JP2009535292A - 水素を反応生成物とする反応を行うための反応装置、及び方法 - Google Patents
水素を反応生成物とする反応を行うための反応装置、及び方法 Download PDFInfo
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Abstract
Description
− 反応室及び燃焼室で、水素透過性膜で互いに分離されており、前記燃焼室が横供給孔を備えた酸素(O2)含有流体のための供給チャンネルを有する、反応室及び燃焼室を与えること;
− 前記反応室で前記反応を行うこと;
− 前記反応室からの水素を前記水素透過性膜を通って前記燃焼室へ移動又は輸送すること;
− 前記供給チャンネルの前記供給孔を通って前記燃焼室へ前記酸素(O2)含有流体を供給すること;
− 前記燃焼室である量の水素を燃焼して熱を発生させること;
− 前記熱を前記反応室へ伝達すること;
を含む方法にも関する。
CH4+H2O+熱 ⇔ CO+3H2
CO+H2O ⇔ CO2+3H2
CH4+2H2O+熱 ⇔ CO+4H2
Claims (30)
- 水素(H2)を反応生成物とする反応室を行うための反応室(2)、燃焼室(5)、及び前記反応室(2)と前記燃焼室(5)との間に与えられた水素透過性膜(3)を有する反応装置(1)であって、前記燃焼室(5)には供給チャンネル(9)が与えられ、その供給チャンネル(9)には前記燃焼室(5)へ酸素(O2)含有流体を供給するための横供給孔(10)が開けられていることを特徴とする、反応装置(1)。
- 燃焼室(5)が水素透過性膜(3)の透過物側に位置する。請求項1に記載の反応装置。
- 燃焼室(5)が水素透過性膜(3)を通って反応室(2)から運び出された水素を燃焼するように設計されている、請求項1又は2に記載の反応装置。
- 燃焼室(5)が水素透過性膜(3)により反応室(2)と熱的に接触している、請求項1〜3のいずれか1項に記載の反応装置。
- 燃焼室(5)が酸素(O2)含有流体のための入り口孔(11)を備え、その入り口孔(11)が横供給孔(10)を有する供給チャンネル(9)に接続されている、請求項1〜4のいずれか1項に記載の反応装置。
- 燃焼室(5)が、水蒸気及び/又は窒素及び/又は酸素(O2)含有流体、例えば空気のようなフラッシュ流体のための入り口(14)を備えている、請求項1〜5のいずれか1項に記載の反応装置。
- 燃焼室(5)が、水素透過性膜(3)を通って反応室(2)から運び出される少なくとも水素のための出口(15)を備えている、請求項1〜6のいずれか1項に記載の反応装置。
- 反応室(2)が、供給流を供給するための供給部(17)を備えている、請求項1〜7のいずれか1項に記載の反応装置。
- 反応室(2)が、反応しなかった供給流、反応生成物、及び副生成物、例えば、CO2、H2O、H2、CH4、及びCOを排出するための排出部(18)を備えている、請求項1〜8のいずれか1項に記載の反応装置。
- 反応室(2)及び/又は燃焼室(5)に、触媒床が与えられている、請求項1〜9のいずれか1項に記載の反応装置。
- 供給チャンネルが管状の供給管(9)を有する、請求項1〜10のいずれか1項に記載の反応装置。
- 反応室(2)が吸熱反応のために設計されている、請求項1〜11のいずれか1項に記載の反応装置。
- 横供給孔(10)が、燃焼室(5)中での水素の燃焼による熱発生が反応室(2)中での吸熱反応に必要な熱条件に適合するような仕方で設計されている、請求項12に記載の反応装置。
- 供給孔(10)が、互いに実質的に不均等な間隔で与えられている、請求項1〜13のいずれか1項に記載の反応装置。
- 酸素(O2)含有流体を供給するための供給部が、反応室(2)に与えられている、請求項1〜14のいずれか1項に記載の反応装置。
- 複数の水素透過性膜(3)で、夫々の膜が燃焼室(5)の境界になっている水素透過性膜が配備された反応容器(20)を有し、然も、前記燃焼室(5)の間に反応室(2)が広がり、各燃焼室(5)には、酸素(O2)含有流体を前記燃焼室へ供給するための横供給孔(10)を備えた供給チャンネル(9)が与えられている、請求項1〜15のいずれか1項に記載の反応装置。
- 反応容器(20)が、供給流のための供給孔(27)で、水素透過性膜(3)を境界とする燃焼室(5)間の反応室(2)中へ開いた供給孔を有する、請求項16に記載の反応装置。
- 水素透過性膜(3)が夫々反応容器(20)中に実質的に垂直に吊るされている、請求項16又は17に記載の反応装置。
- 水素透過性膜(3)が管状燃焼室(5)の境界になっている、請求項1〜18のいずれか1項に記載の反応装置。
- 各管状の供給管(9)に、反応容器(20)の一端部(31)へフラッシュ流体を通過させるための少なくとも一つの中心管(30)が配備されており、前記中心管(30)が、供給管(9)の内部に伸び、前記中心管(30)の末端部(31)近くに各燃焼室(5)のフラッシュ流体のための入り口(14)が設けられている、請求項17〜19のいずれか1項に記載の反応装置。
- 水素(H2)が反応生成物として形成される反応を行う方法において:
− 反応室(2)及び燃焼室(5)で、水素透過性膜(3)で互いに分離されており、前記燃焼室(5)が横供給孔(10)を備えた酸素(O2)含有流体のための供給チャンネル(9)を有する、反応室及び燃焼室を与えること;
− 前記反応室(2)で前記反応を行うこと;
− 前記反応室(2)からの水素を前記水素透過性膜(3)を通って前記燃焼室(5)へ運ぶこと;
− 前記供給チャンネル(9)の前記供給孔(10)を通って前記燃焼室(5)へ酸素(O2)含有流体を供給すること;
− 前記燃焼室(5)で、前記水素透過性膜(3)を通って運ばれた、ある量の水素を燃焼して熱を放出させること;
− 前記熱を前記反応室(2)へ伝達すること;
を含む方法。 - 熱が水素透過性膜(3)を通る熱伝導により燃焼室(5)から反応室(2)へ伝達される、請求項21に記載の方法。
- 反応室(2)で行われる反応が吸熱性であり、反応室(2)へ伝達された熱を前記吸熱反応を維持するために用いられる、請求項21又は22に記載の方法。
- 反応室(2)で行われる反応が発熱性である、請求項21〜23のいずれか1項に記載の方法。
- 反応室(2)で行われる反応が平衡反応である、請求項21〜24のいずれか1項に記載の方法。
- 水蒸気及び/又は窒素及び/又は空気のような酸素(O2)含有流体のようなフラッシュ流体を燃焼室(5)を通って供給する、請求項21〜25のいずれか1項に記載の方法。
- 水素を、燃焼室(5)から出口(15)を通って排出する、請求項21〜26のいずれか1項に記載の方法。
- 燃焼室(5)から排出された水素を発電のためのガスタービンへ供給する、請求項27に記載の方法。
- 燃焼室(5)から排出された水素を、窒素と一緒にアンモニア(NH3)を製造するためのアンモニア反応器へ供給する、請求項27に記載の方法。
- シンガスが反応室(2)から排出部(18)を通って排出される、請求項21〜26のいずれか1項に記載の方法。
Applications Claiming Priority (2)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
NL1031754A NL1031754C2 (nl) | 2006-05-04 | 2006-05-04 | Reactorinrichting, alsmede werkwijze voor het uitvoeren van een reactie met waterstof als reactieproduct. |
PCT/NL2007/050192 WO2007142518A1 (en) | 2006-05-04 | 2007-05-01 | A reactor device, and a method for carrying out a reaction with hydrogen as reaction product |
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JP2009535292A true JP2009535292A (ja) | 2009-10-01 |
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US (1) | US20100044642A1 (ja) |
EP (1) | EP2012912A1 (ja) |
JP (1) | JP2009535292A (ja) |
CN (1) | CN101466462A (ja) |
CA (1) | CA2651336A1 (ja) |
NL (1) | NL1031754C2 (ja) |
NO (1) | NO20084681L (ja) |
WO (1) | WO2007142518A1 (ja) |
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US8506924B2 (en) * | 2010-11-11 | 2013-08-13 | Basf Se | Process and apparatus for preparing acetylene and synthesis gas |
KR101336764B1 (ko) * | 2011-10-28 | 2013-12-05 | 한국에너지기술연구원 | 반응분리동시공정에 의한 수소제조모듈 및 이를 이용한 수조제조반응기 |
WO2016064084A1 (ko) * | 2014-10-22 | 2016-04-28 | 한국에너지기술연구원 | 쉘-앤-튜브형 천연가스 개질용 반응기 및 이를 이용한 합성가스 또는 수소가스의 제조방법 |
US20160251228A1 (en) | 2015-02-26 | 2016-09-01 | Khalid T. Alkusayer | Ammonia synthesis for fertilizer production |
CN107428528B (zh) | 2015-04-08 | 2021-09-10 | 托普索公司 | 包括co2膜的重整器装置 |
RU2650154C1 (ru) * | 2016-12-16 | 2018-04-09 | Общество с ограниченной ответственностью "Биологические Источники Энергии" (ООО "БиоИстЭн") | Устройство с псевдоожиженным фонтанирующим слоем кольцеобразной формы и способ его работы |
RU177152U1 (ru) * | 2017-06-30 | 2018-02-12 | Федеральное государственное бюджетное учреждение науки Институт проблем химической физики Российской академии наук (ИПХФ РАН) | Устройство для получения синтез-газа |
CN109441665A (zh) * | 2018-12-26 | 2019-03-08 | 同济大学 | 高压气态氢氧喷气式发动机装置 |
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- 2007-05-01 CN CNA2007800220194A patent/CN101466462A/zh active Pending
- 2007-05-01 EP EP07747416A patent/EP2012912A1/en not_active Withdrawn
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Also Published As
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CA2651336A1 (en) | 2007-12-13 |
NO20084681L (no) | 2009-02-04 |
EP2012912A1 (en) | 2009-01-14 |
WO2007142518A1 (en) | 2007-12-13 |
NL1031754C2 (nl) | 2007-11-06 |
US20100044642A1 (en) | 2010-02-25 |
CN101466462A (zh) | 2009-06-24 |
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