JP4241372B2 - ポリオールブレンドの製造方法 - Google Patents

ポリオールブレンドの製造方法 Download PDF

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Publication number
JP4241372B2
JP4241372B2 JP2003507170A JP2003507170A JP4241372B2 JP 4241372 B2 JP4241372 B2 JP 4241372B2 JP 2003507170 A JP2003507170 A JP 2003507170A JP 2003507170 A JP2003507170 A JP 2003507170A JP 4241372 B2 JP4241372 B2 JP 4241372B2
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Prior art keywords
polyether
epoxide
weight
blend
initiator
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Expired - Fee Related
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JP2003507170A
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English (en)
Japanese (ja)
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JP2004530767A5 (enExample
JP2004530767A (ja
Inventor
ジャック・アール・リース
スタンリー・エル・ヘイガー
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Bayer Antwerpen NV
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Bayer Antwerpen NV
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    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/2805Compounds having only one group containing active hydrogen
    • C08G18/2815Monohydroxy compounds
    • C08G18/283Compounds containing ether groups, e.g. oxyalkylated monohydroxy compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G65/00Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule
    • C08G65/02Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring
    • C08G65/26Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring from cyclic ethers and other compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00Polymeric products of isocyanates or isothiocyanates
    • C08G18/06Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40High-molecular-weight compounds
    • C08G18/48Polyethers
    • C08G18/4866Polyethers having a low unsaturation value
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G65/00Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule
    • C08G65/02Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring
    • C08G65/26Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring from cyclic ethers and other compounds
    • C08G65/2642Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring from cyclic ethers and other compounds characterised by the catalyst used
    • C08G65/2645Metals or compounds thereof, e.g. salts
    • C08G65/2663Metal cyanide catalysts, i.e. DMC's
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G65/00Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule
    • C08G65/02Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring
    • C08G65/26Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring from cyclic ethers and other compounds
    • C08G65/2696Macromolecular compounds obtained by reactions forming an ether link in the main chain of the macromolecule from cyclic ethers by opening of the heterocyclic ring from cyclic ethers and other compounds characterised by the process or apparatus used
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2110/00Foam properties
    • C08G2110/0008Foam properties flexible
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2110/00Foam properties
    • C08G2110/0041Foam properties having specified density
    • C08G2110/005< 50kg/m3
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G2110/00Foam properties
    • C08G2110/0083Foam properties prepared using water as the sole blowing agent

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Toxicology (AREA)
  • Polyethers (AREA)
  • Polyurethanes Or Polyureas (AREA)
  • Polyesters Or Polycarbonates (AREA)
  • Processes Of Treating Macromolecular Substances (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
JP2003507170A 2001-06-21 2002-06-13 ポリオールブレンドの製造方法 Expired - Fee Related JP4241372B2 (ja)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US09/886,510 US6491846B1 (en) 2001-06-21 2001-06-21 Process for the in-situ production of polyol blends, the in-situ produced polyol blends, and their use in the production of viscoelastic foam
PCT/IB2002/003084 WO2003000770A1 (en) 2001-06-21 2002-06-13 Process for the production of polyol blends

Publications (3)

Publication Number Publication Date
JP2004530767A JP2004530767A (ja) 2004-10-07
JP2004530767A5 JP2004530767A5 (enExample) 2006-01-05
JP4241372B2 true JP4241372B2 (ja) 2009-03-18

Family

ID=25389162

Family Applications (1)

Application Number Title Priority Date Filing Date
JP2003507170A Expired - Fee Related JP4241372B2 (ja) 2001-06-21 2002-06-13 ポリオールブレンドの製造方法

Country Status (18)

Country Link
US (1) US6491846B1 (enExample)
EP (1) EP1401912B1 (enExample)
JP (1) JP4241372B2 (enExample)
KR (1) KR100852527B1 (enExample)
CN (1) CN1235942C (enExample)
AT (1) ATE296849T1 (enExample)
BR (1) BR0210587A (enExample)
CA (1) CA2450785C (enExample)
CZ (1) CZ20033509A3 (enExample)
DE (1) DE60204461T2 (enExample)
ES (1) ES2242871T3 (enExample)
HU (1) HU229655B1 (enExample)
MX (1) MXPA03011866A (enExample)
PL (1) PL207216B1 (enExample)
PT (1) PT1401912E (enExample)
RU (1) RU2312112C2 (enExample)
TW (1) TW593390B (enExample)
WO (1) WO2003000770A1 (enExample)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2004051996A (ja) * 2002-07-19 2004-02-19 Bayer Antwerpen Nv 活性化出発混合物およびその関連方法
US7738815B2 (en) 2007-02-20 2010-06-15 Konica Minolta Business Technologies, Inc. Image forming apparatus including a toner discharge operation

Families Citing this family (39)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DK1507469T3 (da) 2002-05-24 2010-10-18 Tempur World Llc Komfortpude
US7530127B2 (en) 2002-05-24 2009-05-12 Dan-Foam Aps Pillow and method of manufacturing a pillow
ITRM20020471A1 (it) * 2002-09-24 2004-03-25 Adler Plastic S P A Composizione poliuretanica fonoassorbente e fonoisolante.
US7078443B2 (en) * 2003-10-22 2006-07-18 Intellectual Property Holdings, Llc Viscoelastic foam layer and composition
US20050107643A1 (en) * 2003-11-13 2005-05-19 Thomas Ostrowski Preparation of polyether alcohols
WO2005073275A1 (ja) * 2004-01-30 2005-08-11 Kaneka Corporation オキシアルキレン重合体の製造方法
WO2005073276A1 (ja) * 2004-01-30 2005-08-11 Kaneka Corporation 加水分解性珪素基含有オキシアルキレン重合体の製造方法およびその硬化性組成物
EP1889861A4 (en) * 2005-04-21 2012-03-28 Asahi Glass Co Ltd POLYURETHANE FOAMING FUEL WITH LOW RETRACTIVE ELASTICITY AND MANUFACTURING METHOD THEREFOR
US7469437B2 (en) 2005-06-24 2008-12-30 Tempur-Pedic Management, Inc. Reticulated material body support and method
TW200801060A (en) * 2006-02-28 2008-01-01 Asahi Glass Co Ltd Flexible polyurethane foam and process for producing the same
US8656537B2 (en) 2006-04-20 2014-02-25 Dan Foam Aps Multi-component pillow and method of manufacturing and assembling same
US20070299153A1 (en) * 2006-06-23 2007-12-27 Hager Stanley L Viscoelastic foams with slower recovery and improved tear
CN101528800B (zh) 2006-10-25 2012-05-30 旭硝子株式会社 软质聚氨酯泡沫塑料的制造方法
DE502008002134D1 (de) * 2007-01-30 2011-02-10 Basf Se Verfahren zur herstellung von polyethercarbonatpolyolen
JP5303885B2 (ja) * 2007-09-18 2013-10-02 旭硝子株式会社 軟質ポリウレタンフォームの製造方法および軟質ポリウレタンフォーム
KR20100075825A (ko) * 2007-09-28 2010-07-05 아사히 가라스 가부시키가이샤 연질 폴리우레탄 폼 및 열 프레스 성형품의 제조 방법 그리고 열 프레스 성형품
US20090306235A1 (en) * 2008-06-05 2009-12-10 Wang Jin Quan Memory Foam Pad
WO2010009205A1 (en) * 2008-07-18 2010-01-21 Dow Global Technologies Inc. Cellular structures and viscoelastic polyurethane foams
DE102009053218A1 (de) 2009-11-06 2011-07-14 Bayer MaterialScience AG, 51373 Verfahren zur Herstellung eines Polyurethanschaums mittels über- oder nahekritischen Treibmittels
US20110230581A1 (en) * 2010-03-17 2011-09-22 Bayer Materialscience Llc Process for the production of polyether polyols with a high ethylene oxide content
GB2482176A (en) 2010-07-23 2012-01-25 Christopher Wickham Noakes Production of polyols for use in low ball rebound polyurethane foams
US8975335B2 (en) * 2011-09-23 2015-03-10 Bayer Materialscience Llc Process for the production of high air flow polyether foams and the foams produced by this process
US10669368B2 (en) 2013-03-15 2020-06-02 Covestro Llc Method to increase the resistance of double metal cyanide catalysts to deactivation
DE102013224708A1 (de) * 2013-12-03 2015-06-03 Evonik Industries Ag Alkoxysilylhaltige Klebdichtstoffe mit intrinsisch reduzierter Viskosität
EP3087115B1 (en) * 2013-12-23 2018-04-18 Shell International Research Maatschappij B.V. Process for making a flexible flame retardant polyurethane foam
US9951174B2 (en) 2015-05-20 2018-04-24 Covestro Llc Polyol compositions, a process for the production of these polyol compositions, and their use in the production of open celled polyurethane foams having high airflow
WO2017003748A1 (en) * 2015-07-02 2017-01-05 Dow Global Technologies Llc Process for preparing polyether polyol using dmc catalyst and continuous addition of starter
ES2880289T3 (es) 2017-01-17 2021-11-24 Dow Global Technologies Llc Mezclas de poliol útiles para la producción de espuma viscoelástica
CN110402263B (zh) * 2017-03-15 2022-06-07 科思创有限公司 具有降低的温度敏感性的粘弹性聚氨酯泡沫
US10766998B2 (en) 2017-11-21 2020-09-08 Covestro Llc Flexible polyurethane foams
US10793692B2 (en) 2018-10-24 2020-10-06 Covestro Llc Viscoelastic flexible foams comprising hydroxyl-terminated prepolymers
CN109651609B (zh) * 2018-11-28 2021-04-06 山东蓝星东大有限公司 高eo含量聚醚多元醇的制备方法
EP3741788A1 (de) * 2019-05-24 2020-11-25 Covestro Deutschland AG Verfahren zur herstellung von polyoxyalkylenpolyol-mischungen
CN110922579B (zh) * 2019-12-06 2021-12-03 浙江皇马科技股份有限公司 一种低模量密封胶用聚醚的合成方法
CN112552859B (zh) * 2020-12-29 2022-07-15 烟台信友新材料有限公司 一种高初粘低收缩高强度聚氨酯热熔胶及其制备方法
US11572433B2 (en) 2021-03-12 2023-02-07 Covestro Llc In-situ formed polyols, a process for their preparation, foams prepared from these in-situ formed polyols and a process for their preparation
US20230039276A1 (en) 2021-07-28 2023-02-09 Covestro Llc Novel polyether polyol blends, a process for their preparation, foams prepared from these polyether polyol blends and a process for their preparation
US11718705B2 (en) 2021-07-28 2023-08-08 Covestro Llc In-situ formed polyether polyols, a process for their preparation, and a process for the preparation of polyurethane foams
CN115181259B (zh) * 2022-08-11 2024-04-09 万华化学集团股份有限公司 一种连续化制备聚醚的方法

Family Cites Families (14)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB1063525A (en) 1963-02-14 1967-03-30 Gen Tire & Rubber Co Organic cyclic oxide polymers, their preparation and tires prepared therefrom
US3457203A (en) * 1966-04-25 1969-07-22 Olin Mathieson Hydrophilic polyurethane foams and a process for preparing them
US4981880A (en) * 1988-09-23 1991-01-01 The Dow Chemical Company Process for making low density flexible polyisocyanurate-polyurethane foams
US5114619A (en) 1989-07-14 1992-05-19 The Dow Chemical Company Production of polyether polyols with reduced unsaturation
US4950695A (en) 1989-03-06 1990-08-21 Pmc, Inc. Reduction of firmness in flexible polyurethane foam by addition of monofunctional alcohols, polyesters, and polyethers
US5470813A (en) 1993-11-23 1995-11-28 Arco Chemical Technology, L.P. Double metal cyanide complex catalysts
US5777177A (en) 1996-02-07 1998-07-07 Arco Chemical Technology, L.P. Preparation of double metal cyanide-catalyzed polyols by continuous addition of starter
US5689012A (en) * 1996-07-18 1997-11-18 Arco Chemical Technology, L.P. Continuous preparation of low unsaturation polyoxyalkylene polyether polyols with continuous additon of starter
US6077978A (en) * 1997-09-17 2000-06-20 Arco Chemical Technology L.P. Direct polyoxyalkylation of glycerine with double metal cyanide catalysis
US6136879A (en) 1997-10-28 2000-10-24 Tokai Rubber Industries, Ltd. Soft polyurethane foam, method of producing the same and vehicle interior member using the same
US6066683A (en) * 1998-04-03 2000-05-23 Lyondell Chemical Worldwide, Inc. Molded and slab polyurethane foam prepared from double metal cyanide complex-catalyzed polyoxyalkylene polyols and polyols suitable for the preparation thereof
US6063309A (en) 1998-07-13 2000-05-16 Arco Chemical Technology L.P. Dispersion polyols for hypersoft polyurethane foam
DE19834572A1 (de) * 1998-07-31 2000-02-03 Bayer Ag Doppelmetallcyanid-Katalysatoren für die Herstellung von Polyetherpolyolen
US6391935B1 (en) * 2000-01-31 2002-05-21 Bayer Antwerp, N.V. Viscoelastic polyurethane foams

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2004051996A (ja) * 2002-07-19 2004-02-19 Bayer Antwerpen Nv 活性化出発混合物およびその関連方法
US7738815B2 (en) 2007-02-20 2010-06-15 Konica Minolta Business Technologies, Inc. Image forming apparatus including a toner discharge operation

Also Published As

Publication number Publication date
RU2312112C2 (ru) 2007-12-10
BR0210587A (pt) 2004-08-10
HUP0400214A2 (hu) 2004-06-28
HUP0400214A3 (en) 2012-05-29
TW593390B (en) 2004-06-21
US6491846B1 (en) 2002-12-10
MXPA03011866A (es) 2004-03-26
RU2004101635A (ru) 2005-06-27
ES2242871T3 (es) 2005-11-16
CA2450785A1 (en) 2003-01-03
HU229655B1 (en) 2014-03-28
PL207216B1 (pl) 2010-11-30
DE60204461D1 (de) 2005-07-07
CZ20033509A3 (en) 2004-07-14
PT1401912E (pt) 2005-10-31
KR20040030692A (ko) 2004-04-09
KR100852527B1 (ko) 2008-08-14
ATE296849T1 (de) 2005-06-15
CN1235942C (zh) 2006-01-11
EP1401912B1 (en) 2005-06-01
EP1401912A1 (en) 2004-03-31
CN1518572A (zh) 2004-08-04
DE60204461T2 (de) 2006-04-27
HK1068359A1 (en) 2005-04-29
CA2450785C (en) 2011-08-02
WO2003000770A1 (en) 2003-01-03
JP2004530767A (ja) 2004-10-07
PL366781A1 (en) 2005-02-07

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