JP6600300B2 - 固体電解質用多重層配置構成 - Google Patents

固体電解質用多重層配置構成 Download PDF

Info

Publication number
JP6600300B2
JP6600300B2 JP2016514298A JP2016514298A JP6600300B2 JP 6600300 B2 JP6600300 B2 JP 6600300B2 JP 2016514298 A JP2016514298 A JP 2016514298A JP 2016514298 A JP2016514298 A JP 2016514298A JP 6600300 B2 JP6600300 B2 JP 6600300B2
Authority
JP
Japan
Prior art keywords
layer
electrolyte
cathode
metal
oxygen content
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
JP2016514298A
Other languages
English (en)
Japanese (ja)
Other versions
JP2016524282A5 (enExample
JP2016524282A (ja
Inventor
ハイドン、マルクス
オルトナー、カイ
リュッチンガー、マティーアス
フランコ、トーマス
ユング、トーマス
ウーレンブルック、スヴェン
Original Assignee
プランゼー コンポジット マテリアルズ ゲーエムベーハー
フォルシュングスツェントゥルム ユーリッヒ ゲゼルシャフト ミット ベシュレンクテル ハフツング
フラウンホーファー‐ゲゼルシャフト ツア フェルデルング デア アンゲヴァンテン フォルシュング アインゲトラーゲナー フェライン
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by プランゼー コンポジット マテリアルズ ゲーエムベーハー, フォルシュングスツェントゥルム ユーリッヒ ゲゼルシャフト ミット ベシュレンクテル ハフツング, フラウンホーファー‐ゲゼルシャフト ツア フェルデルング デア アンゲヴァンテン フォルシュング アインゲトラーゲナー フェライン filed Critical プランゼー コンポジット マテリアルズ ゲーエムベーハー
Publication of JP2016524282A publication Critical patent/JP2016524282A/ja
Publication of JP2016524282A5 publication Critical patent/JP2016524282A5/ja
Application granted granted Critical
Publication of JP6600300B2 publication Critical patent/JP6600300B2/ja
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Images

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H01M2300/0077—Ion conductive at high temperature based on zirconium oxide
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0088—Composites
    • H01M2300/0094—Composites in the form of layered products, e.g. coatings
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H01M8/1253—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides the electrolyte containing zirconium oxide
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Fuel Cell (AREA)
  • Inert Electrodes (AREA)
  • Conductive Materials (AREA)
JP2016514298A 2013-05-21 2014-05-20 固体電解質用多重層配置構成 Expired - Fee Related JP6600300B2 (ja)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE102013008472.5 2013-05-21
DE102013008472.5A DE102013008472A1 (de) 2013-05-21 2013-05-21 Mehrlagige Schichtanordnung für einen Festkörperelektrolyt
PCT/EP2014/001352 WO2014187559A1 (de) 2013-05-21 2014-05-20 Mehrlagige schichtanordnung für einen festkörperelektrolyt

Publications (3)

Publication Number Publication Date
JP2016524282A JP2016524282A (ja) 2016-08-12
JP2016524282A5 JP2016524282A5 (enExample) 2017-06-08
JP6600300B2 true JP6600300B2 (ja) 2019-10-30

Family

ID=50897525

Family Applications (1)

Application Number Title Priority Date Filing Date
JP2016514298A Expired - Fee Related JP6600300B2 (ja) 2013-05-21 2014-05-20 固体電解質用多重層配置構成

Country Status (10)

Country Link
US (1) US10312540B2 (enExample)
EP (1) EP3000149B1 (enExample)
JP (1) JP6600300B2 (enExample)
KR (1) KR20160010465A (enExample)
CN (1) CN105493327B (enExample)
CA (1) CA2911454A1 (enExample)
DE (1) DE102013008472A1 (enExample)
DK (1) DK3000149T3 (enExample)
TW (1) TWI634696B (enExample)
WO (1) WO2014187559A1 (enExample)

Families Citing this family (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6014807B2 (ja) 2014-11-20 2016-10-26 株式会社プラズマイオンアシスト 燃料電池用セパレータ又は燃料電池用集電部材、及びその製造方法
CN105762391B (zh) * 2016-04-15 2019-01-08 暨南大学 组件组成一体化的质子导体低温固体氧化物电池及其制备
AU2019338937A1 (en) * 2018-09-12 2021-03-18 Gelion Technologies Pty Ltd Battery with halogen sequestering agent
US10930844B2 (en) 2018-10-11 2021-02-23 International Business Machines Corporation Three-terminal oxygen intercalation neuromorphic devices
KR20210076688A (ko) 2019-12-16 2021-06-24 삼성전자주식회사 복합 고체전해질, 이를 포함하는 전기화학 셀, 및 상기 복합 고체전해질의 제조방법

Family Cites Families (27)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5171645A (en) * 1991-01-08 1992-12-15 Gas Research Institute, Inc. Zirconia-bismuth oxide graded electrolyte
WO1997041612A1 (en) 1996-05-01 1997-11-06 Gas Research Institute, Inc. Stable high conductivity functionally gradient compositionally layered solid state electrolytes and membranes
JP3843766B2 (ja) * 2000-07-04 2006-11-08 日産自動車株式会社 固体電解質型燃料電池
US6558831B1 (en) 2000-08-18 2003-05-06 Hybrid Power Generation Systems, Llc Integrated SOFC
JP4840718B2 (ja) * 2001-08-14 2011-12-21 日産自動車株式会社 固体酸化物形燃料電池
JP2003142123A (ja) 2001-11-05 2003-05-16 Nissan Motor Co Ltd 固体電解質型燃料電池
JP4054867B2 (ja) 2001-12-04 2008-03-05 独立行政法人産業技術総合研究所 導電性酸化ジルコニウム
WO2003101629A1 (en) 2002-05-29 2003-12-11 The Board Of Trustees Of The Leland Stanford Junior University Sub-micron electrolyte thin film on nano-porous substrate by oxidation of metal film
DE10227048A1 (de) 2002-06-17 2004-01-08 Fraunhofer-Gesellschaft zur Förderung der angewandten Forschung e.V. Vorrichtung zur Beschichtung von Substraten mittels physikalischer Dampfabscheidung über den Hohlkathodeneffekt
JP4135891B2 (ja) * 2002-11-07 2008-08-20 独立行政法人産業技術総合研究所 固体電解質型燃料電池用電解質材料の製造方法、及び固体電解質型燃料電池セルの製造方法
UA83400C2 (uk) 2003-12-02 2008-07-10 Нанодайнемікс, Інк. Твердооксидні паливні елементи з керметним електролітом та спосіб їх одержання
WO2005122300A2 (en) * 2004-06-10 2005-12-22 Risoe National Laboratory Solid oxide fuel cell
JP2006164801A (ja) 2004-12-08 2006-06-22 Toyota Motor Corp 固体電解質、それを備えた燃料電池およびそれらの製造方法
US7767358B2 (en) 2005-05-31 2010-08-03 Nextech Materials, Ltd. Supported ceramic membranes and electrochemical cells and cell stacks including the same
JP2009512166A (ja) * 2005-10-19 2009-03-19 アイトゲネスィッシェ テヒニッシェ ホーホシューレ チューリッヒ 薄膜及び薄膜から製造される複合素子
AT8975U1 (de) 2006-02-27 2007-03-15 Plansee Se Poröser körper
JP5013748B2 (ja) * 2006-05-23 2012-08-29 新光電気工業株式会社 固体酸化物燃料電池
CN1960048A (zh) 2006-11-23 2007-05-09 上海交通大学 多孔金属支撑的低温固体氧化物燃料电池的结构
DE102007015358A1 (de) 2007-03-30 2008-10-02 Forschungszentrum Jülich GmbH Schichtsystem für einen Elektrolyten einer Hochtemperatur-Brennstoffzelle sowie Verfahren zur Herstellung desselben
EP2083466A1 (en) 2008-01-24 2009-07-29 Institute of Nuclear Energy Research Process for the fabrication of a sputter deposited fully dense electrolyte layer embedded in a high performance membrane electrolyte assembly of solid oxide fuel cell
FR2935843B1 (fr) 2008-09-11 2011-02-11 Commissariat Energie Atomique Electrolyte pour pile sofc et son procede de fabrication.
EP2325931A1 (de) * 2009-11-18 2011-05-25 Plansee Se Anordnung für eine Brennstoffzelle sowie Verfahren zu deren Herstellungen
KR20110101976A (ko) * 2010-03-10 2011-09-16 삼성전자주식회사 고체산화물 연료전지 및 이의 제조방법
KR20120040449A (ko) * 2010-10-19 2012-04-27 삼성전자주식회사 고체산화물 전해질막, 그 제조방법 및 이를 채용한 연료전지
KR20120080375A (ko) * 2011-01-07 2012-07-17 삼성전자주식회사 연료전지용 양극 소재, 이를 포함하는 연료전지용 양극과 그 양극의 제조방법, 및 고체산화물 연료전지
KR101215338B1 (ko) * 2011-06-20 2012-12-26 주식회사 엑스에프씨 고체 산화물 연료전지용 전해질막, 그 제조방법 및 이를 채용한 연료전지
CN102593480B (zh) * 2012-02-23 2014-12-10 上海交通大学 固体氧化物燃料电池掺杂钛酸盐支撑固体电解质多层膜及其制备方法

Also Published As

Publication number Publication date
KR20160010465A (ko) 2016-01-27
WO2014187559A1 (de) 2014-11-27
TW201505246A (zh) 2015-02-01
CN105493327B (zh) 2018-01-30
TWI634696B (zh) 2018-09-01
US10312540B2 (en) 2019-06-04
JP2016524282A (ja) 2016-08-12
US20160118680A1 (en) 2016-04-28
CN105493327A (zh) 2016-04-13
EP3000149B1 (de) 2017-05-10
WO2014187559A8 (de) 2016-02-18
DE102013008472A1 (de) 2014-11-27
DK3000149T3 (en) 2017-08-28
CA2911454A1 (en) 2014-11-27
EP3000149A1 (de) 2016-03-30

Similar Documents

Publication Publication Date Title
JP5421101B2 (ja) 導電性層を製作する方法
Pederson et al. Application of vacuum deposition methods to solid oxide fuel cells
JP5762295B2 (ja) 低温ｓｏｆｃ用の新素材および構造
US9065104B2 (en) Process for manufacturing elementary electrochemical cells for energy- or hydrogen-producing electrochemical systems, in particular of SOFC and HTE type
CN102217130A (zh) 用于生产燃料电池组件的涂覆工艺
US20110262839A1 (en) Proton conducting electrolyte membranes having nano-grain ysz as protective layers, and membrane electrode assemblies and ceramic fuel cells comprising same
JP6600300B2 (ja) 固体電解質用多重層配置構成
JP5552222B2 (ja) セラミック層の加工法及び加工物品
JP5389378B2 (ja) 複合セラミック電解質構造、その製造方法及び関連物品
KR20160030625A (ko) 프로톤 전도체 고체산화물 연료전지의 제조방법과 이 방법에 의해 제조된 프로톤 전도체 고체산화물 연료전지
KR101290577B1 (ko) 고체 산화물 연료전지용 전해질막, 그 제조방법 및 이를 채용한 연료전지
KR101288375B1 (ko) 원자막 증착법으로 형성된 이트리아-안정화 지르코니아 기능층을 포함하는 세리아계 전해질 및 이를 포함하는 고체 산화물 연료전지
KR20100062456A (ko) 전도성 산화물과 비전도성 산화물을 포함하는 치밀한 구조의 복합 산화물의 박막, 이의 제조방법 및 그를 이용한금속 접속자
JP5550223B2 (ja) セラミック電解質の処理方法および関連製品
He Thin coating technologies and applications in high-temperature solid oxide fuel cells
JP5470281B2 (ja) 固体酸化物形燃料電池及びその製造方法
KR20200034344A (ko) 고체산화물 연료 전지용 연결재, 그 제조방법 및 이를 포함하는 고체 산화물 연료 전지
Jaiswal et al. Fabrication of anode supported thick film ceria electrolytes for IT-SOFCs
JP2005078951A (ja) 固体酸化物形燃料電池用単セル及びその製造方法
Tsimekas et al. Morphology and Structure of Solid Oxide Fuel Cell (SOFC) Components Fabricated by Spray Pyrolysis
Haydn et al. Metal Supported Membranes: Development of Metal-Supported Solid Oxide Fuel Cells Based on a Powder-Metallurgical Manufacturing Route
KR20120132058A (ko) 전극 반응층이 개선된 고체산화물 연료 전지 및 그 제조 방법
Martin et al. Ultrathin Solid Oxide Fuel Cell Fabrication
Mukai et al. Improvement of Thermal Reliability and Power Density of SOFCs by Preparing Nano LSC Particles between GDC Electrolyte and LSCF Cathode
Perednis et al. prepared via spray pyrolysis

Legal Events

Date Code Title Description
A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20170411

A621 Written request for application examination

Free format text: JAPANESE INTERMEDIATE CODE: A621

Effective date: 20170411

A131 Notification of reasons for refusal

Free format text: JAPANESE INTERMEDIATE CODE: A131

Effective date: 20180417

A601 Written request for extension of time

Free format text: JAPANESE INTERMEDIATE CODE: A601

Effective date: 20180711

A601 Written request for extension of time

Free format text: JAPANESE INTERMEDIATE CODE: A601

Effective date: 20180914

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20180928

A131 Notification of reasons for refusal

Free format text: JAPANESE INTERMEDIATE CODE: A131

Effective date: 20190219

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20190517

TRDD Decision of grant or rejection written
A01 Written decision to grant a patent or to grant a registration (utility model)

Free format text: JAPANESE INTERMEDIATE CODE: A01

Effective date: 20190924

A61 First payment of annual fees (during grant procedure)

Free format text: JAPANESE INTERMEDIATE CODE: A61

Effective date: 20191004

R150 Certificate of patent or registration of utility model

Ref document number: 6600300

Country of ref document: JP

Free format text: JAPANESE INTERMEDIATE CODE: R150

LAPS Cancellation because of no payment of annual fees