EA200000189A1 - Способ конверсии углеводородов и устройство для его осуществления - Google Patents

Способ конверсии углеводородов и устройство для его осуществления

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Publication number
EA200000189A1
EA200000189A1 EA200000189A EA200000189A EA200000189A1 EA 200000189 A1 EA200000189 A1 EA 200000189A1 EA 200000189 A EA200000189 A EA 200000189A EA 200000189 A EA200000189 A EA 200000189A EA 200000189 A1 EA200000189 A1 EA 200000189A1
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EA
Eurasian Patent Office
Prior art keywords
plasma
hydrocarbons
compartment
products
soot
Prior art date
Application number
EA200000189A
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English (en)
Other versions
EA002038B1 (ru
Inventor
М. Альбин Черниховски
М. Приотр Черниховски
Original Assignee
Лэксарко Холдинг Лимитед
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Publication date
Application filed by Лэксарко Холдинг Лимитед filed Critical Лэксарко Холдинг Лимитед
Priority claimed from PCT/US1998/018027 external-priority patent/WO1999011572A1/en
Publication of EA200000189A1 publication Critical patent/EA200000189A1/ru
Publication of EA002038B1 publication Critical patent/EA002038B1/ru

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    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/36—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents using oxygen or mixtures containing oxygen as gasifying agents
    • C—CHEMISTRY; METALLURGY
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    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/08—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor
    • B01J19/087—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor employing electric or magnetic energy
    • B01J19/088—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor employing electric or magnetic energy giving rise to electric discharges
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    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/342—Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents with the aid of electrical means, electromagnetic or mechanical vibrations, or particle radiations
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2/00—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms
    • C07C2/76—Preparation of hydrocarbons from hydrocarbons containing a smaller number of carbon atoms by condensation of hydrocarbons with partial elimination of hydrogen
    • C07C2/80—Processes with the aid of electrical means
    • H—ELECTRICITY
    • H05—ELECTRIC TECHNIQUES NOT OTHERWISE PROVIDED FOR
    • H05H—PLASMA TECHNIQUE; PRODUCTION OF ACCELERATED ELECTRICALLY-CHARGED PARTICLES OR OF NEUTRONS; PRODUCTION OR ACCELERATION OF NEUTRAL MOLECULAR OR ATOMIC BEAMS
    • H05H1/00—Generating plasma; Handling plasma
    • H05H1/24—Generating plasma
    • H05H1/48—Generating plasma using an arc
    • H05H1/482—Arrangements to provide gliding arc discharges
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J2219/08—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor
    • B01J2219/0894—Processes carried out in the presence of a plasma
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    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0211—Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step
    • C01B2203/0216—Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step containing a non-catalytic steam reforming step
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    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0205—Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0211—Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step
    • C01B2203/0222—Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step containing a non-catalytic carbon dioxide reforming step
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    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/025—Processes for making hydrogen or synthesis gas containing a partial oxidation step
    • C01B2203/0255—Processes for making hydrogen or synthesis gas containing a partial oxidation step containing a non-catalytic partial oxidation step
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    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0283—Processes for making hydrogen or synthesis gas containing a CO-shift step, i.e. a water gas shift step
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    • C01B2203/04—Integrated processes for the production of hydrogen or synthesis gas containing a purification step for the hydrogen or the synthesis gas
    • C01B2203/0465—Composition of the impurity
    • C01B2203/0495—Composition of the impurity the impurity being water
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    • C01B2203/06—Integration with other chemical processes
    • C01B2203/062—Hydrocarbon production, e.g. Fischer-Tropsch process
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    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08—Methods of heating or cooling
    • C01B2203/0805—Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0861—Methods of heating the process for making hydrogen or synthesis gas by plasma
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    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/12—Feeding the process for making hydrogen or synthesis gas
    • C01B2203/1205—Composition of the feed
    • C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
    • C01B2203/1235—Hydrocarbons
    • C01B2203/1241—Natural gas or methane
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    • C01B2203/12—Feeding the process for making hydrogen or synthesis gas
    • C01B2203/1205—Composition of the feed
    • C01B2203/1211—Organic compounds or organic mixtures used in the process for making hydrogen or synthesis gas
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    • C01B2203/16—Controlling the process
    • C01B2203/169—Controlling the feed

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Physics & Mathematics (AREA)
  • Plasma & Fusion (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Inorganic Chemistry (AREA)
  • Combustion & Propulsion (AREA)
  • Toxicology (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Electromagnetism (AREA)
  • Mechanical Engineering (AREA)
  • Physical Or Chemical Processes And Apparatus (AREA)
  • Hydrogen, Water And Hydrids (AREA)
  • Oxygen, Ozone, And Oxides In General (AREA)
  • Carbon And Carbon Compounds (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)

Abstract

В изобретении предложен способ частичного окисления легких углеводородов кислородом с электрическим воздействием. Задачей способа и устройства (1) является содействие при помощи плазмы скользящих электрических разрядов (4) частичному окислению углеводородов, которое сопровождается их паровым риформингом и/или риформингом при помощи CO, чтобы получить газы, богатые CO и H, которые могут также иметь высокие содержания CHи CH, причем без образования сажи или нагара. Указанную смесь продуктов получают в плазменном реакторе со скользящими электрическими разрядами (1), которые тлеют в отсеке (15a), в котором поддерживается температура ниже 1200°C и давление менее 6 бар. Разряды действуют непосредственно в экзотермической реактивной среде, состоящей из углеводородов, перемешанных с газообразным кислородом любого происхождения, и, возможно, с HO и/или CO. Поток продуктов, активизированных плазмой и выходящий из зоны (15a), входит в контакт с металлическим или керамическим материалом (19), размещенным в отсеке (15b), в котором поддерживается температура не более 1100°C. Этот материал становится активным в присутствии потока продуктов и как таковой способствует усилению конверсии продуктов, выходящих из плазменного отсека (15a), в конечный продукт.Международная заявка была опубликована вместе с отчетом о международном поиске.
EA200000189A 1997-09-01 1998-08-28 Способ конверсии углеводородов и устройство для его осуществления EA002038B1 (ru)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
FR9710989A FR2768424B1 (fr) 1997-09-01 1997-09-01 Assistance electrique d'oxydation partielle d'hydrocarbures legers par l'oxygene
PCT/US1998/018027 WO1999011572A1 (en) 1997-09-01 1998-08-28 Electrically assisted partial oxidation of light hydrocarbons by oxygen

Publications (2)

Publication Number Publication Date
EA200000189A1 true EA200000189A1 (ru) 2000-10-30
EA002038B1 EA002038B1 (ru) 2001-12-24

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EA200000189A EA002038B1 (ru) 1997-09-01 1998-08-28 Способ конверсии углеводородов и устройство для его осуществления

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EP (1) EP1012113B1 (ru)
JP (1) JP2001514150A (ru)
KR (1) KR100428402B1 (ru)
CN (1) CN1271329A (ru)
AP (1) AP2000001749A0 (ru)
AU (1) AU740520B2 (ru)
BR (1) BR9812137A (ru)
CA (1) CA2300962C (ru)
DE (1) DE69829481D1 (ru)
EA (1) EA002038B1 (ru)
FR (1) FR2768424B1 (ru)
GE (1) GEP20032949B (ru)
ID (1) ID26947A (ru)
NZ (1) NZ502700A (ru)
OA (1) OA11460A (ru)
UA (1) UA63966C2 (ru)

Cited By (3)

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Publication number Priority date Publication date Assignee Title
RU2665691C2 (ru) * 2012-05-09 2018-09-04 Икспендер Энерджи Инк. Усовершенствованный способ фишера-тропша для составления углеводородного топлива с применением условий gtl
CN110252419A (zh) * 2019-07-11 2019-09-20 广东石油化工学院 一种降低催化重整催化剂积碳失活速率的方法及其应用
CN112689610A (zh) * 2018-08-28 2021-04-20 欧洲等离子公司 通过处理含co2和一种或多种烃的气体流来生产合成气体的方法

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FR2872149B1 (fr) * 2004-06-28 2007-10-19 Physiques Sarl Et Chimiques Conversion plasma-catalytique de matieres carbonees
KR100581476B1 (ko) * 2004-08-23 2006-05-23 엄환섭 전자파 플라즈마 토치를 이용한 메탄의 이산화탄소 개질방법
DE102004063743A1 (de) * 2004-12-29 2006-07-13 Volkswagen Ag Verfahren zur Emissionsverminderung von Fahrzeugen und Vorrichtung zur Durchführung des Verfahrens
US8728180B2 (en) 2006-05-08 2014-05-20 Ceramatec, Inc. Plasma-catalyzed, thermally-integrated reformer for fuel cell systems
US8460409B2 (en) 2006-05-08 2013-06-11 Ceramatec, Inc. Plasma-catalyzed fuel reformer
US8618436B2 (en) * 2006-07-14 2013-12-31 Ceramatec, Inc. Apparatus and method of oxidation utilizing a gliding electric arc
JP5180236B2 (ja) * 2007-02-23 2013-04-10 セラマテック・インク 滑動電気アーク用セラミック電極
JP5496503B2 (ja) * 2008-12-25 2014-05-21 石油資源開発株式会社 水素生成装置を備える燃料電池システム
JP5681357B2 (ja) * 2009-11-24 2015-03-04 愛知電機株式会社 マイクロ波非平衡プラズマを用いた有機物質の処理方法
KR101255152B1 (ko) * 2010-12-01 2013-04-22 한국기초과학지원연구원 플라즈마 가스화기를 이용한 발전 시스템
DE102011002617A1 (de) * 2011-01-13 2012-07-19 Siemens Aktiengesellschaft Verfahren zur Herstellung von Synthesegas enthaltend Kohlenmonoxid (CO) und Wasserstoff (H2)
CN104114264A (zh) * 2012-01-20 2014-10-22 纽卡斯尔大学 用于气体向液体转化的一体化强化生物精炼
US9017437B2 (en) 2012-12-11 2015-04-28 Ceramatec, Inc. Method for forming synthesis gas using a plasma-catalyzed fuel reformer
KR101501261B1 (ko) * 2013-07-05 2015-03-12 한국기계연구원 액화석유가스 개질기
CN103539067A (zh) * 2013-07-26 2014-01-29 路运龙 一种组合电弧放电等离子体解水制氢方法及其制氢系统
KR101471070B1 (ko) * 2013-09-16 2014-12-09 한국기계연구원 플라즈마 반응을 이용한 순환형 가스연료 개질기
CN104528643A (zh) * 2014-12-23 2015-04-22 中山大学 一种等离子体流化床重整垃圾填埋气制合成气方法
CN104528642A (zh) * 2014-12-23 2015-04-22 中山大学 一种等离子体流化床重整沼气制合成气方法
KR102075657B1 (ko) * 2018-10-25 2020-02-10 서강대학교 산학협력단 유전체 장벽 방전 플라즈마 반응기에서 비활성화된 메탄 이량화 반응 베드의 재생방법
EP3705452A1 (en) * 2019-03-05 2020-09-09 Casale Sa A method for the suppression of soot formation in an atr or pox reactor
CN111530509A (zh) * 2020-05-25 2020-08-14 大唐国际化工技术研究院有限公司 一种甲烷化催化剂的保护方法
CN114111028A (zh) * 2021-11-12 2022-03-01 长春大学 热水器

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CA1059065A (en) * 1975-12-12 1979-07-24 Terence E. Dancy Arc reforming of hydrocarbons
NL9300833A (nl) * 1993-05-13 1994-12-01 Gastec Nv Werkwijze voor de produktie van waterstof/koolmonoxide mengsels of waterstof uit methaan.
FR2724806A1 (fr) * 1994-09-16 1996-03-22 Pompes Maupu Entreprise Procede et dispositif d'assistance par plasma au vapo-craquage non-catalytique de composes hydrocarbones et halogeno-organiques

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
RU2665691C2 (ru) * 2012-05-09 2018-09-04 Икспендер Энерджи Инк. Усовершенствованный способ фишера-тропша для составления углеводородного топлива с применением условий gtl
CN112689610A (zh) * 2018-08-28 2021-04-20 欧洲等离子公司 通过处理含co2和一种或多种烃的气体流来生产合成气体的方法
CN112689610B (zh) * 2018-08-28 2023-11-17 欧洲等离子公司 通过处理含co2和一种或多种烃的气体流来生产合成气体的方法
CN110252419A (zh) * 2019-07-11 2019-09-20 广东石油化工学院 一种降低催化重整催化剂积碳失活速率的方法及其应用

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GEP20032949B (en) 2003-04-25
UA63966C2 (en) 2004-02-16
NZ502700A (en) 2002-11-26
BR9812137A (pt) 2000-07-18
AU9126798A (en) 1999-03-22
EP1012113B1 (en) 2005-03-23
EA002038B1 (ru) 2001-12-24
EP1012113A1 (en) 2000-06-28
AP2000001749A0 (en) 2000-02-28
CA2300962A1 (en) 1999-03-11
FR2768424A1 (fr) 1999-03-19
ID26947A (id) 2001-02-22
AU740520B2 (en) 2001-11-08
KR100428402B1 (ko) 2004-04-27
OA11460A (en) 2003-11-18
CA2300962C (en) 2007-09-04
JP2001514150A (ja) 2001-09-11
FR2768424B1 (fr) 1999-10-29
KR20010023517A (ko) 2001-03-26
DE69829481D1 (de) 2005-04-28
CN1271329A (zh) 2000-10-25

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