—Complexes comprising metals of Group VIII as the central metal
- B01J2531/82—Metals of the platinum group
- B01J2531/821—Ruthenium
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
- B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
- B01J31/02—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides
- B01J31/0234—Nitrogen-, phosphorus-, arsenic- or antimony-containing compounds
- B01J31/0235—Nitrogen containing compounds
- B01J31/0254—Nitrogen containing compounds on mineral substrates
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07B—GENERAL METHODS OF ORGANIC CHEMISTRY; APPARATUS THEREFOR
- C07B2200/00—Indexing scheme relating to specific properties of organic compounds
- C07B2200/11—Compounds covalently bound to a solid support
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Inorganic Chemistry (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
- Catalysts (AREA)
- Heterocyclic Carbon Compounds Containing A Hetero Ring Having Nitrogen And Oxygen As The Only Ring Hetero Atoms (AREA)
- Low-Molecular Organic Synthesis Reactions Using Catalysts (AREA)
Abstract
Priority Applications (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
US10/567,742 US20060293526A1 (en) | 2003-08-11 | 2004-07-16 | Immobilised imidazoles and ruthenium catalysts |
JP2006522921A JP2007501695A (ja) | 2003-08-11 | 2004-07-16 | 固定化イミダゾールおよびルテニウム触媒 |
EP04763282A EP1654064A2 (de) | 2003-08-11 | 2004-07-16 | Immobilisierte immidazole und ruthenium-katalysatoren |
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE10337118.4 | 2003-08-11 | ||
DE10337118 | 2003-08-11 |
Publications (2)
Publication Number | Publication Date |
---|---|
WO2005016524A2 WO2005016524A2 (de) | 2005-02-24 |
WO2005016524A3 true WO2005016524A3 (de) | 2005-05-12 |
Family
ID=34177495
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
PCT/EP2004/007939 WO2005016524A2 (de) | 2003-08-11 | 2004-07-16 | Immobilisierte immidazole und ruthenium-katalysatoren |
Country Status (6)
Country | Link |
---|---|
US (1) | US20060293526A1 (de) |
EP (1) | EP1654064A2 (de) |
JP (1) | JP2007501695A (de) |
CN (1) | CN1835801A (de) |
TW (1) | TW200523027A (de) |
WO (1) | WO2005016524A2 (de) |
Families Citing this family (13)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19815275B4 (de) * | 1998-04-06 | 2009-06-25 | Evonik Degussa Gmbh | Alkylidenkomplexe des Rutheniums mit N-heterozyklischen Carbenliganden und deren Verwendung als hochaktive, selektive Katalysatoren für die Olefin-Metathese |
DE102004060247A1 (de) * | 2004-12-15 | 2006-06-29 | Studiengesellschaft Kohle Mbh | Neue N-heterocyclische Carbene und ihre Anwendung in der Katalyse |
AU2007263808B2 (en) * | 2006-06-30 | 2012-04-19 | F. Hoffmann-La Roche Ag | New ruthenium complexes as catalysts for metathesis reactions |
JP5156010B2 (ja) * | 2007-04-20 | 2013-03-06 | 国立大学法人 新潟大学 | オレフィンメタセシス触媒及びそれを用いたメタセシス反応によるオレフィン反応生成物の製造方法 |
EP2082804B1 (de) * | 2008-01-25 | 2012-10-03 | Universite Claude Bernard Lyon 1 | Organisch-anorganische Hybridmaterialien mit stabilisiertem Carben |
EP2506972B1 (de) | 2009-12-03 | 2019-04-17 | Umicore AG & Co. KG | Geträgerte olefinmetathesekatalysatoren |
CN103180332A (zh) * | 2010-10-28 | 2013-06-26 | 巴斯夫欧洲公司 | N-杂环卡宾配合物、其制备及应用 |
US20120289617A1 (en) * | 2011-05-10 | 2012-11-15 | Saudi Arabian Oil Company | Hybrid Catalyst for Olefin Metathesis |
JP5976807B2 (ja) * | 2011-08-15 | 2016-08-24 | ザ・ガヴァニング・カウンシル・オヴ・ユニヴァーシティー・オヴ・トロント | ルテニウム系錯体触媒 |
EP3041812B1 (de) * | 2013-09-04 | 2022-08-10 | California Institute of Technology | Funktionalisierte lineare und cyclische polyolefine |
CN104030973A (zh) * | 2014-06-13 | 2014-09-10 | 上海应用技术学院 | 一种1,4-二氢吡啶类化合物的制备方法 |
CN108043442B (zh) * | 2017-12-07 | 2021-03-19 | 苏州大学 | 碳负载的钌纳米材料及其制备方法与在催化醇与芳香二胺反应中的应用 |
WO2024015248A1 (en) * | 2022-07-13 | 2024-01-18 | Baker Hughes Oilfield Operations Llc | Immobilizing metal catalysts in a porous support via additive manufacturing and chemical vapor transformation |
Citations (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19954485A1 (de) * | 1999-11-12 | 2001-05-17 | Inst Brennstoffchemie Und Phys | Neuartige immobilisierte Ionic Liquids, ihre Darstellung und Verwendung |
US20020198100A1 (en) * | 2001-05-30 | 2002-12-26 | Mehnert Christian Peter | Ionic liquid compositions |
-
2004
- 2004-07-16 WO PCT/EP2004/007939 patent/WO2005016524A2/de not_active Application Discontinuation
- 2004-07-16 US US10/567,742 patent/US20060293526A1/en not_active Abandoned
- 2004-07-16 JP JP2006522921A patent/JP2007501695A/ja active Pending
- 2004-07-16 EP EP04763282A patent/EP1654064A2/de not_active Withdrawn
- 2004-07-16 CN CN200480022981.4A patent/CN1835801A/zh active Pending
- 2004-08-10 TW TW093123927A patent/TW200523027A/zh unknown
Patent Citations (2)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19954485A1 (de) * | 1999-11-12 | 2001-05-17 | Inst Brennstoffchemie Und Phys | Neuartige immobilisierte Ionic Liquids, ihre Darstellung und Verwendung |
US20020198100A1 (en) * | 2001-05-30 | 2002-12-26 | Mehnert Christian Peter | Ionic liquid compositions |
Non-Patent Citations (6)
Title |
---|
CETINKAYA B ET AL: "Synthesis and immobilization of N - heterocyclic carbene complexes of Ru(II): catalytic activity and recyclability for the furan formation", JOURNAL OF MOLECULAR CATALYSIS. A, CHEMICAL, ELSEVIER, AMSTERDAM, NL, vol. 184, 2002, pages 31 - 38, XP002300268, ISSN: 1381-1169 * |
GADENNE, BENOIT ET AL: "Supported ionic liquids : ordered mesoporous silicas containing covalently linked ionic species", CHEMICAL COMMUNICATIONS (CAMBRIDGE, UNITED KINGDOM) , (15), 1768-1769 CODEN: CHCOFS; ISSN: 1359-7345, 30 June 2004 (2004-06-30), XP002311339 * |
HERNDON JAMES W: "The chemistry of the carbon-transition metal double and triple bond: annual survey covering the year 2002", COORDINATION CHEMISTRY REVIEWS, vol. 248, no. 1-2, 21 January 2004 (2004-01-21), pages 3 - 79, XP002311341 * |
HERRMANN W A ET AL: "N-Heterocyclic Carbenes", ANGEWANDTE CHEMIE. INTERNATIONAL EDITION, VERLAG CHEMIE. WEINHEIM, DE, vol. 36, 1997, pages 2162 - 2187, XP002178612, ISSN: 0570-0833 * |
HERRMANN W A: "N-HETEROCYCLIC CARBENES: A NEW CONCEPT IN ORGANOMETALLIC CATALYSIS", ANGEWANDTE CHEMIE. INTERNATIONAL EDITION, VERLAG CHEMIE. WEINHEIM, DE, vol. 41, no. 8, 2002, pages 1291 - 1309, XP001111697, ISSN: 0570-0833 * |
WERNER H ET AL: "Supported rhodium-catalysts: new aspects in the formation of trisubstituted olefins from simple alkenes and diazoalkanes", JOURNAL OF ORGANOMETALLIC CHEMISTRY, vol. 475, no. 1-2, 26 July 1994 (1994-07-26), pages 277 - 282, XP002311340 * |
Also Published As
Publication number | Publication date |
---|---|
EP1654064A2 (de) | 2006-05-10 |
US20060293526A1 (en) | 2006-12-28 |
TW200523027A (en) | 2005-07-16 |
JP2007501695A (ja) | 2007-02-01 |
CN1835801A (zh) | 2006-09-20 |
WO2005016524A2 (de) | 2005-02-24 |
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