RU2016100932A - Регулирование кислого газа в процессе производства жидкого топлива - Google Patents

Регулирование кислого газа в процессе производства жидкого топлива Download PDF

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RU2016100932A
RU2016100932A RU2016100932A RU2016100932A RU2016100932A RU 2016100932 A RU2016100932 A RU 2016100932A RU 2016100932 A RU2016100932 A RU 2016100932A RU 2016100932 A RU2016100932 A RU 2016100932A RU 2016100932 A RU2016100932 A RU 2016100932A
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gasifier
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Шрикар ЧАКРАВАРТИ
Рэймонд Ф. ДРНЕВИЧ
Миниш М. ШАХ
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Праксайр Текнолоджи, Инк.
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    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/22—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by decomposition of gaseous or liquid organic compounds
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    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
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    • C10K—PURIFYING OR MODIFYING THE CHEMICAL COMPOSITION OF COMBUSTIBLE GASES CONTAINING CARBON MONOXIDE
    • C10K1/00—Purifying combustible gases containing carbon monoxide
    • C10K1/002—Removal of contaminants
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    • C10K—PURIFYING OR MODIFYING THE CHEMICAL COMPOSITION OF COMBUSTIBLE GASES CONTAINING CARBON MONOXIDE
    • C10K3/00—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide
    • C10K3/06—Modifying the chemical composition of combustible gases containing carbon monoxide to produce an improved fuel, e.g. one of different calorific value, which may be free from carbon monoxide by mixing with gases
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    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
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    • C01B2203/0227—Processes for making hydrogen or synthesis gas containing a reforming step containing a catalytic reforming step
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    • C01B2203/1205—Composition of the feed
    • C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
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    • C01B2203/14—Details of the flowsheet
    • C01B2203/141—At least two reforming, decomposition or partial oxidation steps in parallel
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    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
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    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
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    • C10J2300/093—Coal
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    • C10J2300/00—Details of gasification processes
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    • C10J2300/00—Details of gasification processes
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    • C10J2300/00—Details of gasification processes
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    • C10J2300/00—Details of gasification processes
    • C10J2300/16—Integration of gasification processes with another plant or parts within the plant
    • C10J2300/164—Integration of gasification processes with another plant or parts within the plant with conversion of synthesis gas
    • C10J2300/1656—Conversion of synthesis gas to chemicals
    • C10J2300/1659—Conversion of synthesis gas to chemicals to liquid hydrocarbons
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    • C10J2300/00—Details of gasification processes
    • C10J2300/16—Integration of gasification processes with another plant or parts within the plant
    • C10J2300/1678—Integration of gasification processes with another plant or parts within the plant with air separation
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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    • Y02E20/00—Combustion technologies with mitigation potential
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    • Y02E20/18—Integrated gasification combined cycle [IGCC], e.g. combined with carbon capture and storage [CCS]
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
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    • Y02P20/145—Feedstock the feedstock being materials of biological origin

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Claims (24)

1. Способ производства жидкого топлива, включающий:
а) конверсию твердого углеродсодержащего материала в блоке газификации с образованием сингаза газификатора;
b) проведение сингаза газификатора в блок обработки газа и обработку в нем сингаза газификатора;
c) образование по меньшей мере потока обработанного сингаза газификатора, содержащего по меньшей мере 50% CО2 сингаза газификатора, газового потока, обогащенного CО2, и потока, обогащенного серой;
d) использование по меньшей мере части обогащенного CО2 газового потока, содержащего по меньшей мере 90% CО2, удаленного из сингаза газификатора, при образовании сингаза газификатора;
e) конверсию легкого ископаемого топлива в блоке конверсии легкого ископаемого топлива с образованием обогащенного H2 сингаза, содержащего H2 и CO в молярном отношении H2/CO по меньшей мере 2:1;
f) объединение обработанного сингаза газификатора и обогащенного H2 сингаза с образованием смешанного сингаза, имеющего более высокое отношение Н2/СО, чем в потоке обработанного сингаза газификатора;
g) конверсию смешанного сингаза с образованием жидкого топливного продукта и потока побочного продукта, содержащего одно или более веществ из водорода, CO, водяного пара, метана и углеводородов, содержащих 2-8 атомов углерода и 0-2 атомов кислорода; и
h) реакцию до 100% потока побочного продукта в блоке конверсии легкого ископаемого топлива, чтобы способствовать образованию обогащенного H2 сингаза.
2. Способ по п.1, дополнительно содержащий реакцию 100% потока побочного продукта в блоке конверсии легкого ископаемого топлива, чтобы способствовать образованию обогащенного H2 сингаза.
3. Способ по п.1, дополнительно включающий использование от 20% до 50% потока побочного продукта в качестве топлива в каком-либо другом месте установки.
4. Способ по п.1, дополнительно включающий реакцию от 50% до 80% потока побочного продукта, направляемого в блок конверсии легкого ископаемого топлива, при этом остальная часть направляемого потока побочного продукта служит в качестве топлива в указанном блоке конверсии легкого ископаемого топлива.
5. Способ по п.1, дополнительно включающий обработку по меньшей мере части потока побочного продукта в блоке удаления CО2 перед осуществлением реакции в блоке конверсии легкого ископаемого топлива.
6. Способ по п.1, в котором по меньшей мере часть обогащенного H2 сингаза обрабатывается в блоке удаления CО2 с образованием обработанного обогащенного H2 сингаза.
7. Способ по п.1, в котором блок конверсии легкого ископаемого топлива включает в себя автотермический реактор, производящий обогащенный H2 сингаз.
8. Способ по п.1, дополнительно содержащий образование обогащенного H2 сингаза в блоке конверсии легкого ископаемого топлива, при этом указанный блок конверсии включает в себя паровой риформер метана, имеющий загруженные катализатором трубки.
9. Способ по п.8, дополнительно включающий образование обогащенного H2 сингаза в блоке конверсии легкого ископаемого топлива, при этом указанный блок конверсии включает в себя автотермический реактор.
10. Способ по п.1, дополнительно включающий направление сингаза газификатора через систему удаления кислого газа, входящую в состав блока обработки газа.
11. Способ по п.1, дополнительно включающий образование обогащенного серой потока из системы извлечения серы, входящей в состав блока обработки.
12. Способ по п.10, дополнительно включающий направление потока, выходящего из системы удаления кислого газа, через блок конечного удаления серы, входящий в состав блока обработки газа, для получения обработанного сингаза газификатора.
13. Способ по п.1, дополнительно включающий рециркуляцию остальной части обогащенного CО2 газового потока в систему удаления кислого газа, тем самым снижая эмиссию серы до почти нулевого уровня.
14. Способ по п.1, дополнительно включающий образование потока обработанного сингаза газификатора, содержащего по меньшей мере 65% CО2 сингаза газификатора.
15. Способ по п.5, в котором блок удаления CО2 представляет собой аминовую систему.
16. Способ по п.10, в котором система удаления кислого газа представляет собой аминовую систему.
RU2016100932A 2013-06-26 2014-06-11 Регулирование кислого газа в процессе производства жидкого топлива RU2670761C9 (ru)

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US13/927,880 US9145525B2 (en) 2013-06-26 2013-06-26 Acid gas management in liquid fuel production process
US13/927,880 2013-06-26
PCT/US2014/041831 WO2014209605A1 (en) 2013-06-26 2014-06-11 Acid gas management in liquid fuel production process

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