JP5698951B2 - 正極活物質及びその製造方法、正極ならびに非水電解質二次電池 - Google Patents

正極活物質及びその製造方法、正極ならびに非水電解質二次電池 Download PDF

Info

Publication number
JP5698951B2
JP5698951B2 JP2010234814A JP2010234814A JP5698951B2 JP 5698951 B2 JP5698951 B2 JP 5698951B2 JP 2010234814 A JP2010234814 A JP 2010234814A JP 2010234814 A JP2010234814 A JP 2010234814A JP 5698951 B2 JP5698951 B2 JP 5698951B2
Authority
JP
Japan
Prior art keywords
positive electrode
source
active material
electrode active
lithium
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
JP2010234814A
Other languages
English (en)
Japanese (ja)
Other versions
JP2012089342A5 (OSRAM
JP2012089342A (ja
Inventor
俊次 末木
俊次 末木
西島　主明
主明 西島
耕司 大平
耕司 大平
正悟 江▲崎▼
正悟 江▲崎▼
田中　功
功 田中
幸典 小山
幸典 小山
勝久 田中
勝久 田中
晃司 藤田
晃司 藤田
俊介 村井
俊介 村井
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Sharp Corp
Original Assignee
Sharp Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sharp Corp filed Critical Sharp Corp
Priority to JP2010234814A priority Critical patent/JP5698951B2/ja
Priority to CA2755059A priority patent/CA2755059C/en
Priority to US13/275,858 priority patent/US9017876B2/en
Priority to DE102011116315A priority patent/DE102011116315A1/de
Priority to CN201110326896.9A priority patent/CN102456878B/zh
Publication of JP2012089342A publication Critical patent/JP2012089342A/ja
Publication of JP2012089342A5 publication Critical patent/JP2012089342A5/ja
Application granted granted Critical
Publication of JP5698951B2 publication Critical patent/JP5698951B2/ja
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/58—Selection of substances as active materials, active masses, active liquids of inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy; of polyanionic structures, e.g. phosphates, silicates or borates
    • H01M4/5825—Oxygenated metallic salts or polyanionic structures, e.g. borates, phosphates, silicates, olivines
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B25/00—Phosphorus; Compounds thereof
    • C01B25/16—Oxyacids of phosphorus; Salts thereof
    • C01B25/26—Phosphates
    • C01B25/45—Phosphates containing plural metal, or metal and ammonium
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B32/00—Carbon; Compounds thereof
    • C01B32/05—Preparation or purification of carbon not covered by groups C01B32/15, C01B32/20, C01B32/25, C01B32/30
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/485—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of mixed oxides or hydroxides for inserting or intercalating light metals, e.g. LiTi2O4 or LiTi2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/50—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese
    • H01M4/505—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese of mixed oxides or hydroxides containing manganese for inserting or intercalating light metals, e.g. LiMn2O4 or LiMn2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/52—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron
    • H01M4/525—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron of mixed oxides or hydroxides containing iron, cobalt or nickel for inserting or intercalating light metals, e.g. LiNiO2, LiCoO2 or LiCoOxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M2004/021—Physical characteristics, e.g. porosity, surface area
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/131—Electrodes based on mixed oxides or hydroxides, or on mixtures of oxides or hydroxides, e.g. LiCoOx
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/136—Electrodes based on inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/621—Binders
    • H01M4/622—Binders being polymers
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/621—Binders
    • H01M4/622—Binders being polymers
    • H01M4/623—Binders being polymers fluorinated polymers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries

Landscapes

  • Chemical & Material Sciences (AREA)
  • Inorganic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Silicon Compounds (AREA)
  • Secondary Cells (AREA)
JP2010234814A 2010-10-19 2010-10-19 正極活物質及びその製造方法、正極ならびに非水電解質二次電池 Expired - Fee Related JP5698951B2 (ja)

Priority Applications (5)

Application Number Priority Date Filing Date Title
JP2010234814A JP5698951B2 (ja) 2010-10-19 2010-10-19 正極活物質及びその製造方法、正極ならびに非水電解質二次電池
CA2755059A CA2755059C (en) 2010-10-19 2011-10-17 Positive electrode active material, production method thereof and its use
US13/275,858 US9017876B2 (en) 2010-10-19 2011-10-18 Positive electrode active material, production method thereof and its use
DE102011116315A DE102011116315A1 (de) 2010-10-19 2011-10-18 Positivelektrodenaktives Material, Herstellungsverfahren dafür und seine Verwendung
CN201110326896.9A CN102456878B (zh) 2010-10-19 2011-10-19 正极活性物质及其制造方法、正极以及非水电解质二次电池

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
JP2010234814A JP5698951B2 (ja) 2010-10-19 2010-10-19 正極活物質及びその製造方法、正極ならびに非水電解質二次電池

Publications (3)

Publication Number Publication Date
JP2012089342A JP2012089342A (ja) 2012-05-10
JP2012089342A5 JP2012089342A5 (OSRAM) 2012-06-21
JP5698951B2 true JP5698951B2 (ja) 2015-04-08

Family

ID=45896051

Family Applications (1)

Application Number Title Priority Date Filing Date
JP2010234814A Expired - Fee Related JP5698951B2 (ja) 2010-10-19 2010-10-19 正極活物質及びその製造方法、正極ならびに非水電解質二次電池

Country Status (5)

Country Link
US (1) US9017876B2 (OSRAM)
JP (1) JP5698951B2 (OSRAM)
CN (1) CN102456878B (OSRAM)
CA (1) CA2755059C (OSRAM)
DE (1) DE102011116315A1 (OSRAM)

Families Citing this family (16)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2011152455A1 (ja) 2010-06-02 2011-12-08 シャープ株式会社 リチウム含有複合酸化物の製造方法
JP5698951B2 (ja) 2010-10-19 2015-04-08 シャープ株式会社 正極活物質及びその製造方法、正極ならびに非水電解質二次電池
JP5478549B2 (ja) * 2011-04-18 2014-04-23 シャープ株式会社 正極活物質の製造方法
US9337478B2 (en) * 2012-02-14 2016-05-10 Shailesh Upreti Composite silicon or composite tin particles
CN103959518B (zh) * 2012-06-06 2016-08-10 夏普株式会社 非水电解质二次电池用正极活性物质、非水电解质二次电池用正极以及非水电解质二次电池
JP2014017199A (ja) * 2012-07-11 2014-01-30 Sharp Corp リチウム二次電池用電極およびその製造方法並びにリチウム二次電池およびその製造方法
CN105122508B (zh) * 2013-04-26 2018-04-06 夏普株式会社 锂离子二次电池用正极以及包括该正极的锂离子二次电池
US10847781B2 (en) * 2017-12-04 2020-11-24 Samsung Sdi Co., Ltd. Positive active material for rechargeable lithium battery, preparing method thereof and rechargeable lithium battery comprising positive electrode including positive active material
US11522189B2 (en) 2017-12-04 2022-12-06 Samsung Sdi Co., Ltd. Positive electrode for rechargeable lithium battery, preparing method thereof, and rechargeable lithium battery comprising positive electrode
US11777075B2 (en) 2017-12-04 2023-10-03 Samsung Sdi Co., Ltd. Positive active material for rechargeable lithium battery, preparing method thereof and rechargeable lithium battery comprising positive electrode including positive active material
KR102424398B1 (ko) 2020-09-24 2022-07-21 삼성에스디아이 주식회사 리튬 이차 전지용 양극, 그 제조 방법, 및 이를 포함한 리튬 이차 전지
KR102853967B1 (ko) 2021-05-28 2025-09-01 삼성에스디아이 주식회사 리튬 이차 전지용 양극 활물질, 이의 제조 방법 및 이를 포함하는 리튬 이차 전지
US11670754B2 (en) 2017-12-04 2023-06-06 Samsung Sdi Co., Ltd. Positive active material for rechargeable lithium battery, preparing method thereof and rechargeable lithium battery comprising positive electrode including positive active material
KR102685070B1 (ko) * 2019-10-02 2024-07-12 에스케이이노베이션 주식회사 리튬 전구체의 회수 방법
CN113582149B (zh) * 2021-05-31 2022-12-30 佛山市德方纳米科技有限公司 一种片状磷酸铁锂材料的制备方法
CN116190641B (zh) * 2023-04-23 2023-08-08 中南大学 一种锂钠钾混合型正极活性材料及其制备方法和应用

Family Cites Families (30)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6085015A (en) * 1997-03-25 2000-07-04 Hydro-Quebec Lithium insertion electrode materials based on orthosilicate derivatives
JP3500424B2 (ja) * 2000-08-31 2004-02-23 独立行政法人産業技術総合研究所 単相リチウムフェライト系複合酸化物
CA2320661A1 (fr) 2000-09-26 2002-03-26 Hydro-Quebec Nouveau procede de synthese de materiaux limpo4 a structure olivine
JP3988374B2 (ja) 2000-10-06 2007-10-10 ソニー株式会社 非水電解液二次電池
JP4686859B2 (ja) 2000-12-27 2011-05-25 株式会社デンソー 正極活物質および非水電解質二次電池
JP2003203632A (ja) 2002-01-09 2003-07-18 Hitachi Ltd リチウム二次電池用正極活物質とその製造法及びそれを用いたリチウム二次電池並びに組電池モジュール
US6815122B2 (en) 2002-03-06 2004-11-09 Valence Technology, Inc. Alkali transition metal phosphates and related electrode active materials
JP4043853B2 (ja) 2002-06-07 2008-02-06 住友大阪セメント株式会社 電極材料の製造方法
JP4695876B2 (ja) 2002-07-22 2011-06-08 エムビーエー ポリマーズ， インコーポレイテッド 輸送可能なプラスチック回収システム
CN1833328B (zh) * 2003-01-31 2012-01-04 三井造船株式会社 蓄电池的阴极材料,生产方法和蓄电池
US7211237B2 (en) * 2003-11-26 2007-05-01 3M Innovative Properties Company Solid state synthesis of lithium ion battery cathode material
CN1926701B (zh) 2003-12-23 2010-12-22 蒙特利尔大学 用于制备电活性嵌入化合物的方法及自其获得的电极材料
JP5428125B2 (ja) * 2005-11-24 2014-02-26 日産自動車株式会社 非水電解質二次電池用正極活物質、および、これを用いた非水電解質二次電池
US7494744B2 (en) 2006-03-08 2009-02-24 Changs-Ascending Enterprise Co. Cathode material for Li-ion battery applications
US8349217B2 (en) * 2007-03-27 2013-01-08 Tokyo Institute Of Technology Method for producing positive electrode material for secondary battery
JP5293936B2 (ja) 2007-05-21 2013-09-18 戸田工業株式会社 非水電解質二次電池用オリビン型複合酸化物及びその製造方法、並びに二次電池
KR20090125278A (ko) 2007-05-28 2009-12-04 비와이디 컴퍼니 리미티드 리튬 이온 2차 전지를 위한 양극 활성 물질로서 리튬 인산철을 제조하는 방법
JP5176400B2 (ja) 2007-06-14 2013-04-03 住友大阪セメント株式会社 電極材料の製造方法と電極材料および電極並びに電池
CN101219360B (zh) 2008-01-24 2010-07-14 同济大学 过渡金属基气凝胶、过渡金属氧化物气凝胶、复合过渡金属氧化物气凝胶的制备方法
JP5383217B2 (ja) * 2008-01-28 2014-01-08 住友化学株式会社 正極活物質およびナトリウム二次電池、ならびにオリビン型リン酸塩の製造方法
EP2231514A4 (en) 2008-04-07 2013-04-10 Byd Co Ltd PROCESS FOR THE PREPARATION OF AN IRON SOURCE FOR PREPARING LITHIUM FERROUS PHOSPHATE, AND PROCESS FOR PREPARING LITHIUM FERROUS PHOSPHATE
CN101339994B (zh) 2008-09-01 2010-12-01 甘肃大象能源科技有限公司 多位掺杂型磷酸铁锂正极材料制备方法及其应用
JP5859855B2 (ja) * 2008-10-20 2016-02-16 キネテイツク・リミテツド 金属化合物の合成
JP5574143B2 (ja) * 2009-02-18 2014-08-20 トヨタ自動車株式会社 正極活物質の製造方法
KR101336562B1 (ko) 2009-05-22 2013-12-03 고쿠리츠 다이가쿠 호진 교토 다이가쿠 정극 활물질, 정극 및 비수 이차 전지
US8993163B2 (en) 2009-07-31 2015-03-31 Toyota Jidosha Kabushiki Kaisha Positive electrode active material and method for producing same
WO2011152455A1 (ja) * 2010-06-02 2011-12-08 シャープ株式会社 リチウム含有複合酸化物の製造方法
JP5683890B2 (ja) * 2010-10-01 2015-03-11 シャープ株式会社 正極材料、その製造方法、正極及び非水電解質二次電池
JP5698951B2 (ja) 2010-10-19 2015-04-08 シャープ株式会社 正極活物質及びその製造方法、正極ならびに非水電解質二次電池
JP5478549B2 (ja) * 2011-04-18 2014-04-23 シャープ株式会社 正極活物質の製造方法

Also Published As

Publication number Publication date
US20120100429A1 (en) 2012-04-26
JP2012089342A (ja) 2012-05-10
CA2755059A1 (en) 2012-04-19
CN102456878A (zh) 2012-05-16
CN102456878B (zh) 2015-06-17
DE102011116315A1 (de) 2012-04-19
US9017876B2 (en) 2015-04-28
CA2755059C (en) 2015-03-24

Similar Documents

Publication Publication Date Title
JP5698951B2 (ja) 正極活物質及びその製造方法、正極ならびに非水電解質二次電池
JP5478549B2 (ja) 正極活物質の製造方法
JP5695842B2 (ja) リチウム含有複合酸化物の製造方法
JP5132727B2 (ja) 正極活物質、正極及び非水電解質二次電池
CN103038169B (zh) 含锂复合氧化物的制造方法
JP2011181452A (ja) リチウムイオン電池用正極活物質の製造方法及びリチウムイオン電池用電極並びにリチウムイオン電池
JP5683890B2 (ja) 正極材料、その製造方法、正極及び非水電解質二次電池
WO2014065117A1 (ja) リチウム二次電池用炭素被覆活物質の製造方法およびそれに用いる製造装置
JP5901492B2 (ja) リチウムシリケート化合物の製造方法、リチウムシリケート化合物凝集体の製造方法及びリチウムイオン電池の製造方法
JP5651377B2 (ja) リチウム含有複合酸化物の製造方法
JP5957536B2 (ja) 正極活物質および正極並びに非水電解質二次電池
JP5539802B2 (ja) 非水電解質二次電池用正極活物質、非水電解質二次電池用正極および非水電解質二次電池
JP5698929B2 (ja) 正極活物質、正極及び非水二次電池
JP6302751B2 (ja) 正極活物質、正極及び非水電解質二次電池
JP5846983B2 (ja) 電極活物質の製造方法
CN103003989B (zh) 正极活性物质、正极和非水电解质二次电池
JP2015092510A (ja) 非水電解質二次電池

Legal Events

Date Code Title Description
A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20120328

A621 Written request for application examination

Free format text: JAPANESE INTERMEDIATE CODE: A621

Effective date: 20130819

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A821

Effective date: 20130819

A711 Notification of change in applicant

Free format text: JAPANESE INTERMEDIATE CODE: A711

Effective date: 20140225

A977 Report on retrieval

Free format text: JAPANESE INTERMEDIATE CODE: A971007

Effective date: 20140226

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A821

Effective date: 20140225

A131 Notification of reasons for refusal

Free format text: JAPANESE INTERMEDIATE CODE: A131

Effective date: 20140507

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20140703

A131 Notification of reasons for refusal

Free format text: JAPANESE INTERMEDIATE CODE: A131

Effective date: 20140819

A521 Request for written amendment filed

Free format text: JAPANESE INTERMEDIATE CODE: A523

Effective date: 20141015

TRDD Decision of grant or rejection written
A01 Written decision to grant a patent or to grant a registration (utility model)

Free format text: JAPANESE INTERMEDIATE CODE: A01

Effective date: 20150120

A61 First payment of annual fees (during grant procedure)

Free format text: JAPANESE INTERMEDIATE CODE: A61

Effective date: 20150216

R150 Certificate of patent or registration of utility model

Ref document number: 5698951

Country of ref document: JP

Free format text: JAPANESE INTERMEDIATE CODE: R150

LAPS Cancellation because of no payment of annual fees